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Clara Saraceno

Publications and source records attributed to Clara Saraceno.

4 recordsLinked to original sources

Self-Supervised Noise2Noise-Enhanced Denoising for Continuous-Scan Air-Plasma THz Spectroscopy

Terahertz time-domain spectroscopy (THz-TDS) based on air-plasma generation and balanced air-biased coherent detection offers gap-free broadband coverage, but individual continuous-scan traces are strongly affected by pulse-to-pulse fluctuations and electronic noise. Reaching a useful signal-to-noise ratio therefore requires averaging multiple traces, which directly increases measurement time. We propose a learned denoising approach that recovers high-quality THz waveforms from as few as one complete continuous delay sweep, referred to here as a single-scan trace. A compact one-dimensional residual U-Net is trained using two complementary strategies: a reference-supervised baseline that maps individual noisy traces to long-average reference waveforms, and a Noise2Noise approach that learns from pairs of independently acquired noisy traces without requiring a clean training target. Averaging the predictions of both models reduces systematic bias and yields a trace-reduction factor of approximately $5.4\times$ at $K=1$, meaning that one denoised trace achieves the reconstruction accuracy of averaging approximately five raw traces. The Noise2Noise model alone achieves $4.9\times$, outperforming both the reference-supervised baseline ($4.6\times$) and classical Wiener filtering ($3.2\times$). These results show that self-supervised learning from repeated noisy measurements can support faster continuous-scan THz-TDS without hardware modification.

eess.SP

Ytterbium-laser-driven THz generation in thin lithium niobate at 1.9 kW average power in a passive enhancement cavity

Single-cycle, high-power, high-repetition-rate THz pulse sources are becoming the cornerstone of several scientific and industrial applications. A promising and versatile method for high-power THz generation is optical rectification in nonlinear crystals pumped by powerful near-infrared ultrafast laser systems. In this context, ytterbium-based laser sources are particularly advantageous in terms of power scalability and technology establishment. However, as the repetition rate increases toward hundreds of MHz, the conversion efficiency typically decreases, as most laser systems do not reach sufficiently high average power to correspondingly enhance the peak power to drive the nonlinear conversion process efficiently. An alternative approach to achieving sufficiently high average power at high repetition rate is based on passive enhancement cavities, which boost the pulse energy of standard watt-level ytterbium lasers by orders of magnitude. We present the first demonstration of optical rectification in a passive enhancement cavity at multi-kW levels, achieved by a 240-fold power enhancement. By irradiating a 50-$μ$m thin lithium niobate plate with 1.9-kW average power inside the enhancement cavity, we generate milliwatt-level THz pulses with 2-THz bandwidth and 93-MHz repetition rate, mostly limited by the driving pulse duration. To the best of our knowledge, this represents the highest driving average power used for OR. This methodology represents a promising new step towards high-repetition-rate and high average power single-cycle THz sources using widely available multi-watt level Yb lasers.

physics.optics

Tracing d-d transitions in FePS$_{3}$ on ultrafast time scales

Excitations between localized 3d states of transition metal ions within crystalline solids, commonly known as d-d transitions, play a pivotal role in diverse phenomena across solid state physics, materials science, and chemistry. These transitions contribute to the coloration in transition metal oxides, catalytic processes on oxide surfaces, and high-temperature superconductivity. They also couple optical excitation to quantized collective phenomena such as phonons and magnons in magnetic systems. Until now, an experimental method to unravel the complex quasiparticle dynamics associated with d-d transitions has remained elusive. We bridge this gap by demonstrating that d-d transitions can be distinctly traced in momentum space and time using time- and angle-resolved photoelectron spectroscopy (trARPES). Through this approach, we can assign specific momentum-dependent characteristics and elucidate the decay mechanisms of specific d-d transitions in FePS$_{3}$, a two-dimensional van der Waals antiferromagnet with a rich array of quantum phenomena stemming from d-d transitions. This study pioneers the use of ARPES in probing the dynamics of d-d transitions across a wide spectrum of solid-state systems.

cond-mat.mtrl-sci

Temperature-independent non-linear terahertz transmission by liquid water

Liquid water is one of the most studied substances, yet many of its properties are difficult to rationalize. The uniqueness of water is rooted in the dynamic network of hydrogen-bonded molecules with relaxation time constants of about one picosecond. Terahertz fields oscillate on a picosecond timescale and are inherently suited to study water. Recent advances in non-linear terahertz spectroscopy have revealed large signals from water, which have been interpreted with different, sometimes competing, theoretical models. Here we show that the non-linear transmission of liquid water at ~1 THz is equal at 21 °C and 4 °C, thus suggesting that the most appropriate microscopic models should depend weakly on temperature. Among the different mechanisms proposed to date, the resonant reorientation of hydrogen-bonded water molecules might be the most appropriate to describe all of the currently available experimental results.

physics.chem-ph