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Cong Xiao

Publications and source records attributed to Cong Xiao.

At least 19 recordsLinked to original sources

Quantum Geometric Origin of Nonlinear Current Induced Orbital Magnetization

Electric generation of magnetization is a focus of condensed matter research, and has recently been advanced into the nonlinear regime. However, due to the nonlocal nature of orbital magnetism, how to properly formulate nonlinear current-induced orbital magnetization remains a fundamental challenge. Here, we develop the proper theory for this effect. This is based on the microscopic derivation of field-corrected orbital magnetic moment of a Bloch electron, a critical missing piece in the present theory. We show that the quantum geometric origin of this phenomenon lies in both the anomalous orbital polarizability and the Berry-connection polarizability, which often provide competing contributions. Combining our theory with first-principles calculations, we predict significant, experimentally accessible nonlinear orbital magnetization generated in strained bilayer graphene, monolayer 1T' $\mathrm{MoS_2}$ and $\mathrm{MoTe_2}$. Remarkably, nonlinear orbital magnetization can dominate over its spin counterpart in materials with topological band features, irrespective of the spin-orbit coupling strength.

cond-mat.mes-hall

Interlayer electric multipole Hall effect in twisted multilayers

Electrons in layered van der Waals materials possess a layer pseudospin characterizing their wave-function distribution among layers. In twisted structures, this pseudospin forms nontrivial textures, leading to intriguing phenomena such as the layer Hall effect (LHE), where distinct layer Hall currents flow despite the presence of time-reversal symmetry. In chiral bilayers, LHE manifests as an interlayer electric dipole Hall effect with Hall counterflows and a concomitant in-plane magnetic dipole. Multilayers host richer layer-dependent Hall currents, generating interlayer electric multipole Hall effects and in-plane magnetic multipoles. We start from exploring the interlayer electric quadrupole Hall effect in mirror-symmetric twisted trilayers. At small twist angles, interlayer translation efficiently tunes layer Hall current magnitudes. At large angles and low doping, the currents can be well accounted for by adding the contributions from the two individual twisted interfaces. This decomposition allows obtaining layer-resolved Hall currents in large-angle twisted multilayers even without well-defined periodicity.

cond-mat.mes-hall

Surface Originated Cross-Field Anomalous Transport in Magnetoelectric Multilayers

In material systems with slab geometry, the surface contribution to physical responses is commonly expected to diminish rapidly with increasing thickness, giving way to the bulk response. Here, we show that this conventional wisdom is violated in a class of gate-induced responses, including gate-induced orbital and spin magnetization as well as cross-field anomalous thermoelectric transport. We develop a general framework for these effects, which naturally decomposes the total response into surface- and bulk-contributions treated on equal footing. Remarkably, the volume-averaged surface contribution remains finite in the thick-slab limit and exhibits the same thickness scaling as the bulk term. Furthermore, the surface response originates from band geometric quantities distinct from those in the bulk, being constrained solely by surface symmetries. As a result, it can dominate the overall response when the bulk contribution is symmetry-forbidden. Taking MnBi$_2$Te$_4$ multilayers as an example, we predict a strong surface-dominated cross-field anomalous Nernst effect arising from surface Berry curvature, which is readily accessible to experimental detection. These findings reveal a previously overlooked significance of surface response and open a new direction in the study of surface quantum geometry.

cond-mat.mes-hall

Zero-Field Thermal Hall Effect in Insulator

Fourier's law dictates that heat flow is usually parallel to the applied temperature gradient. However, under a high magnetic field, heat flow carried by both electrons in conductors and phonons in insulators can be deflected, a phenomenon known as thermal Hall effect. Intriguingly, we observe at zero field a spontaneous thermal Hall effect in an antiferromagnetic insulator. Despite a vanishingly small uncompensated magnetization, the magnitude of this effect is surprisingly large, comparable to typical responses induced by several teslas of external field. This zero-field behavior indicates that charge-neutral heat carriers can be governed by an intrinsic effective field arising from the unique spin arrangement. Our discovery challenges the centuries-old preconception of heat conduction and open up new avenues for exploring non-trivial topological responses in quantum materials.

