arXiv subjects

Christof Eigner

Publications and source records attributed to Christof Eigner.

At least 19 recordsLinked to original sources

arXiv2026

On the temperature dependence of the optical band gap in the material system of lithium niobate and lithium tantalate

Lithium niobate and lithium tantalate see widespread use in optics and electronics, and are increasingly used for cryogenic applications. Despite their broad deployment, their optical band gap and its relation to the crystal stoichiometry are not well characterised as a function of temperature. In this work, we study the optical absorption properties of congruent, stoichiometric, MgO-doped and Er-doped lithium niobate as well as congruent lithium tantalate across the temperature range between 7~K and 1000~K by means of optical transmission spectroscopy. Our results demonstrate that the difference of the optical band gap typically observed at room temperature between different stoichiometries is not primarily attributable to the intrinsic electronic structure, but rather to different electron-phonon couplings and the average phonon energies. Additionally, we exemplarily study the temperature shift of the 523 nm absorption line in Er-doped lithium niobate due to the increased interest in optically active dopants. To facilitate future analyses, we present the open-source software suite PhoQS-Treat (Tauc Regression Edge Analysis Tool), which enables automated Tauc regressions alongside additional analytical capabilities. This work advances the development of high-performance lithium niobate-based devices.

cond-mat.mtrl-sci↗

arXiv2026

A high-performance quantum pulse gate in thin-film lithium niobate

In this work, we demonstrate a quantum pulse gate (QPG) in thin-film lithium niobate. QPGs enable the selective manipulation and detection of temporal modes of quantum light and form the basis of numerous applications in photonic quantum technologies. To date, their widespread adaption is held back by two main limitations: restricted wavelength and polarization combinations of the involved fields and low normalized conversion efficiencies. We overcome these limitations through developing a QPG in thin-film lithium niobate. We design a waveguide geometry that provides the required dispersion properties for a highly efficient type-0 sum-frequency generation.We verify our design through mapping of the phase matching intensity, and demonstrate high-quality QPG operation by measuring a temporal-mode selectivity of (96.8$\pm$1.7)% on par with existing QPGs. Thanks to the strong confinement in thin-film lithium niobate, we succeed in demonstrating an internal conversion efficiency of (89.6$\pm$0.1)% for a pump power of only 20mW in front of our sample. This yields a lower-bound estimate for the normalized conversion efficiency of (1810$\pm$10)$\mathrm{W}^{-1}\mathrm{cm}^{-2}$, three orders of magnitude higher than in previous QPGs. Our results establish thin-film lithium niobate as ideal platform for high-performance QPGs and are a major step towards practical QPGs for photonic quantum technologies.

quant-ph↗

arXiv2026

Photorefraction Management in Lithium Niobate Waveguides: High-Temperature vs. Cryogenic Solutions

Lithium niobate sees widespread use in nonlinear and quantum optical devices, such as for sum- and difference-frequency generation or spontaneous parametric down-conversion. In lithium niobate waveguides, nonlinear optical processes are often limited by the so-called photorefractive effect, which limits the maximum input or output powers and impacts the nonlinear spectral response. Therefore, strategies for the management of photorefractive damage are a key consideration in device design. Usually, the photorefractive damage threshold, i.e. the maximal permissible operating power, can be increased by high temperature operation of devices. This approach, however, is not applicable in cryogenic environments, which may be required for specialized applications. To better understand the impact of photorefraction in nonlinear optical applications, we study the impact of photorefraction on the phase-matching spectra of two nonlinear-optical sum-frequency generation experiments at 1) high temperatures and 2) cryogenic temperatures. Furthermore, we present an approach to reduce the impact of photorefraction which is compatible with cryogenic operation. This comprises an auxiliary light source, propagating in the same waveguide, which is used to restore phase-matching spectra impacted by photorefraction, as well as reduce pyroelectric effects. Our work provides an alternative route to photorefraction management applicable to cryogenic environments, as well as in situations with tight energy budgets like space applications.

physics.optics↗

arXiv2025

Optimizing Ultra-Long Continuous Wafer-Scale Periodic Poling in Thin-Film Lithium Niobate

