SearcharxivSearch

arXiv subjects

Cory Hargus

Publications and source records attributed to Cory Hargus.

7 recordsLinked to original sources

Equation of state for the edge flow of chiral colloidal fluids

We explore the edge flows that emerge at boundaries in nonequilibrium passive and active chiral colloidal fluids. We show that these complex interface currents obey an equation of state that relates their fluxes to bulk observables. For confined fluids, the edge flux is given by the average odd stress in the fluid. In phase-separated systems, the flux along the interface is given by the jump of the odd stress across the interface. We then use the equation of state to reveal, and contrast, the microscopic origins of the edge currents in passive and active systems.

cond-mat.soft

Passive objects in a chiral active bath: from micro to macro

We present a detailed derivation of the Langevin dynamics obeyed by a massive rigid body immersed in a chiral active bath. We show how the antisymmetric nature of the noise leads to an unusual relationship between the Langevin equation describing stochastic trajectories and the Fokker-Planck equation governing the time-evolution of the probability density. The chirality of the bath endows the object dynamics with odd diffusivity, odd mobility, and rotational ratchet effects that depend on the object symmetries. For rotationally-symmetric objects, we show that a hidden time-reversal symmetry leads to separate effective equilibrium descriptions for the translational and rotational degrees of freedom. Finally, starting from the bath dynamics, we construct a multipole expansion to quadrupolar order that allows predicting the far-field current and density modulation induced by the object on the bath.

cond-mat.stat-mech

Odd dynamics of passive objects in a chiral active bath

When submerged in a chiral active bath, a passive object becomes a spinning ratchet imbued with odd transport properties. We present the most general Langevin dynamics for a rigid body in a chiral active bath, in the adiabatic limit of large object mass. For rotationally symmetric objects, odd diffusion and odd mobility are connected by an Einstein relation, that we show numerically to break down outside the adiabatic limit. As the object symmetry decreases, its dynamics becomes increasingly irreversible: a massive disk exhibits an effective equilibrium dynamics, while a rod admits distinct translational and rotational temperatures, and a wedge is fully irreversible.Conversely, this departure from equilibrium can be read in universal far-field currents and density modulations of the bath, which we measure numerically and derive analytically.

cond-mat.stat-mech

Odd Viscodiffusive Fluids

We introduce a theory of "odd viscodiffusive fluids," which exhibit three-dimensional odd transport phenomena through the coupling of viscous and diffusive transport. In these fluids, diffusive fluxes may arise from orthogonal velocity gradients and, reciprocally, stresses may arise from concentration gradients. We examine microscopic fluctuations using the recently proposed "flux hypothesis" to derive Green-Kubo and reciprocal relations for the governing transport coefficients. These relations suggest that only parity symmetry, and not time-reversal symmetry, must be broken at the microscopic scale to observe these couplings. Chiral liquids, whether passive or active, are therefore a natural choice as viscodiffusive fluids. We then introduce two analytically tractable model systems, namely a generator and a corresponding reciprocal engine, which illustrate the nature of viscodiffusive cross-coupling in chiral matter and enable the experimental measurement of the novel transport coefficients. Finally, we make the case for chiral bacterial suspensions to be odd viscodiffusive fluids, and use our theory to predict the behaviors exhibited in prior experimental microfluidic studies involving bacterial migration in response to shearing flows.

cond-mat.soft

The Flux Hypothesis for Odd Transport Phenomena

Onsager's regression hypothesis makes a fundamental connection between macroscopic transport phenomena and the average relaxation of spontaneous microscopic fluctuations. This relaxation, however, is agnostic to odd transport phenomena, in which fluxes run orthogonal to the gradients driving them. To account for odd transport, we generalize the regression hypothesis, postulating that macroscopic linear constitutive laws are, on average, obeyed by microscopic fluctuations, whether they contribute to relaxation or not. From this "flux hypothesis," Green-Kubo and reciprocal relations follow, elucidating the separate roles of broken time-reversal and parity symmetries underlying various odd transport coefficients. As an application, we derive and verify the Green-Kubo relation for odd collective diffusion in chiral active matter, first in an analytically-tractable model and subsequently through molecular dynamics simulations of concentrated active spinners.

cond-mat.stat-mech

Odd Diffusivity of Chiral Random Motion

Diffusive transport is characterized by a diffusivity tensor which may, in general, contain both a symmetric and an antisymmetric component. Although the latter is often neglected, we derive Green-Kubo relations showing it to be a general characteristic of random motion breaking time-reversal and parity symmetries, as encountered in chiral active matter. In analogy with the odd viscosity appearing in chiral active fluids, we term this component the odd diffusivity. We show how odd diffusivity emerges in a chiral random walk model, and demonstrate the applicability of the Green-Kubo relations through molecular dynamics simulations of a passive tracer particle diffusing in a chiral active bath.

cond-mat.stat-mech

Time reversal symmetry breaking and odd viscosity in active fluids: Green-Kubo and NEMD results

Active fluids, which are driven at the microscale by non-conservative forces, are known to exhibit novel transport phenomena due to the breaking of time reversal symmetry. Recently, Epstein and Mandadapu [arXiv:1907.10041] obtained Green-Kubo relations for the full set of viscous coefficients governing isotropic chiral active fluids, including the so-called odd viscosity, invoking Onsager's regression hypothesis for the decay of fluctuations in active non-equilibrium steady states. In this Communication, we test these Green-Kubo relations using molecular dynamics simulations of a canonical model system consisting of actively torqued dumbbells. We find the resulting odd and shear viscosity values from the Green-Kubo relations to be in good agreement with values measured independently through non-equilibrium molecular dynamics (NEMD) flow simulations. This provides a test of the Green-Kubo relations, and lends support to the application of the Onsager regression hypothesis in relation to viscous behaviors of active matter systems.

cond-mat.stat-mech