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Chuan-Feng Li

Publications and source records attributed to Chuan-Feng Li.

At least 37 records · Page 2Linked to original sources

Nonunitary Preparation of Nontrivial States from Trivial Regimes in Two-Dimensional Topological Insulators

While remarkable progress has been achieved in engineering nontrivial Hamiltonians across a wide range of physical platforms, preparing their corresponding nontrivial ground states remains a major experimental challenge. The commonly used strategy for state preparation relies on adiabatic protocols. However, when a trivial initial state is unitarily driven toward nontrivial regimes, the dynamics must cross gap-closing critical points, rendering the process intrinsically nonadiabatic, and the state remains topologically trivial. Here, we present a nonunitary method for dynamically preparing nontrivial states in two-dimensional topological insulators. By introducing dephasing noise into a slowly driven unitary evolution, we demonstrate that the topological number of the resulting dephased states can coincide with that of the target nontrivial Hamiltonian. This nearly adiabatic nonunitary state-preparation protocol provides a powerful alternative to conventional adiabatic approaches for accessing topological states.

quant-ph↗

Global-scale quantum networking using hybrid-channel quantum repeaters with relays based on a chain of balloons

Global-scale entanglement distribution has been a formidable challenge due to the unavoidable losses in communication channels. Here, we propose a novel backbone channel for quantum network based on balloon-based aerial relays. We demonstrate for the first time that the atmospheric disturbances in balloon-based channels can be almost eliminated through optimizing beam waist positions and employing a series of adaptive optics systems, which boosts the channel efficiency to -21 dB over a 10,000 km distance, outperforming satellite-based relays by 12 dB with same device parameters. We then propose a global-scale quantum networking scheme based on hybrid-channel quantum repeaters that combine ground-based quantum repeaters and balloon-based aerial relays. Servers are interconnected globally via a chain of balloons, while clients link to local servers through fiber connections, facilitating rapid client switching and network scalability. Our simulations, employing state-of-the-art Eu$^{3+}$:Y$_2$SiO$_5$ quantum memories and mature entanglement sources based on spontaneous parametric down-conversion, demonstrate an entanglement distribution rate in the sub-Hertz range between clients separated by 10,000 km. This approach offers a practical path toward global quantum networking in the near future.

quant-ph↗

Coherent Spin-Photon Interface of single PL6 Color Centers in Silicon Carbide

The PL6 color center in silicon carbide has recently emerged as a promising platform for quantum information processing, yet its coherent spin--photon interface has remained largely unexplored. Here we present a comprehensive investigation of single PL6 centers, combining spectroscopy with theoretical analysis. The excited-state fine structure is fully resolved using group-theoretical modeling and strain-dependent measurements. Under resonant excitation, we achieve a spin initialization fidelity of $99.69 \pm 0.03\%$ and a readout contrast of $98.31 \pm 1.03\%$. The spin--photon--entangled $A_2$ transition exhibits narrow optical linewidths ($\sim 180$~MHz) and a polarization visibility of $\sim 82\%$. Coherent optical driving enables Rabi frequencies up to $2.895$~GHz, while dynamical decoupling extends the spin coherence time from $0.5$~ms to $5.70$~ms. Our results establish PL6 as a competitive solid-state spin--photon interface hosted in a commercially available semiconductor platform.

quant-ph↗

Decoherence-protected entangling gates in a silicon carbide quantum node

Solid-state color centers are promising candidates for nodes in quantum network architectures. However, realizing scalable and fully functional quantum nodes, comprising both processor and memory qubits with high-fidelity universal gate operations, remains a central challenge in this field. Here, we demonstrate a fully functional quantum node in silicon carbide, where electron spins act as quantum processors and nuclear spins serve as quantum memory. Specifically, we design a pulse sequence that combines dynamical decoupling with hyperfine interactions to realize decoherence-protected universal gate operations between the processor and memory qubits. Leveraging this gate, we deterministically prepare entangled states within the quantum node, achieving a fidelity of 90%, which exceeds the fault-tolerance threshold of certain quantum network architectures. These results open a pathway toward scalable and fully functional quantum nodes based on silicon carbide.

