arXiv subjects

Christoph Hotter

Publications and source records attributed to Christoph Hotter.

17 recordsLinked to original sources

arXiv2026

Input-Output Analysis of Quantum Dot SUPER Excitation

The Swing-UP of the quantum EmitteR population (SUPER) two-color pulsed excitation scheme allows for robust and close to 100\% excitation of a two-level quantum emitter using only red detuned light. We analyze the underlying counterintuitive dynamics using a full quantum input-output description of the in- and outgoing light pulses for the case of two coherent free-space input pulses at realistic photon numbers. At the microscopic level, the SUPER mechanism exhibits its nonlinear three-photon Raman-type character, leading to a net photon-number change of $-2$ in one mode and $+1$ in the other, as was first guessed from cavity-enhanced model descriptions at low photon numbers. We confirm that in free space, a sufficiently high pulse photon number, much larger than one, is required to achieve high-fidelity inversion. To treat the large coherent-state amplitudes (photon numbers) relevant for SUPER, we extend the quantum input-output formalism to include a cumulant expansion approach. With an interaction-picture formulation, the few exchanged photons that govern the nontrivial dynamics enable direct full-quantum calculations in truncated Hilbert spaces, including treatments in a displacement frame and for initial Fock-state pulses.

quant-ph↗

arXiv2026

Realization of waveguide many-body quantum optics

Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.

quant-ph↗

arXiv2025

A Quantum Non-Gaussianity Criterion Based on Photon Correlations $g^{(2)}$ and $g^{(3)}$

Quantum non-Gaussian states, which cannot be written as mixtures of Gaussian states, are necessary to achieve a quantum advantage in continuous variable systems. They represent an important benchmark for the realization of an advanced quantum light source, as they cannot be made by simple means such as displacement and squeezing. We introduce an attenuation-resistant sufficient criterion for quantum non-Gaussian states based on the second- and third-order correlation functions, $g^{(2)}$ and $g^{(3)}$. The general non-linear bound for classical mixtures of Gaussian states is $\sqrt{g^{(3)}} + 3 \sqrt{g^{(2)}} \geq 2$. Any mixture of Gaussian states must fulfill this inequality, thus, the violation of it represents a direct confirmation of quantum non-Gaussianity. We experimentally show the non-Gaussianity of the state produced by a quantum dot single-photon source, where we obtain $\sqrt{g^{(3)}} + 3 \sqrt{g^{(2)}} = 0.174 (13)$, which represents a statistical significance of more than $100$ standard deviations.

quant-ph↗

arXiv2025

Lieb-Mattis states for robust entangled differential phase sensing

We explore a two-node, entanglement-enhanced sensor network for differential phase sensing that exploits decoherence-free subspaces to suppress common-mode noise, a primary limitation of many state-of-the-art quantum sensors. We identify a class of entangled states that, while not strictly optimal, achieve the same asymptotic sensitivity scaling as optimal states and can be prepared efficiently from initially unentangled atomic ensembles. Importantly, the preparation time decreases with increasing system size. This makes the states compatible with realistic noise processes in present-day quantum sensors that operate with large particle numbers but lack full error correction. We illustrate these ideas using two cavity-mediated preparation protocols: (i) coherent, unitary entanglement generation analogous to bosonic two-mode squeezing, yielding Heisenberg scaling; and (ii) dissipative preparation via collective emission into a shared cavity mode, providing a square-root improvement beyond the standard quantum limit. Numerical simulations show that both approaches remain effective at experimentally realistic cavity cooperativities, establishing a practical path toward scalable, quantum-enhanced differential phase sensing.

quant-ph↗

arXiv2025

Quantum Metrology in the Ultrastrong Coupling Regime of Light-Matter Interactions: Leveraging Virtual Excitations without Extracting Them

