arXiv subjects

Colin V. Parker

Publications and source records attributed to Colin V. Parker.

At least 19 recordsLinked to original sources

arXiv2025

Crystal Fields and Zeeman Effect for Thulium in Solid Argon

Optically active defects suspended in an inert solid are an interesting system for sensing and magnetometry at the nanometer scale, in addition to being a potential source of high-density, identical quantum emitters for quantum information. Beyond their response to external fields, the optical absorption and emission spectra also reflect information about the host matrix, which is critical to understand for either application. For the particular system of thulium atoms implanted in solid argon, high resolution laser spectroscopy reveals narrow ensemble linewidths of the 1140 nm f to f ground state spin-orbit transition, which is split due to crystal field effects and hyperfine coupling. Pump-probe spectroscopy is used to identify crystal field levels in at least two stable trapping sites, and the crystal field is determined to be nearly axial in both sites. Strong selection rules indicate that this transition becomes magnetic-electric in the argon host, most likely due to dielectric effects. In the presence of mT magnetic fields, Zeeman shifts are resolvable by laser fluorescence, allowing crystal axis selective polarized spectroscopy. These results show that all-optical detection schemes for DC magnetic fields are already possible with thulium-doped argon, and point towards more informed strategies for monitoring and improving crystal growth and annealing.

physics.atom-ph↗

arXiv2023

High resolution spectroscopy of thulium atoms implanted in solid noble gas crystals

Optically active defects in solid-state systems have many applications in quantum information and sensing. However, unlike free atoms, which have fixed optical transition frequencies, the inhomogeneous broadening of the transitions in solid-state environments limit their use as identical scatterers for such applications. Here we show that crystals of argon and neon prepared in a closed-cycle cryostat doped with thulium atoms at cryogenic temperatures are an exception. High resolution absorption and emission spectroscopy show that the 1140 nm magnetic dipole transition is split into multiple components. The origin of this splitting is likely a combination of different classes of trapping sites, crystal field effects within each site, and hyperfine interactions. The individual lines have ensemble widths as small as 0.6 GHz, which temperature dependence and pump-probe spectroscopy indicate is likely a homogeneous effect, suggesting inhomogeneity is well below the GHz scale.

physics.atom-ph↗

arXiv2023

Instability and Momentum Bifurcation of molecular BEC in Exotic Dispersion with Shaken Lattice

We place a molecular Bose-Einstein condensate in a 1D shaken lattice with a Floquet-engineered dispersion, and observe the dynamics in both position and momentum space. At the initial condition of zero momentum, our engineered dispersion is inverted, and therefore unstable. We observe that the condensate is destabilized by the lattice shaking as expected, but rather than decaying incoherently or producing jets, as in other unstable condensates, under our conditions the condensate bifurcates into two portions in momentum space, with each portion subsequently following semi-classical trajectories that suffer minimal spreading in momentum space as they evolve. We can model the evolution with a Gross-Pitaevskii equation, which suggests the initial bifurcation is facilitate by a nearly linear "inverted V"-shaped dispersion at the zone center, while the lack of spreading in momentum space is facilitated by interactions, as in a soliton. We propose that this relatively clean bifurcation in momentum space has applications for counter-diabatic preparation of exotic ground states in many-body quantum simulation schemes.

cond-mat.quant-gas↗

arXiv2020

Spin Susceptibility Above the Superfluid Onset in Ultracold Fermi Gases

Ultracold atomic Fermi gases can be tuned to interact strongly, where they display spectroscopic signatures above the superfluid transition reminiscent of the pseudogap in cuprates. However, the extent of the analogy can be questioned, since thermodynamic quantities in the low temperature spin-imbalanced normal state can be described successfully using Fermi liquid theory. Here we present spin susceptibility measurements across the interaction strength-temperature phase diagram using a novel radiofrequency technique with ultracold $^6\textrm{Li}$ gases. For all significant interaction strengths and at all temperatures we find the spin susceptibility is reduced compared with the equivalent value for a non-interacting Fermi gas, with the low temperature results consistent with previous studies. However, our measurements extend to higher temperatures, where we find that the reduction persists consistently with a mean-field scenario. At unitarity, we can use the local density approximation to extract the spin susceptibility for the uniform gas, which is well described by mean-field models at temperatures from the superfluid transition to the Fermi temperature.

