arXiv subjects

Craig R. Stark

Publications and source records attributed to Craig R. Stark.

10 recordsLinked to original sources

arXiv2026

Plasma chemistry and electron-moderated pathways in substellar atmospheres: a new perspective on the L/T transition

The long-standing puzzle of the CO/CH$_{4}$ transition in brown dwarfs endures. Although the bulk spectral evolution across an atmosphere can be accounted for through thermal equilibrium cloud models, the behaviour in the NIR remains unaccounted for, indicating that additional, non-thermal processes may influence atmospheric chemistry alongside conventional pathways. We explore cloud-driven electrical activation, where low-energy sparks to full lightning discharges, unlocks non-equilibrium reaction pathways inaccessible under thermal conditions alone. To quantify this, the aim of this paper is to model the electron-moderated atmospheric chemistry with SPARCKS, a bespoke zero-dimensional code that solves the coupled set of particle balance equations for substellar plasma activation and reaction kinetics, focusing on the key CO-CH$_{4}$ electron-moderated chemistry across the parameter ranges $T_{\rm gas} \in [700, 1600]$ K} and $T_{e} \in [2, 5]$ eV. We simulate a 1 microsecond pulse, representing a short dart-stepped leader; and, two pulsed systems with $(t_{\rm on}, t_{\rm off})$ = ($10^{-8}$ s, $10^{-6}$ s) and $(10^{-9}$ s, $10^{-9}$ s), representing small-scale inter-grain discharges, consistent with a typical characteristic substellar atmosphere. Our results show that even modest, physically plausible energies can strongly perturb atmospheric composition: an electron energy of 3.0 eV is sufficient to halve the CH$_{4}$/CO ratio in our sample atmosphere within one microsecond. Beyond the CO-CH$_{4}$ system, electron-moderated plasma chemistry exerts a far-reaching influence on substellar atmospheric composition.

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arXiv2025

Electrostatic instability of non-spherical dust in sub-stellar clouds

Charged dust clouds play an important role in the evolution of sub-stellar atmospheres through electrical discharges such as lightning events or inter-grain discharges. The consequent plasma activation presents an alternative source of disequilibrium chemistry, potentially triggering a set of chemical reactions otherwise energetically unavailable. The aim of this paper is to address the problem of the electrostatic stability of charged spheroidal dust grains in sub-stellar clouds and its impact on inter-grain electrostatic discharges, the available area for atmospheric gas-phase surface chemistry, the particle eccentricity distribution function and observed polarization signatures. This paper has derived the criterion for the allowed values of dust eccentricity that are electrostatically stable as a function of grain size $a\in[0.2,1.8]~\mu$m, floating potential $\phi_{f}\in[1, 10]$~V and tensile strength $\Sigma_{s}=10^{3}$~Pa. As a consequence of electrostatic instability we also calculate the expected electric field enhancement at the spheroidal poles, the increased surface area of a dust grain, the truncation of the particle eccentricity distribution function and the resultant degree of polarization. Dust grains with an eccentricity below a critical value will be electrostatically stable; whereas, grains with an eccentricity above a critical value will be unstable. The results presented here are applicable not only to spheroidal dust grains but any non-spherical dust grains where non-uniform surface electric fields or inhomogeneous tensile strengths could be susceptible to electrostatic instability. In this context electrostatic erosion presents a mechanism that may produce bumpy, irregularly shaped or porous grains.