Virtual excitations, inherent to ultrastrongly coupled light-matter systems, induce measurable modifications in system properties, offering a novel resource for quantum technologies. In this work, we demonstrate how these virtual excitations and their correlations can be harnessed to enhance precision measurements, without the need to extract them. Building on the paradigmatic Dicke model, which describes the interaction between an ensemble of two-level atoms and a single radiation mode, we propose a method to harness hybridized light-matter modes whose renormalized frequencies encode the effects of virtual excitations for quantum metrology. Remarkably, we find that for a fixed squeezing parameter $\xi$, exploiting virtual squeezing through oscillator frequency shifts yields a quadratic enhancement in estimation precision -- scaling as $\exp(4\xi)$ -- compared to the conventional $\exp(2\xi)$ scaling of real squeezed states. These results show that virtual excitations, though unobservable, can drive metrological performance beyond the standard quantum limit. Our approach establishes a broadly applicable framework for high-precision measurements across a wide class of ultrastrongly coupled quantum systems.

quant-ph↗

arXiv2024

Conditional Entanglement Amplification via Non-Hermitian Superradiant Dynamics

Due to the inherently probabilistic nature of quantum mechanics, each experimental realization of a dynamical quantum system may yield a different measurement outcome, especially when the system is coupled to an environment that causes dissipation. Although it is in principle possible that some quantum trajectories lead to exotic highly entangled quantum states, the probability of observing these trajectories is usually extremely low. In this work, we show how to maximize the probability of generating highly entangled states, including maximally entangled cat states, in an ensemble of atoms experiencing superradiant decay. To this end, we analyze an effective non-Hermitian Hamiltonian which governs the dynamics between the quantum jumps associated with photon emission. A key result of our study is that, in order to maximally enhance the probability of cat state generation, the initial state needs to be non-classical. This can be achieved e.g. with one-axis twisting in a cavity-QED system.

quant-ph↗

arXiv2024

Subradiance and Superradiant Long Range Excitation Transport among Quantum Emitter Ensembles in a Waveguide

In contrast to free space, in waveguides the dispersive and dissipative dipole-dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport amongst far-apart ensembles coupled to a waveguide. For sufficiently large ensembles collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that for a large number of emitters a fast transverse coherent pulse can create almost perfect subradiant states with up to $50\%$ excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of $50\%$ we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states as well as the superradiant excitation transfer appear as suitable building blocks in applications like active atomic clocks, quantum batteries, quantum information protocols and quantum metrology procedures such as fiber-based Ramsey schemes.

quant-ph↗

arXiv2024

Combining critical and quantum metrology

Critical metrology relies on the precise preparation of a system in its ground state near a quantum phase transition point where quantum correlations get very strong. Typically this increases the quantum Fisher information with respect to changes in system parameters and thus improves the optimally possible measurement precision limited by the Cramér-Rao bound. Hence critical metrology involves encoding information about the unknown parameter in changes of the system's ground state. Conversely, in conventional metrology methods like Ramsey interferometry, the eigenstates of the system remain unchanged, and information about the unknown parameter is encoded in the relative phases that excited system states accumulate during their time evolution. Here we introduce an approach combining these two methodologies into a unified protocol applicable to closed and driven-dissipative systems. We show that the quantum Fisher information in this case exhibits an additional interference term originating from the interplay between eigenstate and relative phase changes. We provide analytical expressions for the quantum and classical Fisher information in such a setup, elucidating as well a straightforward measurement approach that nearly attains the maximum precision permissible under the Cramér-Rao bound. We showcase these results by focusing on the squeezing Hamiltonian, which characterizes the thermodynamic limit of Dicke and Lipkin-Meshkov-Glick Hamiltonians.

quant-ph↗

arXiv2024

Unique Steady-State Squeezing in a Driven Quantum Rabi Model

Squeezing is essential to many quantum technologies and our understanding of quantum physics. Here we develop a theory of steady-state squeezing that can be generated in the closed and open quantum Rabi as well as Dicke model. To this end, we eliminate the spin dynamics which effectively leads to an abstract harmonic oscillator whose eigenstates are squeezed with respect to the physical harmonic oscillator. The generated form of squeezing has the unique property of time-independent uncertainties and squeezed dynamics, a novel type of quantum behavior. Such squeezing might find applications in continuous back-action evading measurements and should already be observable in optomechanical systems and Coulomb crystals.

