arXiv subjects

Clare C. Yu

Publications and source records attributed to Clare C. Yu.

At least 19 recordsLinked to original sources

arXiv2026

Nearly Isotropic Magnon Transport in Epitaxial Lithium Aluminum Ferrite Thin Films

Low-loss magnetic insulating thin films are promising for information transport via magnons, where isotropic in-plane magnon propagation is desirable. We report nonlocal measurements of electrically and thermally generated magnons in epitaxial (001) lithium aluminum ferrite Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$ thin films with pronounced fourfold in-plane magnetic anisotropy. By measuring the inverse spin Hall signal as a function of the magnon diffusion distance, we deduce magnon diffusion lengths that are nearly identical along the [100] and [110] directions at 250~K. This isotropy is consistent with a nearly isotropic exchange stiffness. These results highlight spinel ferrites as viable platforms for isotropic magnon transport.

cond-mat.mtrl-sci↗

arXiv2026

Understanding Damping Mechanisms via Spin Diffusion Length in Low-damping Li$_{0.5}$Al$_{1.0}$Fe$_{1.5}$O$_4$ Spinel Ferrite Thin Films

The mechanisms underlying magnon damping are of fundamental and technological interest in low-damping materials. We find low-damping ferrimagnetic insulator Li$_{0.5}$Al$_{1.0}$Fe$_{1.5}$O$_4$ (LAFO) thin films to be a promising model system for probing these mechanisms because of its distinct temperature dependent spin diffusion length (SDL) trends for electrically and thermally generated magnons. With increasing temperature, the electrical SDL shows minimal change, while the thermal SDL decreases. We attribute these trends to distinct magnon populations and scattering mechanisms: thermally generated high $k$ magnons are limited by magnon-phonon scattering, whereas electrically generated low $k$ magnons are limited by relaxational scattering from magnetic impurities.

cond-mat.mtrl-sci↗

arXiv2026

Low-temperature spin dynamics in LAFO thin films: from cubic anisotropy to TLS-limited coherence

We investigate the low-temperature spin dynamics of epitaxial lithium aluminum ferrite (LAFO) thin films using broadband ferromagnetic resonance (FMR) spectroscopy from 0.44 K to 68 K. The results reveal a crossover from conventional cubic anisotropy-dominated behavior at higher temperatures to pronounced linewidth broadening and higher-order anisotropy contributions at cryogenic temperatures. With the magnetic field oriented along the [100] crystallographic direction, the resonance is well-captured by four-fold in-plane and out-of-plane uniaxial anisotropies. In contrast, measurements with the field along the [110] direction reveal the presence of an unusually large sixth-order cubic anisotropy term that is symmetry-suppressed for [100] but becomes apparent under this field orientation at ultralow temperatures, indicating a substantial modification of the anisotropy landscape. Independent linewidth analysis shows a pronounced peak near 8 K and a subtle monotonic enhancement with decreasing temperatures below 2 K, features consistent with dissipation mediated by a bath of two-level systems (TLS) arising from antisite defects and localized Fe$^{3+}$ moments. Comparison with TLS-based models demonstrates that both exchange-coupled impurities and nearly free paramagnetic centers contribute to the observed damping. Our results establish LAFO as a model ferrite system where disorder-induced TLS limit spin coherence at ultralow temperatures, providing new insights into anisotropy engineering, magnetic relaxation, and the design of ferrimagnetic insulators for coherent magnonics. These findings offer a framework for future optimization of growth conditions.

cond-mat.mtrl-sci↗

arXiv2025

Excitation of quasiparticle pairs in superconducting nanodevices by 1/f noise

Superconducting nanodevices such as qubits, resonators, and photodetectors, have revolutionized our capabilities for probing and controlling quantum phenomena. Nonequilibrium quasiparticles, which are broken Cooper pairs that cause decoherence and energy loss, can limit their performance. The number of these quasiparticles is often tens of orders of magnitude greater than would be present in thermal equilibrium. Background radiation has been shown to excite quasiparticles, but quasiparticles are observed even when the devices are carefully shielded. Here we show that the high-frequency components of 1/f noise can excite quasiparticle pairs and that this mechanism is consistent with previously unexplained experimental results. We also propose new experiments that exploit this quasiparticle excitation mechanism to non-invasively characterize high-frequency charge noise as well as the locations and nature of the defects producing the noise. The proposed experiments would also investigate how this noise changes as the defects that give rise to it evolve towards thermal equilibrium.

