arXiv subjects
Publications and source records attributed to Claude-Alain Pillet.
We study entropy production (EP) in processes involving repeated quantum measurements of finite quantum systems. Adopting a dynamical system approach, we develop a thermodynamic formalism for the EP and study fine aspects of irreversibility related to the hypothesis testing of the arrow of time. Under a suitable chaoticity assumption, we establish a Large Deviation Principle and a Fluctuation Theorem for the EP.
We study driven finite quantum systems in contact with a thermal reservoir in the regime in which the system changes slowly in comparison to the equilibration time. The associated isothermal adiabatic theorem allows us to control the full statistics of energy transfers in quasi-static processes. Within this approach, we extend Landauer's Principle on the energetic cost of erasure processes to the level of the full statistics and elucidate the nature of the fluctuations breaking Landauer's bound.
We consider a general network of harmonic oscillators driven out of thermal equilibrium by coupling to several heat reservoirs at different temperatures. The action of the reservoirs is implemented by Langevin forces. Assuming the existence and uniqueness of the steady state of the resulting process, we construct a canonical entropy production functional which satisfies the Gallavotti--Cohen fluctuation theorem, i.e., a global large deviation principle with a rate function I(s) obeying the Gallavotti--Cohen fluctuation relation I(-s)-I(s)=s for all s. We also consider perturbations of our functional by quadratic boundary terms and prove that they satisfy extended fluctuation relations, i.e., a global large deviation principle with a rate function that typically differs from I(s) outside a finite interval. This applies to various physically relevant functionals and, in particular, to the heat dissipation rate of the network. Our approach relies on the properties of the maximal solution of a one-parameter family of algebraic matrix Riccati equations. It turns out that the limiting cumulant generating functions of our functional and its perturbations can be computed in terms of spectral data of a Hamiltonian matrix depending on the harmonic potential of the network and the parameters of the Langevin reservoirs. This approach is well adapted to both analytical and numerical investigations.
We characterize the absolutely continuous spectrum of half-line one-dimensional Schrödinger operators in terms of the limiting behavior of the Crystaline Landauer-Büttiker conductance of the associated finite samples.
We study non-equilibrium statistical mechanics of a Gaussian dynamical system and compute in closed form the large deviation functionals describing the fluctuations of the entropy production observable with respect to the reference state and the non-equilibrium steady state. The entropy production observable of this model is an unbounded function on the phase space, and its large deviation functionals have a surprisingly rich structure. We explore this structure in some detail.
The first law of thermodynamics states that the average total energy current between different reservoirs vanishes at large times. In this note we examine this fact at the level of the full statistics of two times measurement protocols also known as the Full Counting Statistics. Under very general conditions, we establish a tight form of the first law asserting that the fluctuations of the total energy current computed from the energy variation distribution are exponentially suppressed in the large time limit. We illustrate this general result using two examples: the Anderson impurity model and a 2D spin lattice model.
We characterize the absolutely continuous spectrum of the one-dimensional Schrödinger operators $h=-Δ+v$ acting on $\ell^2(\mathbb{Z}_+)$ in terms of the limiting behavior of the Landauer-Büttiker and Thouless conductances of the associated finite samples. The finite sample is defined by restricting $h$ to a finite interval $[1,L]\cap\mathbb{Z}_+$ and the conductance refers to the charge current across the sample in the open quantum system obtained by attaching independent electronic reservoirs to the sample ends. Our main result is that the conductances associated to an energy interval $I$ are non-vanishing in the limit $L\to\infty$ iff ${\rm sp}_{\rm ac}(h)\cap I=\emptyset$. We also discuss the relationship between this result and the Schrödinger Conjecture.
We study the problem of exponential mixing and large deviations for discrete-time Markov processes associated with a class of random dynamical systems. Under some dissipativity and regularisation hypotheses for the underlying deterministic dynamics and a non-degeneracy condition for the driving random force, we discuss the existence and uniqueness of a stationary measure and its exponential stability in the Kantorovich-Wasserstein metric. We next turn to the large deviation principle and establish its validity for the occupation measures of the Markov processes in question. The obtained results extend those established earlier for the case of the bounded noise and can be applied to the 2D Navier-Stokes system in a bounded domain and to the complex Ginzburg-Landau equation.
We study a class of dissipative PDE's perturbed by an unbounded kick force. Under some natural assumptions, the restrictions of solutions to integer times form a homogeneous Markov process. Assuming that the noise is rough with respect to the space variables and has a non-degenerate law, we prove that the system in question satisfies a large deviation principle in tau-topology. Under some additional hypotheses, we establish a Gallavotti-Cohen type symmetry for the rate function of an entropy production functional and the strict positivity and finiteness of the mean entropy production in the stationary regime. The latter result is applicable to PDE's with strong nonlinear dissipation.
