arXiv subjects

Coleman Collins

Publications and source records attributed to Coleman Collins.

3 recordsLinked to original sources

arXiv2026

Measuring what matters: A scalable framework for application-level quantum benchmarking

As quantum computing systems continue to mature, there is an increasing need for benchmarking methodologies that capture performance in terms of meaningful, application-level metrics. In this work, we present a scalable framework for application-level quantum benchmarking that is designed to support internal system evaluation and cross-platform comparison across technology providers. Our framework is guided by a set of core principles, including measurability, simplicity, scalability, and extensibility. We present 13 benchmark families that reflect realistic workloads across multiple domains. This enables the systematic evaluation of the quality of solutions, the total execution time, total used energy, as well as Time-to-Solution. The benchmarks are designed to be reproducible, interpretable across stakeholder groups, and adaptable to evolving system capabilities. The framework aims to bridge the gap between low-level performance metrics and real-world value, providing a unified approach to assessing quantum systems. The resulting benchmarks support development and validation and contribute to the foundation of industry-wide benchmarking standards.

quant-ph↗

arXiv2025

Quantum-Classical Auxiliary Field Quantum Monte Carlo with Matchgate Shadows on Trapped Ion Quantum Computers

We demonstrate an end-to-end workflow to model chemical reaction barriers with the quantum-classical auxiliary field quantum Monte Carlo (QC-AFQMC) algorithm with quantum tomography using matchgate shadows. The workflow operates within an accelerated quantum supercomputing environment with the IonQ Forte quantum computer and NVIDIA GPUs on Amazon Web Services. We present several algorithmic innovations and an efficient GPU-accelerated execution, which achieves a several orders of magnitude speedup over the state-of-the-art implementation of QC-AFQMC. We apply the algorithm to simulate the oxidative addition step of the nickel-catalyzed Suzuki-Miyaura reaction using 24 qubits of IonQ Forte with 16 qubits used to represent the trial state, plus 8 additional ancilla qubits for error mitigation, resulting in the largest QC-AFQMC with matchgate shadow experiments ever performed on quantum hardware. We achieve a $9\times$ speedup in collecting matchgate circuit measurements, and our distributed-parallel post-processing implementation attains a $656\times$ time-to-solution improvement over the prior state-of-the-art. Chemical reaction barriers for the model reaction evaluated with active-space QC-AFQMC are within the uncertainty interval of $\pm4$ kcal/mol from the reference CCSD(T) result when matchgates are sampled on the ideal simulator and within 10 kcal/mol from reference when measured on QPU. This work marks a step towards practical quantum chemistry simulations on quantum devices while identifying several opportunities for further development.

quant-ph↗

arXiv2019

Ground-state energy estimation of the water molecule on a trapped ion quantum computer

Quantum computing leverages the quantum resources of superposition and entanglement to efficiently solve computational problems considered intractable for classical computers. Examples include calculating molecular and nuclear structure, simulating strongly-interacting electron systems, and modeling aspects of material function. While substantial theoretical advances have been made in mapping these problems to quantum algorithms, there remains a large gap between the resource requirements for solving such problems and the capabilities of currently available quantum hardware. Bridging this gap will require a co-design approach, where the expression of algorithms is developed in conjunction with the hardware itself to optimize execution. Here, we describe a scalable co-design framework for solving chemistry problems on a trapped ion quantum computer, and apply it to compute the ground-state energy of the water molecule. The robust operation of the trapped ion quantum computer yields energy estimates with errors approaching the chemical accuracy, which is the target threshold necessary for predicting the rates of chemical reaction dynamics.

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