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Christos Panagopoulos

Publications and source records attributed to Christos Panagopoulos.

At least 19 recordsLinked to original sources

Thermal Hall Resistivity as a Unifying Description of Phonon Thermal Hall Effect in Various Insulators

A considerable phonon thermal Hall effect was recently discovered across a diverse collection of materials. To clarify this enigmatic thermal Hall response in various insulators, we investigate the doped Mott insulator La$_{5/3}$Sr$_{1/3}$NiO$_4$ as an example material system and reveal a characteristic phonon-dominated thermal Hall effect. As a sensitive probe of the transverse thermal response, the thermal Hall resistivity $w_{xy}$ exhibits an insulating-like temperature dependence $w_{xy}(T)$, a linear magnetic-field dependence $w_{xy}(H)$ near $H=0$, and a $T$-linear thermal Hall angle at low temperatures. The presence of similar phenomena across a series of insulators suggests that $w_{xy}$ serves as a unifying description of phonon thermal Hall effect, corroborated by an apparent correlation between the insulating-like $w_{xy}(T)$ and material's localized electronic state.

cond-mat.str-el

Magnon Superlattices around Skyrmions in Frustrated Magnets

Dynamic and stable magnetic textures offer a powerful platform for controlling magnon states in the broader context of spin electronics. In this work, we uncover a novel class of dynamical, crystal-like localization patterns in real space, arising from the hybridization of magnons with topologically non-trivial spin textures that possess helicity as an internal degree of freedom. By tuning the magnon wavelength to match the size of these textures, specifically, atomic-scale skyrmions in centrosymmetric frustrated magnets, we achieve strong interference effects. This leads to the emergence of magnon superlattices, shaped by the internal skyrmion structure and the underlying Mexican-hat magnon dispersion. Furthermore, helicity-driven nonlinear dynamics give rise to dispersive magnon bands with nontrivial Chern numbers within the first magnon gap. These findings provide fundamental insights into magnon behavior in complex spin environments and establish frustrated magnets as a versatile platform for manipulating spin excitations at the atomic scale.

cond-mat.mes-hall

Colloquium: Quantum Properties and Functionalities of Magnetic Skyrmions

Competing magnetic interactions may stabilize smooth magnetization textures that can be characterized by a topological winding number. Such textures, which are spatially localized within a two-dimensional plane, are commonly known as skyrmions. On the classical level, their significance for fundamental science and their potential for applications, ranging from spintronic devices to unconventional computation platforms, have been intensively investigated in recent years. This Colloquium considers quantum effects associated with skyrmion textures: their theoretical origins, the experimental and material challenges associated with their detection, and the promise of exploiting them for quantum operations. Starting with classical skyrmions, we discuss their magnon and electron excitations and show how hybrid architectures offer new platforms for engineering quantum orders, including topological superconductivity. We then focus on the quantization of the skyrmion texture itself and formulate the long-time skyrmion dynamics in terms of collective coordinates. Next, we discuss the quantization of helicity and phenomena of macroscopic quantum tunneling: key concepts that fundamentally distinguish quantum skyrmions from their classical counterparts. Looking ahead, we propose material classes suitable for the realization of skyrmions in quantum spin systems and identify device architectures with the promise of achieving quantum operations. We close by addressing the advances in experimental methods which will be a prerequisite for resolving the quantum aspects of topological spin patterns, sensing their local dynamical response, and achieving their predicted functionalities in magnetic systems.

cond-mat.mes-hall

Roadmap for Unconventional Computing with Nanotechnology

In the "Beyond Moore's Law" era, with increasing edge intelligence, domain-specific computing embracing unconventional approaches will become increasingly prevalent. At the same time, adopting a variety of nanotechnologies will offer benefits in energy cost, computational speed, reduced footprint, cyber resilience, and processing power. The time is ripe for a roadmap for unconventional computing with nanotechnologies to guide future research, and this collection aims to fill that need. The authors provide a comprehensive roadmap for neuromorphic computing using electron spins, memristive devices, two-dimensional nanomaterials, nanomagnets, and various dynamical systems. They also address other paradigms such as Ising machines, Bayesian inference engines, probabilistic computing with p-bits, processing in memory, quantum memories and algorithms, computing with skyrmions and spin waves, and brain-inspired computing for incremental learning and problem-solving in severely resource-constrained environments. These approaches have advantages over traditional Boolean computing based on von Neumann architecture. As the computational requirements for artificial intelligence grow 50 times faster than Moore's Law for electronics, more unconventional approaches to computing and signal processing will appear on the horizon, and this roadmap will help identify future needs and challenges. In a very fertile field, experts in the field aim to present some of the dominant and most promising technologies for unconventional computing that will be around for some time to come. Within a holistic approach, the goal is to provide pathways for solidifying the field and guiding future impactful discoveries.