We study a microscopic Hamiltonian model describing an N-level quantum system S coupled to an infinitely extended thermal reservoir R. Initially, the system S is in an arbitrary state while the reservoir is in thermal equilibrium at temperature T. Assuming that the coupled system S+R is mixing with respect to the joint thermal equilibrium state, we study the Full Counting Statistics (FCS) of the energy transfers S->R and R->S in the process of return to equilibrium. The first FCS describes the increase of the energy of the system S. It is an atomic probability measure, denoted $P_{S,λ,t}$, concentrated on the set of energy differences $σ(H_S)-σ(H_S)$ ($σ(H_S)$ is the spectrum of the Hamiltonian of S, $t$ is the length of the time interval during which the measurement of the energy transfer is performed, and $λ$ is the strength of the interaction between S and R). The second FCS, $P_{R,λ,t}$, describes the decrease of the energy of the reservoir R and is typically a continuous probability measure whose support is the whole real line. We study the large time limit $t\rightarrow\infty$ of these two measures followed by the weak coupling limit $λ\rightarrow 0$ and prove that the limiting measures coincide. This result strengthens the first law of thermodynamics for open quantum systems. The proofs are based on modular theory of operator algebras and on a representation of $P_{R,λ,t}$ by quantum transfer operators.
In the independent electron approximation, the average (energy/charge/entropy) current flowing through a finite sample S connected to two electronic reservoirs can be computed by scattering theoretic arguments which lead to the famous Landauer-Büttiker formula. Another well known formula has been proposed by Thouless on the basis of a scaling argument. The Thouless formula relates the conductance of the sample to the width of the spectral bands of the infinite crystal obtained by periodic juxtaposition of S. In this spirit, we define Landauer-Büttiker crystalline currents by extending the Landauer-Büttiker formula to a setup where the sample S is replaced by a periodic structure whose unit cell is S. We argue that these crystalline currents are closely related to the Thouless currents. For example, the crystalline heat current is bounded above by the Thouless heat current, and this bound saturates iff the coupling between the reservoirs and the sample is reflectionless. Our analysis leads to a rigorous derivation of the Thouless formula from the first principles of quantum statistical mechanics.
The Landauer principle asserts that the energy cost of erasure of one bit of information by the action of a thermal reservoir in equilibrium at temperature T is never less than $kTlog 2$. We discuss Landauer's principle for quantum statistical models describing a finite level quantum system S coupled to an infinitely extended thermal reservoir R. Using Araki's perturbation theory of KMS states and the Avron-Elgart adiabatic theorem we prove, under a natural ergodicity assumption on the joint system S+R, that Landauer's bound saturates for adiabatically switched interactions. The recent work of Reeb and Wolf on the subject is discussed and compared.
We study a class of finite dimensional quantum dynamical semigroups exp(tL) whose generators L are sums of Lindbladians satisfying the detailed balance condition. Such semigroup arise in the weak coupling (van Hove) limit of Hamiltonian dynamical systems describing open quantum systems out of equilibrium. We prove a general entropic fluctuation theorem for this class of semigroups by relating the cumulant generating function of entropy transport to the spectrum of a family of deformations of the generator L. We show that, besides the celebrated Evans-Searles symmetry, this cumulant generating function also satisfies the translation symmetry recently discovered by Andrieux et al., and that in the linear regime near equilibrium these two symmetries yield Kubo's and Onsager's linear response relations.
We address the existence of steady state Green-Keldysh correlation functions of interacting fermions in mesoscopic systems for both the partitioning and partition-free scenarios. Under some spectral assumptions on the non-interacting model and for sufficiently small interaction strength, we show that the system evolves to a NESS which does not depend on the profile of the time-dependent coupling strength/bias. For the partitioned setting we also show that the steady state is independent of the initial state of the inner sample. Closed formulae for the NESS two-point correlation functions (Green-Keldysh functions), in the form of a convergent expansion, are derived. In the partitioning approach, we show that the 0th order term in the interaction strength of the charge current leads to the Landauer-Buettiker formula, while the 1st order correction contains the mean-field (Hartree-Fock) results.
We study a class of dissipative PDE's perturbed by a bounded random kick force. It is assumed that the random force is non-degenerate, so that the Markov process obtained by the restriction of solutions to integer times has a unique stationary measure. The main result of the paper is a large deviation principle for occupation measures of the Markov process in question. The proof is based on Kifer's large deviation criterion, a Lyapunov-Schmidt type reduction, and an abstract result on large-time asymptotic for generalised Markov semigroups.
We study the entropy flux in the stationary state of a finite one-dimensional sample S connected at its left and right ends to two infinitely extended reservoirs at distinct temperatures T1, T2 and chemical potentials mu1, mu2. The sample is a free lattice Fermi gas confined to a box [0, L] with energy operator -Δ+ v. The Landauer-Büttiker formula expresses the steady state entropy flux in the coupled system in terms of scattering data. We study the behavior of this steady state entropy flux in the limit L->infinity and relate persistence of transport to norm bounds on the transfer matrices of the limiting half-line Schrödinger operator h. A natural conjecture is that the set of energies at which transport persists in this limit is precisely the essential support of the absolutely continuous spectrum of h. We show that this conjecture is equivalent to the Schrödinger conjecture in spectral theory of one-dimensional Schrödinger operators, thus giving a physically appealing interpretation to the Schrödinger conjecture.
Under certain conditions we prove the existence of a steady-state transport regime for interacting mesoscopic systems coupled to reservoirs (leads). The partitioning and partition-free scenarios are treated on an equal footing. Our time-dependent scattering approach is {\it exact} and proves, among other things the independence of the steady-state quantities from the initial state of the sample. Closed formulas for the steady-state current amenable for perturbative calculations w.r.t. the interaction strength are also derived. In the partitioning case we calculate the first order correction and recover the mean-field (Hartree-Fock) results.
These lecture notes provide an elementary introduction, within the framework of finite quantum systems, to recent developments in the theory of entropic fluctuations.