arXiv subjects

Claudio Castelnovo

Publications and source records attributed to Claudio Castelnovo.

At least 55 records · Page 3Linked to original sources

arXiv2021

Anomalous magnetic noise in imperfect flat bands in the topological magnet Dy2Ti2O7

The spin ice compound Dy_2Ti_2O_7 stands out as the first topological magnet in three dimensions, with its tell-tale emergent fractionalized magnetic monopole excitations. Its real-time dynamical properties have been an enigma from the very beginning. Using ultrasensitive, non-invasive SQUID measurements, we show that Dy_2Ti_2O_7 exhibits a highly anomalous noise spectrum, in three qualitatively different regimes: equilibrium spin ice, a `frozen' regime extending to ultra-low temperatures, as well as a high-temperature `anomalous' paramagnet. We show that in the simplest model of spin ice, the dynamics is not anomalous, and we present several distinct mechanisms which give rise to a coloured noise spectrum. In addition, we identify the structure of the single-ion dynamics as a crucial ingredient for any modelling. Thus, the dynamics of spin ice Dy_2Ti_2O_7 reflects the interplay of local dynamics with emergent topological degrees of freedom and a frustration-generated imperfectly flat energy landscape, and as such should be relevant for a broad class of magnetic materials.

cond-mat.str-el↗

arXiv2021

Enhanced diffusion in soft-walled channels with a periodically varying curvature

In one-dimension, the diffusion of particles along a line is slowed by the addition of energy barriers. The same is true in two-dimensions, provided that the confining channel in which the particles move doesn't change shape. However, if the shape changes then this is no longer necessarily true; adding energy barriers can enhance the rate of diffusion, and even restore free diffusion. We explore these effects for a channel with a sinusoidally varying curvature.

cond-mat.stat-mech↗

arXiv2020

Neural network wave functions and the sign problem

Neural quantum states (NQS) are a promising approach to study many-body quantum physics. However, they face a major challenge when applied to lattice models: Convolutional networks struggle to converge to ground states with a nontrivial sign structure. We tackle this problem by proposing a neural network architecture with a simple, explicit, and interpretable phase ansatz, which can robustly represent such states and achieve state-of-the-art variational energies for both conventional and frustrated antiferromagnets. In the latter case, our approach uncovers low-energy states that exhibit the Marshall sign rule and are therefore inconsistent with the expected ground state. Such states are the likely cause of the obstruction for NQS-based variational Monte Carlo to access the true ground states of these systems. We discuss the implications of this observation and suggest potential strategies to overcome the problem.

cond-mat.str-el↗

arXiv2020

Coherent propagation of quasiparticles in topological spin liquids at finite temperature

The appearance of quasiparticle excitations with fractional statistics is a remarkable defining trait of topologically ordered systems. In this work, we investigate the experimentally relevant finite temperature regime in which one species of quasiparticle acts as a stochastic background for another, more energetically costly, species that hops coherently across the lattice. The nontrivial statistical angle between the two species leads to interference effects that we study using a combination of numerical and analytical tools. In the limit of self-retracing paths, we are able to use a Bethe lattice approximation to construct exact analytical expressions for the time evolution of the site-resolved density profile of a spinon initially confined to a single site. Our results help us to understand the temperature-dependent crossover from ballistic to quantum (sub-)diffusive behaviour as a consequence of destructive interference between lattice walks. The subdiffusive behaviour is most pronounced in the case of semionic mutual statistics, and it may be ascribed to the localised nature of the effective tight-binding description, an effect that is not captured by the Bethe lattice mapping. In addition to quantum spin liquids, our results are directly applicable to the dynamics of isolated holes in the large-$U$ limit of the Hubbard model, relevant to ultracold atomic experiments. A recent proposal to implement $\mathbb{Z}_2$ topologically ordered Hamiltonians using quantum annealers provides a further exciting avenue to test our results.

cond-mat.str-el↗

arXiv2020

Analytical theory of pyrochlore cooperative paramagnets

The pyrochlore lattice is associated with several potential and actual spin liquid phases as a result of its strong geometric frustration. At finite temperature, these can exhibit an unusually broad cross-over regime to a conventional paramagnet. Here, we study this regime analytically by showing how a single-tetrahedron Hamiltonian can extrapolate beyond the first term of a high-temperature expansion and yield insights into the build-up of correlations. We discuss how this unusual behaviour is brought about by the structure of the eigenspaces of the coupling matrix. Further interesting behaviour can appear for parameter values located near phase transitions: we find coexistence of $(111)$ rods and $(220)$ peaks in the structure factor, as observed in neutron scattering experiments on Yb$_2$Ti$_2$O$_7$.

