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Christophe Raufaste

Publications and source records attributed to Christophe Raufaste.

At least 19 recordsLinked to original sources

Quantifying the liquid flow between a soap film and a vertical meniscus

Fluid exchange between a soap film and its bounding menisci governs film drainage and stability, with direct implications for the lifetime of surface bubbles and liquid foams. Despite recent advances, a quantitative characterization of this coupling, associated with the phenomenon of marginal regeneration, remains incomplete. The volumetric flux per unit length of contact follows a well-established scaling law involving geometrical parameters such as the film height and the meniscus radius of curvature. However, the dimensionless prefactor of this relation - the flux coefficient - remains difficult to determine for vertical menisci because of the complex and intermittent flows occurring at the film-meniscus interface. Here, we quantify this flux into the meniscus generated by inserting a solid plate into a vertical soap film. We consider both vertical and inclined plates and further investigate the effects of plate inclination, height, and width. Focusing on the dynamics of the growth of the meniscus driven by liquid supplied by the film, we analyze both steady and transient regimes resulting from the interplay between capillary pressure, gravity, and liquid exchange. Combining experiments, numerical simulations, and theoretical modelling, we determine the flux coefficient using three independent methods and show that it remains constant over the range of parameters explored.

physics.flu-dyn

Soap Film Drainage Using a Centrifugal Thin Film Balance

Surface bubbles are an abundant source of aerosols, with important implications for climate processes. In this context, we investigate the stability and thinning dynamics of soap films under effective gravity fields. Experiments are performed using a centrifugal thin-film balance capable of generating accelerations from 0.2 up to 100 times standard gravity, combined with thin-film interferometry to obtain time-resolved thickness maps. Across all experimental conditions, the drainage dynamics are shown to be governed by capillary suction and marginal regeneration-a mechanism in which thick regions of the film are continuously replaced by thin film elements (TFEs) formed at the meniscus. We consistently recover a thickness ratio of 0.8-0.9 between the TFEs and the adjacent film, in agreement with previous observations under standard gravity. The measured thinning rates also follow the predicted scaling laws. We identified that effective gravity has three distinct effects: (i) it induces a strong stretching of the initial film, extending well beyond the linear-elastic regime; (ii) it controls the meniscus size, and thereby the amplitude of the capillary suction and the drainage rate; and (iii) it reveals an inertia-to-viscous transition in the motion of TFEs within the film. These results are supported by theoretical modeling and highlight the robustness of marginal regeneration and capillary-driven drainage under extreme gravity conditions.

physics.flu-dyn

Flowing menisci: coupled dynamics and liquid exchange with soap films

Liquid foams exhibit menisci whose lengths range from hundreds of microns in microfoams to several centimeters in macroscopic bubble arrangements. These menisci thin under gravity until reaching a steady thickness profile, where hydrostatic and capillary pressures are balanced. While these menisci are in contact with soap films, dynamical liquid exchanges between them are neglected in current drainage models, which assume thin films provide a negligible liquid reservoir. Using controlled experiments, we systematically measure the shape of an isolated meniscus placed in a vertical soap film. By increasing the film thickness, we identify a flowing regime in which the flux from the adjacent film significantly enlarges the meniscus. We present an analytical model that extends the drainage equation to incorporate this film flux and introduce a gravito-exchange length, which sets the minimum meniscus thickness. The model is in quantitative agreement with experiments, capturing the transition between hydrostatic and flowing menisci. This study has implications for flowing or rearranging foams, where thick films are commonly observed.

cond-mat.soft

Undulatory underwater swimming: Linking vortex dynamics, thrust, and wake structure with a biorobotic fish

Flapping-based propulsive systems rely on fluid-structure interactions to produce thrust. At intermediate and high Reynolds numbers, vortex formation and organization in the wake of such systems are crucial for the generation of a propulsive force. In this work, we experimentally investigate the wake produced by a tethered robotic fish immersed in a water tunnel. By systematically varying the amplitude and frequency of the fish tail as well as the free-stream speed, we are able to observe and characterize different vortex streets as a function of the Strouhal number. The produced wakes are three-dimensional and exhibit a classical V-shape, mainly with two oblique trains of vortex rings convecting outward. Using two-dimensional Particle Image Velocimetry (PIV) in the mid-span plane behind the fish and through extensive data processing of the velocity and vorticity fields, we demonstrate the strong couplings at place between vortex dynamics, thrust production and wake structure. We first measure the evolution of the vortex velocity with the Strouhal number, and model it using a momentum balance equation directly related to thrust production. We then focus on the wake structure, such as wake angle as well as vortex ring orientation, diameter and vorticity. The wake structure is modelled in a simple geometrical framework where the vortex ring velocity is composed of the free-stream speed and the ring self-advecting speed. This framework is tested and validated by our experimental measurements as well as literature data collapsing on master curves, highlighting a universal behavior dominated by the Strouhal number. This allows us to establish a comprehensive understanding of how the wake structure varies with this number and, thus, thrust production.

