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Christoph H. Keitel

Publications and source records attributed to Christoph H. Keitel.

At least 55 records · Page 3Linked to original sources
arXiv2024

Photoelectron Polarization Vortexes in Strong-Field Ionization

The spin polarization of photoelectrons induced by an intense linearly polarized laser field is investigated using numerical solutions of the time-dependent Schrödinger equation in companion with our analytic treatment via the spin-resolved strong-field approximation and classical trajectory Monte Carlo simulations. We demonstrate that, even though the total polarization vanishes upon averaging over the photoelectron momentum, momentum-resolved spin polarization is significant, typically exhibiting a vortex structure relative to the laser polarization axis. The polarization arises from the transfer of spin-orbital coupling in the bound state to the spin-correlated quantum orbits in the continuum. The rescattering of photoelectrons at the atomic core plays an important role in forming the polarization vortex structure, while there is no significant effect of the spin-orbit coupling during the continuum dynamics. Furthermore, spin-polarized electron holography is demonstrated, feasible for extracting fine structural information about the atom.

physics.atom-ph↗
arXiv2024

Penning-trap measurement of the $Q$-value of the electron capture in $^{163}\mathrm{Ho}$ for the determination of the electron neutrino mass

The investigation of the absolute scale of the effective neutrino mass remains challenging due to the exclusively weak interaction of neutrinos with all known particles in the standard model of particle physics. Currently, the most precise and least model-dependent upper limit on the electron antineutrino mass is set by the KATRIN experiment from the analysis of the tritium \b{eta}-decay. Another promising approach is the electron capture in $^{163}\mathrm{Ho}$, which is under investigation using microcalorimetry within the ECHo and HOLMES collab orations. An independently measured Q-value of this process is vital for the assessment of systematic uncertainties in the neutrino mass determination. Here, we report a direct, independent determination of this $Q$-value by measuring the free-space cyclotron frequency ratio of highly charged ions of $^{163}\mathrm{Ho}$ and $^{163}\mathrm{Dy}$ in the Penning trap experiment \textsc{Pentatrap}. Combining this ratio with atomic physics calculations of the electronic binding energies yields a $Q$-value of $2863.2(0.6)\,\mathrm{eV}/c^{2}$ - a more than 50-fold improvement over the state-of-the-art. This will enable the determination of the electron neutrino mass on a sub-eV level from the analysis of the electron capture in $^{163}\mathrm{Ho}$.

nucl-ex↗
arXiv2023

Atomic mass determination of uranium-238

The atomic mass of uranium-238 has been determined to be $238.050\,787\,618(15)\,\text{u}$, improving the literature uncertainty by two orders of magnitude. It is obtained from a measurement of the mass ratio of $^{238}$U$^{47+}$ and $^{132}$Xe$^{26+}$ ions with an uncertainty of $3.5\times 10^{-12}$. The measurement was carried out with the Penning-trap mass spectrometer \textsc{Pentatrap} and was accompanied by a calculation of the binding energies $E_{\text{U}}$ and $E_{\text{Xe}}$ of the 47 and 26 missing electrons of the two highly charged ions, respectively. These binding energies were determined using an \textit{ab initio} multiconfiguration Dirac-Hartree-Fock (MCDHF) method to be $E_{\text{U}} = 39\,927(10)\,\text{eV}$ and $E_{\text{Xe}} = 8\,971.2(21)\,\text{eV}$. The new mass value will serve as a reference for high-precision mass measurements in the heavy mass region of the nuclear chart up to transuranium nuclides.

physics.atom-ph↗
arXiv2023

Electron slingshot acceleration in relativistic preturbulent shocks explored via emitted photon polarization

Transient electron dynamics near the interface of counterstreaming plasmas at the onset of a relativistic collisionless shock (RCS) is investigated using particle-in-cell simulations. We identify a slingshot-like injection process induced by the drifting electric field sustained by the flowing focus of backwards-moving electrons, which is distinct from the well-known stochastic acceleration. The flowing focus signifies the plasma kinetic transition from a preturbulent laminar motion to a chaotic turbulence. We find a characteristic correlation between the electron dynamics in the slingshot acceleration and the photon emission features. In particular, the integrated radiation from the RCS exhibits a counterintuitive non-monotonic dependence of the photon polarization degree on the photon energy, which originates from a polarization degradation of relatively high-energy photons emitted by the slingshot-injected electrons. Our results demonstrate the potential of photon polarization as an essential information source in exploring intricate transient dynamics in RCSs with relevance for earth-based plasma and astrophysical scenarios.

physics.plasm-ph↗
arXiv2023

Observation of a low-lying metastable electronic state in highly charged lead by Penning-trap mass spectrometry