cond-mat.str-el

Symplectic connection third-order Hall effect in a room-temperature ferromagnet

Third-order nonlinear Hall effects (THE) have recently attracted considerable experimental interest as powerful probes for quantum geometric properties in emergent quantum materials, encompassing quadrupole moments of quantum metric and Berry curvature. Here, we report a fundamentally new THE in room-temperature van der Waals ferromagnet Fe3GaTe2 from second-order Berry connection polarizability, which manifests a higher-order characterization of band geometry called symplectic connection. Our observations show that the third-order transverse response in Fe3GaTe2 is odd to magnetization, vanishes above the Curie temperature and remains independent of driving current directions. Scaling law analysis combined with first-principles calculations establishes this response as the symplectic-connection-induced THE. This discovery opens the door to probing high-order quantum geometric properties beyond Berry curvature and quantum metric through nonlinear transport, unveiling the potential of exploring nonlinear Hall phenomena in broad classes of magnets without breaking inversion symmetry. Moreover, the room-temperature manipulation of THE holds promises for device applications based on harnessing the quantum-geometric connection structure.

cond-mat.mes-hall

Disorder induced time-reversal-odd nonlinear spin and orbital Hall effects

We develop a theory for the second-order time-reversal-odd ($\mathcal{T}$-odd) angular-momentum current, incorporating both spin and orbital components. We reveal that besides spin and orbital Berry curvature dipoles, $\mathcal{T}$-odd nonlinear angular-momentum current can originate from disorder-induced mechanisms including coordinate shift, side-jump spin and orbital currents, anomalous scattering amplitude, and skew scattering. A general scaling relation is derived to help distinguish some of these contributions in experiments. Model calculations demonstrate that the orbital component can be comparable to and much larger than the spin component. Our theory lays the groundwork for $\mathcal{T}$-odd nonlinear spin and orbital transport.

cond-mat.mes-hall

Nonlinear Magnetic Orbital Hall Effect Induced by Spin-Orbit Coupling

Electrical readout of 180$^\circ$ switching in strictly compensated collinear antiferromagnets remains a major challenge in antiferromagnetic spintronics. Electrical writing of perpendicularly magnetized ferromagnets by out-of-plane orbital torque remains an important challenge in orbitronics. In this work, we propose a second-order nonlinear magnetic orbital Hall effect in the source antiferromagnet as a simultaneous recipe for both difficulties. This orbitronics effect is induced by spin-orbit coupling and is odd in the N\'eel vector, thus is a unique effect that integrates both functionalities via electric control of the N\'eel vector in the source antiferromagnet. Our first-principles calculations in CuMnAs predict significant non-perturbative orbital effects from spin-orbit coupling, with a orbital Berry-curvature dipole mechanism. These findings unveil new possibilities opened by topological antiferromagnetic orbitronics.

cond-mat.mtrl-sci

Electron Dynamics Reconstruction and Nontrivial Transport by Acoustic Waves

Surface acoustic waves (SAWs) become a popular driving source in modern condensed matter physics, but most existing theories simplify them as electric fields and ignore the non-uniform Brillouin zone folding effect. We develop a semiclassical framework and reconstruct the electron dynamics by treating SAW as a quasi-periodic potential modulating electronic momentum distribution. This framework naturally explains the experimentally observed DC drag current and predicts acousto-electric Hall effect. The theory further reveals various SAW-driven transport phenomena, emerging anomalous Hall, thermal Hall, and Nernst effects within time-reversal symmetric systems. Illustrated in bilayer graphene and $\mathrm{MX_2}$ (M = Mo, W; X = S, Se, Te), the angular-dependent acousto-electric Hall effect provides an experimental probe for Berry curvature distribution.

cond-mat.mes-hall

Eccentricity valley Hall effect

Valleytronics harnesses the valley degree of freedom -- energy-degenerate extrema in the electronic band structure -- for information storage and processing. Valley Hall effect (VHE) is a cornerstone of valleytronics, enabling electric generation of pure valley currents. While extensively studied in systems with valleys located at time-reversal-breaking points, here, we shift the paradigm to valleytronic platforms with time-reversal-invariant valleys (TRIVs), revealing a novel phenomenon: eccentricity VHE. Unlike conventional VHE, the valley Hall angle for eccentricity VHE is an intrinsic geometric property, governed solely by the eccentricity of the valley Fermi surface, rendering it highly robust against variations in temperature or carrier density. Eccentricity VHE emerges universally across all 25 layer groups supporting TRIVs. We demonstrate these distinctive features in monolayer GeS$_{2}$ via first-principles calculations, predicting a significant valley Hall angle of 0.74. This effect can be detected through nonlocal transport measurements exhibiting characteristic scaling behavior, or, in certain cases, through valley-layer coupling. Our findings reveal a critical overlooked facet of valley Hall physics, transcend the established VHE paradigm, and significantly broadens the scope of valleytronics.