quant-ph↗

arXiv2023

Threshold studies for a hot beam superradiant laser including an atomic guiding potential

Recent theoretical predictions hint at an implementation of a superradiant laser based on narrow optical clock transitions by using a filtered thermal beam at high density. Corresponding numerical studies give encouraging results but the required very high densities are sensitive to beam collimation errors and inhomogeneous shifts. Here we present extensive numerical studies of threshold conditions and the predicted output power of such a superradiant laser involving realistic particle numbers and velocities along the cavity axis. Detailed studies target the threshold scaling as a function of temperature as well as the influence of eliminating the hottest part of the atomic distribution via velocity filtering and the benefits of additional atomic beam guiding. Using a cumulant expansion approach allows us to quantify the significance of atom-atom and atom-field correlations in such configurations. We predict necessary conditions to achieve a certain threshold photon number depending on the atomic temperature and density. In particular, we show that the temperature threshold can be significantly increased by using more atoms. Interestingly, a velocity filter removing very fast atoms has only almost negligible influence despite their phase perturbing properties. On the positive side an additional conservative optical guiding towards cavity mode antinodes leads to significantly lower threshold and higher average photon number. Interestingly we see that higher order atom-field and direct atom-atom quantum correlations play only a minor role in the laser dynamics, which is a bit surprising in the superradiant regime.

physics.atom-ph↗

arXiv2023

Collectively enhanced Ramsey readout by cavity sub- to superradiant transition

When an inverted ensemble of atoms is tightly packed on the scale of its emission wavelength or when the atoms are collectively strongly coupled to a single cavity mode, their dipoles will align and decay rapidly via a superradiant burst. However, a spread-out dipole phase distribution theory predicts a required minimum threshold of atomic excitation for superradiance to occur. Here we experimentally confirm this predicted threshold for superradiant emission on a narrow optical transition when exciting the atoms transversely and show how to take advantage of the resulting sub- to superradiant transition. A $π/2$-pulse places the atoms in a subradiant state, protected from collective cavity decay, which we exploit during the free evolution period in a corresponding Ramsey pulse sequence. The final excited state population is read out via superradiant emission from the inverted atomic ensemble after a second $π/2$-pulse, and with minimal heating this allows for multiple Ramsey sequences within one experimental cycle. Our scheme is a fundamentally new approach to atomic state readout characterized by its speed, simplicity, and high sensitivity. It demonstrates the potential of sensors using collective effects in cavity-coupled quantum emitters.

quant-ph↗

arXiv2022

Cavity Sub- and Superradiance Enhanced Ramsey Spectroscopy

Ramsey spectroscopy in large, dense ensembles of ultra-cold atoms trapped in optical lattices suffers from dipole-dipole interaction induced shifts and collective superradiance limiting its precision and accuracy. We propose a novel geometry implementing fast signal readout with minimal heating for large atom numbers at lower densities via an optical cavity operated in the weak single atom but strong collective coupling regime. The key idea is controlled collective transverse $\pi/2$-excitation of the atoms to prepare a macroscopic collective spin protected from cavity superradiance. This requires that the two halves of the atomic ensemble are coupled to the cavity mode with opposite phase, which is naturally realized for a homogeneously filled volume covering odd and even sites of the cavity mode along the cavity axis. The origin of the superior precision can be traced back to destructive interference among sub-ensembles in the complex nonlinear collective atom field dynamics. In the same configuration we find surprising regular self-pulsing of the cavity output for suitable continuous illumination. Our simulations for large atom numbers employing a cumulant expansion are qualitatively confirmed by a full quantum treatment of smaller ensembles.

cond-mat.quant-gas↗

arXiv2021

QuantumCumulants.jl: A Julia framework for generalized mean-field equations in open quantum systems

