arXiv subjects

Christoph H. Keitel

Publications and source records attributed to Christoph H. Keitel.

At least 91 records · Page 5Linked to original sources

arXiv2020

Construction of Dirac spinors for electron vortex beams in background electromagnetic fields

Exact solutions of the Dirac equation, a system of four partial differential equations, are rare. The vast majority of them are for highly symmetric stationary systems. Moreover, only a handful of solutions for time dependent dynamics exists. Given the growing number of applications of high energy electron beams interacting with a variety of quantum systems in laser fields, novel methods for finding exact solutions to the Dirac equation are called for. We present a method for building up solutions to the Dirac equation employing a recently introduced approach for the description of spinorial fields and their driving electromagnetic fields in terms of geometric algebras. We illustrate the method by developing several stationary as well as non-stationary solutions of the Dirac equation with well defined orbital angular momentum along the electron's propagation direction. The first set of solutions describe free electron beams in terms of Bessel functions as well as stationary solutions for both a homogeneous and an inhomogeneous magnetic field. The second set of solutions are new and involve a plane electromagnetic wave combined with a generally inhomogeneous longitudinal magnetic field. Moreover, the developed technique allows us to derive general physical properties of the dynamics in such field configurations, as well as provides physical predictions on the self-consistent electromagnetic fields induced by the dynamics.

quant-ph↗

arXiv2020

Sub-barrier pathways to Freeman resonances

The problem of Freeman resonances [R. R. Freeman \textit{et al.}, Phys. Rev. Lett. \textbf{59}, 1092 (1987)] when strong field ionization is enhanced due to the transient population of excited states during the ionization, is revisited. An intuitive model is put forward which explains the mechanism of the intermediate population of excited states during nonadiabatic tunneling ionization via the under-the-barrier recollision and recombination. The theoretical model is based on perturbative strong-field approximation (SFA), where the sub-barrier bound-continuum-bound pathway is described in the second-order SFA, while the further ionization from the excited state by an additional perturbative step. The enhancement of ionization is shown to arise due to the constructive interference of contributions into the excitation amplitudes originating from different laser cycles. The applied model provides an intuitive understanding of the electron dynamics during a Freeman resonance in strong-field ionization, as well as means of enhancing the process and possible applications to related processes.

physics.atom-ph↗

arXiv2020

A cosmic Zevatron based on cyclotron auto-resonance

A Zevatron is an accelerator scheme envisaged to accelerate particles to ZeV energies (1 ZeV = $10^{21}$ eV). Schemes, most notably the internal shock model, have been proposed to explain the acceleration of ultra-high-energy cosmic-ray (UHECR) particles that have been sporadically detected reaching Earth since 1962. Here, the cyclotron auto-resonance acceleration (CARA) mechanism is tailored and used to demonstrate possible acceleration of particles ejected as a result of violent astrophysical processes such as the merger of a binary system or a supernova explosion. Such events result in emission of highly-energetic particles and ultra-intense beamed radiation. In the simultaneous presence of a super-strong magnetic field, the condition for cyclotron auto-resonance may be met. Thus CARA can act like a {\it booster} for particles pre-accelerated inside their progenitor by shock waves, possibly among other means. As examples, it is shown that nuclei of hydrogen, helium, and iron-56, may reach ZeV energies by CARA, under which conditions the particles, while gyrating around the lines of an ultra-strong magnetic field, also surf on the waves of a super-intense radiation field. When radiation-reaction is taken into account, it is shown that the ZeV energy gained by a particle can fall off by less than an order-of-magnitude if the resonance condition is missed by roughly less than 20\%.

astro-ph.HE↗

arXiv2020

Interrogating the temporal coherence of EUV frequency combs with highly charged ions

A scheme to infer the temporal coherence of EUV frequency combs generated from intra-cavity high-order harmonic generation is put forward. The excitation dynamics of highly charged Mg-like ions, interacting with EUV pulse trains featuring different carrier-envelope-phase fluctuations, are simulated. While demonstrating the microscopic origin of the macroscopic equivalence between excitations induced by pulse trains and continuous-wave lasers, we show that the coherence time of the pulse train can be determined from the spectrum of the excitations. The scheme will provide a verification of the comb temporal coherence at time scales several orders of magnitude longer than current state of the art, and at the same time will enable high-precision spectroscopy of EUV transitions with a relative accuracy up to $δω/ω\sim10^{-17}$.