physics.flu-dyn

Multiscale stress dynamics in sheared liquid foams revealed by tomo-rheoscopy

Rheology aims at quantifying the response of materials to mechanical forcing. However, standard rheometers provide only global macroscopic quantities, such as viscoelastic moduli. They fail to capture the heterogeneous flow of soft amorphous materials at the mesoscopic scale, arising from the rearrangements of the microstructural elements, that must be accounted for to build predictive models. To address this experimental challenge, we have combined shear rheometry and time-resolved X-ray micro-tomography on 3D liquid foams used as model glassy materials, yielding a unique access to the stresses and contact network topology at the bubble scale. We reveal a universal scaling behavior of the local stress build-up and relaxation associated with topological modifications. Moreover, these plastic events redistribute stress non-locally, as if the foam were an elastic medium subjected to a quadrupolar deformation. Our findings clarify how the macroscopic elastoplastic behavior of amorphous materials emerges from the spatiotemporal stress variations induced by microstructural rearrangements.

cond-mat.soft

Self-similar and Universal Dynamics in Drainage of Mobile Soap Films

Vertical soap films drain under the influence of gravity, as indicated by the downward motion of colorful horizontal interference fringes observed on their surfaces. In this study conducted with rectangular soap films, we experimentally characterize the descent dynamics of these isothickness fringes and report its self-similar nature. We also show that this result is equivalent to thickness profiles exhibiting a separation of space and time. By integrating new measurements with data from the literature across various conditions, we validate these properties and establish the universality of the dynamics, governed by a single physical scalar. Our findings provide new insights for proposing a drainage model and understanding the mechanism of marginal regeneration at the origin of the process.

cond-mat.soft

Scaling the tail beat frequency and swimming speed in underwater undulatory swimming

Due to its great efficiency and maneuverability, undulatory swimming is the predominant form of locomotion in aquatic vertebrates. A myriad of animals of different species and sizes oscillate their bodies to propel themselves in aquatic environments with swimming speed scaling as the product of the animal length by the oscillation frequency. Although frequency tuning is the primary means by which a swimmer selects its speed, there is no consensus on the mechanisms involved. In this article, we propose scaling laws for undulatory swimmers that relate oscillation frequency to length by taking into account both the biological characteristics of the muscles and the interaction of the moving swimmer with its environment. Results are supported by an extensive literature review including approximately 1200 individuals of different species, sizes and swimming environments. We highlight a crossover in length around 0.5-1 m. Below this value, the frequency can be tuned between 2-20 Hz due to biological constraints and the interplay between slow and fast muscles. Above this value, the fluid-swimmer interaction must be taken into account and the frequency is inversely proportional to the length of the animal. This approach predicts a maximum swimming speed around 5-10 m.s$^{-1}$ for large swimmers, consistent with the threshold to prevent bubble cavitation.

physics.flu-dyn

Collapse of a hemicatenoid bounded by a solid wall: instability and dynamics driven by surface Plateau border friction

The collapse of a catenoidal soap film when the rings supporting it are moved beyond a critical separation is a classic problem in interface motion in which there is a balance between surface tension and the inertia of the surrounding air, with film viscosity playing only a minor role. Recently [Goldstein, et al., Phys. Rev. E 104, 035105 (2021)], we introduced a variant of this problem in which the catenoid is bisected by a glass plate located in a plane of symmetry perpendicular to the rings, producing two identical hemicatenoids, each with a surface Plateau border (SPB) on the glass plate. Beyond the critical ring separation, the hemicatenoids collapse in a manner qualitatively similar to the bulk problem, but their motion is governed by the frictional forces arising from viscous dissipation in the SPBs. Here we present numerical studies of a model that includes classical friction laws for SPB motion on wet surfaces and show consistency with our experimental measurements of the temporal evolution of this process. This study can help explain the fragmentation of bubbles inside very confined geometries such as porous materials or microfluidic devices.