quant-ph↗

3D imaging of the biphoton spatiotemporal wave packet

Photons are among the most important carriers of quantum information owing to their rich degrees of freedom (DoFs), including various spatiotemporal structures. The ability to characterize these DoFs, as well as the hidden correlations among them, directly determines whether they can be exploited for quantum tasks. While various methods have been developed for measuring the spatiotemporal structure of classical light fields, owing to the technical challenges posed by weak photon flux, there have so far been no reports of observing such structures in their quantum counterparts, except for a few studies limited to correlations within individual DoFs. Here, we propose and experimentally demonstrate a self-referenced, high-efficiency, and all-optical method, termed 3D imaging of photonic wave packets, for comprehensive characterization of the spatiotemporal structure of a quantum light field, i.e., the biphoton spatiotemporal wave packet. Benefiting from this developed method, we successfully observe the spatial-spatial, spectral-spectral, and spatiotemporal correlations of biphotons generated via spontaneous parametric down-conversion, revealing rich local and nonlocal spatiotemporal structure in quantum light fields. This method will further advance the understanding of the dynamics in nonlinear quantum optics and expand the potential of photons for applications in quantum communication and quantum computing.

quant-ph↗

Experimental Certification of Quantum Measurements with Maximally Mixed States

So far, certifying quantum devices from their input-output statistics, under minimal assumptions, required the preparation of specific pure quantum states. Recently, Xu et al. [Phys. Rev. Lett. 132, 140201 (2024)] have demonstrated that certain sets of quantum observables can be certified using any state of full rank. However, their method is restricted to ideal conditions. Here, we address this problem and present an experimentally robust method that eliminates the need of preparing states with high fidelity with respect to specific pure states. We demonstrate the feasibility of the method by experimentally certifying photonic devices implementing Peres' set of 24 ququart observables [J. Phys. A 24, L175 (1991)] and Yu and Oh's set of 13 qutrit observables [Phys. Rev. Lett. 108, 030402 (2012)], using maximally mixed states as input. This approach offers a crucial advantage for certifying high-dimensional quantum systems, since it works with maximally mixed and thermal states.

quant-ph↗

Informationally Complete Distributed Metrology Without a Shared Reference Frame

In quantum information processing, implementing arbitrary preparations and measurements on qubits necessitates precise information to identify a specific reference frame (RF). In space quantum communication and sensing, where a shared RF is absent, the interplay between locality and symmetry imposes fundamental restrictions on physical systems. A restriction on realizable unitary operations results in a no-go theorem prohibiting the extraction of locally encoded information in RF-independent distributed metrology. Here, we propose a reversed-encoding method applied to two copies of local-unitary-invariant network states. This approach circumvents the no-go theorem while simultaneously mitigating decoherence-like noise caused by RF misalignment, thereby enabling the complete recovery of the quantum Fisher information (QFI). Furthermore, we confirm local Bell-state measurements as an optimal strategy to saturate the QFI. Our findings pave the way for the field application of distributed quantum sensing, which is inherently subject to unknown RF misalignment and was previously precluded by the no-go theorem.

quant-ph↗

Binarisation-loophole-free observation of high-dimensional quantum nonlocality

Bell inequality tests based on high-dimensional entanglement usually require measurements that can resolve multiple possible outcomes. However, the implementation of high-dimensional multi-outcome measurements is often only emulated via a collection of ``click or no-click'' measurements. This reduction of multi-outcome measurements to binary-outcome measurements opens a loophole in high-dimensional tests Bell inequalities which can be exploited by local hidden variable models [Tavakoli et al., Phys. Rev. A 111, 042433 (2025)]. Here, we close this loophole by using four-dimensional photonic path-mode entanglement and multi-outcome detection. We test both the well-known Collins-Gisin-Linden-Massar-Popescu inequality and a related Bell inequality tailored for maximally entangled states in high-dimension. We observe violations that are large enough to also rule out any quantum model based on entanglement of lower dimension, thereby demonstrating genuinely high-dimensional nonlocality free of the binarisation loophole.

quant-ph↗

Measuring Mixed-State Topological Invariant in Open Photonic Quantum Walk

Pure-state manifestations of geometric phase are well established and have found applications across essentially all branches of physics, yet their generalization to mixed-state regimes remains largely unexplored experimentally. The Uhlmann geometric phase offers a natural extension of pure-state paradigms and can exhibit a topological character. However, observation of this invariant is impeded by the incompatibility between Uhlmann parallel transport and Hamiltonian dynamics, as well as the difficulty of preparing topologically nontrivial mixed states. To address this challenge, we report an experimentally accessible protocol for directly measuring the mixed-state topological invariant. By engineering controlled nonunitary dynamics in a photonic quantum walk, we prepare topologically nontrivial mixed states from a trivial initial state. Furthermore, by machine-learning the full density matrix in momentum space, we directly extract the quantized geometric phase of the nontrivial mixed states. These results highlight a geometric phase framework that naturally extends to open quantum systems both in and out of thermal equilibrium.

