arXiv subjects

Christoph H. Keitel

Publications and source records attributed to Christoph H. Keitel.

At least 19 recordsLinked to original sources

arXiv2026

Time delay in nonadiabatic tunneling ionization

The under-the-barrier recollision pathway during the tunneling ionization of an atom, despite its minuscule amplitude, leaves its signature on the observable photoelectron momentum distribution due to a phase shift relative to the direct ionization path, that can be interpreted as a tunneling time delay. We investigate how this time delay is modified in the nonadiabatic regime, where the tunneling barrier evolves dynamically during the ionization process. Our analysis is based on a simple model of a one-dimensional short-range potential driven by a strong laser pulse which remains amenable to a systematic analytical treatment with the strong field approximation (SFA). We show a significant contribution of the high-order SFA corrections, which describes the recollision channel with recombination and further ionization, and is additional to the rescattering. Whereas the recombination channel dominates over the rescattering for the tunneling time delay in the quasistatic regime at relatively large laser fields, their contributions are reversed in weak fields.

physics.atom-ph↗

arXiv2026

Radiation-induced electron spin polarization in ultrarelativistic kinetic turbulence

Electron spin polarization in radiative plasmas with ultrarelativistic kinetic turbulence under highly magnetized conditions is investigated using particle-in-cell simulations. We observe that a significant spin polarization can be sustained when the leptons undergo energetic photon emission accompanied by spin flips during the nonequilibrium turbulent evolution. By analyzing the time evolution of spatially dependent spin polarization, we identify an electromagnetic (EM) regime of kinetic turbulence, distinct from the well-known density-dominated regime characterized by vortex currents and magnetic islands. While in the latter regime the spin polarization exists only transiently, in the EM regime significant anisotropic net polarization emerges and persists in non-dissipative scenarios. The correlation between spin signals and turbulence features is leveraged to introduce the characteristic parameter delimiting the EM regime via the ratio of electric and magnetic energy densities and to gain insight into complex plasma turbulence. This study demonstrates the versatility of a spin-resolved study of the plasma turbulence in extreme environments, such as black holes and magnetar magnetospheres.

physics.plasm-ph↗

arXiv2026

Nondipole Coulomb effects in strong x-ray field ionization

Atomic ionization in superintense x-ray fields is studied through numerical solutions of the time-dependent Schrödinger equation including nondipole corrections. The role of the Coulomb potential of the atomic core in the nondipole regime is analyzed for a linearly polarized laser field. In the considered high-frequency and high-intensity stabilization regime, the photoelectron spectra are dominated by a near-zero-energy structure, while above-threshold ionization peaks are suppressed. Two sub-regimes in the nondipole case are identified based on the scaling of the Coulomb momentum transfer, when the Coulomb effect during the interaction with the laser field is either significant or minor. The Coulomb influenced regime sets in within the realm of relatively low field strengths, high laser frequencies, and long pulse durations. An intuitive model explaining the distinct features in the photoelectron momentum distributions and the Coulomb effect scaling is provided.

physics.atom-ph↗

arXiv2026

Intrinsic Nonlocality of Spin- and Polarization-Resolved Probabilities in Strong-Field Quantum Electrodynamics

Spin and polarization are central to precision tests of fundamental physics and for interpreting radiation from astrophysical sources and ultraintense laser-matter experiments. Here, focusing on the fundamental process of nonlinear Compton scattering, we demonstrate that a key assumption underlying current strong-field quantum electrodynamics (SFQED) models, i.e., that emission can be treated as an instantaneous random event sampled from a local differential rate, is inconsistent once emission angles, electron spin, and/or photon polarization are resolved. Namely, even in strictly constant and uniform fields, the resulting fully differential distribution is sign-indefinite, yielding negative inferred probabilities. The physical reason is that the photon emission probability builds up over a finite length of the electron trajectory, the formation region, during which the electron direction changes by roughly the same small angle that defines the radiation cone. Therefore, we put forward a new method where we integrate over this formation region analytically to obtain a physically consistent electron spin and photon polarization model. Simulations of a GeV-class electron-laser collision accessible at current petawatt facilities and of emission in a pulsar-like magnetic field are shown to reveal spin and polarization patterns that differ even qualitatively from state-of-the-art local models. In particular, our new model predicts substantial angle-dependent circular photon polarization where the well-known collinear-emission approach yields none, and a pronounced helicity bias in the recoiling electrons absent from current predictions. These findings have direct implications for upcoming strong-field QED experiments and for interpreting polarized radiation from extreme astrophysical environments.