cond-mat.mes-hall↗

arXiv2025

Philip Warren Anderson

Philip Warren Anderson was a pioneering theoretical physicist whose work fundamentally shaped our understanding of complex systems. Anderson received the Nobel Prize in Physics in 1977 for his groundbreaking research on localization and magnetism, yet he did so much more. His work on magnetism included antiferromagnetism, superexchange, the Kondo problem and local magnetic moments in metals. Anderson pointed out the importance of disorder through his work on localization, non-crystalline solids and spin glasses. In superconductivity, he is known for the dirty superconductor theorem, showing the gauge-invariance of the BCS theory, his study of flux creep, and for his collaboration with experimentalists to realize the Josephson effect. Anderson's resonating valence bond theory may yet play an important role in high temperature superconductivity. Anderson was also fascinated by broken symmetry, and he laid the theoretical groundwork for what is now known as the Anderson-Higgs mechanism, showing how gauge bosons can acquire mass - an insight that played a foundational role in the Standard Model of particle physics. In his seminal "More is Different" paper, Anderson argued that the collective emergent phenomena that arise in complex interacting systems cannot be deduced from their fundamental parts. Anderson's legacy endures not only through the lasting impact of his scientific work but also through his influence on generations of physicists who continue to explore the rich landscape of collective behavior in nature.

physics.hist-ph↗

arXiv2024

Why Superconducting Ta Qubits Have Fewer Tunneling Two-Level Systems at the Air-Oxide Interface Than Nb Qubits

Superconducting qubits are a key contender for quantum computing elements, but they often face challenges like noise and decoherence from two-level systems (TLS). Tantalum (Ta) qubits are notable for their long T$_1$ coherence times nearing milliseconds, mainly due to fewer TLS, though the cause was unclear. Our research explored this by analyzing the air-oxide interface with density functional theory, particularly comparing Nb oxide (Nb$_2$O$_5$) and Ta oxide (Ta$_2$O$_5$). We discovered that Ta$_2$O$_5$ forms a smoother surface with fewer dangling O atoms and TLS than Nb$_2$O$_5$. The greater atomic mass of Ta also lowers the TLS tunnel splittings below the qubit's operating frequency. Furthermore, using external electric fields or SO$_2$ passivation can significantly reduce TLS on Nb surfaces, potentially improving their coherence times.

cond-mat.mtrl-sci↗

arXiv2024

Monte Carlo Spin Simulations of Magnetic Noise -- The Search for Pivoting

Superconducting quantum interference devices (SQUIDs) show great promise as quantum bits (qubits) but continue to be hindered by flux noise. The flux noise power spectra of SQUIDs go as $1/f^\alpha$, where $\alpha$ is the temperature-dependent noise exponent. Experiments find $0.5 \lesssim \alpha \lesssim 1$. Furthermore, experiments find that the noise power spectra versus frequency at different temperatures pivot about or cross at a common point for each SQUID. To try to better understand the results and motivated by experimental evidence that magnetic moments on the surface of SQUIDS produce flux noise, we present the results of our Monte Carlo simulations of various spin systems on 2D lattices. We find that only spin glasses produce $\alpha \sim 1$ at low temperature. We find that aliasing of the noise power spectra at high frequencies can lead to spectral pivoting if it is in proximity to a knee at a slightly lower frequency. We show that the pivot frequency depends on the method of site selection and how often the magnetization is recorded. The spectral pivoting that occurs in our simulations is due to aliasing and does not explain the spectral pivoting of experiments.

cond-mat.mes-hall↗

arXiv2023

Interacting Two-Level Systems as a Source of 1/f Charge Noise in Quantum Dot Qubits

Charge noise in semiconducting quantum dots has been observed to have a 1/f spectrum. We propose a model in which a pair of quantum dots are coupled to a 2D bath of fluctuating two level systems (TLS) that have electric dipole moments and that interact with each other, i.e., with the other fluctuators. These interactions are primarily via the elastic strain field. We use a 2D nearest-neighbor Ising spin glass to represent these elastic interactions and to simulate the dynamics of the bath of electric dipole fluctuators in the presence of a ground plane representing metal gates above the oxide layer containing the fluctuators. The interactions between the TLS cause the energy splitting of individual fluctuators to change with time. We calculate the resulting fluctuations in the electric potential at the two quantum dots that lie below the oxide layer. We find that 1/f electric potential noise spectra at the quantum dots and cross correlation in the noise between the two quantum dots are in qualitative agreement with experiment. Our simulations find that the cross correlations decrease exponentially with increasing quantum dot separation.