cond-mat.quant-gas↗

arXiv2020

Enhanced principle component method for fringe removal in cold atom images

Many powerful imaging techniques for cold atoms are based on determining the optical density by comparing a beam image having passed through the atom cloud to a reference image taken under similar conditions with no atoms. In practice the beam profile typically contains interference fringes whose phase is not stable between camera exposures. To reduce the error of these fringes in the computed optical density, an algorithm based on principle component analysis (PCA) is often employed. However, PCA is general purpose and not tailored to the specific case of interference fringes. Here we demonstrate an algorithm that takes advantage of the Fourier-space structure of interference fringes to further reduce the residual fringe signatures in the optical density.

physics.atom-ph↗

arXiv2019

Sub-nanometer optical linewidth of thulium atoms in rare gas crystals

We investigate the 1140 nm magnetic dipole transition of thulium atoms trapped in solid argon and neon. These solids can be straightforwardly grown on any substrate at cryogenic temperatures, making them prime targets for surface sensing applications. Our data are well described by a splitting of the single vacuum transition into three components in both argon and neon, with each component narrower than the 0.8 nm spectrometer resolution. The lifetime of the excited states is 14.6(0.5) ms in argon and 27(3) ms in neon, shorter than in vacuum or in solid helium. We also collected visible laser-induced fluorescence spectroscopy showing broader emission features in the range of 580-600 nm. The narrow infrared features in particular suggest a range of possible applications.

physics.atom-ph↗

arXiv2018

All-optical production of ${}^6\textrm{Li}$ molecular BEC in excited hyperfine levels

We present an all-optical method for achieving molecular Bose-Einstein condensates of ${}^6\textrm{Li}$. We demonstrate this with mixtures in the lowest two (1-2), and second lowest two (2-3) hyperfine states. For the 1-2 mixture, we can achieve condensate fractions of 36\%, with $9\times10^4$ atoms at $0.05\textrm{ }μ\textrm{K}$ temperature. For the 2-3 mixture, we have 28\% condensed with $3.2\times10^4$ atoms at $0.05\textrm{ }μ\textrm{K}$ temperature. We use mostly standard methods, but make a number of refinements in the magnetic bias coils compared with earlier work. Our method imposes minimal constraints on subsequent experiments by allowing plenty of optical access while requiring only one high-vacuum chamber. We use an optical system designed around minimizing the number of active elements, and we can accomplish slowing and sub-Doppler cooling with a single tapered amplifier

physics.atom-ph↗

arXiv2015

Mobile magnetic impurities in a Fermi superfluid: a route to designer molecules

A magnetic impurity in a fermionic superfluid hosts bound quasiparticle states known as Yu-Shiba-Rusinov (YSR) states. We argue here that, if the impurity is mobile (i.e., has a finite mass), the impurity and its bound YSR quasiparticle move together as a midgap molecule, which has an unusual "Mexican-hat" dispersion that is tunable via the fermion density. We map out the impurity dispersion, which consists of an "atomic" branch (in which the impurity is dressed by quasiparticle pairs) and a "molecular" branch (in which the impurity binds a quasiparticle). We discuss the experimental realization and detection of midgap Shiba molecules, focusing on lithium-cesium mixtures, and comment on the prospects they offer for realizing exotic many-body states.

cond-mat.quant-gas↗

arXiv2015

Roton-Maxon Excitation Spectrum of Bose Condensates in a Shaken Optical Lattice

We present experimental evidence showing that an interacting Bose condensate in a shaken optical lattice develops a roton-maxon excitation spectrum, a feature normally associated with superfluid helium. The roton-maxon feature originates from the double-well dispersion in the shaken lattice, and can be controlled by both the atomic interaction and the lattice shaking amplitude. We determine the excitation spectrum using Bragg spectroscopy and measure the critical velocity by dragging a weak speckle potential through the condensate - both techniques are based on a digital micromirror device. Our dispersion measurements are in good agreement with a modified-Bogoliubov model.

cond-mat.quant-gas↗

arXiv2015

Simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K on the D$_1$ line: Theory and Experiment