Highly charged ions (HCIs) offer many opportunities for next-generation clock research due to the vast landscape of available electronic transitions in different charge states. The development of XUV frequency combs has enabled the search for clock transitions based on shorter wavelengths in HCIs. However, without initial knowledge of the energy of the clock states, these narrow transitions are difficult to be probed by lasers. In this Letter, we provide experimental observation and theoretical calculation of a long-lived electronic state in Nb-like Pb$^{41+}$ which could be used as a clock state. With the mass spectrometer Pentatrap, the excitation energy of this metastable state is directly determined as a mass difference at an energy of 31.2(8) eV, corresponding to one of the most precise relative mass determinations to date with a fractional uncertainty of $4\times10^{-12}$. This experimental result agrees within 1 $σ$ with two partially different \textit{ab initio} multi-configuration Dirac-Hartree-Fock calculations of 31.68(13) eV and 31.76(35) eV, respectively. With a calculated lifetime of 26.5(5.3) days, the transition from this metastable state to the ground state bears a quality factor of $1.1\times10^{23}$ and allows for the construction of a HCI clock with a fractional frequency instability of $<10^{-19}/\sqrtτ$.

physics.atom-ph↗
arXiv2023

Nonspreading relativistic electron wavepacket in a strong laser field

A solution of the Dirac equation in a strong laser field presenting a nonspreading wave packet in the rest frame of the electron is derived. It consists of a generalization of the self-accelerating free electron wave packet [Kaminer et al. Nature Phys. 11, 261 (2015)] to the case with the background of a strong laser field. Built upon the notion of nonspreading for an extended relativistic wavepacket, the concept of Born rigidity for accelerated motion in relativity is the key ingredient of the solution. At its core, the solution comes from the connection between the self-accelerated free electron wave packet and the eigenstate of a Dirac electron in a constant and homogeneous gravitational field via the equivalence principle. The solution is an essential step towards the realization of the laser-driven relativistic collider [Meuren et al. PRL 114, 143201 (2015)], where the large spreading of a common Gaussian wave packet during the excursion in a strong laser field strongly limits the expectable yields.

quant-ph↗
arXiv2023

Spin-polarized electron beam generation in the colliding-pulse injection scheme

Employing colliding-pulse injection has been shown to enable high-quality electron beams to be generated from laser-plasma accelerators. Here by leveraging test particle simulations, Hamiltonian analysis, and multidimensional particle-in-cell (PIC) simulations, we lay the theoretical framework of spin-polarized electron beam generation in the colliding-pulse injection scheme. Furthermore, we show that this scheme enables the production of quasi-monoenergetic electron beams in excess of 80\% polarization and tens pC charge with commercial 10-TW-class laser systems.

physics.acc-ph↗
arXiv2023

Enhanced signature of vacuum birefringence in a plasma wakefield

Vacuum birefringence (VB) is a basic phenomenon predicted in quantum electrodynamics (QED). However, due to the smallness of the signal, conventional magnet-based and extremely intense laser-driven detection methods are still very challenging. This is because in the first case the interaction length is large but the field is limited, and vice versa in the second case. We put forward a method to generate and detect VB in a plasma bubble wakefield, which combines both advantages, providing large fields along large interaction lengths. A polarized $γ$-photon beam is considered to probe the wakefield along a propagation distance of millimeters to centimeters in the plasma bubble. We find via plasma particle-in-cell simulations that the VB signal in terms of Stokes parameters can reach about $ 10^{-5}$ ($10^{-3}$-$10^{-2}$) for tens of MeV (GeV) probe photons with moderately intense lasers ($10^{20}$-$10^{21}~\mathrm{W/cm^2}$). The main source of noise from plasma electrons is mitigated, in particular, by a choice of $γ$-photon polarization and by proper modulation of the plasma density. The proposed method represents an attractive alternative for the experimental observation of VB via laser-plasma interaction.

physics.plasm-ph↗
arXiv2023

Laser-driven lepton polarization in the quantum radiation-dominated reflection regime

Generation of ultrarelativistic polarized leptons during interaction of an ultrarelativistic electron beam with a counterpropagating ultraintense laser pulse is investigated in the quantum radiation-dominated domain. While the symmetry of the laser field tends to average the radiative polarization of leptons to zero, we demonstrate the feasibility of sizable radiative polarization through breaking the symmetry of the process in the reflection regime. After the reflection, the off-axis particles escape the tightly focused beam with polarization correlated to the emission angle, while the particles at the beam center are more likely to be captured in the laser field with unmatched polarization and kinetic motion. Meanwhile, polarization along the electric field emerges due to the spin rotation in the transverse plane via precession. In this way, the combined effects of radiative polarization, spin precession and the laser field focusing are shaping the angle-dependent polarization for outgoing leptons. Our spin-resolved Monte Carlo simulations demonstrate an angle-dependent polarization degree up to $\sim20\%$ for both electrons and positrons, with a yield of one pair per seed electron. It provides a new approach for producing polarized high density electron and positron jets at ultraintense laser facilities.