cond-mat.str-el↗

arXiv2019

Correlated Quantum Tunnelling of Monopoles in Spin Ice

The spin ice materials Ho$_{2}$Ti$_{2}$O$_{7}$ and Dy$_{2}$Ti$_{2}$O$_{7}$ are by now perhaps the best-studied classical frustrated magnets. A crucial step towards the understanding of their low temperature behaviour -- both regarding their unusual dynamical properties and the possibility of observing their quantum coherent time evolution -- is a quantitative understanding of the spin-flip processes which underpin the hopping of magnetic monopoles. We attack this problem in the framework of a quantum treatment of a single-ion subject to the crystal, exchange and dipolar fields from neighbouring ions. By studying the fundamental quantum mechanical mechanisms, we discover a bimodal distribution of hopping rates which depends on the local spin configuration, in broad agreement with rates extracted from experiment. Applying the same analysis to Pr$_{2}$Sn$_{2}$O$_{7}$ and Pr$_{2}$Zr$_{2}$O$_{7}$, we find an even more pronounced separation of timescales signalling the likelihood of coherent many-body dynamics.

cond-mat.str-el↗

arXiv2019

Seeing beyond the light: Vison and photon electrodynamics in quantum spin ice

Understanding the nature and behaviour of excitations in quantum spin liquids, and in topological phases of matter in general, is of fundamental importance and has proven crucial for experimental detection and characterisation of candidate materials. Current theoretical and numerical techniques, however, have limited capabilities, especially when it comes to studying gapped excitations. Here, we propose a semiclassical numerical method to study systems whose spin liquid behaviour is underpinned by perturbative ring-exchange Hamiltonians. Our method can readily access both thermodynamic and spectral properties. We focus in particular on quantum spin ice and its photon and vison excitations. After benchmarking the method against existing results on photons, we use it to characterise visons and their thermodynamic behaviour, which remained hitherto largely unexplored. We find that visons, in contrast to spinons in classical spin ice, form a weak electrolyte: vison pairs are the dominant population at low temperatures. This is reflected in the behaviour of thermodynamic quantities, such as pinch point motifs in the relevant correlators. Visons also appear to strongly hybridise with the photon background, a phenomenon that affects the way these quasiparticles may show up in inelastic response measurements. Our results demonstrate that the method, and generalisations thereof, can substantially help our understanding of quasiparticles and their interplay in quantum spin ice and other quantum spin liquids, quantum dimer models, and lattice gauge theories in general.

cond-mat.str-el↗

arXiv2019

Generalised route to effective field theories for quantum systems with local constraints

Some of the exciting phenomena uncovered in strongly correlated systems in recent years - for instance quantum topological order, deconfined quantum criticality, and emergent gauge symmetries -- appear in systems in which the Hilbert space is effectively projected at low energies in a way that imposes local constraints on the original degrees of freedom. Cases in point include spin liquids, valence bond systems, dimer models, and vertex models. In this work, we use a slave boson description coupled to a large-$S$ path integral formulation to devise a generalised route to obtain effective field theories for such systems. We demonstrate the validity and capability of our approach by studying quantum dimer models and by comparing our results with the existing literature. Field-theoretic approaches to date are limited to bipartite lattices, they depend on a gauge-symmetric understanding of the constraint, and they lack generic quantitative predictive power for the coefficients of the terms that appear in the Lagrangians of these systems. Our method overcomes all these shortcomings and we show how the results up to quadratic order compare with the known height description of the square lattice quantum dimer model, as well as with the numerical estimate of the speed of light of the photon excitations on the diamond lattice. Finally, instanton considerations allow us to infer properties of the finite-temperature behaviour in two dimensions.