We report on simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K using the D$_1$ optical transitions. We compare experimental results to a numerical simulation of the cooling process applying a semi-classical Monte Carlo wavefunction method. The simulation takes into account the three dimensional optical molasses setup and the dipole interaction between atoms and the bichromatic light field driving the D$_1$ transitions. We discuss the physical mechanisms at play, we identify the important role of coherences between the ground state hyperfine levels and compare D$_1$ and D$_2$ sub-Doppler cooling. In 5 ms, the D$_1$ molasses phase largely reduces the temperature for both $^6$Li and $^{40}$K at the same time, with a final temperature of 44 $μ$K and 11 $μ$K, respectively. For both species this leads to a phase-space density close to $10^{-4}$. These conditions are well suited to directly load an optical or magnetic trap for efficient evaporative cooling to quantum degeneracy.

physics.atom-ph↗

arXiv2014

Geometric scaling of Efimov states in a $^{6}\textrm{Li}$-$^{133}\textrm{Cs}$ mixture

In few-body physics, Efimov states are an infinite series of three-body bound states that obey universal discrete scaling symmetry when pairwise interactions are resonantly enhanced. Despite abundant reports of Efimov states in recent cold atom experiments, direct observation of the discrete scaling symmetry remains an elusive goal. Here we report the observation of three consecutive Efimov resonances in a heteronuclear Li-Cs mixture near a broad interspecies Feshbach resonance. The positions of the resonances closely follow a geometric series $1$, $λ$, $λ^2$. The observed scaling constant $λ_{\rm exp} = 4.9(4)$ is in good agreement with the predicted value of 4.88.

cond-mat.quant-gas↗

arXiv2013

Efficient Continuous-Duty Bitter-Type Electromagnets for Cold Atom Experiments

We present the design, construction and characterization of Bitter-type electromagnets which can generate high magnetic fields under continuous operation with efficient heat removal for cold atom experiments. The electromagnets are constructed from a stack of alternating layers consisting of copper arcs and insulating polyester spacers. Efficient cooling of the copper is achieved via parallel rectangular water cooling channels between copper layers with low resistance to flow; a high ratio of the water-cooled surface area to the volume of copper ensures a short length scale ~1 mm to extract dissipated heat. High copper fraction per layer ensures high magnetic field generated per unit energy dissipated. The ensemble is highly scalable and compressed to create a watertight seal without epoxy. From our measurements, a peak field of 770 G is generated 14 mm away from a single electromagnet with a current of 400 A and a total power dissipation of 1.6 kW. With cooling water flowing at 3.8 l/min, the coil temperature only increases by 7 degrees Celsius under continuous operation.

physics.ins-det↗

arXiv2013

In situ observation of strongly interacting ferromagnetic domains in a shaken optical lattice

Solid state systems derive their richness from the interplay between interparticle interactions and novel band structures that deviate from those of free particles. Strongly interacting systems, where both of these phenomena are of equal importance, exhibit a variety of theoretically interesting and practically useful phases. Systems of ultracold atoms are rapidly emerging as precise and controllable simulators, and it is precisely in this strongly interacting regime where simulation is the most useful. Here we demonstrate how to hybridize Bloch bands in optical lattices to introduce long-range ferromagnetic order in an itinerant atomic system. We find spontaneously broken symmetry for bosons with a double-well dispersion condensing into one of two distinct minima, which we identify with spin-up and spin-down. The density dynamics following a rapid quench to the ferromagnetic state confirm quantum interference between the two states as the mechanism for symmetry breaking. Unlike spinor condensates, where interaction is driven by small spin-dependent differences in scattering length, our interactions scale with the scattering length itself, leading to domains which equilibrate rapidly and develop sharp boundaries characteristic of a strongly interacting ferromagnet.

cond-mat.quant-gas↗

arXiv2011

Scattering from incipient stripe order in the high-temperature superconductor Bi2Sr2CaCu2O8+d