hep-ph↗
arXiv2023

Energy enhancement of laser-driven ions by radiation reaction and Breit-Wheeler pair production in the ultra-relativistic transparency regime

The impact of radiation reaction and Breit-Wheeler pair production on acceleration of fully ionized Carbon ions driven by an intense linearly-polarized laser pulse has been investigated in the ultra-relativistic transparency regime. Against initial expectations radiation reaction and pair production at ultra-high laser intensities is found to enhance the energy gained by the ions. The electrons lose most of their transverse momentum and the additionally produced pair plasma of Breit-Wheeler electrons and positrons co-stream in the forward direction as opposed to the existing electrons streaming at an angle above zero. We discuss how these observations could be explained by the changes in the phase velocity of the Buneman instability, that is known to aid ion acceleration in the Breakout-Afterburner regime, by tapping the free energy in the relative electron and ion streams. We present evidence that these non-classical effects can further improve the highest Carbon ion energies in this transparency regime.

physics.plasm-ph↗
arXiv2023

Ultrastable optical, XUV and soft-x-ray clock transitions in open-shell highly charged ions

Highly charged ions (HCIs) are insensitive to external perturbations and are attractive for the development of ultrastable clocks. However, only a few HCI candidates are known to provide optical clock transitions. In this Letter, we show that, as a result of strong relativistic effects, there are more than 100 suitable optical HCI clock candidates in more than 70 elements. Their transitions are embedded in the fine-structure splitting of the $nd^4$, $nd^5$ and $nd^6$ ground-state configurations with $n=3,4,5$ being the principal quantum numbers. The corresponding high multipolarity transitions in these ions have lifetimes and quality factors many orders of magnitude longer and larger, respectively, than those in state-of-the-art clocks. Their polarizabilities are also orders of magnitude smaller, rendering them more stable against external electromagnetic fields. Furthermore, within the same electronic configurations, the clock transitions in heavy ions scale up to the XUV and soft-x-ray region, thus enable the development of clocks based on shorter wavelengths. The existence of multiple clock transitions in different charge states of a single element, as well as in a whole isoelectronic sequence, would significantly enrich the detection of fine-structure constant variations, the search for new physics and the test of nuclear theories via high-precision spectroscopy.

physics.atom-ph↗
arXiv2023

Certifying multi-mode light-matter interaction in lossy resonators

Quantum models based on few-mode Master equations have been a central tool in the study of resonator quantum electrodynamics, extending the seminal single-mode Jaynes-Cummings model to include loss and multiple modes. Despite their broad application range, previous approaches within this framework have either relied on a Markov approximation or a fitting procedure. By combining ideas from pseudomode and quasinormal mode theory, we develop a certification criterion for multi-mode effects in lossy resonators. It is based on a witness observable, and neither requires a fitting procedure nor a Markov approximation. Using the resulting criterion, we demonstrate that such multi-mode effects are important for understanding previous experiments in X-ray cavity QED with Mössbauer nuclei and that they allow one to tune the nuclear ensemble properties.

quant-ph↗
arXiv2023

Relativistic analytical R-matrix (ARM) theory for strong-field ionization

The analytical R-matrix (ARM) theory has been known for an efficient description of the Coulomb effects of the atomic core in strong-field ionization in the nonrelativistic regime. We generalize the ARM theory into the relativistic domain aiming at the application to strong-field ionization of highly-charged ions in ultrastrong laser fields. Comparison with the relativistic Coulomb-corrected strong field approximations (SFA) is provided, highlighting the advantages and disadvantages. The weakly relativistic asymptotics and its accordance with the nondipole Coulomb-corrected SFA are examined. As an example of a physical application of the relativistic ARM, the Coulomb enhancement of tunneling ionization probability for highly-charged ions at the cutoff of the direct channel is discussed.

physics.atom-ph↗
arXiv2023

High-order harmonic generation enhanced by XUV light

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the first electron performs a HHG three-step process whereas, the second electron Rabi flops between the core and the valence vacancy. The modified HHG spectrum due to recombination with the valence and the core is determined and analyzed for krypton on the 3d -- > 4p resonance in the ion. We assume an 800 nm laser with an intensity of about 10^14 W/cm^2 and XUV radiation from the Free Electron Laser in Hamburg (FLASH) with an intensity in the range 10^13--10^16 W/cm^2. Our prediction opens perspectives for nonlinear XUV physics, attosecond x rays, and HHG-based spectroscopy involving core orbitals.

