arXiv subjects

Cleaven Chia

Publications and source records attributed to Cleaven Chia.

14 recordsLinked to original sources

arXiv2025

Purcell-enhanced spin-phonon coupling with a single color center

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely used in quantum computing and communication to channel photons emitted by atoms into well-defined modes and control atom-photon interactions. For solid-state artificial atoms, such as color-centers, the host lattice introduces an acoustic environment, allowing excited atoms to relax by emitting phonons. Here we observe the acoustic Purcell effect by constructing a specially engineered, microwave-frequency nanomechanical resonator around a color-center spin qubit in diamond. Using a co-localized optical mode of the structure that strongly couples to the color-center's excited state, we perform single-photon-level laser spectroscopy at milliKelvin temperatures and observe ten-fold faster spin relaxation when the spin qubit is tuned into resonance with a 12 GHz acoustic mode. Additionally, we use the color-center as an atomic-scale probe to measure the broadband phonon spectrum of the nanostructure up to a frequency of 28 GHz. Our work establishes a new regime of control for quantum defects in solids and paves the way for interconnects between atomic-scale quantum memories and qubits encoded in acoustic and superconducting devices.

quant-ph↗

arXiv2024

Limitations in design and applications of ultra-small mode volume photonic crystals

Ultra-small mode volume nanophotonic crystal cavities have been proposed as powerful tools for increasing coupling rates in cavity quantum electrodynamics systems. However, their adoption in quantum information applications remains elusive. In this work, we investigate possible reasons why, and analyze the impact of different low mode volume resonator design choices on their utility in quantum optics experiments. We analyze band structure features and loss rates of low mode volume bowtie cavities in diamond and demonstrate independent design control over cavity-emitter coupling strength and loss rates. Further, using silicon vacancy centers in diamond as exemplary emitters, we investigate the influence of placement imprecision. We find that the benefit on photon collection efficiency and indistinguishability is limited, while the fabrication complexity of ultra-small cavity designs increases substantially compared to conventional photonic crystals. We conclude that ultra-small mode volume designs are primarily of interest for dispersive spin-photon interactions, which are of great interest for future quantum networks.

quant-ph↗

arXiv2024

Hybrid quantum systems with artificial atoms in solid state

The development of single-platform qubits, predominant for most of the last few decades, has driven the progress of quantum information technologies but also highlighted the limitations of various platforms. Some inherent issues such as charge/spin noise in materials hinder certain platforms, while increased decoherence upon attempts to scale-up severely impact qubit quality and coupling on others. In addition, a universal solution for coherent information transfer between quantum systems remains lacking. By combining one or more qubit platforms, one could potentially create new hybrid platforms that might alleviate significant issues that current single platform qubits suffer from, and in some cases, even facilitate the conversion of static to flying qubits on the same hybrid platform. While nascent, this is an area of rising importance that could shed new light on robust and scalable qubit development and provide new impetus for research directions. Here, we define the requirements for hybrid systems with artificial atoms in solid state, exemplify them with systems that have been proposed or attempted, and conclude with our outlook for such hybrid quantum systems.

quant-ph↗

arXiv2023

High Q-factor diamond optomechanical resonators with silicon vacancy centers at millikelvin temperatures

Phonons are envisioned as coherent intermediaries between different types of quantum systems. Engineered nanoscale devices such as optomechanical crystals (OMCs) provide a platform to utilize phonons as quantum information carriers. Here we demonstrate OMCs in diamond designed for strong interactions between phonons and a silicon vacancy (SiV) spin. Using optical measurements at millikelvin temperatures, we measure a linewidth of 13 kHz (Q-factor of ~440,000) for 6 GHz acoustic modes, a record for diamond in the GHz frequency range and within an order of magnitude of state-of-the-art linewidths for OMCs in silicon. We investigate SiV optical and spin properties in these devices and outline a path towards a coherent spin-phonon interface.

