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Christopher L. Holloway

Publications and source records attributed to Christopher L. Holloway.

At least 37 records · Page 2Linked to original sources
arXiv2025

Angle-of-arrival detection of radio-frequency waves via Rydberg atom fluorescence imaging of standing waves in a glass vapor cell

We present a method for measuring the angle-of-arrival of 40 GHz radio-frequency (RF) radiation by mapping the standing waves generated in a rectangular glass vapor cell. These standing waves have regular and well-defined structure from which we can infer the angle and sign of the wavevector of the RF field. We map the field using spatially resolved light sheet spectroscopy of Rydberg states of rubidium atoms in the cell. Unlike traditional phased arrays, this detection scheme is compact and low-complexity, has an active area of nearly 4$π$ steradians, and is sensitive to all RF polarizations. For in-plane measurements ($ϕ= 0$), we demonstrate quantitative angle-of-arrival measurements with an uncertainty on the order of one degree in an 11~s measurement, and for out-of-plane measurements (arbitrary $θ$,$ϕ$), we demonstrate angle-of-arrival detection with uncertainty on the order of several degrees.

physics.atom-ph↗
arXiv2025

Determining angle of arrival of radio frequency fields using subwavelength, amplitude-only measurements of standing waves in a Rydberg atom sensor

Deep subwavelength RF imaging with atomic Rydberg sensors has overcome fundamental limitations of traditional antennas and enabled ultra-wideband detection of omni-directional time varying fields all in a compact form factor. However, in most applications, Rydberg sensors require the use of a secondary strong RF reference field to serve as a phase reference. Here, we demonstrate a new type of Rydberg sensor for angle-of-arrival (AoA) sensing which utilizes subwavelength imaging of standing wave fields. By placing a metallic plate within the Rydberg cell, we can determine the AoA independent of the strength of incoming RF field and without requiring a secondary strong RF phase reference field. We perform precision AoA measurements with a robotic antenna positioning system for 4.2, 5.0, and 5.7 GHz signals and demonstrate a 1.7 deg polar angular resolution from 0 deg to 60 deg AoA and 4.1 deg over all possible angles.

physics.atom-ph↗
arXiv2025

Imaging of induced surface charge distribution effects in glass vapor cells used for Rydberg atom-based sensors

We demonstrate the imaging of localized surface electric (E) field effects on the atomic spectrum in a vapor cell used in Rydberg atom-based sensors. These surface E-fields can result from an induced electric charge distribution on the surface. Induced surface charge distributions can dramatically perturb the atomic spectrum, hence degrading the ability to perform electrometry. These effects become pronounced near the walls of the vapor cell, posing challenges for vapor cell miniaturization. Using a fluorescence imaging technique, we investigate the effects of surface charge on the atomic spectrum generated with electromagnetically induced transparency (EIT). Our results reveal that visible light (480 nm and 511 nm), i.e., the coupling laser used in two-photon Rydberg EIT schemes, generates localized patches of charge or dipoles where this light interacts with the glass walls of the vapor cell, while a three-photon Rydberg EIT scheme using only near-infrared wavelength lasers shows no measurable field induction. Additionally, imaging in a vacuum chamber where a glass plate is placed between large electrodes confirms that the induced charge is positive. We further validate these findings by studying the photoelectric effect with broadband light during EIT and impedance measurements. These results demonstrate the power of the fluorescence imaging technique to study localized E-field distributions in vapor cells and to target the photoelectric effect of the alkali-exposed glass of vapor cells as a major disruptor in Rydberg atom-based sensors.

physics.atom-ph↗
arXiv2024

Two-dimensional imaging of electromagnetic fields via light sheet fluorescence imaging with Rydberg atoms

The ability to image electromagnetic fields holds key scientific and industrial applications, including electromagnetic compatibility, diagnostics of high-frequency devices, and experimental scientific work involving field interactions. Generally electric and magnetic field measurements require conductive elements which significantly distort the field. However, electromagnetic fields can be measured without altering the field via the shift they induce on Rydberg states of alkali atoms in atomic vapor, which are highly sensitive to electric fields. Previous field measurements using Rydberg atoms utilized electromagnetically induced transparency to read out the shift on the states induced by the fields, but did not provide spatial resolution. In this work, we demonstrate that electromagnetically induced transparency can be spatially resolved by imaging the fluorescence of the atoms. We demonstrate that this can be used to image $\sim$ V/cm scale electric fields in the DC-GHz range and $\sim$ mT scale static magnetic fields, with minimal distortion to the fields. We also demonstrate the ability to image $\sim$ 5 mV/cm scale fields for resonant microwave radiation and measure standing waves generated by the partial reflection of the vapor cell walls in this regime. With additional processing techniques like lock-in detection, we predict that our sensitivities could reach down to nV/cm levels. We perform this field imaging with a spatial resolution of 160 $μ$m, limited by our imaging system, and estimate the fundamental resolution limitation to be 5 $μ$m.

