arXiv subjects

Claudiu Genes

Publications and source records attributed to Claudiu Genes.

At least 19 recordsLinked to original sources

arXiv2026

Microscopic theory of a radiation-balanced solar laser

We develop a microscopic open-quantum-system theory for a radiation-balanced solar laser (RBSL) based on ytterbium-doped yttrium aluminum garnet (Yb:YAG), in which optical gain, thermal redistribution among sublevels of the electronic ground and excited manifolds, and lattice-temperature dynamics are treated within a unified framework. Starting from a Lindblad master equation for a multilevel gain medium coupled to a cavity mode, we include incoherent solar pumping, spontaneous emission, cavity loss, and phonon-assisted intra-manifold relaxation obeying detailed balance. In the regime of fast thermalization within each electronic manifold, a compact temperature-dependent two-level model is derived, in which the gain, inversion, and lasing threshold are controlled by Boltzmann occupation factors and partition functions of the electronic sublevels. This microscopic reduction is then coupled self-consistently to a thermal balance equation accounting for anti-Stokes fluorescence cooling, quantum-defect heating, parasitic absorption, and heat exchange with the environment. The theory predicts several operating regimes, including pure cooling, lasing with net cooling, and lasing with net heating, as well as dynamical effects such as delayed lasing onset induced by self-cooling into threshold. In contrast to earlier radiation-balanced laser (RBL) models based mainly on macroscopic rate equations and thermodynamic balance arguments, the present approach provides a microscopic description of the feedback between quantum optical dynamics and temperature redistribution. It therefore offers a physically transparent framework for analyzing RBSLs and for identifying design strategies that exploit level structure, thermalization, and photonic-environment engineering to stabilize laser operation while minimizing internal heat load.

physics.optics↗

arXiv2026

A solid-state quantum memory based on a continuous optoacoustic system

Quantum memories for optical states are essential resources for quantum communication and information processing. We propose a quantum memory protocol based on coherent photon-phonon transduction in a Brillouin-active optical waveguide supporting traveling acoustic modes. A pulsed pump drives an effective beam-splitter interaction between optical and acoustic fields, enabling the mapping of a propagating optical quantum state onto a traveling phononic excitation and its subsequent retrieval on demand. Using a continuum optoacoustic model, we show that the protocol enables broadband quantum state storage in a distributed medium without relying on discrete cavity modes. Analytical and numerical results demonstrate high-fidelity storage and retrieval of squeezed and entangled states under experimentally realistic parameters. The memory bandwidth is set by the Brillouin interaction and can reach hundreds of MHz. Our results identify continuum Brillouin optomechanical systems as a scalable platform for broadband quantum memories and multimode quantum signal processing.

quant-ph↗

arXiv2026

Dicke superradiance in degenerate quantum matter: interplay of exchange statistics and spatial confinement

Collective radiance effects in quantum degenerate systems, such as superradiance and subradiance of a partially inverted ensemble, are shaped by the interplay of spatial confinement and exchange statistics. We investigate this interplay using a purely dissipative field theoretic quartic Lindblad master equation, which captures the nonlinear dynamics of the combined motional and electronic manifolds. This approach captures the interplay between the permutational symmetry of the Lindbladian and the exchange symmetry of the particles, quantifying how bosonic enhancement and Pauli blocking dictate superradiant and subradiant scaling. We identify two distinct routes to distinguishable dynamics: thermal dilution of the initial state at high temperatures and the dynamical breakdown of collective order via recoil induced transport in soft traps. This analysis provides a benchmark for collective emission in quantum-degenerate atomic systems with coupled motional and internal dynamics, such as optical lattice clocks and spinor gases, when dissipation is engineered to control recoil and motional heating.

