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Christopher Eckberg

Publications and source records attributed to Christopher Eckberg.

15 recordsLinked to original sources
arXiv2026

Probing the Penetration Depth of Topological Surface States by Magnetic Impurity Scattering in V-doped Sb$_2$Te$_3$

Topological insulators host Dirac surface states (SS) protected by time-reversal symmetry. Inter-surface hybridization can gap the SS and give rise to the quantum spin Hall effect in films that are sufficiently thin compared to the SS penetration depth. However, quantifying the SS penetration depth typically requires painstaking synthesis of multiple films with varying thickness. Here we introduce a direct method to probe the SS penetration depth in bulk crystals, by studying the interplay between SS and magnetic impurities in \SVT. Using scanning tunneling microscopy and spectroscopy, we find that even sparse magnetic impurities ($\lesssim0.25\%$ vanadium) can gap the Dirac SS. However, a single V impurity induces only localized states, and does not form an impurity band, so the gapped Dirac dispersion is preserved away from the impurity. In high magnetic fields, we observe an energy shift of the $0^\text{th}$ Landau level and a suppression of quasiparticle lifetime at the Dirac point, indicating \newtext{magnetic} scattering of the SS. Crucially, by employing V impurities at different depths as precise scattering probes, we reveal the SS penetration depth on the sub-nanometer scale in a bulk crystal.

cond-mat.mes-hall↗
arXiv2025

Charge order-driven nematicity in the nickel-pnictide superconductor Ba$_{1-x}$Sr$_x$Ni$_2$As$_2$

Nematic order refers to the spontaneous breaking of rotational symmetry while preserving translational symmetry. First identified in classical liquid crystals, nematic order arises from the collective alignment of anisotropic molecules. Its quantum counterpart, electronic nematicity, has been observed in a variety of quantum materials, ranging from unconventional superconductors to kagome metals. Despite its prevalence, there is no universal understanding of the conditions under which nematic order occurs. Electronic nematicity is most firmly established in iron-based superconductors, where it is understood to be a consequence of vestigial spin density wave (SDW) order. However, direct evidence for nematicity arising from other types of order are lacking. Here, we report direct evidence for charge-order-driven electronic nematicity in Ba$_{1-x}$Sr$_x$Ni$_2$As$_2$, a nickel-based analog of the iron pnictides known to exhibit charge density wave (CDW) order. Using x-ray diffraction under applied uniaxial strain, we observe a pronounced symmetry-breaking response-up to $\sim 50 \%$-in the intensity of incommensurate CDW Bragg peaks, even at small strain levels ($\epsilon_{xy} \sim 10^{-3}$). This effect occurs within the same region of the phase diagram where a giant nematic susceptibility is observed in transport measurements. These results provide direct evidence that long-range CDW order can drive nematic behavior in quantum materials.

cond-mat.str-el↗
arXiv2024

Field-Resilient Supercurrent Diode in a Multiferroic Josephson Junction

The research on supercurrent diodes has surged rapidly due to their potential applications in electronic circuits at cryogenic temperatures. To unlock this functionality, it is essential to find supercurrent diodes that can work consistently at zero magnetic field and under ubiquitous stray fields generated in electronic circuits. However, a supercurrent diode with robust field tolerance is currently lacking. Here, we demonstrate a field-resilient supercurrent diode by incorporating a multiferroic material into a Josephson junction. We first observed a pronounced supercurrent diode effect at zero magnetic field. More importantly, the supercurrent rectification persists over a wide and bipolar magnetic field range beyond industrial standards for field tolerance. By theoretically modeling a multiferroic Josephson junction, we unveil that the interplay between spin-orbit coupling and multiferroicity underlies the unusual field resilience of the observed diode effect. This work introduces multiferroic Josephson junctions as a new field-resilient superconducting device for cryogenic electronics.

cond-mat.supr-con↗
arXiv2024

Precision frequency tuning of tunable transmon qubits using alternating-bias assisted annealing

