arXiv subjects

Christopher Mudry

Publications and source records attributed to Christopher Mudry.

At least 37 records · Page 2Linked to original sources

arXiv2018

Giant pressure dependence and dimensionality switching in a metal-organic quantum antiferromagnet

We report an extraordinary pressure dependence of the magnetic interactions in the metal-organic system [(CuF$_2$(H$_2$O)$_2$)$_2$pyrazine]. At zero pressure, this material realizes a quasi-two-dimensional (Q2D) spin-1/2 square-lattice Heisenberg antiferromagnet. By high-pressure, high-field susceptibility measurements we show that the dominant exchange parameter is reduced continuously by a factor of 2 upon compression. Above 18 kbar, a phase transition occurs, inducing an orbital re-ordering that switches the dimensionality, transforming the Q2D lattice into weakly coupled chains (Q1D). We explain the microscopic mechanisms for both phenomena by combining detailed x-ray and neutron diffraction results with quantitative modeling using spin-polarized density functional theory.

cond-mat.mtrl-sci↗

arXiv2017

Fractional Abelian topological phases of matter for fermions in two-dimensional space

These notes constitute chapter 7 from "l'Ecole de Physique des Houches" Session CIII, August 2014 dedicated to Topological Aspects of Condensed matter physics. The tenfold way in quasi-one-dimensional space is presented. The method of chiral Abelian bosonization is reviewed. It is then applied to the stability analysis for the edge theory in symmetry class AII, and for the construction of two-dimensional topological phases from coupled wires.

cond-mat.str-el↗

arXiv2017

Weyl-type topological phase transitions in fractional quantum Hall like systems

We develop a method to characterize topological phase transitions for strongly correlated Hamiltonians defined on two-dimensional lattices based on the many-body Berry curvature. Our goal is to identify a class of quantum critical points between topologically nontrivial phases with fractionally quantized Hall (FQH) conductivity and topologically trivial gapped phases through the discontinuities of the many-body Berry curvature in the so-called flux Brillouin zone (fBZ), the latter being defined by imposing all possible twisted boundary conditions. For this purpose, we study the finite-size signatures of several quantum phase transitions between fractional Chern insulators and charge-ordered phases for two-dimensional lattices by evaluating the many-body Berry curvature numerically using exact diagonalization. We observe degeneracy points (nodes) of many-body energy levels at high-symmetry points in the fBZ, accompanied by diverging Berry curvature. We find a correspondence between the number and order of these nodal points, and the change of the topological invariants of the many-body ground states across the transition, in close analogy with Weyl nodes in non-interacting band structures. This motivates us to apply a scaling procedure, originally developed for non-interacting systems, for the Berry curvature at the nodal points. This procedure offers a useful tool for the classification of topological phase transitions in interacting systems harboring FQH-like topological order.

cond-mat.str-el↗

arXiv2017

A model of chiral spin liquids with Abelian and non-Abelian topological phases

We present a two-dimensional lattice model for quantum spin-1/2 for which the low-energy limit is governed by four flavors of strongly interacting Majorana fermions. We study this low-energy effective theory using two alternative approaches. The first consists of a mean-field approximation. The second consists of a Random Phase approximation (RPA) for the single-particle Green's functions of the Majorana fermions built from their exact forms in a certain one-dimensional limit. The resulting phase diagram consists of two competing chiral phases, one with Abelian and the other with non-Abelian topological order, separated by a continuous phase transition. Remarkably, the Majorana fermions propagate in the two-dimensional bulk, as in the Kitaev model for a spin liquid on the honeycomb lattice. We identify the vison fields, which are mobile (they are static in the Kitaev model) domain walls propagating along only one of the two space directions.

cond-mat.str-el↗

arXiv2016

Multiferroic magnetic spirals induced by random magnetic exchanges

Multiferroism can originate from the breaking of inversion symmetry caused by magnetic-spiral order. The usual mechanism for stabilizing a magnetic spiral is competition between magnetic exchange interactions differing by their range and sign, such as nearest-neighbor and next-nearest- neighbor interactions. Since the latter are usually weak the onset temperatures for multiferroism via this mechanism are typically low. By considering a realistic model for YBaCuFeO$_5$ we propose an alternative mechanism for magnetic-spiral order, and hence for multiferroism, that occurs at much higher temperatures. We show using Monte-Carlo simulations and electronic structure calculations based on density functional theory that the Heisenberg model on a geometrically non-frustrated lattice with only nearest-neighbor interactions can have a spiral phase up to high temperature when frustrating bonds are introduced randomly along a single crystallographic direction as caused, e.g., by a particular type of chemical disorder. This long-range correlated pattern of frustration avoids ferroelectrically inactive spin glass order. Finally, we provide an intuitive explanation for this mechanism and discuss its generalization to other materials.