Recently we have used spectroscopic mapping with the scanning tunneling microscope to probe modulations of the electronic density of states in single crystals of the high temperature superconductor Bi2Sr2CaCu2O8+d (Bi-2212) as a function of temperature [C. V. Parker et al., Nature (London) 468, 677 (2010)]. These measurements showed Cu-O bond-oriented modulations that form below the pseudogap temperature with a temperature-dependent energy dispersion displaying different behaviors in the superconducting and pseudogap states. Here we demonstrate that quasiparticle scattering off impurities does not capture the experimentally observed energy- and temperature-dependence of these modulations. Instead, a model of scattering of quasiparticles from short-range stripe order, with periodicity near four lattice constants (4a), reproduces the experimentally observed energy dispersion of the bond-oriented modulations and its temperature dependence across the superconducting critical temperature, Tc. The present study confirms the existence of short-range stripe order in Bi-2212.

cond-mat.str-el↗

arXiv2010

Appearance of fluctuating stripes at the onset of the pseudogap in the high-Tc Superconductor Bi2Sr2CaCu2O8+x

Doped Mott insulators have been shown to have a strong propensity to form patterns of holes and spins often referred to as stripes. In copper-oxides, doping also gives rise to the pseudogap state, which transforms into a high temperature superconductor with sufficient doping or by reducing the temperature. A long standing question has been the interplay between pseudogap, which is generic to all hole-doped cuprates, and stripes, whose static form occurs in only one family of cuprates over a narrow range of the phase diagram. Here we examine the spatial reorganization of electronic states with the onset of the pseudogap state at T* in the high-temperature superconductor Bi2Sr2CaCu2O8+x using spectroscopic mapping with the scanning tunneling microscope (STM). We find that the onset of the pseudogap phase coincides with the appearance of electronic patterns that have the predicted characteristics of fluctuating stripes. As expected, the stripe patterns are strongest when the hole concentration in the CuO2 planes is close to 1/8 (per Cu). While demonstrating that the fluctuating stripes emerge with the onset of the pseudogap state and occur over a large part of the cuprate phase diagram, our experiments indicate that they are a consequence of pseudogap behavior rather than its cause.

cond-mat.supr-con↗

arXiv2010

Visualizing the Formation of the Kondo Lattice and the Hidden Order in URu2Si2

Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope (STM) to examine the novel electronic states that emerge from the uranium f states in URu2Si2. We find that as the temperature is lowered, partial screening of the f electrons' spins gives rise to a spatially modulated Kondo-Fano resonance that is maximal between the surface U atoms. At T=17.5 K, URu2Si2 is known to undergo a 2nd order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states.

cond-mat.str-el↗

arXiv2010

Nanoscale Proximity Effect in the High Temperature Superconductor Bi-2212

High temperature cuprate superconductors exhibit extremely local nanoscale phenomena and strong sensitivity to doping. While other experiments have looked at nanoscale interfaces between layers of different dopings, we focus on the interplay between naturally inhomogeneous nanoscale regions. Using scanning tunneling microscopy to carefully track the same region of the sample as a function of temperature, we show that regions with weak superconductivity can persist to elevated temperatures if bordered by regions of strong superconductivity. This suggests that it may be possible to increase the maximum possible transition temperature by controlling the distribution of dopants.

cond-mat.supr-con↗

arXiv2009

Topological Surface States Protected From Backscattering by Chiral Spin Texture

Topological insulators are a new class of insulators in which a bulk gap for electronic excitations is generated by strong spin orbit coupling. These novel materials are distinguished from ordinary insulators by the presence of gapless metallic boundary states, akin to the chiral edge modes in quantum Hall systems, but with unconventional spin textures. Recently, experiments and theoretical efforts have provided strong evidence for both two- and three-dimensional topological insulators and their novel edge and surface states in semiconductor quantum well structures and several Bi-based compounds. A key characteristic of these spin-textured boundary states is their insensitivity to spin-independent scattering, which protects them from backscattering and localization. These chiral states are potentially useful for spin-based electronics, in which long spin coherence is critical, and also for quantum computing applications, where topological protection can enable fault-tolerant information processing. Here we use a scanning tunneling microscope (STM) to visualize the gapless surface states of the three-dimensional topological insulator BiSb and to examine their scattering behavior from disorder caused by random alloying in this compound. Combining STM and angle-resolved photoemission spectroscopy, we show that despite strong atomic scale disorder, backscattering between states of opposite momentum and opposite spin is absent. Our observation of spin-selective scattering demonstrates that the chiral nature of these states protects the spin of the carriers; they therefore have the potential to be used for coherent spin transport in spintronic devices.

cond-mat.mtrl-sci↗