hep-ph↗

arXiv2026

Quasiperiodic nondipole ionization dynamics in the x-ray stabilization regime

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties in the nondipole regime for long laser pulses remains unknown. Here, we numerically investigate the strong-field ionization of an atom in a long XUV laser pulse in the nondipole regime. Our study of the time-dependent quantum dynamics reveals a quasiperiodic modulation of the ionization yield as a function of pulse duration. We demonstrate that the Coulomb-field-induced slow oscillation of the ionized electron wave packet during the interaction is responsible for the observed modulation of the ionization yield. Furthermore, we scrutinize the unusual photon momentum sharing between the photoelectron and the ion in this extreme regime. These effects are observable in upcoming x-ray free-electron laser facilities.

physics.atom-ph↗

arXiv2026

Strong-field focusing of high-energy particles in beam-multifoil collisions

Extreme beams of charged particles and photons, reaching ultrahigh densities or producing intense gamma-ray bursts, are central to accelerator physics, laboratory astrophysics, and strong-field quantum electrodynamics research. Yet their generation is hindered by conventional focusing methods at multi-GeV energies that rely on massive magnetic assemblies, limiting compactness and attainable density. Here we report the first experimental observation of a fundamentally new focusing mechanism, in which a high-energy charged-particle beam is focused by its own magnetic field reflected from a stack of thin metallic foils via near-field coherent-transition-radiation. The experiment, performed at SLAC's FACET-II facility, reveals strong, cumulative focusing across a broad range of beam configurations, enabled by the delivered 10 GeV, 1 nC, 10 Hz electron beam. The measurements closely agree with predictions from an analytical model and particle-in-cell simulations. These results demonstrate that multifoil focusing is a remarkably straightforward, self-aligned approach to the generation of ultrahigh density beams, opening a path to explore unprecedented regimes of beam-matter interaction and high-energy radiation.

physics.acc-ph↗

arXiv2026

Single-shot sorting of Mössbauer time-domain data at X-ray free-electron lasers

Mössbauer spectroscopy is widely used to study structure and dynamics of matter with remarkably high energy resolution, provided by the narrow nuclear resonance line widths. However, the narrow width implies low count rates, such that experiments commonly average over extended measurement times or many x-ray pulses (``shots''). This averaging impedes the study of non-equilibrium phenomena. It has been suggested that X-ray free-electron lasers (XFELs) could enable Mössbauer single-shot measurements without averaging, and a proof-of-principle demonstration has been reported. However, so far, only a tiny fraction of all shots resulted in signal-photon numbers which are sufficiently high for a single-shot analysis. Here, we demonstrate coherent nuclear-forward-scattering of self-seeded XFEL radiation, with up to 900 signal-photons per shot. We develop a sorting approach which allows us to include all data on a single-shot level, independent of the signal content of the individual shots. It utilizes the presence of different dynamics classes, i.e. different nuclear evolutions after each excitation. Each shot is assigned to one of the classes, which can then be analyzed separately. Our approach determines the classes from the data without requiring theory modeling nor prior knowledge on the dynamics, making it also applicable to unknown phenomena. We envision that our approach opens up new grounds for Mössbauer science, enabling the study of out-of-equilibrium transient dynamics of the nuclei or their environment.