quant-ph↗

High-fidelity realisation of CNOT gate in Majorana-based optical platform

We present the experimental realisation of a robust CNOT quantum gate using Majorana zero modes simulated on a photonic platform. Three Kitaev chains supporting Majorana zero modes at their endpoints are used to encode two logical qubits, and both intra-chain and inter-chain braiding operations are performed to implement the CNOT gate. While the topological encoding of quantum information in Majorana fermions does not offer full topological protection in our non-interacting photonic setting, it nevertheless exhibits a natural resilience to the dominant noise and decoherence effects present in the experiment. Consequently, the fidelity of the CNOT gate is significantly enhanced, surpassing 0.992 and addressing a key limitation in the path toward scalable quantum computation. These results represent a major advancement in topological quantum computing with Majorana fermions and underscore the potential of photonic platforms for realising high-fidelity quantum gates.

quant-ph↗

Minute-Scale Photonic Quantum Memory

Long-lived storage of single photons is a fundamental requirement for enabling quantum communication and foundational tests of quantum physics over extended distances. While the implementation of a global-scale quantum network requires quantum storage times on the order of seconds to minutes, existing photonic quantum memories have so far been limited to subsecond lifetimes. Although $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystals exhibit substantially extended spin coherence times at the `magic' magnetic field, the concomitant weak optical absorption has until now prevented single-photon storage. Here, we overcome this challenge by integrating a noiseless photon echo protocol--which makes full use of the crystal's natural absorption for photonic storage--with a universally robust dynamical decoupling sequence incorporating adiabatic pulses to efficiently protect delocalized spin-wave excitation, enabling long-lived quantum storage at the `magic' magnetic field. At a storage time of 5.6 s, we achieve a time-bin qubit storage fidelity of 88.0 $\pm$ 2.1%, surpassing the maximum fidelity attainable via classical strategies. Our device reaches a $1/e$ storage lifetime of 27.6 $\pm$ 0.5 s, enabling single-photon-level storage for 42 s with a signal-to-noise ratio greater than unity. This work establishes photonic quantum memory in the minute-scale regime, laying a solid foundation for global-scale quantum network and deep-space quantum experiments.

quant-ph↗

Invested and Potential Magic Resources in Measurement-Based Quantum Computation

Magic states and magic gates are crucial for achieving universal quantum computation, but important questions about how magic resources should be implemented to attain maximal quantum advantage have remained unexplored, especially in the context of measurement-based quantum computation (MQC). This work bridges the gap between MQC and the resource theory of magic by introducing the key concepts of "invested" and "potential" magic resources. The former quantifies the magic cost associated with MQC, serving as both a resource witness and a feasible upper bound for the practical realization, and is gate-order independent; The latter represents the maximal achievable magic resource in a given graph structure defining MQC. We utilize both concepts to analyze the quantum Fourier transform (QFT) and provide a fresh perspective on the universality of MQC, highlighting the crucial role of non-Pauli measurements in injecting magic. In particular, we theoretically prove that high-dimensional graphs can generate an exponential advantage of MQC compared to classical computing. We demonstrate experimentally our theoretical findings in a high-fidelity four-photon setup, surpassing conventional magic state injection (MSI) methods in both qubit efficiency and resource utilization. Our findings pave the way for future research exploring magic resource optimization and novel distillation schemes within the MQC framework, advancing fault-tolerant universal quantum computation.

quant-ph↗

Observation of Non-Hermitian Spectral Deformation in Complex Momentum Space

Open systems feature a variety of phenomena that arise from non-Hermitian physics. Recent theoretical studies have offered much insights into these phenomena through the non-Bloch band theory, though many of the theory's key features are experimentally elusive. For instance, the correspondence between complex momenta and non-Hermitian bands, while central to non-Bloch band theory, has so far defied direct experimental observation. Here we experimentally study the non-Hermitian spectral deformation in complex-momentum space, by implementing a non-Hermitian lattice with long-range couplings in the synthetic orbital-angular-momentum (OAM) dimension of photons inside a degenerate cavity. Encoding the complex momenta in the phase and amplitude modulations of the OAM modes, and devising a complex-momentum-resolved projective detection, we reconstruct the spectral deformation in momentum space, where the eigenspectrum on the complex plane morphs through distinct geometries. This enables us to experimentally extract key information of the system under the non-Bloch band theory, including exceptional points in the complex-momentum space, the open-boundary spectra, and the generalized Brillouin zone. Our work demonstrates a versatile platform for exploring non-Hermitian physics and non-Bloch band theory, and opens the avenue for direct experimental investigation of non-Bloch features in the complex-momentum space.