physics.atom-ph↗
arXiv2024

Compact Blackbody Radiation Atomic Sensor: Measuring Temperature using Optically Excited Atoms in Vapor Cells

We demonstrate a blackbody radiation thermometer based on optically excited rubidium atoms in a vapor cell. The temperature measurement is fast, with statistical uncertainty as low as 0.1% in one second. We resolve temperature with a precision of 0.04% in the range 308 K to 344 K when averaging for several seconds. Additionally, we describe an extension to this measurement scheme where the device operates as a self-calibrated, or primary, thermometer. We make progress toward realizing a primary thermometer by demonstrating a temperature-dependent self-consistent calibration scheme, with temperature accuracy of order 1% limited by the uncertainty in atomic transition dipole matrix elements.

physics.atom-ph↗
arXiv2024

Primary quantum thermometry of mm-wave blackbody radiation via induced state transfer in Rydberg states of cold atoms

Rydberg states of alkali atoms are highly sensitive to electromagnetic radiation in the GHz-to-THz regime because their transitions have large electric dipole moments. Consequently, environmental blackbody radiation (BBR) can couple Rydberg states together at $μ$s timescales. Here, we track the BBR-induced transfer of a prepared Rydberg state to its neighbors and use the evolution of these state populations to characterize the BBR field at the relevant wavelengths, primarily at 130 GHz. We use selective field ionization readout of Rydberg states with principal quantum number $n\sim30$ in $^{85}$Rb and substantiate our ionization signal with a theoretical model. With this detection method, we measure the associated blackbody-radiation-induced time dynamics of these states, reproduce the results with a simple semi-classical population transfer model, and demonstrate that this measurement is temperature sensitive with a statistical sensitivity to the fractional temperature uncertainty of 0.09 Hz$^{-1/2}$, corresponding to 26 K$\cdot$Hz$^{-1/2}$ at room temperature. This represents a calibration-free SI-traceable temperature measurement, for which we calculate a systematic fractional temperature uncertainty of 0.006, corresponding to 2 K at room temperature when used as a primary temperature standard.

physics.atom-ph↗
arXiv2024

Multichannel, ultra-wideband Rydberg Electrometry with an Optical Frequency Comb

While Rydberg atoms have shown tremendous potential to serve as accurate and sensitive detectors of microwaves and millimeter waves, their response is generally limited to a single narrow frequency band around a chosen microwave transition. As a result, their potential to serve as agile and wideband electromagnetic receivers has not been fully realized. Here we demonstrate the use of a mid-infrared, frequency agile optical frequency comb as the coupling laser for three-photon Rydberg atom electrometry. This approach allows us to simultaneously prepare as many as seven individual Rydberg states, allowing for multichannel detection across a frequency range from 1 GHz to 40 GHz. The generality and flexibility of this method for wideband multiplexing is anticipated to have transformative effects in the field of Rydberg electrometry, paving the way for advanced information coding and arbitrary signal detection.

physics.atom-ph↗
arXiv2024

Revisiting collisional broadening of $^{85}$Rb Rydberg levels: conclusions for vapor cell manufacture

Electrometry based on electromagnetically induced transparency (EIT) in alkali Rydberg vapor cells may suffer reduced sensitivity due to spurious line broadening effects, caused by surface charges, contaminant gases, or other manufacturing defects. In order to draw conclusions about the deleterious effects of potential contaminant gases inside Rydberg electrometry vapor cells, we revisit collisional broadening and shifts of both the D$_2$ line and Rydberg levels of rubidium. Specifically, we measure the broadening and shifts of the $5{\rm S}_{1/2}\rightarrow 5{\rm P}_{3/2}$ (i.e., the D$_2$ line) and $5{\rm S}_{1/2}\rightarrow 5{\rm P}_{3/2}\rightarrow (25{\rm D},27{\rm S},30{\rm D},32{\rm S},35{\rm D},37{\rm S})$ transitions of $^{85}$Rb due to He, Ne, N$_2$ and Ar. By combining these measurements with observations of velocity changing collisions in the sub-Doppler spectrum of the D$_2$ line, we conclude the following: (1) that contaminant gases are most likely not the cause of irregular line shapes or shifts of Rydberg transitions due to the high pressures required, and (2) the sub-Doppler spectrum of the D$_2$ line, through its accompanying loss of contrast at high pressures, can validate that a vapor cell is sufficiently free of contaminant gas for EIT electrometry. We use the theory of Omont, J. Phys. France 38, 1343 (1977), to extend our results to a wide variety of possible contaminant gases and further derive scaling laws applicable to all gases.