cond-mat.quant-gas↗

arXiv2025

Symbolic Quantum-Trajectory Method for Multichannel Dicke Superradiance

We solve Dicke superradiance with two or more competing collective decay channels of tunable rates using a symbolic quantum-trajectory construction. The method yields closed time-domain populations and observables as finite combinations of exponential terms for arbitrary numbers of emitters and arbitrary decay rates. For two channels, the behavior of the stationary ground-state distribution resembles a first-order phase transition at the point where the channel-rate ratio is equal to unity. For balanced $d$-channel decay, we obtain scaling laws for the superradiant peak time and intensity. These results unify and extend single-channel Dicke dynamics to multilevel emitters and provide a compact tool for cavity and waveguide experiments, where permutation-symmetric reservoirs engineer multiple collective decay paths.

quant-ph↗

arXiv2025

Phase-adaptive cooling of fringe-trapped nanoparticles at room temperature in hollow-core photonic crystal fiber

Active feedback cooling of levitated dielectric particles is a pivotal technique for creating ultrasensitive sensors and probing fundamental physics. Here we demonstrate phase-adaptive feedback cooling of silica nanoparticles optically trapped in standing-wave potential formed by two co-linearly polarized counterpropagating diffraction-free guided modes in a hollow-core photonic crystal fiber at room temperature. Unlike standard laser intensity- or Coulomb force-based feedback, our approach modulates the relative optical phase between the counterpropagating fundamental modes proportionally to the particle's axial momentum. This generates a Stokes-like dissipative force which effectively damps the center-of-mass motion without introducing excess heating and can also work with uncharged particles. At 2 mbar air pressure, the axial center-of-mass temperature of a 195 nm silica particle is reduced by half upon application of the feedback and to 58.6 K at 0.5 mbar. The measured mechanical spectra agree well with our analytical model, validating the cooling mechanism. We envision this approach will open up pathways towards long-range, coherent control of mesoscopic particles inside hollow-core fibers, offering a fiber-integrated versatile platform for future quantum manipulation.

physics.optics↗

arXiv2025

Solving Dicke superradiance analytically: A compendium of methods

We present several analytical approaches to the Dicke superradiance problem, which involves determining the time evolution of the density operator for an initially inverted ensemble of $N$ identical two-level systems undergoing collective spontaneous emission. This serves as one of the simplest cases of open quantum system dynamics that allows for a fully analytical solution. We explore multiple methods to tackle this problem, yielding a solution valid for any time and any number of spins. These approaches range from solving coupled rate equations and identifying exceptional points in non-Hermitian evolution to employing combinatorial and probabilistic techniques, as well as utilizing a quantum jump unraveling of the master equation. The analytical solution is expressed as a residue sum obtained from a contour integral in the complex plane, suggesting the possibility of fully analytical solutions for a broader class of open quantum system dynamics problems.

quant-ph↗

arXiv2024

An exact analytical solution for Dicke superradiance

We revisit the Dicke superradiance problem, where an ensemble of N identical two-level systems undergoes collective spontaneous decay. While an exact analytical solution has been known since 1977, its algebraic complexity has hindered practical use. Here we present a compact, closed-form solution that expresses the dynamics as a finite sum over residues or, equivalently, a complex contour integral. The method yields explicit populations of all Dicke states at arbitrary times and system sizes, and generalizes naturally to arbitrary initial conditions. Our formulation is computationally efficient and offers structural insights into the role of spectral degeneracies and Lindbladian eigenmodes in collective decay.

quant-ph↗

arXiv2024

Optoacoustic entanglement in a continuous Brillouin-active solid state system

Entanglement in hybrid quantum systems comprised of fundamentally different degrees of freedom, such as light and mechanics is of interest for a wide range of applications in quantum technologies. Here, we propose to engineer bipartite entanglement between traveling acoustic phonons in a Brillouin active solid state system and the accompanying light wave. The effect is achieved by applying optical pump pulses to state-of-the-art waveguides, exciting a Brillouin Stokes process. This pulsed approach, in a system operating in a regime orthogonal to standard optomechanical setups, allows for the generation of entangled photon-phonon pairs, resilient to thermal fluctuations. We propose an experimental platform where readout of the optoacoustics entanglement is done by the simultaneous detection of Stokes and Anti-Stokes photons in a two-pump configuration. The proposed mechanism presents an important feature in that it does not require initial preparation of the quantum ground state of the phonon mode.