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arXiv2020

Evolution of spheroidal dust in electrically active sub-stellar atmospheres

Understanding the source of sub-stellar polarimetric observations in the optical and near-infrared is key to characterizing sub-stellar objects and developing potential diagnostics for determining properties of their atmospheres. Differential scattering from a population of aligned, non-spherical dust grains is a potential source of polarization that could be used to determine geometric properties of the dust clouds. This paper addresses the problem of the spheroidal growth of dust grains in electrically activated sub-stellar atmospheres. It presents the novel application of a mechanism whereby non-spherical, elongated dust grains can be grown via plasma deposition as a consequence of the surface electric field effects of charged dust grains. We numerically solve the differential equations governing the spheroidal growth of charged dust grains via plasma deposition as a result of surface electric field effects in order to determine how the dust eccentricity and the dust particle eccentricity distribution function evolve with time. From these results, we determine the effect of spheroidal dust on the observed linear polarization. Numerical solutions show that $e\approx 0.94$ defines a watershed eccentricity, where the eccentricity of grains with an initial eccentricity less than (greater than) this value decreases (increases) and spherical (spheroidal) growth occurs. This produces a characteristic bimodal eccentricity distribution function yielding a fractional change in the observed linear polarization of up to $\approx0.1$ corresponding to dust grains of maximal eccentricity at wavelengths of $\approx1 μ$m, consistent with the near infrared observational window. The results presented here are relevant to the growth of non-spherical, irregularly shaped dust grains of general geometry where non-uniform surface electric field effects of charged dust grains are significant.

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arXiv2020

The effect of internal gravity waves on cloud evolution in sub-stellar atmospheres

Sub-stellar objects exhibit photometric variability, which is believed to be caused by a number of processes, such as magnetically-driven spots or inhomogeneous cloud coverage. Recent models have shown that turbulent flows and waves, including internal gravity waves, may play an important role in cloud evolution. The aim of this paper is to investigate the effect of IGW on dust nucleation and dust growth, and whether observations of the resulting cloud structures could be used to recover atmospheric density information. For a simplified atmosphere in two dimensions, we numerically solved the governing fluid equations to simulate the effect on dust nucleation and mantle growth as a result of the passage of an IGW. Furthermore, we derived an expression that relates the properties of the wave-induced cloud structures to observable parameters in order to deduce the atmospheric density. Numerical simulations show that the $ρ, p, T$ variations caused by gravity waves lead to an increase of the nucleation rate by up to a factor 20, and an increase of the mantle growth rate by up to a factor 1.6, compared to their equilibrium values. An exploration of the wider parameter space shows that in absolute terms, the increase in nucleation due to IGW is stronger in cooler (T dwarfs) and TiO2-rich sub-stellar atmospheres. The relative increase, however, is greater in warmer (L dwarf) and TiO2-poor atmospheres due to conditions less suited for efficient nucleation at equilibrium. These variations lead to banded areas in which dust formation is much more pronounced, similar to the cloud structures observed on Earth. We show that IGW in the atmosphere of sub-stellar objects can produce banded clouds structures similar to that observed on Earth. We propose a method with which potential observations of banded clouds could be used to estimate the atmospheric density of sub-stellar objects.

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arXiv2017

Dust cloud evolution in sub-stellar atmospheres via plasma deposition and plasma sputtering

In contemporary sub-stellar model atmospheres, dust growth occurs through neutral gas-phase surface chemistry. Recently, there has been a growing body of theoretical and observational evidence suggesting that ionisation processes can also occur. As a result, atmospheres are populated by regions composed of plasma, gas and dust, and the consequent influence of plasma processes on dust evolution is enhanced. This paper aims to introduce a new model of dust growth and destruction in sub-stellar atmospheres via plasma deposition and plasma sputtering. Using example sub-stellar atmospheres from Drift-Phoenix, we have compared plasma deposition and sputtering timescales to those from neutral gas-phase surface chemistry to ascertain their regimes of influence. We calculated the plasma sputtering yield and discuss the circumstances where plasma sputtering dominates over deposition. Within the highest dust density cloud regions, plasma deposition and sputtering dominates over neutral gas-phase surface chemistry if the degree of ionisation is $\gtrsim10^{-4}$. Loosely bound grains with surface binding energies of the order of $0.1-1$ eV are susceptible to destruction through plasma sputtering for feasible degrees of ionisation and electron temperatures; whereas, strong crystalline grains with binding energies of the order $10$ eV are resistant to sputtering. The mathematical framework outlined sets the foundation for the inclusion of plasma deposition and plasma sputtering in global dust cloud formation models of sub-stellar atmospheres.