cond-mat.mes-hall↗

arXiv2023

Effects of Temperature Fluctuations on Charge Noise in Quantum Dot Qubits

Silicon quantum dot qubits show great promise but suffer from charge noise with a 1/f^\alpha spectrum, where f is frequency and \alpha \lesssim 1. It has recently been proposed that 1/f^\alpha noise spectra can emerge from a few thermally activated two-level fluctuators in the presence of sub-bath temperature fluctuations associated with a two-dimensional electron gas (2DEG)~\cite{Ahn2021}. We investigate this proposal by doing Monte Carlo simulations of a single Ising spin in a bath with a fluctuating temperature. We find that to obtain noise with a $1/f^\alpha$ spectrum with $alpha \lesssim 1 down to low frequencies, the duration of temperature fluctuations must be comparable to the inverse of the lowest frequency at which the noise is measured. This result is consistent with an analytic calculation in which the fluctuator is a two-state system with dynamics governed by time-dependent switching rates. In this case we find that the noise spectrum follows a Lorentzian at frequencies lower than the inverse of the average duration of the lowest switching rate. We then estimate relaxation times of thermal fluctuations by considering thermal diffusion in an electron gas in a confined geometry. We conclude that temperature fluctuations in a 2DEG sub-bath would require an unphysically long duration to be consistent with experimental measurements of 1/f-like charge noise in quantum dots at frequencies extending well below 1 Hz.

cond-mat.mes-hall↗

arXiv2021

Two-Level Systems and the Tunneling Model: A Critical View

The thermal and acoustic properties displayed by a wide variety of glasses at low temperatures are well described by the model of tunneling two level systems (TLS). We review the standard TLS model as well as developments that have occurred since the earlier work. In spite of half a century of effort and impressive successes, mysteries still remain. We discuss some of these longstanding puzzles about glasses at low temperatures and speculate about future directions.

cond-mat.dis-nn↗

arXiv2019

Physics Approaches to the Spatial Distribution of Immune Cells in Tumors

The goal of immunotherapy is to enhance the ability of the immune system to kill cancer cells. Immunotherapy is more effective and, in general, the prognosis is better, when more immune cells infiltrate the tumor. We explore the question of whether the spatial distribution rather than just the density of immune cells in the tumor is important in forecasting whether cancer recurs. After reviewing previous work on this issue, we introduce a novel application of maximum entropy to quantify the spatial distribution of discrete point-like objects. We apply our approach to B and T cells in images of tumor tissue taken from triple negative breast cancer (TBNC) patients. We find that there is a distinct difference in the spatial distribution of immune cells between good clinical outcome (no recurrence of cancer within at least 5 years of diagnosis) and poor clinical outcome (recurrence within 3 years of diagnosis). Our results highlight the importance of spatial distribution of immune cells within tumors with regard to clinical outcome, and raise new questions on their role in cancer recurrence.

physics.bio-ph↗

arXiv2019

Why phonon scattering in glasses is universally small at low temperatures

We present a novel view of the standard model of tunneling two level systems (TLS) to explain the puzzling universal value of a quantity, $C\sim 3\times 10^{-4}$, that characterizes phonon scattering in glasses below 1 K as reflected in thermal conductivity, ultrasonic attenuation, internal friction, and the change in sound velocity. Physical considerations lead to a broad distribution of phonon-TLS couplings that (1) exponentially renormalize tunneling matrix elements, and (2) reduce the TLS density of states through TLS-TLS interactions. We find good agreement between theory and experiment for a variety of individual glasses.

cond-mat.dis-nn↗

arXiv2017

Hydrogen as a Source of Flux Noise in SQUIDs

Superconducting qubits are hampered by flux noise produced by surface spins from a variety of microscopic sources. Recent experiments indicated that hydrogen (H) atoms may be one of those sources. Using density functional theory calculations, we report that H atoms either embedded in, or adsorbed on, an a-Al2O3(0001) surface have sizeable spin moments ranging from 0.81 to 0.87 uB with energy barriers for spin reorientation as low as ~10 mK. Furthermore, H adatoms on the surface attract gas molecules such as O2, producing new spin sources. We propose coating the surface with graphene to eliminate H-induced surface spins and to protect the surface from other adsorbates.