physics.atom-ph↗

arXiv2020

Ab initio quantum models for thin-film x-ray cavity QED

We develop two ab initio quantum approaches to thin-film x-ray cavity quantum electrodynamics with spectrally narrow x-ray resonances, such as those provided by Mössbauer nuclei. The first method is based on a few-mode description of the cavity, and promotes and extends existing phenomenological few-mode models to an ab initio theory. The second approach uses analytically-known Green's functions to model the system. The two approaches not only enable one to ab initio derive the effective few-level scheme representing the cavity and the nuclei in the low-excitation regime, but also provide a direct avenue for studies at higher excitation, involving non-linear or quantum phenomena. The ab initio character of our approaches further enables direct optimizations of the cavity structure and thus of the photonic environment of the nuclei, to tailor the effective quantum optical level scheme towards particular applications. To illustrate the power of the ab initio approaches, we extend the established quantum optical modeling to resonant cavity layers of arbitrary thickness, which is essential to achieve quantitative agreement for cavities used in recent experiments. Further, we consider multi-layer cavities featuring electromagnetically induced transparency, derive their quantum optical few-level systems ab initio, and identify the origin of discrepancies in the modeling found previously using phenomenological approaches as arising from cavity field gradients across the resonant layers.

quant-ph↗

arXiv2020

High Resolution Photoexcitation Measurements Exacerbate the Long-Standing Fe XVII Oscillator Strength Problem

For more than 40 years, most astrophysical observations and laboratory studies of two key soft x-ray diagnostic $2p-3d$ transitions, $3C$ and $3D$, in Fe XVII ions found oscillator strength ratios $f(3C)/f(3D)$ disagreeing with theory, but uncertainties had precluded definitive statements on this much studied conundrum. Here, we resonantly excite these lines using synchrotron radiation at PETRA III, and reach, at a millionfold lower photon intensities, a 10 times higher spectral resolution, and 3 times smaller uncertainty than earlier work. Our final result of $f(3C)/f(3D) = 3.09(8)(6)$ supports many of the earlier clean astrophysical and laboratory observations, while departing by five sigmas from our own newest large-scale ab initio calculations, and excluding all proposed explanations, including those invoking nonlinear effects and population transfers.

physics.atom-ph↗

arXiv2020

High-energy gamma-photon polarization in nonlinear Breit-Wheeler pair production and gamma-polarimetry

The interaction of an unpolarized electron beam with a counterpropagating ultraintense linearly polarized laser pulse is investigated in the quantum radiation-dominated regime. We employ a semiclassical Monte Carlo method to describe spin-resolved electron dynamics, photon emissions and polarization, and pair production. Abundant high-energy linearly polarized gamma photons are generated intermediately during this interaction via nonlinear Compton scattering, with an average polarization degree of more than 50%, which further interacting with the laser fields produce electron-positron pairs due to nonlinear Breit-Wheeler process. The photon polarization is shown to significantly affect the pair yield by a factor beyond 10%. The considered signature of the photon polarization in the pair's yield can be experimentally identified in a prospective two-stage setup. Moreover, the signature can serve also for the polarimetry of high-energy high-flux gamma photons with a resolution well below 1% with currently achievable laser facilities.

physics.plasm-ph↗

arXiv2020

Skyrme-type nuclear interaction as a tool for calculating the finite nuclear size correction to atomic energy levels and the bound-electron $g$ factor

A state-of-the-art approach for calculating the finite nuclear size correction to atomic energy levels and the bound-electron $g$ factor is introduced and demonstrated for a series of highly charged hydrogen-like ions. Firstly, self-consistent mean-field calculations based on the Skyrme-type nuclear interaction are employed in order to produce a realistic nuclear proton distribution. In the second step, the obtained nuclear charge density is used to construct the potential of an extended nucleus, and the Dirac equation is solved numerically. The ambiguity in the choice of a Skyrme parametrization is supressed by fine-tuning of only one parameter of the Skyrme force in order to accurately reproduce the experimental values of nuclear radii in each particular case. The homogeneously charged sphere approximation, the two-parameter Fermi distribution and experimental nuclear charge distributions are used for comparison with our approach, and the uncertainties of the presented calculations are estimated. In addition, suppression of the finite nuclear size effect for the specific differences of $g$ factors is demonstrated.

physics.atom-ph↗

arXiv2019

Electron acceleration in direct laser-solid interactions far beyond the ponderomotive limit

In laser-solid interactions, electrons may be generated and subsequently accelerated to energies of the order-of-magnitude of the ponderomotive limit, with the underlying process dominated by direct laser acceleration. Breaking this limit, realized here by a radially-polarized laser pulse incident upon a wire target, can be associated with several novel effects. Three-dimensional Particle-In-Cell simulations show a relativistic intense laser pulse can extract electrons from the wire and inject them into the accelerating field. Anti-dephasing, resulting from collective plasma effects, are shown here to enhance the accelerated electron energy by two orders of magnitude compared to the ponderomotive limit. It is demonstrated that ultra-short radially polarized pulses produce super-ponderomotive electrons more efficiently than pulses of the linear and circular polarization varieties.