Superconducting quantum processors are one of the leading platforms for realizing scalable fault-tolerant quantum computation (FTQC). The recent demonstration of post-fabrication tuning of Josephson junctions using alternating-bias assisted annealing (ABAA) technique and a reduction in junction loss after ABAA illuminates a promising path towards precision tuning of qubit frequency while maintaining high coherence. Here, we demonstrate precision tuning of the maximum $|0\rangle\rightarrow |1\rangle$ transition frequency ($f_{01}^{\rm max}$) of tunable transmon qubits by performing ABAA at room temperature using commercially available test equipment. We characterize the impact of junction relaxation and aging on resistance spread after tuning, and demonstrate a frequency equivalent tuning precision of 7.7 MHz ($0.17\%$) based on targeted resistance tuning on hundreds of qubits, with a resistance tuning range up to $18.5\%$. Cryogenic measurements on tuned and untuned qubits show evidence of improved coherence after ABAA with no significant impact on tunability. Despite a small global offset, we show an empirical $f_{01}^{\rm max}$ tuning precision of 18.4 MHz by tuning a set of multi-qubit processors targeting their designed Hamiltonians. We experimentally characterize high-fidelity parametric resonance iSWAP gates on two ABAA-tuned 9-qubit processors with fidelity as high as $99.51\pm 0.20\%$. On the best-performing device, we measured across the device a median fidelity of $99.22\%$ and an average fidelity of $99.13\pm 0.12 \%$. Yield modeling analysis predicts high detuning-edge-yield using ABAA beyond the 1000-qubit scale. These results demonstrate the cutting-edge capability of frequency targeting using ABAA and open up a new avenue to systematically improving Hamiltonian targeting and optimization for scaling high-performance superconducting quantum processors.

quant-ph↗
arXiv2024

Ultrafast dynamics of wavelength-sensitive magnons in unconventional compensated semiconducting antiferromagnet

Antiferromagnet is a promising candidate for the next generation spintronic devices, benefiting from its ultrafast dynamics and spontaneous zero stray field. However, the understanding of their ultrafast spin behaviors is lacking due to the challenges of controlling/detecting the quenched net magnetization. Unconventional compensated semiconducting antiferromagnets present strong time-reversal symmetry breaking, spin splitting in the momentum space, and suitable bandgap for optical control/detection. Thus, it is a powerful platform to uncover the ultrafast dynamics of antiferromagnets. Here, we show an exotic wavelength-dependent spin dynamic in the unconventional compensated semiconducting antiferromagnet α-MnTe via time-resolved quadratic magneto-optical Kerr effect measurement, where the probing photon energy of the laser matches its bandgap. This direct excitation and detection of distinct magnon modes reveal varying spin behaviors and time characteristics in a broad temperature range. It originates from the spins triggered at different bands of electronic structures and is depicted in an energy transfer model among electrons, phonons, and magnons. Our study of exotic optical properties in this unconventional semiconducting antiferromagnet fulfills the missing information of spin evolution in the time domain and paves the way for its utilization in ultrafast spintronic devices.

physics.app-ph↗
arXiv2023

Potential Lifshitz transition at optimal substitution in nematic pnictide Ba$_{1-x}$Sr$_x$Ni$_2$As$_2$

BaNi$_2$As$_2$ is a structural analog of the pnictide superconductor BaFe$_2$As$_2$, which, like the iron-based superconductors, hosts a variety of ordered phases including charge density waves (CDWs), electronic nematicity, and superconductivity. Upon isovalent Sr substitution on the Ba site, the charge and nematic orders are suppressed, followed by a sixfold enhancement of the superconducting transition temperature ($T_c$). To understand the mechanisms responsible for enhancement of $T_c$, we present high-resolution angle-resolved photoemission spectroscopy (ARPES) measurements of the Ba$_{1-x}$Sr$_{x}$Ni$_2$As$_2$ series, which agree well with our density functional theory (DFT) calculations throughout the substitution range. Analysis of our ARPES-validated DFT results indicates a Lifshitz transition and reasonably nested electron and hole Fermi pockets near optimal substitution where $T_c$ is maximum. These nested pockets host Ni $d_{xz}$/$d_{yz}$ orbital compositions, which we associate with the enhancement of nematic fluctuations, revealing unexpected connections to the iron-pnictide superconductors. This gives credence to a scenario in which nematic fluctuations drive an enhanced $T_c$.