quant-ph↗

arXiv2026

Pair beams unlock beyond-terawatt attosecond free-electron laser pulses

Free-electron lasers (FELs) generate the brightest coherent X-ray pulses available, enabling atomic-resolution and femtosecond-timescale studies across physics, chemistry, and biology. Realising their full potential at extreme peak powers and attosecond pulse durations critically depends on sustaining coherent gain across the full bunch length. Yet, the quasi-static longitudinal space-charge field in the ultrahigh-current regime imprints a slice-dependent energy detuning that quenches gain growth, so that current schemes typically sustain efficient lasing only across a limited fraction of the bunch. Here we demonstrate that a quasi-neutral electron-positron pair beam cancels this self-field and enables full-bunch high-gain lasing in ultracompressed beams without external compensation. Three-dimensional particle-in-cell simulations in a single-pass, untapered undulator confirm the mechanism across operating regimes: in the soft X-ray regime, the pair beam reaches $1.85\,\mathrm{TW}$ at $345\,\mathrm{as}$ with enhanced odd-harmonic emission and improved spatial coherence, while the electron-only beam fails to saturate; and a high-harmonic pair-cascade configuration yields ${\sim}10\,\mathrm{TW}$ in isolated ${\sim}3.5\,\mathrm{as}$ spikes with coherent amplification extending to photon energies of ${\sim}177\,\mathrm{keV}$. These results establish a new operating regime for ultrahigh-power attosecond light sources and open a direct route to coherent gamma-ray emission ($\geq\!100\,\mathrm{keV}$) currently inaccessible to magnetic-undulator FELs, with broad implications for ultrafast structural, electronic, and nuclear sciences.

physics.acc-ph↗

arXiv2026

Stringent Constraints on New Pseudoscalar & Vector Bosons from Precision Hyperfine Splitting Measurements

Axion-like particles and similar new pseudoscalar as well as vector bosons coupled to nucleons and electrons are predicted to lead to spin-dependent forces in atoms and ions. We argue that hyperfine structure measurements in hydrogen- and lithium-like charge states are a sensitive probe to this effect. Employing specific differences of these splittings reduces uncertainties due to nuclear effects in hyperfine structure calculations and measurements. Using this, we show that existing measurements on Be provide competitive limits in the region $m_ϕ\gtrsim 100 {\rm keV}$, confirming, or improving by up to a factor of 2, existing constraints for pseudoscalar couplings, depending on the nuclear model. We also find that future measurements on Cs have a further factor of $2-2.5$ improved discovery potential for pseudoscalars and an order of magnitude for new vector bosons when compared with the corresponding current constraints.

hep-ph↗

arXiv2026

Observation of quantum effects on radiation reaction in strong fields

Radiation reaction, the force experienced by an accelerated charge due to radiation emission, has long been the subject of extensive theoretical and experimental research. Experimental verification of a quantum, strong-field description of radiation reaction is fundamentally important, and has wide-ranging implications for astrophysics, laser-driven particle acceleration, next-generation particle colliders and inverse-Compton photon sources for medical and industrial applications. However, the difficulty of accessing regimes where strong field and quantum effects dominate inhibited previous efforts to observe quantum radiation reaction in charged particle dynamics with high significance. We report the first high significance (> 5σ) observation of strong-field radiation reaction on electron spectra where quantum effects are substantial. We obtain the first, quantitative, strong evidence favouring the quantum-continuous and quantum-stochastic models over the classical model; the quantum models perform comparably. The lower electron energy losses predicted by the quantum models accounts for their improved performance. Model comparison was performed using a novel Bayesian framework which has widespread utility for laser-particle collision experiments, including those utilising conventional accelerators, where some collision parameters cannot be measured directly.

