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Christopher Pasco

Publications and source records attributed to Christopher Pasco.

4 recordsLinked to original sources

Ta-based S-I-S junctions for integrated superconducting Electronics

In this work, we have presented S-I-S Josephson junctions with $\rmα$-Ta electrodes and a ${\rm TaO}_x$ barrier. We grew base and top $α$-Ta electrodes using seed layer engineering, showing both Nb and ${\rm TaN}_x$ are viable seed layer choices, and particularly emphasize that at room temperature a re-seed layer is required to nucleate $\rmα$-Ta for the top electrode. However, we note that the choice of seed layer can have subtle implications on the electrical tunneling behavior of the junctions. We used room-temperature probing of variable junction areas, combined with Ambegaokar-Baratoff physics, to characterize the wafer scale critical current densities. For 0.4 $μ$m$^2$ junctions, we found junction spreads as low as 2.0% across the 20 x 20 mm chip relevant for device performance. The entire process was carried out using standard industry foundry processing using 150 mm wafer tooling, which is an important step towards proving that Ta-based junctions can be implemented at scale. We have successfully fabricated and tested junctions with $\rmα$-Ta electrodes and a ${\rm TaO}_x$ insulating tunnel barrier, demonstrating that this is a material platform which merits further investigation and studies for potential application in classical and quantum superconducting technologies.

cond-mat.supr-con↗

An Algorithm for Subtraction of Doublet Emission Lines in Angle-Resolved Photoemission Spectroscopy

Plasma discharge lamps are widely utilized in the practice of angle-resolved photoemission spectroscopy (ARPES) experiments as narrow-linewidth ultraviolet photon sources. However, many emission lines such as Ar-I, Ne-I, and Ne-II have closely spaced doublet emission lines, which result in superimposed replica on the measured ARPES spectra. Here, we present a simple method for subtracting the contribution of these doublet emission lines from photoemission spectra. Benchmarking against ARPES spectra of well-characterized 2D materials, we demonstrate that this algorithm manages to subtract the doublet signal and reproduce the key features of the monochromated He-I$α$ spectra in a physically sound manner that reliably reproduces quantifiable dispersion relations and quasiparticle lifetimes.

physics.ins-det↗

Magnetic phase crossover in strongly correlated EuMn2P2

Strong electron correlations underlie a plethora of electronic and magnetic components and devices and are often used to identify and probe novel ground states in quantum materials. Herein we report a magnetic phase crossover in EuMn2P2, an insulator which shows Eu antiferromagnetism at TN=17K, but no phase transition attributed to Mn magnetism. The absence of a Mn magnetic phase transition contrasts with the formation of long-range Mn order at T=130K in isoelectronic EuMn2Sb2 and EuMn2As2. Temperature-dependent specific heat and 31P NMR measurements provide evidence for the development of Mn magnetic correlations from T=250-100 K. Density functional theory calculations demonstrate an unusual sensitivity of the band structure to the details of the imposed Mn and Eu magnetic order, with antiferromagnetic Mn order required to recapitulate an insulating state. Our results imply a picture in which long range Mn magnetic order is suppressed by chemical pressure, but that magnetic correlations persist, narrowing bands and producing an insulating state.

cond-mat.str-el↗

Image registration of low signal-to-noise cryo-STEM data

Combining multiple fast image acquisitions to mitigate scan noise and drift artifacts has proven essential for picometer precision, quantitative analysis of atomic resolution scanning transmission electron microscopy (STEM) data. For very low signal-to-noise ratio (SNR) image stacks - frequently required for undistorted imaging at liquid nitrogen temperatures - image registration is particularly delicate, and standard approaches may either fail, or produce subtly specious reconstructed lattice images. We present an approach which effectively registers and averages image stacks which are challenging due to their low-SNR and propensity for unit cell misalignments. Registering all possible image pairs in a multi-image stack leads to significant information surplus. In combination with a simple physical picture of stage drift, this enables identification of incorrect image registrations, and determination of the optimal image shifts from the complete set of relative shifts. We demonstrate the effectiveness of our approach on experimental, cryogenic STEM datasets, highlighting subtle artifacts endemic to low-SNR lattice images and how they can be avoided. High-SNR average images with information transfer out to 0.72 A are achieved at 300 kV and with the sample cooled to near liquid nitrogen temperature.

eess.SP↗