physics.atom-ph↗
arXiv2024

Observation of Asymmetric Sideband Generation in Strongly-driven Rydberg Atoms

Improving the bandwidth of Rydberg atom-based receivers is an ongoing challenge owing to the long-lived Rydberg state lifetimes that limit the refresh rate of ground state atoms. In particular, the LO-based Rydberg mixer approach allows for bandwidths into the few-MHz range. Here, we use heterodyne detection of the Rydberg atom receiver probe laser to separate the negative and positive sidebands that originate from distinct six wave mixing processes, in order to investigate their individual bandwidths. We experimentally confirm the prediction that the negative sideband exhibits a higher bandwidth than the positive sideband. We further explore the effect of coupling and probe laser Rabi frequency on the bandwidth, which we find to be in good agreement with our model. We achieved a maximum experimental (and theoretical) bandwidth of about 11 (11) MHz and 3.5 (5) MHz for the negative and positive sidebands, respectively, from the -3dB roll-off point for optimized field parameters. This work provides insight into the bandwidth-limiting features of Rydberg atom receivers and points the way towards further optimization of their response.

physics.atom-ph↗
arXiv2024

Independent Rydberg Atom Sensing using a Dual-Ladder Scheme

Rydberg atom-based electric field sensing can provide all-optical readout of radio frequency fields in a dielectric environment. However, because a single set of optical fields is typically used to prepare the Rydberg state and read out its response to RF fields, it is challenging to perform simultaneous and independent measurements of the RF field(s). Here we show that using two independent schemes to prepare and read out the same Rydberg state can be used to perform independent measurements in general, which we demonstrate specifically by resolving the the RF polarization. We expect this work will be useful for fiber-coupled sensor heads where spatial multiplexing is challenging, as well as for complex multi-level sensing schemes.

physics.atom-ph↗
arXiv2024

Investigation of fluorescence versus transmission readout for three-photon Rydberg excitation used in electrometry

We present a three-photon based fluorescence readout method where the strength of the fluorescence scales with the strength of the radio-frequency (RF) field being applied. We compare this method to conventional three-photon electromagnetically-induced transparency (EIT) and electromagnetically-induced absorption (EIA). Our demonstrated EIA/EIT sensitivity in the collinear three-photon Cesium system is the best reported to date at roughly 30 uVm^{-1}Hz^{-1/2}. The fluorescence is nearly 4 fold better in sensitivity compared to EIA/EIT readout.

quant-ph↗
arXiv2023

Zeeman-resolved Autler-Townes splitting in Rydberg atoms with tunable resonances and a single transition dipole moment

Applying a magnetic field as a method for tuning the frequency of Autler-Townes splitting for Rydberg electrometry has recently been demonstrated. In this paper we provide a theoretical understanding of EIT signals in the presence of a large magnetic field, as well as demonstrate some advantages of this technique over traditional Autler-Townes based electrometry. We show that a strong magnetic field provides a well-defined quantization axis regardless of the optical field polarizations, we demonstrate that by separating the $m_J$ levels of the Rydberg state we can perform an Autler-Townes splitting with a single participating dipole moment, and we demonstrate recovery of signal strength by populating a single $m_J$ level using circularly polarized light.

physics.atom-ph↗
arXiv2023

High angular momentum coupling for enhanced Rydberg-atom sensing in the VHF band

Recent advances in Rydberg atom electrometry detail promising applications in radio frequency (RF) communications. Presently, most applications use carrier frequencies greater than 1~GHz where resonant Autler-Townes splitting provides the highest sensitivity. This letter documents a series of experiments with Rydberg atomic sensors to collect and process waveforms from the automated identification system (AIS) used in maritime navigation in the Very High Frequency (VHF) band. Detection in this band is difficult with conventional resonant Autler-Townes based Rydberg sensing and requires a new approach. We show the results from a new method called High Angular Momentum Matching Excited Raman (HAMMER), which enhances low frequency detection and exhibits superior sensitivity compared to the traditional AC Stark effect. From measurements of electromagnetically induced transparency (EIT) in rubidium and cesium vapor cells, we show the relationship between incident electric field strength and observed signal-to-noise ratio and find that the sensitivity of the HAMMER scheme in rubidium achieved an equivalent single VHF tone sensitivity of $\mathrm{100~μV/m/\sqrt{Hz}}$. With these results, we estimate the usable range of the atomic vapor cell antenna for AIS waveforms given current technology and detection techniques.