physics.plasm-ph↗

arXiv2019

X-ray assisted nuclear excitation by electron capture in optical laser-generated plasmas

X-ray assisted nuclear excitation by electron capture (NEEC) into inner-shell atomic holes in a plasma environment generated by strong optical lasers is investigated theoretically. The considered scenario involves the interaction of a strong optical laser with a solid-state nuclear target leading to the generation of a plasma. In addition, intense x-ray radiation from an X-ray Free Electron Laser (XFEL) produces inner-shell holes in the plasma ions, into which NEEC may occur. As case study we consider the $4.85$-keV transition starting from the 2.4 MeV long-lived $^{\mathrm{93m}}$Mo isomer that can be used to release the energy stored in this metastable nuclear state. We find that the recombination into $2p_{1/2}$ inner-shell holes is most efficient in driving the nuclear transition. Already at few hundred eV plasma temperature, the generation of inner-shell holes can allow optimal conditions for NEEC, otherwise reached for steady-state plasma conditions in thermodynamical equilibrium only at few keV. The combination of x-ray and optical lasers presents two advantages: first, NEEC rates can be maximized at plasma temperatures where the photoexcitation rate remains low. Second, with mJ-class optical lasers and an XFEL repetition rate of $10$ kHz, the NEEC excitation number can reach $\sim 1$ depleted isomer per second and is competitive with scenarios recently envisaged at petawatt-class lasers.

physics.plasm-ph↗

arXiv2019

Polarized ultrashort brilliant multi-GeV $γ$-rays via single-shot laser-electron interaction

Generation of circularly-polarized (CP) and linearly-polarized (LP) $γ$-rays via the single-shot interaction of an ultraintense laser pulse with a spin-polarized counterpropagating ultrarelativistic electron beam has been investigated in nonlinear Compton scattering in the quantum radiation-dominated regime. For the process simulation a Monte Carlo method is developed which employs the electron-spin-resolved probabilities for polarized photon emissions. We show efficient ways for the transfer of the electron polarization to the high-energy photon polarization. In particular, multi-GeV CP (LP) $γ$-rays with polarization of up to about 95\% can be generated by a longitudinally (transversely) spin-polarized electron beam, with a photon flux at a single shot meeting the requirements of recent proposals for the vacuum birefringence measurement in ultrastrong laser fields. Such high-energy, high-brilliance, high-polarization $γ$-rays are also beneficial for other applications in high-energy physics, nuclear physics, and laboratory astrophysics.

physics.plasm-ph↗

arXiv2019

Roadmap on STIRAP applications

STIRAP (Stimulated Raman Adiabatic Passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of population between quantum states. A particularly interesting feature is the fact that the coupling between the initial and the final quantum states is via an intermediate state even though the lifetime of the latter can be much shorter than the interaction time with the laser radiation. Nevertheless, spontaneous emission from the intermediate state is prevented by quantum interference. Maintaining the coherence between the initial and final state throughout the transfer process is crucial. STIRAP was initially developed with applications in chemical dynamics in mind. That is why the original paper of 1990 was published in The Journal of Chemical Physics. However, as of about the year 2000, the unique capabilities of STIRAP and its robustness with respect to small variations of some experimental parameters stimulated many researchers to apply the scheme in a variety of other fields of physics. The successes of these efforts are documented in this collection of articles.

quant-ph↗

arXiv2019

Collisionless shocks in laboratory astrophysics experiments

Influence of the plasma collisions on the laser-driven collisionless shock formation and subsequent ion acceleration is studied on the basis of two different collisional algorithms and their implementations in two well-known particle-in-cell codes EPOCH and SMILEI. In this setup, an ultra-intense incident laser pulse generates hot-electrons in a thick target, launching an electrostatic shock at the laser-plasma interface while also pushing the interface through the hole-boring effect. We observe, to varying degrees, the weakening of the space-charge effects due to collisions and improvements ($\ge 10\%$) in the energy spectra of quasi-monoenergetic ions in both PIC codes EPOCH and SMILEI. These results establish the `collisionlessness' of the collisionless shocks in laboratory astrophysics experiments.

physics.plasm-ph↗

arXiv2019

Holographic interferences in strong-field ionization beyond the dipole approximation: The influence of the peak and focal volume averaged laser intensity