Periodically poled thin-film lithium niobate (TFLN) crystals are the fundamental building block for highly-efficient quantum light sources and frequency converters. The efficiency of these devices is strongly dependent on the interaction length between the light and the nonlinear material, scaling quadratically with this parameter. Nevertheless, the fabrication of long, continuously poled areas in TFLN remains challenging, the length of continuously poled areas rarely exceeds 10 mm. In this work, we demonstrate a significant progress in this field achieving the periodic poling of continuous poled areas of 70 mm length with a 3 microns poling period and a close to 50 % duty cycle. We compare two poling electrode design approaches to fabricate long, continuous poled areas. The first approach involves the poling of a single, continuous 70 mm long electrode. The second utilize a segmented approach including the poling of more than 20 individual sections forming together a 70 mm long poling area with no stitching errors. While the continuous electrode allows for faster fabrication, the segmented approach allows to individually optimize the poling resulting in less duty cycle variation. A detailed analysis of the periodic poling results reveals that the results of both are consistent with previously reported poling outcomes for shorter devices. Thus, we demonstrate wafer-scale periodic poling exceeding chiplet-size without any loss in the periodic poling quality. Our work presents a key step towards highly-efficient, narrowbandwidth and low-pump power nonlinear optical devices.

physics.app-ph↗

arXiv2025

Widely non-degenerate nonlinear frequency conversion in cryogenic titanium in-diffused lithium niobate waveguides

The titanium in-diffused lithium niobate waveguide platform is well-established for reliable prototyping and packaging of many quantum photonic components at room temperature. Nevertheless, compatibility with certain quantum light sources and superconducting detectors requires operation under cryogenic conditions. We characterize alterations in phase-matching and mode guiding of a non-degenerate spontaneous parametric down-conversion process emitting around 1556 nm and 950 nm, under cryogenic conditions. Despite the effects of pyroelectricity and photorefraction, the spectral properties match our theoretical model. Nevertheless, these effects cause small but significant variations within and between cooling cycles. These measurements provide a first benchmark against which other nonlinear photonic integration platforms, such as thin-film lithium niobate, can be compared.

quant-ph↗

arXiv2025

Towards integrated sensors for optimized OCT with undetected photons

The development of practical sensors for optical coherence tomography (OCT) with undetected photons requires miniaturization via integration. To be practical, these sensors must exhibit a large spectral bandwidth and a high brightness, which are linked to a high axial resolution and a sufficient signal to noise ratio, respectively. Here, we combine these requirements in a scheme for OCT-measurements with undetected photons based on nonlinear Ti:LiNbO$_3$ waveguides. We investigate the performance benchmarks of the commonly used SU(1,1) scheme in comparison to an induced coherence scheme and find that the latter is actually better suited when implementing measurements with undetected photons in integrated systems. In both schemes, we perform pump gain optimization and OCT measurements with undetected photons with an axial resolution as low as 28 $\mathrm{\mu}$m.

quant-ph↗

arXiv2025

A ultrabright, two-colour photon pair source based on thin-film lithium niobate for bridging visible and telecom wavelengths

We present the design and characterisation of a guided-wave, bright and highly frequency non-degenerate parametric down-conversion source in thin-film lithium niobate. The source generates photon pairs with wavelengths of 815$\,\mathrm{nm}$ and 1550$\,\mathrm{nm}$ linking the visible wavelength regime with telecommunication wavelengths. We confirm the high quality of the generated single photons by determining a value for the heralded second-order correlation function as low as $g^{(2)}_h(0) = (6.7\pm1.1)\cdot10^{-3}$. Furthermore, we achieve a high spectral brightness of 0.44$\cdot$10$^{7}$$\frac{\text{pairs}}{\text{s} \cdot \text{mW} \cdot \text{GHz}}$ which is two orders of magnitude higher than sources based on weakly guiding waveguides. The almost perfect sinc-shape and the strong agreement between the effective and nominal bandwidth highlights the success of our integrated workflow, which begins with device design and continues through precise fabrication to detailed quantum-state characterization. This comprehensive approach enables targeted optimization of the source, resulting in excellent quantum state generation. Our results set a new standard for on-chip, non-degenerate photon-pair sources and represent a crucial step towards practical, scalable quantum communication networks and photonic quantum computing.

