arXiv subjects

Christoph Kurz

Publications and source records attributed to Christoph Kurz.

10 recordsLinked to original sources

arXiv2019

Precision frequency-comb terahertz spectroscopy on pure quantum states of a single molecular ion

Spectroscopy is a powerful tool for studying molecules and is commonly performed on large thermal molecular ensembles that are perturbed by motional shifts and interactions with the environment and one another, resulting in convoluted spectra and limited resolution. Here, we use generally applicable quantum-logic techniques to prepare a trapped molecular ion in a single quantum state, drive terahertz rotational transitions with an optical frequency comb, and read out the final state non-destructively, leaving the molecule ready for further manipulation. We resolve rotational transitions to 11 significant digits and derive the rotational constant of CaH+ to be B_R = 142501777.9(1.7) kHz. Our approach suits a wide range of molecular ions, including polyatomics and species relevant for tests of fundamental physics, chemistry, and astrophysics.

physics.atom-ph↗

arXiv2017

Subgroup Identification and Interpretation with Bayesian Nonparametric Models in Health Care Claims Data

Inpatient care is a large share of total health care spending, making analysis of inpatient utilization patterns an important part of understanding what drives health care spending growth. Common features of inpatient utilization measures include zero inflation, over-dispersion, and skewness, all of which complicate statistical modeling. Mixture modeling is a popular approach that can accommodate these features of health care utilization data. In this work, we add a nonparametric clustering component to such models. Our fully Bayesian model framework allows for an unknown number of mixing components, so that the data determine the number of mixture components. When we apply the modeling framework to data on hospital lengths of stay for patients with lung cancer, we find distinct subgroups of patients with differences in means and variances of hospital days, health and treatment covariates, and relationships between covariates and length of stay.

stat.ML↗

arXiv2017

Preparation and coherent manipulation of pure quantum states of a single molecular ion

Laser cooling and trapping of atoms and atomic ions has led to numerous advances including the observation of exotic phases of matter, development of exquisite sensors and state-of-the-art atomic clocks. The same level of control in molecules could also lead to profound developments such as controlled chemical reactions and sensitive probes of fundamental theories, but the vibrational and rotational degrees of freedom in molecules pose a formidable challenge for controlling their quantum mechanical states. Here, we use quantum-logic spectroscopy (QLS) for preparation and nondestructive detection of quantum mechanical states in molecular ions. We develop a general technique to enable optical pumping and preparation of the molecule into a pure initial state. This allows for the observation of high-resolution spectra in a single ion (here CaH+) and coherent phenomena such as Rabi flopping and Ramsey fringes. The protocol requires a single, far-off resonant laser, which is not specific to the molecule, so that many other molecular ions, including polyatomic species, could be treated with the same methods in the same apparatus by changing the molecular source. Combined with long interrogation times afforded by ion traps, a broad range of molecular ions could be studied with unprecedented control and precision, representing a critical step towards proposed applications, such as precision molecular spectroscopy, stringent tests of fundamental physics, quantum computing, and precision control of molecular dynamics.

physics.atom-ph↗

arXiv2016

Survival Prediction with Limited Features: a Top Performing Approach from the DREAM ALS Stratification Prize4Life Challenge

Survival prediction with small sets of features is a highly relevant topic for decision-making in clinical practice. I describe a method for predicting survival of amyotrophic lateral sclerosis (ALS) patients that was developed as a submission to the DREAM ALS Stratification Prize4Life Challenge held in summer 2015 to find the most accurate prediction of ALS progression and survival. ALS is a neurodegenerative disease with very heterogeneous survival times. Based on patient data from two national registries, solvers were asked to predict survival for three different time intervals, which was then evaluated on undisclosed information from additional data. I describe methods used to generate new features from existing ones from longitudinal data, selecting the most predictive features, and developing the best survival model. I show that easily obtainable engineered features can significantly improve prediction and could be incorporated into clinical practice. Furthermore, my prediction model confirms previous reports suggesting that past disease progression measured by the ALSFRS (ALS functional rating scale score), time since disease onset, onset site, and age are strong predictors for survival. Regarding prediction accuracy, this approach ranked second.

stat.AP↗

arXiv2016

Tweedie distributions for fitting semicontinuous health care utilization cost data

We explore a statistical distribution that can simultaneously model the probability of zero outcome for non-users of health care utilization and continuous costs for users. We compare this distribution to other com- monly used models on example data and show that it fits cost data well and has some appealing properties that provide flexible use.

stat.AP↗

arXiv2016

Programmable atom-photon quantum interface

We present the implementation of a programmable atom-photon quantum interface, employing a single trapped $^{40}$Ca$^+$ ion and single photons. Depending on its mode of operation, the interface serves as a bi-directional atom-photon quantum-state converter, as a source of entangled atom-photon states, or as a quantum frequency converter of single photons. The interface lends itself particularly to interfacing ions with single or entangled photons in hybrid quantum networks.

quant-ph↗

arXiv2014

Experimental protocol for high-fidelity heralded photon-to-atom quantum state transfer

A quantum network combines the benefits of quantum systems regarding secure information transmission and calculational speed-up by employing quantum coherence and entanglement to store, transmit, and process information. A promising platform for implementing such a network are atom-based quantum memories and processors, interconnected by photonic quantum channels. A crucial building block in this scenario is the conversion of quantum states between single photons and single atoms through controlled emission and absorption. Here we present an experimental protocol for photon-to-atom quantum state conversion, whereby the polarization state of an absorbed photon is mapped onto the spin state of a single absorbing atom with >95% fidelity, while successful conversion is heralded by a single emitted photon. Heralded high-fidelity conversion without affecting the converted state is a main experimental challenge, in order to make the transferred information reliably available for further operations. We record >80/s successful state transfer events out of 18,000/s repetitions.

quant-ph↗

arXiv2014

Quantum interference in the absorption and emission of single photons by a single ion

We investigate quantum beats in the arrival-time distribution of single photons from a single trapped $^{40}$Ca$^+$ ion, revealing their fundamentally different physical origins in two distinct experimental situations: In a $Λ$-type level scheme the interference of two 854-nm absorption amplitudes suppresses and enhances the emission process of Raman-scattered 393-nm photons; in a V-type level scheme the interference of two 393-nm emission amplitudes causes a rotation of their dipole emission pattern resulting in a temporal modulation of the detected photons. For both cases we demonstrate coherent control over the quantum-beat phase through the phases of the atomic and photonic input states, which also allows controlled adjustment of the total photon detection efficiency.

quant-ph↗

arXiv2013

Heralded photonic interaction between distant single ions

We establish heralded interaction between two remotely trapped single 40Ca+ ions through the exchange of single photons. In the sender ion, we release single photons with controlled temporal shape on the P_3/2 to D_5/2 transition and transmit them to the distant receiver ion. Individual absorption events in the receiver ion are detected by quantum jumps. For continuously generated photons, the absorption reduces significantly the lifetime of the long-lived D_5/2 state. For triggered single-photon transmission, we observe coincidence between the emission at the sender and quantum jump events at the receiver.

quant-ph↗

arXiv2012

A high-rate source for single photons in a pure quantum state

We report on the efficient generation of single photons, making use of spontaneous Raman scattering in a single trapped ion. The photons are collected through in-vacuum high-NA objectives. Photon frequency, polarization and temporal shape are controlled through appropriate laser parameters, allowing for photons in a pure quantum state.

quant-ph↗