In strong-field ionization interferences between electron trajectories create a variety of interference structures in the final momentum distributions. Among them, the interferences between electron pathways that are driven directly to the detector and the ones that rescatter significantly with the parent ion lead to holography-type interference patterns that received great attention in recent years. In this work, we study the influence of the magnetic field component onto the holographic interference pattern, an effect beyond the electric dipole approximation, in experiment and theory. The experimentally observed nondipole signatures are analyzed via quantum trajectory Monte Carlo simulations. We provide explanations for the experimentally demonstrated asymmetry in the holographic interference pattern and its non-uniform photoelectron energy dependence as well as for the variation of the topology of the holography-type interference pattern along the laser field direction. Analytical scaling laws of the interference features are derived, and their direct relation to either the focal volume averaged laser intensities, or to the peak intensities are identified. The latter, in particular, provides a direct access to the peak intensity in the focal volume.

physics.atom-ph↗

arXiv2019

$^{93m}$Mo isomer depletion via beam-based nuclear excitation by electron capture

A recent nuclear physics experiment [C. J. Chiara {\it et al.}, Nature (London) {\bf 554}, 216 (2018)] reports the first direct observation of nuclear excitation by electron capture (NEEC) in the depletion of the $^{93m}$Mo isomer. The experiment used a beam-based setup in which Mo highly charged ions with nuclei in the isomeric state $^{93m}$Mo at 2.4 MeV excitation energy were slowed down in a solid-state target. In this process, nuclear excitation to a higher triggering level led to isomer depletion. The reported excitation probability $P_{\rm{exc}} = 0.01$ was solely attributed to the so-far unobserved process of NEEC in lack of a different known channel of comparable efficiency. In this work, we investigate theoretically the beam-based setup and calculate excitation rates via NEEC using state-of-the-art atomic structure and ion stopping power models. For all scenarios, our results disagree with the experimental data by approximately nine orders of magnitude. This stands in conflict with the conclusion that NEEC was the excitation mechanism behind the observed depletion rate.

nucl-th↗

arXiv2019

Ultrarelativistic polarized positron jets via collision of electron and ultraintense laser beams

Relativistic spin-polarized positron beams are indispensable for future electron-positron colliders to test modern high-energy physics theory with high precision. However, present techniques require very large scale facilities for those experiments. We put forward a novel efficient way for generating ultrarelativistic polarized positron beams employing currently available laser fields. For this purpose the generation of polarized positrons via multiphoton Breit-Wheeler pair production and the associated spin dynamics in single-shot interaction of an ultraintense laser pulse with an ultrarelativistic electron beam is investigated in the quantum radiation-dominated regime. A specifically tailored small ellipticity of the laser field is shown to promote splitting of the polarized particles along the minor axis of laser polarization into two oppositely polarized beams. In spite of radiative de-polarization, a dense positron beam with up to about 90\% polarization can be generated in tens of femtoseconds. The method may eventually usher high-energy physics studies into smaller-scale laser laboratories.

physics.plasm-ph↗

arXiv2019

Polarized laser-wakefield-accelerated kiloampere electron beams

High-flux polarized particle beams are of critical importance for the investigation of spin-dependent processes, such as in searches of physics beyond the Standard Model, as well as for scrutinizing the structure of solids and surfaces in material science. Here we demonstrate that kiloampere polarized electron beams can be produced via laser-wakefield acceleration from a gas target. A simple theoretical model for determining the electron beam polarization is presented and supported with self-consistent three-dimensional particle-in-cell simulations that incorporate the spin dynamics. By appropriately choosing the laser and gas parameters, we show that the depolarization of electrons induced by the laser-wakefield-acceleration process can be as low as 10%. Compared to currently available sources of polarized electron beams, the flux is increased by four orders of magnitude.

physics.plasm-ph↗

arXiv2019

Polarized positron beams via intense two-color laser pulses

Generation of ultrarelativistic polarized positrons during interaction of an ultrarelativistic electron beam with a counterpropagating two-color petawatt laser pulse is investigated theoretically. Our Monte Carlo simulation based on a semi-classical model, incorporates photon emissions and pair productions, using spin-resolved quantum probabilities in the local constant field approximation, and describes the polarization of electrons and positrons for the pair production and photon emission processes, as well as the classical spin precession in-between. The main reason of the polarization is shown to be the spin-asymmetry of the pair production process in strong external fields, combined with the asymmetry of the two-color laser field. Employing a feasible scenario, we show that highly polarized positron beams, with a polarization degree of $ζ\approx 60\%$, can be produced in a femtosecond time scale, with a small angular divergence, $\sim 74$ mrad, and high density $\sim 10^{14}$ cm$^{-3}$. The laser-driven positron source, along with laser wakefield acceleration, may pave the way to small scale facilities for high energy physics studies.

physics.plasm-ph↗