cs.ET

Skyrmion Qubits: Challenges For Future Quantum Computing Applications

Magnetic nano-skyrmions develop quantized helicity excitations, and the quantum tunneling between nano-skyrmions possessing distinct helicities is indicative of the quantum nature of these particles. Experimental methods capable of non-destructively resolving the quantum aspects of topological spin textures, their local dynamical response, and their functionality now promise practical device architectures for quantum operations. With abilities to measure, engineer, and control matter at the atomic level, nano-skyrmions present opportunities to translate ideas into solid-state technologies. Proof-of-concept devices will offer electrical control over the helicity, opening a promising new pathway towards functionalizing collective spin states for the realization of a quantum computer based on skyrmions. This Perspective aims to discuss developments and challenges in this new research avenue in quantum magnetism and quantum information.

cond-mat.mes-hall

Doubling of the superconducting transition temperature in ultra-clean wafer-scale aluminum nanofilms

Superconducting properties of thin films can be vastly different from those of bulk materials. Seminal work has shown the critical temperature Tc of elemental superconductors decreases with decreasing film thickness when the normal-state sheet resistance is lower than the quantum resistance h/(4e2). Sporadic examples on disordered films, however, hinted an enhancement in Tc although, structural and strain characterization was not possible since samples were prepared on a cold substrate in situ. To clarify the role of reduced dimensionality and disorder on the superconducting properties of thin films we employed molecular beam epitaxy to grow wafer-scale high-quality aluminum (Al) nanofilms with normal-state sheet resistance at least 20 times lower than h/(4e2) and investigated their electronic and structural properties ex situ. Defying general expectations, Tc increases with decreasing Al film thickness, reaching 2.4 K for 3.5-nm-thick Al film grown on GaAs: twice that of bulk Al (1.2 K). DFT calculations indicate surface phonon softening impacts superconductivity in pure ultra-thin films, offering a new route for materials engineering in two dimensions.

cond-mat.supr-con

Skyrmion Helicity: Quantization and Quantum Tunneling Effects

We derive the quantization of magnetic helicity in the solid-state and demonstrate tunable macroscopic quantum tunneling, coherence, and oscillation for a skyrmion spin texture stabilized in frustrated magnets. We also discuss the parameter space for the experimental realization of quantum effects. Typically, for a skyrmion of 5 nm radius, quantum tunneling between two macroscopic states with distinct helicities occurs with an inverse escape rate within seconds below 100 mK, and an energy splitting in the MHz regime. Feasibility of quantum tunneling of an ensemble of magnetic spins inspires new platforms for quantum operations utilizing topologically protected chiral spin configurations.

cond-mat.mes-hall

Tailoring magnetic order via atomically stacking 3d/5d electrons

The ability to tune magnetic orders, such as magnetic anisotropy and topological spin texture, is desired in order to achieve high-performance spintronic devices. A recent strategy has been to employ interfacial engineering techniques, such as the introduction of spin-correlated interfacial coupling, to tailor magnetic orders and achieve novel magnetic properties. We chose a unique polar-nonpolar LaMnO3/SrIrO3 superlattice because Mn (3d)/Ir (5d) oxides exhibit rich magnetic behaviors and strong spin-orbit coupling through the entanglement of their 3d and 5d electrons. Through magnetization and magnetotransport measurements, we found that the magnetic order is interface-dominated as the superlattice period is decreased. We were able to then effectively modify the magnetization, tilt of the ferromagnetic easy axis, and symmetry transition of the anisotropic magnetoresistance of the LaMnO3/SrIrO3 superlattice by introducing additional Mn (3d) and Ir (5d) interfaces. Further investigations using in-depth first-principles calculations and numerical simulations revealed that these magnetic behaviors could be understood by the 3d/5d electron correlation and Rashba spin-orbit coupling. The results reported here demonstrate a new route to synchronously engineer magnetic properties through the atomic stacking of different electrons, contributing to future applications.

cond-mat.str-el

Skyrmion Qubits: A New Class of Quantum Logic Elements Based on Nanoscale Magnetization