cond-mat.str-el↗

arXiv2019

Supercooling and fragile glassiness in a dipolar kagome Ising magnet

We study equilibration and ordering in the classical dipolar kagome Ising antiferromagnet, which we show behaves as a disorder-free fragile spin glass. By identifying an appropriate order parameter, we demonstrate a transition to the ordered state proposed by Chioar et al. [Phys. Rev. B 93, 214410 (2016)] with a 12-site unit cell that breaks time-reversal and sublattice symmetries, and further provide evidence that the nature of the transition is first order. Upon approaching the transition, the spin dynamics slow dramatically. The system readily falls out of equilibrium, overshooting the transition and entering a supercooled liquid regime. Using extensive Monte Carlo simulations, we show that the system exhibits super-Arrhenius behaviour above the ordering transition. The relaxation time diverges according to a Vogel-Fulcher form at a finite `glass transition' temperature in the supercooled regime. Such behaviour, characteristic of fragile glasses, is particularly remarkable as the model is free of quenched disorder, does not straightforwardly conform to the avoided criticality paradigm, and is simple and eminently realisable in engineered nanomagnetic arrays.

cond-mat.str-el↗

arXiv2019

Rod motifs in neutron scattering in spin ice

In classical and quantum spin ice, rod-like features appear in the neutron scattering structure factor when the pinchpoints characteristic of classical spin ice get washed out. We show that these features do not indicate the absence of spin correlations between planes perpendicular to the rods. Rather, they arise because unpolarised neutron scattering is largely insensitive to the three-dimensional correlations which are present throughout. We present two very simple models which exhibit a pristine incarnation of such scattering rods. This provides a physical picture for their appearance, elucidates the role played by monopole excitations and identifies conditions conducive to their observation.

cond-mat.str-el↗

arXiv2019

Quantum oscillations and criticality in a fermionic and bosonic dimer model for the cuprates

We study quantum oscillations for a system of fermionic and bosonic dimers and compare the results to those experimentally observed in the cuprate superconductors in their underdoped regime. Based on gauge invariance, we argue that the charge carriers obey the Onsager quantization condition and quantum oscillations take on a Lifshitz-Kosevich form. We obtain the effective mass and find good qualitative agreement with experiments if we tune the model to the point where the observed mass divergence at optimum doping is associated to a van Hove singularity at which four free-dimer Fermi pockets touch pairwise in the interior of the Brillouin zone. The same van Hove singularity leads to a maximum in the d-wave superconducting pairing amplitude when anti-ferromagnetic interactions are included. Our combined results therefore suggest that a quantum critical point separating the underdoped and overdoped regimes is marked by the location of the van Hove saddle point in the fermionic dimer dispersion.

cond-mat.str-el↗

arXiv2019

Topological many-body scar states in dimensions 1, 2, and 3

We propose an exact construction for atypical excited states of a class of non-integrable quantum many-body Hamiltonians in one dimension (1D), two dimensions (2D), and three dimensins (3D) that display area law entanglement entropy. These examples of many-body `scar' states have, by design, other properties, such as topological degeneracies, usually associated with the gapped ground states of symmetry protected topological phases or topologically ordered phases of matter.

cond-mat.other↗

arXiv2018

Steady-state superconductivity in electronic materials with repulsive interactions

We study the effect of laser driving on a minimal model for a hexagonal two-dimensional material with broken inversion symmetry. Through the application of circularly polarised light and coupling to a thermal free electron bath, the system is driven into a nonequilibrium steady state with asymmetric, nonthermal carrier populations in the two valleys. We show that, in this steady state, interband superconducting correlations between electrons can develop independent of the sign of the electron-electron interactions. We discuss how our results apply, for example, to transition metal dichalcogenides. This work opens the door to technological applications of superconductivity in a range of materials that were hitherto precluded from it.

cond-mat.str-el↗

arXiv2018

Phases of quantum dimers from ensembles of classical stochastic trajectories

We study the connection between the phase behaviour of quantum dimers and the dynamics of classical stochastic dimers. At the so-called Rokhsar-Kivelson (RK) point a quantum dimer Hamiltonian is equivalent to the Markov generator of the dynamics of classical dimers. A less well understood fact is that away from the RK point the quantum-classical connection persists: in this case the Hamiltonian corresponds to a non-stochastic "tilted" operator that encodes the statistics of time-integrated observables of the classical stochastic problem. This implies a direct relation between the phase behaviour of quantum dimers and properties of ensembles of stochastic trajectories of classical dimers. We make these ideas concrete by studying fully packed dimers on the square lattice. Using transition path sampling - supplemented by trajectory umbrella sampling - we obtain the large deviation statistics of dynamical activity in the classical problem, and show the correspondence between the phase behaviour of the classical and quantum systems. The transition at the RK point between quantum phases of distinct order corresponds, in the classical case, to a trajectory phase transition between active and inactive dynamical phases. Furthermore, from the structure of stochastic trajectories in the active dynamical phase we infer that the ground state of quantum dimers has columnar order to one side of the RK point. We discuss how these results relate to those from quantum Monte Carlo, and how our approach may generalise to other problems.