cond-mat.mes-hall

Nonperturbative Magnetic Orbital Hall Effect in Altermagnets

Recent studies on altermagnets have focused considerable attention on nonrelativistic effects that persist in the absence of spin-orbit coupling (SOC). As a result, the relative importance of various phenomena in altermagnets has commonly been judged by their dependence on SOC. Here, we challenge this common wisdom by uncovering the magnetic orbital Hall effect, which is nonperturbative in SOC strength. We establish the symmetry properties of this effect, demonstrating that it is strictly forbidden in conventional collinear antiferromagnets yet universally allowed in all ten spin-Laue classes of collinear altermagnets. Counterintuitively, although SOC-induced, it reaches giant magnitudes in altermagnets-comparable to or even exceeding the nonrelativistic spin Hall effect. Moreover, altermagnetic symmetry enables unconventional collinear-polarized orbital currents, allowing field-free manipulation of perpendicular magnetization. Our first-principles calculations predict strong room-temperature responses in the experimentally established altermagnets CrSb and FeSb2. These findings reveal the previously overlooked potential of altermagnetic orbitronics and broaden the horizons for altermagnets in high-performance magnetic memory applications.

cond-mat.mtrl-sci

Semiclassical theory for proximity-induced superconducting systems with spin-orbit coupling

We develop a semiclassical theory of superconducting quasiparticles for proximity-induced superconducting systems, where spin-orbit coupling plays a critical role in shaping the quasiparticle dynamics. We reveal the structure of superconducting Berry curvatures in such systems, and derived the superconducting Berry curvature induced thermal Edelstein effect and spin Nernst effect. We calculate these two thermo-spin responses with model systems where Rashba spin-orbit coupling, proximity induced superconductivity, and ferromagnetic order are coexisting.

cond-mat.supr-con

Out-of-Plane Nonlinear Orbital Hall Torque

Despite recent advances in orbitronics, generating out-of-plane orbital torques essential for field-free deterministic switching of perpendicular magnetization remains a key challenge. Here, we propose a strategy to produce such unconventional torques across broad classes of materials, by leveraging the nonlinear orbital Hall effect. We demonstrate that this nonlinear orbital response is dramatically amplified by topological band degeneracies, where it overwhelmingly dominates the spin response even in systems with strong spin-orbit coupling. These features are confirmed via a quantitative investigation of representative topological metals RhSi, YPtBi, and PbTaSe$_2$, by combining our theory with first-principles calculations. The resulting orbital torques substantially surpass those from linear mechanisms reported thus far. These findings propel the research of orbital transport into the nonlinear regime, broaden the scope of orbital source materials, and establish a new pathway towards high-performance orbitronic devices.

cond-mat.mtrl-sci

Lorentz Skew Scattering Nonreciprocal Magneto-Transport

In materials with broken inversion symmetry, nonreciprocal magneto-transport (NRMT) manifests as a bilinear dependence of charge conductivity on applied electric (E) and magnetic (B) fields. This phenomenon is deeply rooted in symmetry and electronic quantum geometry, holding promise for novel rectification and detector technologies. Existing experimental studies generally attribute NRMT to Zeeman-driven mechanisms and exhibit quadratic scaling with conductivity. Here, we report a previously unknown NRMT microscopic mechanism - Lorentz skew scattering (LSK) - revealed through the discovery of an unprecedented quartic scaling law of NRMT as well as quantitative agreement between theory and experiment in BiTeBr. LSK emerges from the interplay of Lorentz force and skew scattering, bridging classical field effect to quantum scattering effect on the Fermi surface. We demonstrate that the LSK dominates NRMT in BiTeBr, and elucidate that this dominance over other possible contributions stems from high mobility and strong Rashba splitting. The finding of LSK mechanism is of unique importance because it unveils the leading NRMT effect in high-mobility systems and suggests a universal principle towards strong NRMT by enhancing electronic relaxation time in topological materials, rendering a new designing idea for low-dissipation rectifiers and high-performance quantum electronics.

cond-mat.mes-hall

Giant field-tunable nonlinear Hall effect by Lorentz skew scattering in a graphene moire superlattice

The nonlinear Hall effect (NHE) can enable rectification and energy harvesting, and its control by external fields, including gate, strain and magnetic field, has been pursued intensively. However, existing tuning pathways rely predominantly on fully quantum mechanical effects and are typically inefficient, resulting in weak NHE signals that limit further progress. In this work, we report the discovery of a distinct type of NHE in a graphene-hBN moire superlattice, which arises from a classical-quantum cooperative effect called Lorentz skew scattering (LSK), induced by a perpendicular magnetic field. This field-driven NHE exhibits a linear dependence on magnetic field and a pronounced unidirectional angular dependence. Remarkably, its magnitude reaches up to 32% of the linear Hall signal. We show that this giant, field-tunable NHE originating from LSK follows a unique quartic scaling law and produces a record-high nonlinear Hall conductivity (36000 {\mu}mV-1{\Omega}-1) near van Hove singularities of moire minibands, which is over an order of magnitude larger than all previously reported NHEs. Our findings establish an efficient, magnetic-field-driven route to giant Hall rectification in high-mobility materials, offering a broadly applicable paradigm for modulating the NHE beyond electrostatic gating.