cond-mat.mtrl-sci↗

arXiv2016

Coupled spin-1/2 ladders as microscopic models for non-Abelian chiral spin liquids

We construct a two-dimensional (2D) lattice model that is argued to realize a gapped chiral spin liquid with (Ising) non-Abelian topological order. The building blocks are spin-1/2 two-leg ladders with $SU(2)$-symmetric spin-spin interactions. The two-leg ladders are then arranged on rows and coupled through SU(2)-symmetric interactions between consecutive ladders. The intra-ladder interactions are tuned so as to realize the c = 1/2 Ising conformal field theory, a fact that we establish numerically via Density Matrix Renormalization Group (DMRG) studies. Time-reversal breaking inter-ladder interactions are tuned so as to open a bulk gap in the 2D lattice system. This 2D system supports gapless chiral edge modes with Ising non-Abelian excitations but no charge excitations, in contrast to the Pfaffian non-Abelian fractional quantum Hall state.

cond-mat.str-el↗

arXiv2016

Heavy going

Chiral symmetry breaking is imaged in graphene which, through a mechanism analogous to mass generation in quantum electrodynamics, could provide a means for making it semiconducting.

cond-mat.mtrl-sci↗

arXiv2016

Wire constructions of Abelian topological phases in three or more dimensions

Coupled-wire constructions have proven to be useful tools to characterize Abelian and non-Abelian topological states of matter in two spatial dimensions. In many cases, their success has been complemented by the vast arsenal of other theoretical tools available to study such systems. In three dimensions, however, much less is known about topological phases. Since the theoretical arsenal in this case is smaller, it stands to reason that wire constructions, which are based on one-dimensional physics, could play a useful role in developing a greater microscopic understanding of three-dimensional topological phases. In this paper, we provide a comprehensive strategy, based on the geometric arrangement of commuting projectors in the toric code, to generate and characterize coupled-wire realizations of strongly-interacting three-dimensional topological phases. We show how this method can be used to construct pointlike and linelike excitations, and to determine the topological degeneracy. We also point out how, with minor modifications, the machinery already developed in two dimensions can be naturally applied to study the surface states of these systems, a fact that has implications for the study of surface topological order. Finally, we show that the strategy developed for the construction of three-dimensional topological phases generalizes readily to arbitrary dimensions, vastly expanding the existing landscape of coupled-wire theories. Throughout the paper, we discuss $\mathbb{Z}^{\,}_m$ topological order in three and four dimensions as a concrete example of this approach, but the approach itself is not limited to this type of topological order.

cond-mat.str-el↗

arXiv2016

Non-Abelian topological spin liquids from arrays of quantum wires or spin chains

We construct two-dimensional non-Abelian topologically ordered states by strongly coupling arrays of one-dimensional quantum wires via interactions. In our scheme, all charge degrees of freedom are gapped, so the construction can use either quantum wires or quantum spin chains as building blocks, with the same end result. The construction gaps the degrees of freedom in the bulk, while leaving decoupled states at the edges that are described by conformal field theories (CFT) in $(1+1)$-dimensional space and time. We consider both the cases where time-reversal symmetry (TRS) is present or absent. When TRS is absent, the edge states are chiral and stable. We prescribe, in particular, how to arrive at all the edge states described by the unitary CFT minimal models with central charges $c<1$. These non-Abelian spin liquid states have vanishing quantum Hall conductivities, but non-zero thermal ones. When TRS is present, we describe scenarios where the bulk state can be a non-Abelian, non-chiral, and gapped quantum spin liquid, or a gapless one. In the former case, we find that the edge states are also gapped. The paper provides a brief review of non-Abelian bosonization and affine current algebras, with the purpose of being self-contained. To illustrate the methods in a warm-up exercise, we recover the ten-fold way classification of two-dimensional non-interacting topological insulators using the Majorana representation that naturally arises within non-Abelian bosonization. Within this scheme, the classification reduces to counting the number of null singular values of a mass matrix, with gapless edge modes present when left and right null eigenvectors exist.