quant-ph↗

arXiv2024

Cryogenic Feedforward of a Photonic Quantum State

Modulation conditioned on measurements on entangled photonic quantum states is a cornerstone technology of optical quantum information processing. Performing this task with low latency requires combining single-photon-level detectors with both electronic logic processing and optical modulation in close proximity. In the technologically relevant telecom wavelength band, detection of photonic quantum states is best performed with high-efficiency, low-noise, and high-speed detectors based on the photon-induced breakdown of superconductivity. Therefore, using these devices for feedforward requires mutual compatibility of all components under cryogenic conditions. Here, we demonstrate low-latency feedforward using a quasi-photon-number-resolved measurement on a quantum light source. Specifically, we use a multipixel superconducting nanowire single-photon detector, amplifier, logic, and an integrated electro-optic modulator in situ below 4K. We modulate the signal mode of a spontaneous parametric down-conversion source, conditional on a photon-number measurement of the idler mode, with a total latency of (23+/-3)ns. The photon-number discrimination actively manipulates the signal mode photon statistics, which is itself a central component in photonic quantum computing reliant on heralded single-photon sources. This represents an important benchmark for the fastest quantum photonic feedforward experiments comprising measurement, amplification, logic and modulation. This has direct applications in quantum computing, communication, and simulation protocols.

quant-ph↗

arXiv2024

Programmable time-frequency mode-sorting of single photons with a multi-output quantum pulse gate

We demonstrate a high-dimensional mode-sorter for single photons based on a multi-output quantum pulse gate, which we can program to switch between different temporal-mode encodings including pulse modes, frequency bins, time bins, and their superpositions. This device can facilitate practical realizations of quantum information applications such as high-dimensional quantum key distribution, and thus enables secure communication with enhanced information capacity. We characterize the mode-sorter through a detector tomography in 3 and 5 dimensions and find a fidelity up to $0.958\pm 0.030$ at the single-photon level.

quant-ph↗

arXiv2024

Ultra-broadband non-degenerate guided-wave bi-photon source in the near and mid-infrared

The latest applications in ultrafast quantum metrology require bright, broadband bi-photon sources with one of the photons in the mid-infrared and the other in the visible to near infrared. However, existing sources based on bulk crystals are limited in brightness due to the short interaction length and only allow for limited dispersion engineering. Here, we present an integrated PDC source based on a Ti:LiNbO$_3$ waveguide that generates broadband bi-photons with central wavelengths at $860\,\mathrm{nm}$ and $2800\,\mathrm{nm}$. Their spectral bandwidth exceeds $25\,\mathrm{THz}$ and is achieved by simultaneous matching of the group velocities and cancellation of group velocity dispersion for the signal and idler field. We provide an intuitive understanding of the process by studying our source's behaviour at different temperatures and pump wavelengths, which agrees well with simulations.

quant-ph↗

arXiv2024

Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals

Lithium niobate and lithium tantalate are among the most widespread materials for nonlinear, integrated photonics. Mixed crystals with arbitrary Nb-Ta ratios provide a new degree of freedom to tune materials properties, such as the birefringence, but also leverage the advantages of the singular compounds, for example, by combining the thermal stability of lithium tantalate with the larger nonlinear or piezoelectric constants of lithium niobate. Periodic poling is the prerequisite for any nonlinear optical application. For mixed crystals this has been challenging so far due to the lack of homogeneous, mono-domain crystals, which severely inhibit domain growth and nucleation. In this work we demonstrate that surface-near ($< 1$~$\mu$m depth) periodic poling on x-cut lithium niobate tantalate mixed crystals can be achieved via electric field poling and lithographically structured electrodes. We find that naturally occurring head-to-head or tail-to-tail domain walls in the as-grown crystal inhibit domain inversion at a larger scale. However, periodic poling is possible, if the gap size between the poling electrodes is of the same order of magnitude or smaller than the average size of naturally occurring domains. This work provides the basis for the nonlinear optical application of lithium niobate tantalate mixed crystals.

physics.optics↗

arXiv2024

Integrated, bright, broadband parametric down-conversion source for quantum metrology and spectroscopy

Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness $1.52\cdot10^6\frac{\mathrm{pairs}}{\mathrm{s\,mW\,GHz}}$ and large bandwidth ($7.8\,$THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of $\Delta \tau \approx 120\,\text{fs}$ while maintaining the narrow bandwidth $\Delta \omega_p \ll 1\,\text{MHz}$ of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.

quant-ph↗

arXiv2023

Pyroelectric Influence on Lithium Niobate During the Thermal Transition for Cryogenic Integrated Photonics

Lithium niobate has emerged as a promising platform for integrated quantum optics, enabling efficient generation, manipulation, and detection of quantum states of light. However, integrating single-photon detectors requires cryogenic operating temperatures, since the best performing detectors are based on narrow superconducting wires. While previous studies have demonstrated the operation of quantum light sources and electro-optic modulators in LiNbO3 at cryogenic temperatures, the thermal transition between room temperature and cryogenic conditions introduces additional effects that can significantly influence device performance. In this paper, we investigate the generation of pyroelectric charges and their impact on the optical properties of lithium niobate waveguides when changing from room temperature to 25K, and vice versa. We measure the generated pyroelectric charge flow and correlate this with fast changes in the birefringence acquired through the Senarmont method. Both electrical and optical influence of the pyroelectric effect occurs predominantly at temperatures above 100K.