cond-mat.mes-hall

Intrinsic Nernst Effect from Berry Curvature in Superconductors

The Nernst effect in superconductors is typically linked to fluctuating Cooper pairs above $T_c$ or vortex motion below $T_c$. We show instead that Berry curvature of Bogoliubov quasiparticles can generate an intrinsic Nernst response in a clean, vortex-free superconducting state. Focusing on two-dimensional systems with Ising spin-orbit coupling, relevant to transition-metal dichalcogenides, we identify two regimes: an intervalley $s$-wave paired state where a weak magnetic field activates the effect, and an intravalley chiral $p$-wave paired state that exhibits a spontaneous charge or spin Nernst response without a field. We propose an experimental setup that circumvents screening and provide estimates of the signal magnitude. Our results establish the Nernst effect as a direct probe of Berry curvature and pairing symmetry in two-dimensional spin-orbit-coupled superconductors.

cond-mat.supr-con

Intrinsic nonlinear valley Nernst effect

We investigate the intrinsic nonlinear valley Nernst effect, which induces a transverse valley current via a second-order thermoelectric response to a longitudinal temperature gradient. The effect arises from the Berry connection polarizability dipole of valley electrons and is permissible in both inversion-symmetric and inversion-asymmetric materials. We demonstrate that the response tensor is connected to the intrinsic nonlinear valley Hall conductivity through a generalized Mott relation, with the two being directly proportional at low temperatures, scaled by the Lorenz number. We elucidate the symmetry constraints governing this effect and develop a theory for its nonlocal measurement, revealing a nonlocal second-harmonic signal with a distinct $\rho^2$ scaling. This signal comprises two scaling terms, with their ratio corresponding to the square of the thermopower normalized by the Lorenz number. Key characteristics are demonstrated using a tilted Dirac model and first-principles calculations on bilayer WTe$_2$. Possible extrinsic contributions and alternative experimental detection methods, e.g., by valley pumping and by nonreciprocal directional dichroism, are discussed. These findings underscore the significance of band quantum geometry on electron dynamics and establish a theoretical foundation for nonlinear valley caloritronics.

cond-mat.mes-hall

Giant magneto-cubic in-plane Hall effect in a nonmagnetic material

In-plane Hall effect (IPHE) triggered by an external magnetic field applied in the transport plane has attracted significant experimental attentions in recent few years 1-6. However, most experiments focus on magnetic materials, where the existence of magnetic ordering may complicate understanding the physics behind, and the relatively small signal magnitudes limit the application of the effect. Here, we report a giant IPHE in a nonmagnetic half-Heusler compound LuAuSn, with a magnitude exceeding all the previously reported values. A -period of IPHE and the consistent cubic dependence on the magnetic field are observed, realizing the long-sought theoretical prediction of magneto-cubic IPHE under threefold rotational symmetry7-9 in an unexpected material. The scaling law analysis and first-principles calculations indicate that extrinsic side jump and skew scattering processes from both impurity and phonon scatterings dominate the observed effect. These findings unravel a new type of magneto-nonlinear IPHE, and its large magnitude and wide-temperature operation may open the door to practical applications of IPHE.

cond-mat.mtrl-sci

Room-temperature intrinsic nonlinear planar Hall effect in TaIrTe$_4$

Intrinsic responses are of paramount importance in physics research, as they represent the inherent properties of materials, independent of extrinsic factors that vary from sample to sample, and often reveal the intriguing quantum geometry of the band structure. Here, we report the experimental discovery of a new intrinsic response in charge transport, specifically the intrinsic nonlinear planar Hall effect (NPHE), in the topological semimetal TaIrTe$_4$. This effect is characterized by an induced Hall current that is quadratic in the driving electric field and linear in the in-plane magnetic field. The response coefficient is determined by the susceptibility tensor of Berry-connection polarizability dipole, which is an intrinsic band geometric quantity. Remarkably, the signal persists up to room temperature. Our theoretical calculations show excellent agreement with the experimental results and further elucidate the significance of a previously unknown orbital mechanism in intrinsic NPHE. This finding not only establishes a novel intrinsic material property but also opens a new route toward innovative nonlinear devices capable of operating at room temperature.

cond-mat.mes-hall