cond-mat.str-el↗

arXiv2016

Wire deconstructionism of two-dimensional topological phases

A scheme is proposed to construct integer and fractional topological quantum states of fermions in two spatial dimensions. We devise models for such states by coupling wires of non-chiral Luttinger liquids of electrons, that are arranged in a periodic array. Which inter-wire couplings are allowed is dictated by symmetry and the compatibility criterion that they can simultaneously acquire a finite expectation value, opening a spectral gap between the ground state(s) and all excited states in the bulk. First, with these criteria at hand, we reproduce the tenfold classification table of integer topological insulators, where their stability against interactions becomes immediately transparent in the Luttinger liquid description. Second, we construct an example of a strongly interacting fermionic topological phase of matter with short-range entanglement that lies outside of the tenfold classification. Third, we expand the table to long-range entangled topological phases with intrinsic topological order and fractional excitations.

cond-mat.str-el↗

arXiv2015

Breakdown of the topological classification Z for gapped phases of noninteracting fermions by quartic interactions

The conditions for both the stability and the breakdown of the topological classification of gapped ground states of noninteracting fermions, the tenfold way, in the presence of quartic fermion-fermion interactions are given for any dimension of space. This is achieved by encoding the effects of interactions on the boundary gapless modes in terms of boundary dynamical masses. Breakdown of the noninteracting topological classification occurs when the quantum nonlinear sigma models for the boundary dynamical masses favor quantum disordered phases. For the tenfold way, we find that (i) the noninteracting topological classification $\mathbb{Z}^{\,}_{2}$ is always stable, (ii) the noninteracting topological classification $\mathbb{Z}$ in even dimensions is always stable, (iii) the noninteracting topological classification $\mathbb{Z}$ in odd dimensions is unstable and reduces to $\mathbb{Z}^{\,}_{N}$ that can be identified explicitly for any dimension and any defining symmetries. We also apply our method to the three-dimensional topological crystalline insulator SnTe from the symmetry class AII$+R$, for which we establish the reduction $\mathbb{Z}\to\mathbb{Z}^{\,}_{8}$ of the noninteracting topological classification.

cond-mat.str-el↗

arXiv2015

Anderson localization and the topology of classifying spaces

We construct the generic phase diagrams encoding the topologically distinct localized and delocalized phases of noninteracting fermionic quasiparticles for any symmetry class from the tenfold way in one, two, and three dimensions. To this end, we start from a massive Dirac Hamiltonian perturbed by a generic disorder for any dimension of space and for any one of the ten symmetry classes from the tenfold way. The physics of Anderson localization is then encoded by a two-dimensional phase diagram that we deduce from the topology of the space of normalized Dirac masses. This approach agrees with previously known results and gives an alternative explanation for the even-odd effect in the one-dimensional chiral symmetry classes. We also give a qualitative explanation for the Gade singularity and Griffiths effects in the density of states using the first homotopy group of the normalized Dirac masses in two dimensions. Finally, this approach is used to analyze the stability of massless Dirac fermions on the surface of three-dimensional topological crystalline insulators.

cond-mat.mes-hall↗

arXiv2015

Topological BF theory of the quantum hydrodynamics of incompressible polar fluids

We analyze a hydrodynamical model of a polar fluid in (3+1)-dimensional spacetime. We explore a spacetime symmetry -- volume preserving diffeomorphisms -- to construct an effective description of this fluid in terms of a topological BF theory. The two degrees of freedom of the BF theory are associated to the mass (charge) flows of the fluid and its polarization vorticities. We discuss the quantization of this hydrodynamic theory, which generically allows for fractionalized excitations. We propose an extension of the Girvin-MacDonald-Platzman algebra to (3+1)-dimensional spacetime by the inclusion of the vortex-density operator in addition to the usual charge density operator and show that the same algebra is obeyed by massive Dirac fermions that represent the bulk of $\mathbb{Z}^{\,}_{2}$ topological insulators in three-dimensional space.