quant-ph↗

Efficient integrated quantum memory for light

Scalable implementation of quantum networks and photonic processors require integrated photonic memories with high efficiency, yet current integrated systems have been limited to storage efficiencies below 27.8%. Here, we demonstrate highly efficient integrated quantum memories based on rare-earth-iondoped crystals coupled with impedance-matched microcavities, realized in two novel architectures: 200-micrometer-thin membranes of Eu3+:Y2SiO5 integrated with fiber-based microcavities, and waveguide-based cavities fabricated using femtosecond lasers. Our approach achieves reliable integrated quantum storage with record efficiencies of 80.3(7)% for weak coherent pulses and 69.8(1.6)% for telecom-heralded single photons, alongside the storage of 20 temporal modes with an average efficiency of 51.3(2)%. Moreover, the thin-membrane Eu3+:Y2SiO5 architecture enables spectrally tunable efficient quantum storage via variable strain, providing a flexible interface for quantum networks. By combining high efficiency, large multimode capacity, and tunability, our devices establish a versatile hardware foundation for scalable quantum repeaters and chip-scale photonic processors.

quant-ph↗

Design and Fabrication of Metal-Shielded Fiber-Cavity Mirrors for Ion-Trap Systems

Trapped ions in micro-cavities constitute a key platform for advancing quantum information processing and quantum networking. By providing an efficient light-matter interface within a compact architecture, they serve as highly efficient quantum nodes with strong potential for scalable quantum network. However, in such systems, ion trapping stability is often compromised by surface charging effects, and nearby dielectric materials are known to cause a dramatic increase in the ion heating rate by several orders of magnitude. These challenges significantly hinder the practical implementation of ion trap systems integrated with micro-cavities. To overcome these limitations, we present the design and fabrication of metal-shielded micro-cavity mirrors, enabling the stable realization of ion trap systems integrated with micro cavities. Using this method, we constructed a needle ion trap integrated with fiber Fabry-Perot cavity and successfully achieved stable trapping of a single ion within the cavity. The measured ion heating rate was reduced by more than an order of magnitude compared with unshielded configurations. This work establishes a key technique toward fully integrated ion-photon interfaces for scalable quantum network.

quant-ph↗

Nonlinear-linear duality for multipath quantum interference

In quantum optics, the postselection amplitude of a nondegenerate parametric down-conversion (PDC) process is linked to a beamsplitter (BS) via partial time reversal, up to a normalization coefficient which is related to the parametric gain [Proc. Natl. Acad. Sci. USA 117, 33107 (2020)]. A special example where the gain is low is reminiscent of Klyshko's advanced-wave picture in quantum imaging. Here, we propose and prove a generalized duality for multiple spatial paths connecting a quantum nonlinear interference setup consisting of nondegenerate PDCs and linear optical systems to a linear one, where the PDCs are directly replaced by hypothetical wavelength-shifting BSs. This replacement preserves the geometry of the original setup, and cascaded PDCs become optical cavities whose calculation involves the Redheffer star product. Additional terms in the normalization coefficient are related to the contribution of looping photons inside the cavities. Then, we discuss the case of coherent state input and postselection for $Q$-function calculation. This theorem will be helpful in the development of quantum photonic devices beyond the low-gain limit.

quant-ph↗

Implementation of multiparticle quantum speed limits on observables

The energy-time uncertainty relation limits the maximum speed of quantum system evolution and is crucial for determining whether quantum tasks can be accelerated. However, multiparticle quantum speed limits have not been experimentally explored. In this work, we experimentally verify that both multiparticles and entanglement can accelerate the quantum speed on observables in two-particle systems based on ultrahigh precision control of quantum evolution time. Furthermore, we experimentally prove that the initial quantum state plays a critical role in the quantum speed limits of the entangled systems. In addition, we experimentally demonstrate that the upper bound and lower bound of the quantum speed are workable even in a nonunitary Markovian open system with two photons. The results obtained based on two-photon experiments have been shown to be generalizable to more particles. Our work facilitates the characterization of the dynamic transient properties of complex quantum systems and the control of the quantum speed of large-scale quantum systems.

quant-ph↗

Nanoscale positioning and in-situ enhancement of single G center in silicon using a fluorescence-localization technique

Silicon-based semiconductor nanofabrication technology has achieved a remarkable level of sophistication and maturity, and color centers in silicon naturally inherit this advantage. Besides, their emissions appear in telecommunication bands, which makes them play a crucial role in the construction of quantum network. To address the challenge of weak spontaneous emission, different optical cavities are fabricated to enhance the emission rate. However, the relative location between cavity and emitter is random, which greatly reduce the success probability of enhancement. Here, we report on a fluorescence-localization technique (FLT) for precisely locating single G center in silicon and embedding it in the center of a circular Bragg grating cavity in situ, achieving 240-times improvement of the success probability. We observe a 30-fold enhancement in luminescence intensity, 2.5-fold acceleration of the emission from single G center, corresponding to a Purcell factor exceeding 11. Our findings pave the way for the large-scale integration of quantum light sources including those with spins.

physics.optics↗