physics.atom-ph↗
arXiv2022

New Measurement Resolves Key Astrophysical Fe XVII Oscillator Strength Problem

One of the most enduring and intensively studied problems of X-ray astronomy is the disagreement of state-of-the art theory and observations for the intensity ratio of two Fe XVII transitions of crucial value for plasma diagnostics, dubbed 3C and 3D. We unravel this conundrum at the PETRA III synchrotron facility by increasing the resolving power two and a half times and the signal-to-noise ratio thousand-fold compared to our previous work. The Lorentzian wings had hitherto been indistinguishable from the background and were thus not modeled, resulting in a biased line-strength estimation. The present experimental oscillator-strength ratio $R_\mathrm{exp}=f_{\mathrm{3C}}/f_{\mathrm{3D}}=3.51(2)_{\mathrm{stat}}(7)_{\mathrm{sys}}$ agrees with our state-of-the-art calculation of $R_\mathrm{th}=3.55(2)$, as well as with some previous theoretical predictions. To further rule out any uncertainties associated with the measured ratio, we also determined the individual natural linewidths and oscillator strengths of 3C and 3D transitions, which also agree well with the theory. This finally resolves the decades-old mystery of Fe XVII oscillator strengths.

physics.atom-ph↗
arXiv2022

Electron polarization in ultrarelativistic plasma current filamentation instabilities

Plasma current filamentation of an ultrarelativistic electron beam impinging on an overdense plasma is investigated, with emphasis on radiation-induced electron polarization. Particle-in-cell simulations provide the classification and in-depth analysis of three different regimes of the current filaments, namely, the normal filament, abnormal filament, and quenching regimes. We show that electron radiative polarization emerges during the instability along the azimuthal direction in the momentum space, which significantly varies across the regimes. We put forward an intuitive Hamiltonian model to trace the origin of the electron polarization dynamics. In particular, we discern the role of nonlinear transverse motion of plasma filaments, which induces asymmetry in radiative spin flips, yielding an accumulation of electron polarization. Our results break the conventional perception that quasi-symmetric fields are inefficient for generating radiative spin-polarized beams, suggesting the potential of electron polarization as a source of new information on laboratory and astrophysical plasma instabilities.

physics.plasm-ph↗
arXiv2022

High-precision mass measurement of doubly magic $^{208}$Pb

The absolute atomic mass of $^{208}$Pb has been determined with a fractional uncertainty of $7\times 10^{-11}$ by measuring the cyclotron-frequency ratio $R$ of $^{208}$Pb$^{41+}$ to $^{132}$Xe$^{26+}$ with the high-precision Penning-trap mass spectrometer Pentatrap and computing the binding energies $E_{\text{Pb}}$ and $E_{\text{Xe}}$ of the missing 41 and 26 atomic electrons, respectively, with the ab initio fully relativistic multi-configuration Dirac-Hartree-Fock (MCDHF) method. $R$ has been measured with a relative precision of $9\times 10^{-12}$. $E_{\text{Pb}}$ and $E_{\text{Xe}}$ have been computed with an uncertainty of 9.1 eV and 2.1 eV, respectively, yielding $207.976\,650\,571(14)$ u (u$=9.314\,941\,024\,2(28)\times 10^{8}$ eV/c$^2$) for the $^{208}$Pb neutral atomic mass. This result agrees within $1.2σ$ with that from the Atomic-Mass Evaluation (AME) 2020, while improving the precision by almost two orders of magnitude. The new mass value directly improves the mass precision of 14 nuclides in the region of Z=81-84 and is the most precise mass value with A>200. Thus, the measurement establishes a new region of reference mass values which can be used e.g. for precision mass determination of transuranium nuclides, including the superheavies.

nucl-ex↗
arXiv2022

Reconciling conflicting approaches for the tunneling time delay in strong field ionization

Several recent attoclock experiments have investigated the fundamental question of a quantum mechanically induced time delay in tunneling ionization via extremely precise photoelectron momentum spectroscopy. The interpretations of those attoclock experimental results were controversially discussed, because the entanglement of the laser and Coulomb field did not allow for theoretical treatments without undisputed approximations. The method of semiclassical propagation matched with the tunneled wavefunction, the quasistatic Wigner theory, the analytical R-matrix theory, the backpropagation method, and the under-the-barrier recollision theory are the leading conceptual approaches put forward to treat this problem, however, with seemingly conflicting conclusions on the existence of a tunneling time delay. To resolve the contradicting conclusions of the different approaches, we consider a very simple tunneling scenario which is not plagued with complications stemming from the Coulomb potential of the atomic core, avoids consequent controversial approximations and, therefore, allows us to unequivocally identify the origin of the tunneling time delay.

quant-ph↗