physics.optics↗

arXiv2023

All optical operation of a superconducting photonic interface

Advanced electro-optic processing combines electrical control with optical modulation and detection. For quantum photonic applications these processes must be carried out at the single photon level with high efficiency and low noise. Integrated quantum photonics has made great strides achieving single photon manipulation by combining key components on integrated chips which are operated by external driving electronics. Nevertheless, electrical interconnects between driving electronics and the electro-optic components, some of which require cryogenic operating conditions, can introduce parasitic effects. Here we show an all-optical interface which simultaneously delivers the operation power to, and extracts the measurement signal from, an advanced photonic circuit, namely, bias and readout of a superconducting nanowire single photon detector (SNSPD) on a single stage in a 1K cryostat. To do so, we supply all power for the single photon detector, output signal conditioning, and electro-optic readout using optical interconnects alone, thereby fully decoupling the cryogenic circuitry from the external environment. This removes the need to heatsink electrical connections, and potentially offers low-loss, high-bandwidth signal processing. This method opens the possibility to operate other advanced electrically decoupled photonic circuits such as optical control and readout of superconducting circuits, and feedforward for photonic quantum computing.

quant-ph↗

arXiv2022

Demonstration of Hong-Ou-Mandel interference in an LNOI directional coupler

Interference between single photons is key for many quantum optics experiments and applications in quantum technologies, such as quantum communication or computation. It is advantageous to operate the systems at telecommunication wavelengths and to integrate the setups for these applications in order to improve stability, compactness and scalability. A new promising material platform for integrated quantum optics is lithium niobate on insulator (LNOI). Here, we realise Hong-Ou-Mandel (HOM) interference between telecom photons from an engineered parametric down-conversion source in an LNOI directional coupler. The coupler has been designed and fabricated in house and provides close to perfect balanced beam splitting. We obtain a raw HOM visibility of (93.5+/-0.7)%, limited mainly by the source performance and in good agreement with off-chip measurements. This lays the foundation for more sophisticated quantum experiments in LNOI

quant-ph↗

arXiv2022

Realization of a multi-output quantum pulse gate for decoding high-dimensional temporal modes of single-photon states

Temporal modes (TMs) of photons provide an appealing high-dimensional encoding basis for quantum information. While techniques to generate TM states have been established, high-dimensional decoding of single-photon TMs remains an open challenge. In this work, we experimentally demonstrate demultiplexing of five-dimensional TMs of single photons with an average fidelity of 0.96 $\pm$ 0.01, characterized via measurement tomography. This is achieved using a newly developed device, the multi-output quantum pulse gate (mQPG). We demonstrate a proof-of-principle complete decoder based on the mQPG that operates on any basis from a set of 6 five-dimensional MUBs and is therefore suitable as a receiver for high-dimensional quantum key distribution. Furthermore, we confirm the high-quality operation of the mQPG by performing resource-efficient state tomography with an average fidelity of 0.98 $\pm$ 0.02.

quant-ph↗

arXiv2022

Cryogenic electro-optic modulation in titanium in-diffused lithium niobate waveguides

Lithium niobate is a promising platform for integrated quantum optics. In this platform we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage $V_{π/2}$ of these modulators increases due to the decrease of the electro-optic effect by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5$\,\mathrm{K}$. The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85$\,\mathrm{nm}$ while cooling the device down to 5$\,\mathrm{K}$. The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the used poling changes by 112$\,\mathrm{nm}$ when cooling to 5$\,\mathrm{K}$

physics.optics↗

arXiv2021

Cryogenic integrated spontaneous parametric down-conversion

Scalable quantum photonics relies on interfacing many optical components under mutually compatible operating conditions. To that end, we demonstrate that spontaneous parametric down-conversion (SPDC) in nonlinear waveguides, a standard technology for generating entangled photon pairs, squeezed states, and heralded single photons, is fully compatible with cryogenic operating conditions required for superconducting detectors. This is necessary for the proliferation of integrated quantum photonics in integration platforms exploiting quasi-phase-matched second-order nonlinear interactions. We investigate how cryogenic operation at 4 K affects the SPDC process by comparing the heralding efficiency, second-order correlation function and spectral properties with operation at room temperature.

quant-ph↗