physics.optics↗

arXiv2023

Engineering Phonon-Qubit Interactions using Phononic Crystals

The ability to control phonons in solids is key for diverse quantum applications, ranging from quantum information processing to sensing. Often, phonons are sources of noise and decoherence, since they can interact with a variety of solid-state quantum systems. To mitigate this, quantum systems typically operate at milli-Kelvin temperatures to reduce the number of thermal phonons. Here we demonstrate an alternative approach that relies on engineering phononic density of states, drawing inspiration from photonic bandgap structures that have been used to control the spontaneous emission of quantum emitters. We design and fabricate diamond phononic crystals with a complete phononic bandgap spanning 50 - 70 gigahertz, tailored to suppress interactions of a single silicon-vacancy color center with resonant phonons of the thermal bath. At 4 Kelvin, we demonstrate a reduction of the phonon-induced orbital relaxation rate of the color center by a factor of 18 compared to bulk. Furthermore, we show that the phononic bandgap can efficiently suppress phonon-color center interactions up to 20 Kelvin. In addition to enabling operation of quantum memories at higher temperatures, the ability to engineer qubit-phonon interactions may enable new functionalities for quantum science and technology, where phonons are used as carriers of quantum information.

quant-ph↗

arXiv2023

Integrated Phononic Waveguides in Diamond

Efficient generation, guiding, and detection of phonons, or mechanical vibrations, are of interest in various fields including radio frequency communication, sensing, and quantum information. Diamond is an important platform for phononics because of the presence of strain-sensitive spin qubits, and its high Young's modulus which allows for low-loss gigahertz devices. We demonstrate a diamond phononic waveguide platform for generating, guiding, and detecting gigahertz-frequency surface acoustic wave (SAW) phonons. We generate SAWs using interdigital transducers integrated on AlN/diamond and observe SAW transmission at 4-5 GHz through both ridge and suspended waveguides, with wavelength-scale cross sections (~1 μm2) to maximize spin-phonon interaction. This work is a crucial step for developing acoustic components for quantum phononic circuits with strain-sensitive color centers in diamond.

physics.app-ph↗

arXiv2022

Development of hard masks for reactive ion beam angled etching of diamond

Diamond offers good optical properties and hosts bright color centers with long spin coherence times. Recent advances in angled-etching of diamond, specifically with reactive ion beam angled etching (RIBAE), have led to successful demonstration of quantum photonic devices operating at visible wavelengths. However, larger devices operating at telecommunication wavelengths have been difficult to fabricate due to the increased mask erosion, arising from the increased size of devices requiring longer etch times. We evaluated different mask materials for RIBAE of diamond photonic crystal nanobeams and waveguides, and how their thickness, selectivity, aspect ratio and sidewall smoothness affected the resultant etch profiles and optical performance. We found that a thick hydrogen silesquioxane (HSQ) layer on a thin alumina adhesion layer provided the best etch profile and optical performance. The techniques explored in this work can also be adapted to other bulk materials that are not available heteroepitaxially or as thin films-on-insulator.

physics.app-ph↗

arXiv2021

Telecommunication-wavelength two-dimensional photonic crystal cavities in a thin single-crystal diamond membrane

We demonstrate two-dimensional photonic crystal cavities operating at telecommunication wavelengths in a single-crystal diamond membrane. We use a high-optical-quality and thin (~ 300 nm) diamond membrane, supported by a polycrystalline diamond frame, to realize fully suspended two-dimensional photonic crystal cavities with a high theoretical quality factor of ~ $8\times10^6$ and a relatively small mode volume of ~2$(λ/n)^3$. The cavities are fabricated in the membrane using electron-beam lithography and vertical dry etching. We observe cavity resonances over a wide wavelength range spanning the telecommunication O- and S-bands (1360 nm-1470 nm) with Q factors of up to ~1800. Our method offers a new direction for on-chip diamond nanophotonic applications in the telecommunication-wavelength range.

physics.optics↗

arXiv2021

Coupling of a Single Tin-vacancy Center to a Photonic Crystal Cavity in Diamond

We demonstrate optical coupling between a single tin-vacancy (SnV) center in diamond and a free-standing photonic crystal nanobeam cavity. The cavities are fabricated using quasi-isotropic etching and feature experimentally measured quality factors as high as ~11,000. We investigate the dependence of a single SnV center's emission by controlling the cavity wavelength using a laser-induced gas desorption technique. Under resonance conditions, we observe an intensity enhancement of the SnV emission by a factor of 12 and a 16-fold reduction of the SnV lifetime. Based on the large enhancement of the SnV emission rate inside the cavity, we estimate the Purcell factor for the SnV zero-phonon line to be 37 and the coupling efficiency of the SnV center to the cavity, the beta factor, to be 95%. Our work paves the way for the realization of quantum photonic devices and systems based on efficient photonic interfaces using the SnV color center in diamond.