hep-ph↗

arXiv2025

Relativistic Lindblad description of the electron's radiative dynamics

An effective model for describing the relativistic quantum dynamics of a radiating electron is developed via a relativistic generalization of the Lindblad master equation. By incorporating both radiation reaction and vacuum fluctuations into the Dirac equation within an open quantum system framework, our approach captures the Zitterbewegung of the electron, ensuing noncommutativity of its effective spatial coordinates, and provides the quantum analogue of the Landau-Lifshitz (LL) classical equation of motion with radiation reaction. We develop the corresponding phase-space representation via the relativistic Wigner function and derive the semiclassical limit through a Foldy-Wouthuysen transformation. The latter elucidates the signature of quantum vacuum fluctuations in the LL equation, and shows its relationship with the corrected Sokolov equation. Our results offer a robust framework for investigating quantum radiation reaction effects in ultrastrong laser fields.

quant-ph↗

arXiv2025

Role of quantum dynamics in coherent and incoherent radiation during tunneling ionization

Radiation during strong-field tunneling ionization is investigated. The spontaneous as well as the coherent components of the radiation are calculated describing the ionization dynamics via the strong field approximation and the role of the quantum dynamics at tunneling is analyzed. The competition between different mechanisms in different spectral regions is examined. Transition-like radiation (Brunel radiation) is dominated at low-frequencies, Thomson scattering at the laser frequency, and radiative recombination via the three-step process at high-order harmonics. To distinguish the role of the quantum dynamics, simple man Drude models are developed for the coherent as well as for spontaneous radiation, which are based on the electron trajectory out of the tunneling barrier. The quantum dynamics is shown to modify the coherent Brunel radiation for near-zero-frequencies in asymmetric laser pulses. The significant role of free-free transitions is demonstrated for the spontaneous radiation in the low-frequency region.

physics.atom-ph↗

arXiv2025

Fermion selective tests of new physics with the bound electron g-factor

The use of high-precision measurements of the $g$ factor of single-electron ions is considered as a detailed probe for physics beyond the Standard Model. The contribution of the exchange of a hypothetical force-carrying scalar boson to the $g$ factor is calculated for the ground state of H-like ions and used to derive bounds on the parameters of that force. Similarly to the isotope shift, we employ the nuclide shift, i.e. the difference for elements with different proton and/or neutron numbers, in order to increase the experimental sensitivity to the new physics contribution. In particular we find, combining available measurements with current precision with different ions, that the coupling constant for the interaction between an electron and a proton can be constrained up to three orders of magnitude better than with the best current atomic data and theory.

physics.atom-ph↗

arXiv2025

Enhanced One-Color-Two-Photon Resonant Ionization in Highly Charged Ions by Fine-Structure Effects

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from the neutral to the final highly charged states make a comparison with theory enormously difficult. We resolve these pathways by preparing highly charged ions in an electron beam ion trap before exposing them to the pulsed radiation. This reveals how relativistic fine-structure effects shift electronic energies, largely compensate the core-screening potential, and enable the consecutive, resonant absorption of two quasi-monochromatic X-ray photons that would generally be unfeasible. This doubly-resonant channel enhances the efficiency of two-photon ionization by more than two orders of magnitude, dominating in this regime the nonlinear interaction of light and matter with possible application for future precision X-ray metrology.

physics.atom-ph↗

arXiv2025

Dark-fringe interferometer with dynamic phase control for Mössbauer science

Interference is a powerful tool for measuring and control. In Mössbauer science, interference effects are essential to most applications, due to the coherent scattering nature. However, Mössbauer interferometry remains challenging, due to stability requirements imposed by the short x-ray wavelength. Here, we put forward a ``dark fringe'' interferometer with vanishing transmission in the empty state, thereby facilitating sensitive measurements. The relative interferometer phase can dynamically be tuned by displacing a Mössbauer target. We experimentally demonstrate the tuning capabilities of this interferometer by controlling the transmitted x-ray intensity on nanosecond time scales. Then, we demonstrate sensitive measurements by observing the propagation of impulsively launched sound waves in the target over $\sim 10\,μs$. The interferometer concept opens avenues towards polarization-sensitive phase measurements, the generation of coherent multi-pulse sequences for controlling nuclear dynamics, and the implementation of feedback loops to adaptively optimize the interferometer, thereby fueling the further development of nuclear quantum optics.