cond-mat.stat-mech↗

arXiv2018

Color-dependent interactions in the three coloring model

Since it was first discussed by Baxter in 1970, the three coloring model has been studied in several contexts, from frustrated magnetism to superconducting devices and glassiness. In presence of interactions, when the model is no longer exactly soluble, it was already observed that the phase diagram is highly non-trivial. Here we discuss the generic case of `color-dependent' nearest-neighbor interactions between the vertex chiralities. We uncover different critical regimes merging into one another: c=1/2 free fermions combining into c=1 free bosons; c=1 free bosons combining into c=2 critical loop models; as well as three separate c=1/2 critical lines merging at a supersymmetric c=3/2 critical point. When the three coupling constants are tuned to equal one another, transfer-matrix calculations highlight a puzzling regime where the central charge appears to vary continuously from 3/2 to 2.

cond-mat.stat-mech↗

arXiv2018

Entanglement negativity and sudden death in the toric code at finite temperature

We study the fate of quantum correlations at finite temperature in the two-dimensional toric code using the logarithmic entanglement negativity. We are able to obtain exact results that give us insight into how thermal excitations affect quantum entanglement. The toric code has two types of elementary excitations (defects) costing different energies. We show that an $O(1)$ density of the lower energy defect is required to degrade the zero-temperature entanglement between two subsystems in contact with one another. However, one type of excitation alone is not sufficient to kill all quantum correlations, and an $O(1)$ density of the higher energy defect is required to cause the so-called sudden death of the negativity. Interestingly, if the energy cost of one of the excitations is taken to infinity, quantum correlations survive up to arbitrarily high temperatures, a feature that is likely shared with other quantum spin liquids and frustrated systems in general, when projected down to their low-energy states. We demonstrate this behaviour both for small subsystems, where we can prove that the negativity is a necessary and sufficient condition for separability, as well as for extended subsystems, where it is only a necessary condition. We further observe that the negativity per boundary degree of freedom at a given temperature increases (parametrically) with the size of the boundary, and that quantum correlations between subsystems with extended boundaries are more robust to thermal fluctuations.

cond-mat.str-el↗

arXiv2018

Dynamic scaling of topological ordering in classical systems

We analyze scaling behaviors of simulated annealing carried out on various classical systems with topological order, obtained as appropriate limits of the toric code in two and three dimensions. We first consider the three-dimensional $\mathbb{Z}_2$ (Ising) lattice gauge model, which exhibits a continuous topological phase transition at finite temperature. We show that a generalized Kibble-Zurek scaling ansatz applies to this transition, in spite of the absence of a local order parameter. We find perimeter-law scaling of the magnitude of a non-local order parameter (defined using Wilson loops) and a dynamic exponent $z=2.70 \pm 0.03$, the latter in good agreement with previous results for the equilibrium dynamics (autocorrelations). We then study systems where (topological) order forms only at zero temperature---the Ising chain, the two-dimensional $\mathbb{Z}_2$ gauge model, and a three-dimensional star model (another variant of the $\mathbb{Z}_2$ gauge model). In these systems the correlation length diverges exponentially, in a way that is non-smooth as a finite-size system approaches the zero temperature state. We show that the Kibble-Zurek theory does not apply in any of these systems. Instead, the dynamics can be understood in terms of diffusion and annihilation of topological defects, which we use to formulate a scaling theory in good agreement with our simulation results. We also discuss the effect of open boundaries where defect annihilation competes with a faster process of evaporation at the surface.

cond-mat.stat-mech↗

arXiv2017

Dephasing with strings attached

Motivated by the existence of mobile low-energy excitations like domain walls in one dimension or gauge-charged fractionalized particles in higher dimensions, we compare quantum dynamics in the presence of weak Markovian dephasing for a particle hopping on a chain and for an Ising domain wall whose motion leaves behind a string of flipped spins. Exact solutions show that the two models have near identical transport responses in the bulk. On the other hand, in finite-length chains, the broadening of discrete spectral lines is much more noticeable in the case of a domain wall. These results may be of relevance to a broad class of systems including quasi-1D antiferromagnets, polymer chains, and even retinal systems.

cond-mat.mes-hall↗