arXiv subjects

Cord Arnold

Publications and source records attributed to Cord Arnold.

6 recordsLinked to original sources

arXiv2026

Enhanced dynamic range spatio-spectral metrology of few-cycle laser pulses

Accurate spatio-temporal and spatio-spectral metrology is critical to the characterization and use of ultra-short, high-power lasers. The emergence of few cycle pulses, with bandwidths of tens or hundreds of nanometers, poses a significant challenge to existing metrology techniques. This is due both to large discrepancies in the sensitivities of the measurements at different wavelengths and to variation in the spectral intensity at those wavelengths. In this paper, the authors propose spectral filtering and stitching of the measurements as a robust, simple solution that enhances the dynamic range of the measurements, allowing accurate few-cycle pulse reconstruction. This enhancement is demonstrated using INSIGHT -- the most commonly used spatio-spectral measurement device -- as well as using IMPALA and spatially resolved Fourier transform spectrometry.

physics.optics↗

arXiv2025

Influence of the laser pulse duration in high-order harmonic generation

High-order harmonic generation (HHG) in gases has been studied for almost 40 years in many different conditions, varying the laser wavelength, intensity, focusing geometry, target design, gas species, etc. However, no systematic investigation of the effect of the pulse duration has been performed in spite of its expected impact on phase-matching of the high-order harmonics. Here, we develop a compact post-compression method based on a bulk multi-pass cell enabling tunable Fourier-limited pulse durations. We examine the HHG yield as a function of the pulse duration, ranging from 42 fs to 180 fs, while maintaining identical focusing conditions and generating medium. Our findings reveal that, for a given intensity, there exists an optimum pulse duration - not necessarily the shortest - that maximizes conversion efficiency. This optimum pulse duration increases as the intensity decreases. The experimental results are corroborated by numerical simulations, which show the dependence of HHG yield on the duration and peak intensity of the driving laser and underscore the importance of the interplay between light-matter interaction and phase-matching in the non-linear medium. Our conclusion explains why HHG could be demonstrated in 1988 with pulses as long as 40 ps and intensities of just a few $10^{13}$ W/cm${^2}$.

physics.optics↗

arXiv2023

Measurement of Ultrashort Laser Pulses With a Time-Dependent Polarization State Using the D-Scan Technique

The dispersion scan (d-scan) technique is extended to measurement of the timedependent polarization state of ultrashort laser pulses. In the simplest implementation for linearly polarized ultrashort pulses, the d-scan technique records the second harmonic generation (SHG) spectrum as a function of a known spectral phase manipulation. By applying this method to two orthogonally polarized projections of an arbitrary polarized electric field and by measuring the spectrum at an intermediate angle, we can reconstruct the evolution over time of the polarization state. We demonstrate the method by measuring a polarization gate generated from 6 fs pulses with a combination of waveplates. The measurements are compared to simulations, showing an excellent agreement.

physics.optics↗

arXiv2022

Continuous variable quantum state tomography of photoelectrons

We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct calculation of the quantum state of photoelectrons ejected from helium and argon in the vicinity of a Fano resonance. In the latter case, we furthermore distill ion-photoelectron entanglement due to spin-orbit splitting. This opens new routes towards the investigation of quantum coherence and entanglement properties on the ultrafast timescale.

physics.atom-ph↗

arXiv2021

Probing electronic decoherence with high-resolution attosecond photoelectron interferometry

Quantum coherence plays a fundamental role in the study and control of ultrafast dynamics in matter. In the case of photoionization, entanglement of the photoelectron with the ion is a well known source of decoherence when only one of the particles is measured. Here we investigate decoherence due to entanglement of the radial and angular degrees of freedom of the photoelectron. We study two-photon ionization via the 2s2p autoionizing state in He using high spectral resolution photoelectron interferometry. Combining experiment and theory, we show that the strong dipole coupling of the 2s2p and 2p$^2$ states results in the entanglement of the angular and radial degrees of freedom. This translates, in angle integrated measurements, into a dynamic loss of coherence during autoionization.

physics.atom-ph↗

arXiv2011

Simultaneous compression and characterization of ultrashort laser pulses using chirped mirrors and glass wedges

We present a simple and robust technique to retrieve the phase of ultrashort laser pulses, based on a chirped mirror and glass wedges compressor. It uses the compression system itself as a diagnostic tool, thereby making unnecessary the use of complementary diagnostic tools. We used this technique to compress and characterize 7.1 fs laser pulses from an ultrafast laser oscillator.

physics.optics↗