A full quantum mechanical treatment of open quantum systems via a Master equation is often limited by the size of the underlying Hilbert space. As an alternative, the dynamics can also be formulated in terms of systems of coupled differential equations for operators in the Heisenberg picture. This typically leads to an infinite hierarchy of equations for products of operators. A well-established approach to truncate this infinite set at the level of expectation values is to neglect quantum correlations of high order. This is systematically realized with a so-called cumulant expansion, which decomposes expectation values of operator products into products of a given lower order, leading to a closed set of equations. Here we present an open-source framework that fully automizes this approach: first, the equations of motion of operators up to a desired order are derived symbolically using predefined canonical commutation relations. Next, the resulting equations for the expectation values are expanded employing the cumulant expansion approach, where moments up to a chosen order specified by the user are included. Finally, a numerical solution can be directly obtained from the symbolic equations. After reviewing the theory we present the framework and showcase its usefulness in a few example problems.

quant-ph↗

arXiv2021

Superradiant lasing in inhomogeneously broadened ensembles with spatially varying coupling

Theoretical studies of superradiant lasing on optical clock transitions predict a superb frequency accuracy and precision closely tied to the bare atomic linewidth. Such a superradiant laser is also robust against cavity fluctuations when the spectral width of the lasing mode is much larger than that of the atomic medium. Recent predictions suggest that this unique feature persists even for a hot and thus strongly broadened ensemble, provided the effective atom number is large enough. Here we use a second-order cumulant expansion approach to study the power, linewidth and lineshifts of such a superradiant laser as a function of the inhomogeneous width of the ensemble including variations of the spatial atom-field coupling within the resonator. We present conditions on the atom numbers, the pump and coupling strengths required to reach the buildup of collective atomic coherence as well as scaling and limitations for the achievable laser linewidth.

quant-ph↗

arXiv2021

Continuous multi-step pumping of the optical clock transition in alkaline-earth atoms with minimal perturbation

A suitable scheme to continuously create inversion on an optical clock transition with negligible perturbation is a key missing ingredient required to build an active optical atomic clock. Re- pumping of the atoms on the narrow transition typically needs several pump lasers in a multi step process involving several auxiliary levels. In general this creates large effective level shifts and a line broadening, strongly limiting clock accuracy. Here we present an extensive theoretical study for a realistic multi-level implementation in search of parameter regimes where a sufficient inversion can be achieved with minimal perturbations. Fortunately we are able to identify a useful operating regime, where the frequency shifts remain small and controllable, only weakly perturbing the clock transition for useful pumping rates. For practical estimates of the corresponding clock performance we introduce a straightforward mapping of the multilevel pump scheme to an effective energy shift and broadening parameters for the reduced two-level laser model system. This allows to evaluate the resulting laser power and spectrum using well-known methods.

quant-ph↗

arXiv2021

Continuous narrowband lasing with coherently driven V-level atoms

Simultaneous strong coherent pumping of the two transitions of a V-level atom with very differentdecay rates has been predicted to create almost perfect inversion on the narrower transition. Usingthe example of the blue and red transitions in Strontium we show that for suitable operatingconditions the corresponding resonant gain can be used to continuously operate a laser on thenarrow transition. In particular, for a strong detuning of the pump field with respect to the narrowtransition, coherent laser emission occurs close to the bare atomic transition frequency exhibitingonly a negligible contribution from coherent pump light scattered into the lasing mode.Calculations of the cavity output spectrum show that the resulting laser linewidth can get muchsmaller than the bandwidth of the pump light and even the natural linewidth of the narrow atomictransition. Its frequency is closely tied to the atomic transition frequency for properly chosen atomnumbers. Simulations including atomic motionshow Doppler cooling on the strong transitionwith minor motion heating on the lasing transition, so that continuous laser operation in thepresence of a magneto-optical trap should be possible with current experimental technology.

quant-ph↗

arXiv2019

Superradiant Cooling, Trapping, and Lasing of Dipole-Interacting Clock Atoms

A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such a configuration using a semiclassical description of particle motion along the cavity axis. In extension of earlier work we include free space atomic and cavity decay as well as atomic dipole-dipole interactions and their corresponding forces. We show that for a proper choice of parameters even in the bad cavity limit the atoms can create a sufficiently strong field inside the resonator such that they are trapped and cooled via the superradiant lasing action with less than one photon on average inside the cavity.

quant-ph↗