cond-mat.soft

Stress-Induced Dinoflagellate Bioluminescence at the Single Cell Level

One of the characteristic features of many marine dinoflagellates is their bioluminescence, which lights up nighttime breaking waves or seawater sliced by a ship's prow. While the internal biochemistry of light production by these microorganisms is well established, the manner by which fluid shear or mechanical forces trigger bioluminescence is still poorly understood. We report controlled measurements of the relation between mechanical stress and light production at the single-cell level, using high-speed imaging of micropipette-held cells of the marine dinoflagellate $Pyrocystis~lunula$ subjected to localized fluid flows or direct indentation. We find a viscoelastic response in which light intensity depends on both the amplitude and rate of deformation, consistent with the action of stretch-activated ion channels. A phenomenological model captures the experimental observations.

cond-mat.soft

Three-dimensional foam flow resolved by fast X-ray tomographic microscopy

Thanks to ultra fast and high resolution X-ray tomography, we managed to capture the evolution of the local structure of the bubble network of a 3D foam flowing around a sphere. As for the 2D foam flow around a circular obstacle, we observed an axisymmetric velocity field with a recirculation zone, and indications of a negative wake downstream the obstacle. The bubble deformations, quantified by a shape tensor, are smaller than in 2D, due to a purely 3D feature: the azimuthal bubble shape variation. Moreover, we were able to detect plastic rearrangements, characterized by the neighbor-swapping of four bubbles. Their spatial structure suggest that rearrangements are triggered when films faces get smaller than a characteristic area.

physics.flu-dyn

Two dimensional Leidenfrost Droplets in a Hele Shaw Cell

We experimentally and theoretically investigate the behavior of Leidenfrost droplets inserted in a Hele-Shaw cell. As a result of the confinement from the two surfaces, the droplet has the shape of a flattened disc and is thermally isolated from the surface by the two evaporating vapor layers. An analysis of the evaporation rate using simple scaling arguments is in agreement with the experimental results. Using the lubrication approximation we numerically determine the shape of the droplets as a function of its radius. We furthermore find that the droplet width tends to zero at its center when the radius reaches a critical value. This prediction is corroborated experimentally by the direct observation of the sudden transition from a flattened disc into an expending torus. Below this critical size, the droplets are also displaying capillary azimuthal oscillating modes reminiscent of a hydrodynamic instability.

physics.flu-dyn

Jet impact on a soap film

We experimentally investigate the impact of a liquid jet on a soap film. We observe that the jet never breaks the film and that two qualitatively different steady regimes may occur. The first one is a refraction-like behavior obtained at small incidence angles when the jet crosses the film and is deflected by the film-jet interaction. For larger incidence angles, the jet is absorbed by the film, giving rise to a new class of flow in which the jet undulates along the film with a characteristic wavelength. Besides its fundamental interest, this study presents a new way to guide a micro-metric flow of liquid in the inertial regime and to probe foam stability submitted to violent perturbations at the soap film scale.

cond-mat.soft

Deformation of a free interface pierced by a tilted cylinder

We investigate the interaction between an infinite cylinder and a free fluid-fluid interface governed only by its surface tension. We study the deformation of an initially flat interface when it is deformed by the presence of a cylindrical object, tilted at an arbitrary angle, that the interface "totally wets". Our simulations predict all significant quantities such as the interface shape, the position of the contact line, and the force exerted by the interface on the cylinder. These results are compared with an experimental study of the penetration of a soap film by a cylindrical liquid jet. This dynamic situation exhibits all the characteristics of a totally wetting interface. We show that whatever the inclination, the force is always perpendicular to the plane of the interface, and its amplitude diverges as the inclination angle increases. Such results should bring new insights in both fluid and solid mechanics, from animal locomotion to surface micro-processing.-processing.

cond-mat.soft

The mechanism of porosity formation during solvent-mediated phase transformations