physics.optics↗

arXiv2019

Coherent Acoustic Control of a Single Silicon Vacancy Spin in Diamond

Phonons are considered to be universal quantum transducers due to their ability to couple to a wide variety of quantum systems. Among these systems, solid-state point defect spins are known for being long-lived optically accessible quantum memories. Recently, it has been shown that inversion-symmetric defects in diamond, such as the negatively charged silicon vacancy center (SiV), feature spin qubits that are highly susceptible to strain. Here, we leverage this strain response to achieve coherent and low-power acoustic control of a single SiV spin, and perform acoustically driven Ramsey interferometry of a single spin. Our results demonstrate a novel and efficient method of spin control for these systems, offering a path towards strong spin-phonon coupling and phonon-mediated hybrid quantum systems.

quant-ph↗

arXiv2019

Microwave-to-optical conversion using lithium niobate thin-film acoustic resonators

We demonstrate conversion of up to 4.5 GHz-frequency microwaves to 1500 nm-wavelength light using optomechanical interactions on suspended thin-film lithium niobate. Our method utilizes an interdigital transducer that drives a free-standing 100 $μ$m-long thin-film acoustic resonator to modulate light travelling in a Mach-Zehnder interferometer or racetrack cavity. Owing to the strong microwave-to-acoustic coupling offered by the transducer in conjunction with the strong photoelastic, piezoelectric, and electro-optic effects of lithium niobate, we achieve a half-wave voltage of $V_π$ = 4.6 V and $V_π$ = 0.77 V for the Mach-Zehnder interferometer and racetrack resonator, respectively. The acousto-optic racetrack cavity exhibits an optomechancial single-photon coupling strength of 1.1 kHz. Our integrated nanophotonic platform coherently leverages the compelling properties of lithium niobate to achieve microwave-to-optical transduction. To highlight the versatility of our system, we also demonstrate a lossless microwave photonic link, which refers to a 0 dB microwave power transmission over an optical channel.

physics.app-ph↗

arXiv2019

Quantum interference of electromechanically stabilized emitters in nanophotonic devices

Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical transitions. Here we present a nano-electromechanical platform for stabilization and tuning of optical transitions of silicon-vacancy (SiV) color centers in diamond nanophotonic devices by dynamically controlling their strain environments. This strain-based tuning scheme has sufficient range and bandwidth to alleviate the spectral mismatch between individual SiV centers. Using strain, we ensure overlap between color center optical transitions and observe an entangled superradiant state by measuring correlations of photons collected from the diamond waveguide. This platform for tuning spectrally stable color centers in nanophotonic waveguides and resonators constitutes an important step towards a scalable quantum network.

physics.app-ph↗

arXiv2018

Strain engineering of the silicon-vacancy center in diamond

We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system. This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multi-qubit networks. In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states. We identify regimes where the spin-orbit interaction results in a large strain suseptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator.

quant-ph↗

arXiv2016

Diamond optomechanical crystals

Cavity-optomechanical systems realized in single-crystal diamond are poised to benefit from its extraordinary material properties, including low mechanical dissipation and a wide optical transparency window. Diamond is also rich in optically active defects, such as the nitrogen-vacancy (NV) and silicon-vacancy (SiV) centers, which behave as atom-like systems in the solid state. Predictions and observations of coherent coupling of the NV electronic spin to phonons via lattice strain has motivated the development of diamond nanomechanical devices aimed at realization of hybrid quantum systems, in which phonons provide an interface with diamond spins. In this work, we demonstrate diamond optomechanical crystals (OMCs), a device platform to enable such applications, wherein the co-localization of ~ 200 THz photons and few to 10 GHz phonons in a quasi-periodic diamond nanostructure leads to coupling of an optical cavity field to a mechanical mode via radiation pressure. In contrast to other material systems, diamond OMCs operating in the resolved-sideband regime possess large intracavity photon capacity (> 10$^5$) and sufficient optomechanical coupling rates to reach a cooperativity of ~ 20 at room temperature, allowing for the observation of optomechanically induced transparency and the realization of large amplitude optomechanical self-oscillations.

cond-mat.mes-hall↗