quant-ph↗

arXiv2023

Purcell modified Doppler cooling of quantum emitters inside optical cavities

Standard cavity cooling of atoms or dielectric particles is based on the action of dispersive optical forces in high-finesse cavities. We investigate here a complementary regime characterized by large cavity losses, resembling the standard Doppler cooling technique. For a single two-level emitter a modification of the cooling rate is obtained from the Purcell enhancement of spontaneous emission in the large cooperativity limit. This mechanism is aimed at cooling of quantum emitters without closed transitions, which is the case for molecular systems, where the Purcell effect can mitigate the loss of population from the cooling cycle. We extend our analytical formulation to the many particle case governed by weak individual coupling but exhibiting collective strong Purcell enhancement to a cavity mode.

quant-ph↗

arXiv2023

Metasurface-based hybrid optical cavities for chiral sensing

Quantum metasurfaces, i.e., two-dimensional subwavelength arrays of quantum emitters, can be employed as mirrors towards the design of hybrid cavities, where the optical response is given by the interplay of a cavity-confined field and the surface modes supported by the arrays. We show that, under external magnetic field control, stacked layers of quantum metasurfaces can serve as helicity-preserving cavities. These structures exhibit ultranarrow resonances and can enhance the intensity of the incoming field by orders of magnitude, while simultaneously preserving the handedness of the field circulating inside the resonator, as opposed to conventional cavities. The rapid phase shift in the cavity transmission around the resonance can be exploited for the sensitive detection of chiral scatterers passing through the cavity. We discuss possible applications of these resonators as sensors for the discrimination of chiral molecules.

quant-ph↗

arXiv2023

Scaling law for Kasha's rule in photoexcited molecular aggregates

We study the photophysics of molecular aggregates from a quantum optics perspective, with emphasis on deriving scaling laws for the fast non-radiative relaxation of collective electronic excitations, referred to as Kasha's rule. Aggregates exhibit an energetically broad manifold of collective states with delocalized electronic excitations originating from near field dipole-dipole exchanges between neighboring monomers. Photo-excitation at optical wavelengths, much larger than the monomer-monomer average separation, addresses almost exclusively symmetric collective states, which for an arrangement known as H-aggregate, show an upward hypsochromic shift. The extremely fast subsequent non-radiative relaxation via intramolecular vibrational modes populates lower energy, subradiant states, resulting in an effective inhibition of fluorescence. Our analytical treatment allows for the derivation of an approximate scaling law of this relaxation process, linear in the number of available low energy vibrational modes and directly proportional to the dipole-dipole interaction strength between neighbouring monomers.

quant-ph↗

arXiv2023

Hybrid THz architectures for molecular polaritonics

Physical and chemical properties of materials can be modified by a resonant optical mode. Such recent demonstrations have mostly relied on a planar cavity geometry, others have relied on a plasmonic resonator. However, the combination of these two device architectures have remained largely unexplored, especially in the context of maximizing light-matter interactions. Here, we investigate several schemes of electromagnetic field confinement aimed at facilitating the collective coupling of a localized photonic mode to molecular vibrations in the terahertz region. The key aspects are the use of metasurface plasmonic structures combined with standard Fabry-Perot configurations and the deposition of a thin layer of glucose, via a spray coating technique, within a tightly focused electromagnetic mode volume. More importantly, we demonstrate enhanced vacuum Rabi splittings reaching up to 200 GHz when combining plasmonic resonances, photonic cavity modes and low-energy molecular resonances. Furthermore, we demonstrate how a cavity mode can be utilized to enhance the zero-point electric field amplitude of a plasmonic resonator. Our study provides key insight into the design of polaritonic platforms with organic molecules to harvest the unique properties of hybrid light-matter states.