Solvent-mediated solid-solid phase transformations often result in the formation of a porous medium, which may be stable on long time scales or undergo ripening and consolidation. We have studied replace- ment processes in the KBr-KCl-H2O system using both in situ and ex situ experiments. The replacement of a KBr crystal by a K(Br,Cl) solid solution in the presence of an aqueous solution is facilitated by the gen- eration of a surprisingly stable, highly anisotropic and connected pore structure that pervades the product phase. This pore structure ensures efficient solute transport from the bulk solution to the reacting KBr and K(Br,Cl) surfaces. The compositional profile of the K(Br,Cl) solid solu- tion exhibits striking discontinuities across disc-like cavities in the product phase. Similar transformation mechanisms are probably important in con- trolling phase transformation processes and rates in a variety of natural and man-made systems.

physics.chem-ph

Discrete rearranging disordered patterns: Prediction of elastic and plastic behaviour, and application to two-dimensional foams

We study the elasto-plastic behaviour of materials made of individual (discrete) objects, such as a liquid foam made of bubbles. The evolution of positions and mutual arrangements of individual objects is taken into account through statistical quantities, such as the elastic strain of the structure, the yield strain and the yield function. The past history of the sample plays no explicit role, except through its effect on these statistical quantities. They suffice to relate the discrete scale with the collective, global scale. At this global scale, the material behaves as a continuous medium; it is described with tensors such as elastic strain, stress and velocity gradient. We write the differential equations which predict their elastic and plastic behaviour in both the general case and the case of simple shear. An overshoot in the shear strain or shear stress is interpreted as a rotation of the deformed structure, which is a purely tensorial effect that exists only if the yield strain is at least of order 0.3. We suggest practical applications, including: when to choose a scalar formalism rather than a tensorial one; how to relax trapped stresses; and how to model materials with a low, or a high, yield strain.

cond-mat.soft

Discrete rearranging disordered patterns, part II: 2D plasticity, elasticity and flow of a foam

The plastic flow of a foam results from bubble rearrangements. We study their occurrence in experiments where a foam is forced to flow in 2D: around an obstacle; through a narrow hole; or sheared between rotating disks. We describe their orientation and frequency using a topological matrix defined in the companion paper (Graner et al., preprint), which links them with continuous plasticity at large scale. We then suggest a phenomenological equation to predict the plastic strain rate: its orientation is determined from the foam's local elastic strain; and its rate is determined from the foam's local elongation rate. We obtain a good agreement with statistical measurements. This enables us to describe the foam as a continuous medium with fluid, elastic and plastic properties. We derive its constitutive equation, then test several of its terms and predictions.

cond-mat.soft

Discrete rearranging disordered patterns, part I: Robust statistical tools in two or three dimensions

Discrete rearranging patterns include cellular patterns, for instance liquid foams, biological tissues, grains in polycrystals; assemblies of particles such as beads, granular materials, colloids, molecules, atoms; and interconnected networks. Such a pattern can be described as a list of links between neighbouring sites. Performing statistics on the links between neighbouring sites yields average quantities (hereafter "tools") as the result of direct measurements on images. These descriptive tools are flexible and suitable for various problems where quantitative measurements are required, whether in two or in three dimensions. Here, we present a coherent set of robust tools, in three steps. First, we revisit the definitions of three existing tools based on the texture matrix. Second, thanks to their more general definition, we embed these three tools in a self-consistent formalism, which includes three additional ones. Third, we show that the six tools together provide a direct correspondence between a small scale, where they quantify the discrete pattern's local distortion and rearrangements, and a large scale, where they help describe a material as a continuous medium. This enables to formulate elastic, plastic, fluid behaviours in a common, self-consistent modelling using continuous mechanics. Experiments, simulations and models can be expressed in the same language and directly compared. As an example, a companion paper (Marmottant, Raufaste and Graner, joint paper) provides an application to foam plasticity.

cond-mat.soft

Yield drag in a two-dimensional foam flow around a circular obstacle: Effect of liquid fraction

We study the two-dimensional flow of foams around a circular obstacle within a long channel. In experiments, we confine the foam between liquid and glass surfaces. In simulations, we use a deterministic software, the Surface Evolver, for bubble details and a stochastic one, the extended Potts model, for statistics. We adopt a coherent definition of liquid fraction for all studied systems. We vary it in both experiments and simulations, and determine the yield drag of the foam, that is, the force exerted on the obstacle by the foam flowing at very low velocity. We find that the yield drag is linear over a large range of the ratio of obstacle to bubble size, and is independent of the channel width over a large range. Decreasing the liquid fraction, however, strongly increases the yield drag; we discuss and interpret this dependence.

cond-mat.soft