cond-mat.supr-con↗
arXiv2023

Concurrent Ferromagnetism and Superconductivity in Fe(Te,Se) van der Waals Josephson Junctions

Ferromagnetism and superconductivity are two key ingredients to create non-Abelian quasiparticle excitations that are expected as building blocks to construct topological quantum computers. Adversely, ferromagnetism and superconductivity are typically also two hostile orderings competing to align spins in different configurations, making the material design and experimental implementation extremely challenging. Recently, iron-based superconductor Fe(Te,Se) has emerged as a connate topological superconductor (TSC), which differentiates itself from other hybrid TSCs by self-proximitizing its Dirac surface states with bulk superconductivity. So far, the efforts to search for Majorana states in this material are prevalently focused on spectroscopy techniques. In this paper, we present the global transport signature of interfacial magnetism coexisting with superconductivity. Time-reversal symmetry breaking superconducting states are confirmed through device level transport measurements for the first time in a van der Waals (vdW) Josephson junction structure. Magnetic hysteresis is observed in this device scheme, which only appears below the superconducting critical temperature, leading to potential Fulde-Ferrell (FF) superconducting pairing mechanisms. The 0-π phase mixing in the Fraunhofer patterns pinpoints the ferromagnetic state dwelling on the surface. Furthermore, a stochastic field-free superconducting diode effect also confirms the spontaneous time-reversal symmetry breaking which reflects the behavior of the ferromagnetism. Our work paves a new way to explore topological superconductivity in iron-based superconductors for future high Tc fault-tolerant qubit implementations from a device perspective.

cond-mat.supr-con↗
arXiv2023

Charge Order Evolution of Superconducting BaNi2As2 Under High Pressure

BaNi$_2$As$_2$, a non-magnetic superconductor counterpart to BaFe$_2$As$_2$, has been shown to develop nematic order, multiple charge orders, and a dramatic six-fold enhancement of superconductivity via isovalent chemical substitution of Sr for Ba. Here we present high pressure single-crystal and powder x-ray diffraction measurements of BaNi$_2$As$_2$ to study the effects of tuning lattice density on the evolution of charge order in this system. Single-crystal X-ray experiments track the evolution of the incommensurate (Q=0.28) and commensurate (Q=0.33 and Q=0.5) charge orders, and the tetragonal-triclinic distortion as a function of temperature up to pressures of 10.4 GPa, and powder diffraction experiments at 300 K provide lattice parameters up to 17 GPa. We find that applying pressure to BaNi$_2$As$_2$ produces a similar evolution of structural and charge-ordered phases as found as a function of chemical pressure in Ba$_{1-x}$Sr$_{x}$Ni$_2$As$_2$ , with coexisting commensurate charge orders appearing on increasing pressure. These phases also exhibit a similar abrupt cutoff at a critical pressure of (9 $\pm$ 0.5) GPa, where powder diffraction experiments indicate a collapse of the tetragonal structure at higher temperatures. We discuss the relationship between this collapsed tetragonal phase and the discontinuous phase boundary observed at the optimal substitution value for superconductivity in Ba$_{1-x}$Sr$_{x}$Ni$_2$As$_2$