quant-ph↗

arXiv2025

$^{208}$Pb nuclear charge radius revisited: closing the fine-structure-anomaly gap

A comprehensive reevaluation of the root-mean-square nuclear charge radius is presented for the doubly magic $^{208}$Pb extracted from muonic spectroscopy measurements. By integrating rigorous theoretical quantum electrodynamics calculations, state-of-the-art numerical methods, and a systematic reanalysis of the uncertainties, we reduced the long-standing muonic fine-structure anomaly and improved the goodness of fit by a factor of twenty. The resulting value of 5.5062(5)~fm for a Fermi distribution is fairly consistent with the previously reported muonic spectroscopy value, and three standard deviations larger than the commonly used compilation data, which indicates that the current value and its uncertainty could be significantly underestimated. Attributing the remaining discrepancy to theory errors which can not be rigorously calculated we suggest the rms charge radius with reduced model dependence to be 5.5062(17) fm. This work sets an improved benchmark for charge radius extraction in heavy nuclei and paves a path for systematic reevaluations across the nuclear chart.

physics.atom-ph↗

arXiv2025

Bright 25-attosecond light pulses reach the one atomic unit of time

Generating ever-shorter and brighter light pulses has long been a central pursuit in ultrafast science, as it benchmarks our ability to create and manipulate the coherence on the intrinsic timescale of sub-atomic electron motion. The current state-of-the-art in attosecond pulse generation reaches durations of 40-50 attoseconds (1 as = $10^{-18}$ seconds), produced via high-order harmonic generation (HHG) driven by secondary mid-infrared light sources. However, these sources often suffer from low stability and poor HHG conversion efficiency. In this work, we demonstrate the generation of 25$\pm$2 attosecond light pulses, a new world record for the shortest light pulse, driven by a post-compressed, industrial-grade Yb-based laser system. The resulting high-harmonic spectrum spans photon energies from 50 eV to 320 eV, covering the carbon K-edge, with a calibrated photon flux exceeding $10^{12}$ photons per second, approximately three orders of magnitude higher than previous studies. The pulse duration was characterized using an angle-resolved photoelectron streaking camera on helium atoms and systematically optimized through the use of dielectric filters of varying thicknesses to compensate the attochirp. Our study reaches the threshold of one atomic unit of time (24.2 attoseconds), the boundary between atomic and ionic physics, opening the door to resolving exciting ionic quantum dynamics with tabletop lasers.

physics.atom-ph↗

arXiv2025

Broadband coherent XUV light from $e^-/e^+$ microbunching in an intense laser pulse

Attosecond pulses of coherent extreme ultraviolet (XUV) light are instrumental for investigating subatomic dynamics and can be produced using a free-electron laser (FEL). It has been suggested that an optical FEL, which employs a laser pulse in place of a conventional undulator, could enable a dramatically more compact implementation of such a light source. Yet, the high electron density and subsequent high emittance implied by an optical FEL makes this concept challenging to realize with an electron beam. There has been impressive progress in recent years producing collimated dense and relativistic beams of electrons and positrons in the laboratory. As we demonstrate here, the inherent stability of a quasi-neutral electron-positron beam mitigates Coulomb expansion, and renders it a promising alternative source of coherent light. Specifically, we show via computer simulations that broadband coherent light in the XUV domain, which takes the form of 8-as pulses at 92-as intervals, can be generated by microbunching of relativistic electrons and positrons in a laser pulse. This process occurs over a sub-millimeter length scale, enabling the development of light sources which are orders-of-magnitude more compact than existing sources, with potential applications in physics, chemistry, biology, and industry.

physics.plasm-ph↗