physics.optics↗

arXiv2022

Linear optical elements based on cooperative subwavelength emitter arrays

We describe applications of two-dimensional subwavelength quantum emitter arrays as efficient optical elements in the linear regime. For normally incident light, the cooperative optical response, stemming from emitter-emitter dipole exchanges, allows the control of the array's transmission, its resonance frequency, and bandwidth. Operations on fully polarized incident light, such as generic linear and circular polarizers as well as phase retarders can be engineered and described in terms of Jones matrices. Our analytical approach and accompanying numerical simulations identify optimal regimes for such operations and reveal the importance of adjusting the array geometry and of the careful tuning of the external magnetic fields amplitude and direction.

quant-ph↗

arXiv2022

Theory of phase-adaptive parametric cooling

We propose an adaptive phase technique for the parametric cooling of mechanical resonances. This involves the detection of the mechanical quadratures, followed by a sequence of periodic controllable adjustments of the phase of a parametric modulation. The technique allows the preparation of the quantum ground state with an exponential loss of thermal energy, similarly to the case of cold-damping or cavity self-cooling. Analytical derivations are presented for the cooling rate and final occupancies both in the classical and quantum regimes.

quant-ph↗

arXiv2022

Cooperative subwavelength molecular quantum emitter arrays

Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom. While vibrations are typically considered detrimental to coherent dynamics, we show that molecular dimers or rings can be operated as platforms for the preparation of long-lived dark superposition states aided by vibrational relaxation. In closed ring configurations, we extend previous predictions for the generation of coherent light from ideal quantum emitters to molecular emitters, quantifying the role of vibronic coupling onto the output intensity and coherence.

quant-ph↗

arXiv2021

Molecular polaritonics in dense mesoscopic disordered ensembles

We study the dependence of the vacuum Rabi splitting (VRS) on frequency disorder, vibrations, near-field effects and density in molecular polaritonics. In the mesoscopic limit, static frequency disorder alone can already introduce a loss mechanism from polaritonic states into a dark state reservoir, which we quantitatively describe, providing an analytical scaling of the VRS with the level of disorder. Disorder additionally can split a molecular ensemble into donor-type and acceptor-type molecules and the combination of vibronic coupling, dipole-dipole interactions and vibrational relaxation induces an incoherent FRET (Förster resonance energy transfer) migration of excitations within the collective molecular state. This is equivalent to a dissipative disorder and has the effect of saturating and even reducing the VRS in the mesoscopic, high-density limit. Overall, this analysis allows to quantify the crucial role played by dark states in cavity quantum electrodynamics with mesoscopic, disordered ensembles.

quant-ph↗

arXiv2021

Cooperative quantum phenomena in light-matter platforms

Quantum cooperativity is evident in light-matter platforms where quantum emitter ensembles are interfaced with confined optical modes and are coupled via the ubiquitous electromagnetic quantum vacuum. Cooperative effects can find applications, among other areas, in topological quantum optics, in quantum metrology or in quantum information. This tutorial provides a set of theoretical tools to tackle the behavior responsible for the onset of cooperativity by extending open quantum system dynamics methods, such as the master equation and quantum Langevin equations, to electron-photon interactions in strongly coupled and correlated quantum emitter ensembles. The methods are illustrated on a wide range of current research topics such as the design of nanoscale coherent light sources, highly-reflective quantum metasurfaces or low intracavity power superradiant lasers. The analytical approaches are developed for ensembles of identical two-level quantum emitters and then extended to more complex systems where frequency disorder or vibronic couplings are taken into account. The relevance of the approach ranges from atoms in optical lattices to quantum dots or molecular systems in solid-state environments.

quant-ph↗

arXiv2021

Excitation transport with collective radiative decay

We investigate a one-dimensional quantum emitter chain where transport of excitations and correlations takes place via nearest neighbor, dipole-dipole interactions. In the presence of collective radiative emission, we show that a phase imprinting wavepacket initialization procedure can lead to subradiant transport and can preserve quantum correlations. In the context of cavity mediated transport, where emitters are coupled to a common delocalized optical mode, we analyze the effect of frequency disorder and nonidentical photon-emitter couplings on excitation transport.

quant-ph↗