cond-mat.str-el↗
arXiv2023

Structural tuning magnetism and topology in a magnetic topological insulator

To date, the most widely-studied quantum anomalous Hall insulator (QAHI) platform is achieved by dilute doping of magnetic ions into thin films of the alloyed tetradymite topological insulator (TI) (Bi$_{1-x}$Sb$_x$)$_2$Te$_3$ (BST). In these films, long-range magnetic ordering of the transition metal substituants opens an exchange gap $Δ$ in the topological surface states, stabilizing spin-polarized, dissipationless edge channels with a nonzero Chern number $\mathcal{C}$. The long-range ordering of the spatially separated magnetic ions is itself mediated by electronic states in the host TI, leading to a sophisticated feedback between magnetic and electronic properties. Here we present a study of the electronic and magnetic response of a BST-based QAHI system to structural tuning via hydrostatic pressure. We identify a systematic closure of the topological gap under compressive strain accompanied by a simultaneous enhancement in the magnetic ordering strength. Combining these experimental results with first-principle calculations we identify structural deformation as a strong tuning parameter to traverse a rich topological phase space and modify magnetism in the magnetically doped BST system.

cond-mat.mes-hall↗
arXiv2022

Distinguishing two-component anomalous Hall effect from topological Hall effect

In transport, the topological Hall effect (THE) presents itself as non-monotonic features (or humps and dips) in the Hall signal and is widely interpreted as a sign of chiral spin textures, like magnetic skyrmions. However, when anomalous Hall effect (AHE) is also present, the co-existence of two AHEs could give rise to similar artifacts, making it difficult to distinguish between genuine THE with AHE and two-component AHE. Here we confirm genuine THE with AHE by means of transport and magneto-optical Kerr effect (MOKE) microscopy, in which magnetic skyrmions are directly observed, and find that genuine THE occurs in the transition region of the AHE. In sharp contrast, the artifact "THE", or two-component AHE occurs well beyond the saturation of the "AHE component" (under the false assumption of THE+AHE). Furthermore, we distinguish artifact "THE" from genuine THE by three methods: 1. Minor loops, 2. Temperature dependence, 3. Gate dependence. Minor loops of genuine THE with AHE are always within the full loop, while minor loops of the artifact "THE" may reveal a single loop that cannot fit into the "AHE component". Besides, the temperature or gate dependence of the artifact "THE" may also be accompanied by a polarity change of the "AHE component", as the non-monotonic features vanish, while the temperature dependence of genuine THE with AHE reveals no such change. Our work may help future researchers to exercise cautions and use these methods to examine carefully in order to ascertain genuine THE.

cond-mat.mtrl-sci↗
arXiv2022

Exchange-biased quantum anomalous Hall effect

The quantum anomalous Hall (QAH) effect is characterized by a dissipationless chiral edge state with a quantized Hall resistance at zero magnetic field. Manipulating the QAH state is of great importance in both the understanding of topological quantum physics and the implementation of dissipationless electronics. Here, we realized the QAH effect in the magnetic topological insulator Cr-doped (Bi,Sb)2Te3 (CBST) grown on an uncompensated antiferromagnetic insulator Al-doped Cr2O3. Through polarized neutron reflectometry (PNR), we find a strong exchange coupling between CBST and Al-Cr2O3 surface spins fixing interfacial magnetic moments perpendicular to the film plane. The interfacial coupling results in an exchange-biased QAH effect. We further demonstrate that the magnitude and sign of the exchange bias can be effectively controlled using a field training process to set the magnetization of the Al-Cr2O3 layer. Our work demonstrates the use of the exchange bias effect to effectively manipulate the QAH state, opening new possibilities in QAH-based spintronics.

cond-mat.mes-hall↗
arXiv2021

Mesoscopic Transport of Quantum Anomalous Hall Effect in Sub-Micron Size Regime

The quantum anomalous Hall (QAH) effect has been demonstrated in two-dimensional topological insulator systems incorporated with ferromagnetism. However, a comprehensive understanding of mesoscopic transport in sub-micron QAH devices has yet been established. Here we fabricated miniaturized QAH devices with channel widths down to 600 nm, where the QAH features are still preserved. A back-scattering channel is formed in narrow QAH devices through percolative hopping between 2D compressible puddles. Large resistance fluctuations are observed in narrow devices near the coercive field, which is associated with collective interference between intersecting paths along domain walls when the device geometry is smaller than the phase coherence length $L_ϕ$. Through measurement of size-dependent breakdown current, we confirmed that the chiral edge states are confined at the physical boundary with its width on the order of Fermi wavelength.