cond-mat.mes-hall↗

arXiv2014

Accessing topological order in fractionalized liquids with gapped edges

We consider manifestations of topological order in time-reversal-symmetric fractional topological liquids (TRS-FTLs), defined on planar surfaces with holes. We derive a formula for the topological ground state degeneracy of such a TRS-FTL, which applies to cases where the edge modes on each boundary are fully gapped by appropriate backscattering terms. The degeneracy is exact in the limit of infinite system size, and is given by $q^{N^{\,}_{\mathrm{h}}}$, where $N^{\,}_{\mathrm{h}}$ is the number of holes and $q$ is an integer that is determined by the topological field theory. When the degeneracy is lifted by finite-size effects, the holes realize a system of $N^{\,}_{\mathrm{h}}$ coupled spin-like $q$-state degrees of freedom. In particular, we provide examples where $\mathbb Z^{\,}_{q}$ quantum clock models are realized on the low-energy manifold of states. We also investigate the possibility of measuring the topological ground state degeneracy with calorimetry, and briefly revisit the notion of topological order in $s$-wave BCS superconductors.

cond-mat.str-el↗

arXiv2014

Fractional (Chern and topological) insulators

We review various features of interacting Abelian topological phases of matter in two spatial dimensions, placing particular emphasis on fractional Chern insulators (FCIs) and fractional topological insulators (FTIs). We highlight aspects of these systems that challenge the intuition developed from quantum Hall physics - for instance, FCIs are stable in the limit where the interaction energy scale is much larger than the band gap, and FTIs can possess fractionalized excitations in the bulk despite the absence of gapless edge modes.

cond-mat.str-el↗

arXiv2014

Effective field theory for the bulk-edge correspondence in a two-dimensional Z_2 topological insulator with Rashba interactions

We determine the effective field theory in (2+1)-dimensional space and time that captures the long wave length and low-energy limit of fermions hopping on a honeycomb lattice at half-filling when both a dominant intrinsic and subdominant Rashba spin-orbit couplings are present. This effective field theory for a Z_2 topological insulator (the Kane-Mele model at vanishing uniform and staggered chemical potentials) is a perturbation around a double Chern-Simons theory, with the U(1) gauge invariance associated to spin conservation explicitly broken due to the Rashba spin orbit coupling. Nonetheless, we find that the effective field theory has a BRST symmetry that allows us to construct the bulk-edge correspondence.

cond-mat.str-el↗

arXiv2014

Symmetry-protected entangling boundary zero modes in crystalline topological insulators

Crystalline topological insulators owe their topological character to the protection that certain boundary states acquire because of certain point-group symmetries. We first show that a Hermitian operator obeying supersymmetric quantum mechanisms (SUSY QM) delivers the entanglement spectrum. We then show that such an entanglement spectrum that is compatible with a certain point-group symmetry obeys a certain local spectral symmetry. The latter result is applied to the stability analysis of four fermionic non-interacting Hamiltonians, the last of which describes graphene with a Kekule distortion. All examples have the remarkable property that their entanglement spectra inherit a local spectral symmetry from either an inversion or reflection symmetry that guarantees the stability of gapless boundary entangling states, even though all examples fail to support protected gapless boundary states at their physical boundaries.

cond-mat.str-el↗

arXiv2014

Magnetic nano-fluctuations in a frustrated magnet

Frustrated systems exhibit remarkable properties due to the high degeneracy of their ground states. Stabilised by competing interactions, a rich diversity of typically nanometre-sized phase structures appear in polymer and colloidal systems, while the surface of ice pre-melts due to geometrically frustrated interactions. Atomic spin systems where magnetic interactions are frustrated by lattice geometry provide a fruitful source of emergent phenomena, such as fractionalised excitations analogous to magnetic monopoles. The degeneracy inherent in frustrated systems may prevail all the way down to absolute zero temperature, or it may be lifted by small perturbations or entropic effects. In the geometrically frustrated Ising--like magnet Ca3Co2O6, we follow the temporal and spatial evolution of nanoscale magnetic fluctuations firmly embedded inside the spin--density--wave magnetic structure. These fluctuations are a signature of a competing ferrimagnetic phase with an incommensurability that is different from, but determined by the host. As the temperature is lowered, the fluctuations slow down into a super-paramagnetic regime of stable spatiotemporal nano-structures.

cond-mat.str-el↗