physics.atom-ph↗
arXiv2023

Phase-Resolved Rydberg Atom Field Sensing using Quantum Interferometry

Although Rydberg atom-based electric field sensing provides key advantages over traditional antenna-based detection, it remains limited by the need for a local oscillator (LO) for low-field and phase resolved detection. In this work, we demonstrate that closed-loop quantum interferometric schemes can be used to generate a system-internal reference that can directly replace an external LO for Rydberg field sensing. We reveal that this quantum-interferometrically defined internal reference phase and frequency can be used analogously to a traditional LO for atom-based down-mixing to an intermediate frequency for lock-in phase detection. We demonstrate that this LO-equivalent functionality provides analogous benefits to an LO, including full 360$^\circ$ phase resolution as well as improved sensitivity. The general applicability of this approach is confirmed by demodulating a four phase-state signal broadcast on the atoms. Our approach opens up new sensing schemes and provides a clear path towards all-optical Rydberg atom sensing implementations.

physics.atom-ph↗
arXiv2023

EIT spectra of Rydberg atoms dressed with dual-tone radio-frequency fields

We examine spectral signatures of Rydberg atoms driven with near-resonant dual-tone radio-frequency (RF) fields in the regime of strong driving. We experimentally demonstrate and theoretically model a variety of nonlinear and multiphoton phenomena in the atomic Rydberg response that manifest in the EIT spectra. Our results echo previous studies of two-level atoms driven with bichromatic optical fields. In comparison to the optical studies, the RF-driven Rydberg system utilizes a more complex excitation pathway, and electromagnetic fields from two different spectral regimes: a two-photon optical excitation continuously creates highly excited Rydberg atoms, while RF fields drive resonant coupling between the Rydberg levels and generate strong mixing. Yet, our spectra reflect nearly identical effects of the dual-tone RF fields on the atomic Rydberg observables, showing detuning-dependent splittings and Rabi frequency dependent peak numbers and relative strengths, and avoided crossings at subharmonic resonances. We thus validate previous two-state models in this more complex physical system. In the context of Rydberg electrometry, we use these investigations to explore a technique where we tune a known RF field to observe spectra which give frequency and power of an unknown RF field using the complex dual-tone spectra.

physics.atom-ph↗
arXiv2023

Inverse Transform Sampling for Efficient Doppler-Averaged Spectroscopy Simulations

We present a thermal velocity sampling method for calculating Doppler-broadened atomic spectra, which more efficiently reaches a smooth limit than regular velocity weighted sampling. The method uses equal-population sampling of the 1-D thermal distribution, sampling the 'inverse transform' of the cumulative distribution function, and is broadly applicable to normal distributions. We also discuss efficiencies from eliminating velocity classes which don't significantly contribute to observed atomic lines, and comment on the application of this method in 2- and 3-dimensions.

physics.atom-ph↗
arXiv2023

Detection of HF and VHF Fields through Floquet Sideband Gaps by `Rabi Matching' Dressed Rydberg Atoms

Radio frequencies in the HF and VHF (3 MHz to 300 MHz) bands are challenging for Rydberg atom-based detection schemes, as resonant detection requires exciting the atoms to extremely high energy states. We demonstrate a method for detecting and measuring radio frequency (RF) carriers in the HF and VHF bands via a controlled Autler-Townes line splitting. Using a resonant, high-frequency (GHz) RF field, the absorption signal from Townes-Merrit sidebands created by a low frequency, non-resonant RF field can be enhanced. Notably, this technique uses a measurement of the optical frequency separation of an avoided crossing to determine the amplitude of a non-resonant, low frequency RF field. This technique also provides frequency-selective measurements of low frequency RF electric fields. To show this, we demonstrate amplitude modulated signal transduction on a low frequency VHF carrier. We further demonstrate reception of multiple tones simultaneously, creating a Rydberg `spectrum analyzer' over the VHF range.

physics.atom-ph↗