cond-mat.mes-hall↗
arXiv2019

Extreme magnetic field-boosted superconductivity

Applied magnetic fields underlie exotic quantum states, such as the fractional quantum Hall effect and Bose-Einstein condensation of spin excitations. Superconductivity, on the other hand, is inherently antagonistic towards magnetic fields. Only in rare cases can these effects be mitigated over limited fields, leading to reentrant superconductivity. Here, we report the unprecedented coexistence of multiple high-field reentrant superconducting phases in the spin-triplet superconductor UTe2. Strikingly, we observe superconductivity in the highest magnetic field range identified for any reentrant superconductor, beyond 65 T. These extreme properties reflect a new kind of exotic superconductivity rooted in magnetic fluctuations and boosted by a quantum dimensional crossover.

cond-mat.supr-con↗
arXiv2017

Superconductivity and magnetism in Iron Sulfides Intercalated by Metal Hydroxides

Inspired by naturally occurring sulfide minerals, we present a new family of iron-based superconductors. A metastable form of FeS known as the mineral mackinawite forms two-dimensional sheets that can be readily intercalated by various cationic guest species. Under hydrothermal conditions using alkali metal hydroxides, we prepare three different cation and metal hydroxide-intercalated FeS phases including (Li$_{1-x}$Fe$_x$OH)FeS, [(Na$_{1-x}$Fe$_x$)(OH)$_2$]FeS, and K$_x$Fe$_{2-y}$S$_2$. Upon successful intercalation of the FeS layer, the superconducting critical temperature $T_c$ of mackinawite is enhanced from 5 K to 8 K for the (Li$_{1-x}$Fe$_x$OH)$^{δ+}$ intercalate. Layered heterostructures of [(Na$_{1-x}$Fe$_x$)(OH)$_2$]FeS resemble the natural mineral tochilinite, which contains an iron square lattice interleaved with a hexagonal hydroxide lattice. Whilst heterostructured [(Na$_{1-x}$Fe$_x$)(OH)$_2$]FeS displays long-range magnetic ordering near 15 K, K$_x$Fe$_{2-y}$S$_2$ displays short range antiferromagnetism.

cond-mat.supr-con↗
arXiv2016

Strong anisotropy in nearly ideal-tetrahedral superconducting FeS single crystals

We report the novel preparation of single crystals of tetragonal iron sulfide, FeS, which exhibits a nearly ideal tetrahedral geometry with S--Fe--S bond angles of 110.2(2) $^\circ$ and 108.1(2) $^\circ$. Grown via hydrothermal de-intercalation of K${_x}$Fe${_{2-y}}$S${_2}$ crystals under basic and reducing conditions, the silver, plate-like crystals of FeS remain stable up to 200 $^\circ$C under air and 250 $^\circ$C under inert conditions, even though the mineral "mackinawite" (FeS) is known to be metastable. FeS single crystals exhibit a superconducting state below $T_c=4$ K as determined by electrical resistivity, magnetic susceptibility, and heat capacity measurements, confirming the presence of a bulk superconducting state. Normal state measurements yield an electronic specific heat of 5~mJ/mol-K$^2$, and paramagnetic, metallic behavior with a low residual resistivity of 250~$μΩ\cdot$cm. Magnetoresistance measurements performed as a function of magnetic field angle tilted toward both transverse and longitudinal orientations with respect to the applied current reveal remarkable two-dimensional behavior. This is paralleled in the superconducting state, which exhibits the largest known upper critical field $H_{c2}$ anisotropy of all iron-based superconductors, with $H_{c2}^{||ab}(0) / H_{c2}^{||c}(0)=$(2.75~T)/(0.275~T)=10. Comparisons to theoretical models for 2D and anisotropic-3D superconductors, however, suggest that FeS is the latter case with a large effective mass anisotropy. We place FeS in context to other closely related iron-based superconductors and discuss the role of structural parameters such as anion height on superconductivity.

cond-mat.supr-con↗