We introduce a new class of primitive building blocks for realizing quantum logic elements based on nanoscale magnetization textures called skyrmions. In a skyrmion qubit, information is stored in the quantum degree of helicity, and the logical states can be adjusted by electric and magnetic fields, offering a rich operation regime with high anharmonicity. By exploring a large parameter space, we propose two skyrmion qubit variants depending on their quantized state. We discuss appropriate microwave pulses required to generate single-qubit gates for quantum computing, and skyrmion multiqubit schemes for a scalable architecture with tailored couplings. Scalability, controllability by microwave fields, operation time scales, and readout by nonvolatile techniques converge to make the skyrmion qubit highly attractive as a logical element of a quantum processor.

cond-mat.mes-hall

Microwave resonances of magnetic skyrmions in thin film multilayers

Non-collinear magnets exhibit a rich array of dynamic properties at microwave frequencies. They can host nanometre-scale topological textures known as skyrmions, whose spin resonances are expected to be highly sensitive to their local magnetic environment. Here, we report a magnetic resonance study of an [Ir/Fe/Co/Pt] multilayer hosting Néel skyrmions at room temperature. Experiments reveal two distinct resonances of the skyrmion phase during in-plane ac excitation, with frequencies between 6-12 GHz. Complementary micromagnetic simulations indicate that the net magnetic dipole moment rotates counterclockwise (CCW) during both resonances. The magnon probability distribution for the lower-frequency resonance is localised within isolated skyrmions, unlike the higher-frequency mode which principally originates from areas between skyrmions. However, the properties of both modes depend sensitively on the out-of-plane dipolar coupling, which is controlled via the ferromagnetic layer spacing in our heterostructures. The gyrations of stable isolated skyrmions reported in this room temperature study encourage the development of new material platforms and applications based on skyrmion resonances. Moreover, our material architecture enables the resonance spectra to be tuned, thus extending the functionality of such applications over a broadband frequency range.

cond-mat.mes-hall

Magnetization Reversal Signatures of Hybrid and Pure Néel Skyrmions in Thin Film Multilayers

We report a study of the magnetization reversals and skyrmion configurations in two systems - Pt/Co/MgO and Ir/Fe/Co/Pt multilayers, where magnetic skyrmions are stabilized by a combination of dipolar and Dzyaloshinskii-Moriya interactions (DMI). First Order Reversal Curve (FORC) diagrams of low-DMI Pt/Co/MgO and high-DMI Ir/Fe/Co/Pt exhibit stark differences, which are identified by micromagnetic simulations to be indicative of hybrid and pure Néel skyrmions, respectively. Tracking the evolution of FORC features in multilayers with dipolar interactions and DMI, we find that the negative FORC valley, typically accompanying the positive FORC peak near saturation, disappears under both reduced dipolar interactions and enhanced DMI. As these conditions favor the formation of pure Neel skyrmions, we propose that the resultant FORC feature - a single positive FORC peak near saturation - can act as a fingerprint for pure Néel skyrmions in multilayers. Our study thus expands on the utility of FORC analysis as a tool for characterizing spin topology in multilayer thin films.

cond-mat.mes-hall

Current-induced spin torques on single GdFeCo magnetic layers

Spintronics exploits spin-orbit coupling (SOC) to generate spin currents, spin torques, and, in the absence of inversion symmetry, Rashba, and Dzyaloshinskii-Moriya interactions (DMI). The widely used magnetic materials, based on 3d metals such as Fe and Co, possess a small SOC. To circumvent this shortcoming, the common practice has been to utilize the large SOC of nonmagnetic layers of 5d heavy metals (HMs), such as Pt, to generate spin currents by Spin Hall Effect (SHE) and, in turn, exert spin torques on the magnetic layers. Here, we introduce a new class of material architectures, excluding nonmagnetic 5d HMs, for high-performance spintronics operations. We demonstrate very strong current-induced torques exerted on single GdFeCo layers due to the combination of large SOC of the Gd 5d states, and inversion symmetry breaking mainly engineered by interfaces. These "self-torques" are enhanced around the magnetization compensation temperature (close to room temperature) and can be tuned by adjusting the spin absorption outside the GdFeCo layer. In other measurements, we determine the very large emission of spin current from GdFeCo. This material platform opens new perspectives to exert "self-torques" on single magnetic layers as well as to generate spin currents from a magnetic layer.