cond-mat.mtrl-sci↗

arXiv2015

Candidate source of flux noise in SQUIDs: adsorbed oxygen molecules

A major obstacle to using SQUIDs as qubits is flux noise. We propose that the heretofore mysterious spins producing flux noise could be $O_2$ molecules adsorbed on the surface. Using density functional theory calculations, we find that an $O_2$ molecule adsorbed on an α-alumina surface has a magnetic moment of ~1.8 μB. When the spin is oriented perpendicular to the axis of the O-O bond, the barrier to spin rotations is about 10 mK. Monte Carlo simulations of ferromagnetically coupled, anisotropic XY spins on a square lattice find 1/f magnetization noise, consistent with flux noise in Al SQUIDs.

cond-mat.supr-con↗

arXiv2012

Modeling Flux Noise in SQUIDs Due to Hyperfine Interactions

Recent experiments implicate spins on the surface of metals as the source of flux noise in SQUIDs, and indicate that these spins are able to relax without conserving total magnetization. We present a model of $1/f$ flux noise in which electron spins on the surface of metals can relax via hyperfine interactions. Our results indicate that flux noise would be significantly reduced in superconducting materials where the most abundant isotopes do not have nuclear moments such as zinc and lead.

cond-mat.mes-hall↗

arXiv2011

How Stress Can Reduce Dissipation in Glasses

We propose that stress can decrease the internal friction of amorphous solids, either by increasing the potential barriers of defects, thus reducing their tunneling and thermal activation that produce loss, or by decreasing the coupling between defects and phonons. This stress can be from impurities, atomic bonding constraints, or externally applied stress. Externally applied stress also reduces mechanical loss through dissipation dilution. Our results are consistent with the experiments, and predict that stress could substantially reduce dielectric loss and increase the thermal conductivity.

cond-mat.dis-nn↗

arXiv2011

The Widom line and noise power spectral analysis of a supercritical fluid

We have performed extensive molecular dynamics simulations to study noise power spectra of density and potential energy fluctuations of a Lennard-Jones model of a fluid in the supercritical region. Emanating from the liquid-vapor critical point, there is a locus of isobaric specific heat maxima, called the Widom line, which is often regarded as an extension of the liquid-vapor coexistence line. Our simulation results show that the noise power spectrum of the density fluctuations on the Widom line of the liquid-vapor transition exhibits three distinct $1/f^γ$ behaviors with exponents $γ$= 0, 1.2 and 2, depending on the frequency $f$. We find that the intermediate frequency region with an exponent $γ\sim$ 1 appears as the temperature approaches the Widom temperature from above or below. On the other hand, we do not find three distinct regions of $1/f^γ$ in the power spectrum of the potential energy fluctuations on the Widom line. Furthermore, we find that the power spectra of both the density and potential energy fluctuations at low frequency have a maximum on the Widom line, suggesting that the noise power can provide an alternative signature of the Widom line.

cond-mat.stat-mech↗

arXiv2009

Saturation of Two Level Systems and Charge Noise in Josephson Junction Qubits

We study the charge noise $S_Q$ in Josephson qubits produced by fluctuating two level systems (TLS) with electric dipole moments in the substrate. The TLS are driven by an alternating electric field of angular frequency $Ω$ and electric field intensity $I$. It is not widely appreciated that TLS in small qubits can easily be strongly saturated if $I\gg I_c$, where $I_c$ is the critical electric field intensity. To investigate the effect of saturation on the charge noise, we express the noise spectral density in terms of density matrix elements. To determine the dependence of the density matrix elements on the ratio $I/I_c$, we find the steady state solution for the density matrix using the Bloch-Redfield differential equations. We then obtain an expression for the spectral density of charge fluctuations as a function of frequency $f$ and the ratio $I/I_c$. We find $1/f$ charge noise at low frequencies, and that the charge noise is white (constant) at high frequencies. Using a flat density of states, we find that TLS saturation has no effect on the charge noise at either high or low frequencies.

cond-mat.supr-con↗