cond-mat.mes-hall

Physical foundations and basic properties of magnetic skyrmions

Magnetic skyrmions (or vortices) are spatially inhomogeneous spin textures localized in nanoscale cylindrical regions. Topological protection and small size make skyrmions especially attractive for the study of spin topology and technologies wherein information is carried by the electron spin further to, or instead of the electron charge. Despite achievements in the synthesis of materials where axisymmetric magnetic skyrmions can be stabilized and characterized, there is disproportionate progress in elucidating the basic properties. The Perspective aims to bridge this gap and deliver an intelligible guide on the physical principles governing these magnetic whirls.

cond-mat.mes-hall

The emergence of magnetic skyrmions

This is a narrative of the basic theoretical ideas of axisymmetric two-dimensional solitons and of their connection to basic experiments on magnetic compounds. A shortened and edited version appeared in Physics Today.

cond-mat.mes-hall

Angle-resolved broadband ferromagnetic resonance apparatus enabled through a spring-loaded sample mounting manipulator

Broadband ferromagnetic resonance is a useful technique to determine the magnetic anisotropy and study the magnetization dynamics of magnetic thin films. We report a spring-loaded sample loading manipulator for reliable sample mounting and rotation. The manipulator enables maximum signal, enhances system stability and is particularly useful for fully automated in-plane-field angle-resolved measurements. This angle-resolved broadband ferromagnetic resonance apparatus provides a viable method to study anisotropic damping and weak magnetic anisotropies, both vital for fundamental research and applications.

physics.app-ph

Stabilizing zero-field skyrmions in Ir/Fe/Co/Pt thin film multilayers by magnetic history control

We present a study of the stability of room-temperature skyrmions in [Ir/Fe/Co/Pt] thin film multilayers, using the First Order Reversal Curve (FORC) technique and magnetic force microscopy (MFM). FORC diagrams reveal irreversible changes in magnetization upon field reversals, which can be correlated with the evolution of local magnetic textures probed by MFM. Using this approach, we have identified two different mechanisms - (1) skyrmion merger and (2) skyrmion nucleation followed by stripe propagation - which facilitate magnetization reversal in a changing magnetic field. Analysing the signatures of these mechanisms in the FORC diagram allows us to identify magnetic "histories" - i.e. precursor field sweep protocols - capable of enhancing the final zero-field skyrmion density. Our results indicate that FORC measurements can play a useful role in characterizing spin topology in thin film multilayers, and are particularly suitable for identifying samples in which skyrmion populations can be stabilized at zero field.

cond-mat.mes-hall

Quadratic to linear magnetoresistance tuning in TmB4

The change of a material's electrical resistance (R) in response to an external magnetic field (B) provides subtle information for the characterization of its electronic properties and has found applications in sensor and storage related technologies. In good metals, Boltzmann's theory predicts a quadratic growth in magnetoresistance (MR) at low B, and saturation at high fields. On the other hand, a number of nonmagnetic materials with weak electronic correlation and low carrier concentration for metallicity, such as inhomogeneous conductors, semimetals, narrow gap semiconductors and topological insulators, two-dimensional electron gas (2DEG) show positive, non-saturating linear magnetoresistance (LMR). However, observation of LMR in single crystals of a good metal is rare. Here we present low-temperature, angle dependent magnetotransport in single crystals of the antiferromagnetic metal, TmB4. We observe large, positive and anisotropic MR(B), which can be tuned from quadratic to linear by changing the direction of the applied field. In view of the fact that isotropic, single crystalline metals with large Fermi surface (FS) are not expected to exhibit LMR, we attribute our observations to the anisotropic FS topology of TmB4. Furthermore, the linear MR is found to be temperature-independent, suggestive of quantum mechanical origin.

cond-mat.str-el

Degeneracy of the 1/8 plateau and antiferromagnetic phases in the Shastry-Sutherland magnet TmB4

The 1/8 fractional plateau phase (1/8-FPP) in Shastry-Sutherland Lattice (SSL) spin systems has been viewed an exemplar of emergence on an Archimedean lattice. Here we explore this phase in the Ising magnet TmB4 using high-resolution specific heat (C) and magnetization (M) in the field-temperature plane. We show that the 1/8-FPP is smoothly connected to the antiferromagnetic (AF) phase on ramping the field from H= 0. Thus, the 1/8-FPP is not a distinct ground state of TmB4. The implication of these results for Heisenberg spins on the SSL is discussed.

cond-mat.str-el