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arXiv2015

Particle-in-Cell Simulations of Collisionless Magnetic Reconnection with a Non-Uniform Guide Field

Results are presented of a first study of collisionless magnetic reconnection starting from a recently found exact nonlinear force-free Vlasov-Maxwell equilibrium. The initial state has a Harris sheet magnetic field profile in one direction and a non-uniform guide field in a second direction, resulting in a spatially constant magnetic field strength as well as a constant initial plasma density and plasma pressure. It is found that the reconnection process initially resembles guide field reconnection, but that a gradual transition to anti-parallel reconnection happens as the system evolves. The time evolution of a number of plasma parameters is investigated, and the results are compared with simulations starting from a Harris sheet equilibrium and a Harris sheet plus constant guide field equilibrium.

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arXiv2015

Inhomogeneous cloud coverage through the Coulomb explosion of dust in substellar atmospheres

Recent observations of brown dwarf spectroscopic variability in the infrared infer the presence of patchy cloud cover. This paper proposes a mechanism for producing inhomogeneous cloud coverage due to the depletion of cloud particles through the Coulomb explosion of dust in atmospheric plasma regions. Charged dust grains Coulomb-explode when the electrostatic stress of the grain exceeds its mechanical tensile stress, which results in grains below a critical radius $a<a^{\rm Coul}_{\rm crit}$ being broken up. This work outlines the criteria required for the Coulomb explosion of dust clouds in substellar atmospheres, the effect on the dust particle size distribution function, and the resulting radiative properties of the atmospheric regions. Our results show that for an atmospheric plasma region with an electron temperature of $T_{e}=10$~eV ($\approx10^{5}$~K), the critical grain radius varies from $10^{-7}$ to $10^{-4}$~cm, depending on the grains' tensile strength. Higher critical radii up to $10^{-3}$~cm are attainable for higher electron temperatures. We find that the process produces a bimodal particle size distribution composed of stable nanoscale seed particles and dust particles with $a\geq a^{\rm Coul}_{\rm crit}$, with the intervening particle sizes defining a region devoid of dust. As a result, the dust population is depleted, and the clouds become optically thin in the wavelength range $0.1-10~μ$m, with a characteristic peak that shifts to higher wavelengths as more sub-micrometer particles are destroyed. In an atmosphere populated with a distribution of plasma volumes, this will yield regions of contrasting radiative properties, thereby giving a source of inhomogeneous cloud coverage. The results presented here may also be relevant for dust in supernova remnants and protoplanetary disks.

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arXiv2014

Jupiter as a Giant Cosmic Ray Detector

We explore the feasibility of using the atmosphere of Jupiter to detect Ultra-High-Energy Cosmic Rays (UHECR's). The large surface area of Jupiter allows us to probe cosmic rays of higher energies than previously accessible. Cosmic ray extensive air showers in Jupiter's atmosphere could in principle be detected by the Large Area Telescope (LAT) on the Fermi observatory. In order to be observed, these air showers would need to be oriented toward the Earth, and would need to occur sufficiently high in the atmosphere that the gamma rays can penetrate. We demonstrate that, under these assumptions, Jupiter provides an effective cosmic ray "detector" area of $3.3 \times 10^7$ km$^2$. We predict that Fermi-LAT should be able to detect events of energy $>10^{21}$ eV with fluence $10^{-7}$ erg cm$^{-2}$ at a rate of about one per month. The observed number of air showers may provide an indirect measure of the flux of cosmic rays $\gtrsim 10^{20}$ eV. Extensive air showers also produce a synchrotron signature that may be measurable by ALMA. Simultaneous observations of Jupiter with ALMA and Fermi-LAT could be used to provide broad constraints on the energies of the initiating cosmic rays.

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arXiv2013

Electrostatic activation of prebiotic chemistry in substellar atmospheres

Charged dust grains in the atmospheres of exoplanets may play a key role in the formation of prebiotic molecules, necessary to the origin of life. Dust grains submerged in an atmospheric plasma become negatively charged and attract a flux of ions that are accelerated from the plasma. The energy of the ions upon reaching the grain surface may be sufficient to overcome the activation energy of particular chemical reactions that would be unattainable via ion and neutral bombardment from classical, thermal excitation. As a result, prebiotic molecules or their precursors could be synthesised on the surface of dust grains that form clouds in exoplanetary atmospheres. This paper investigates the energization of the plasma ions, and the dependence on the plasma electron temperature, in the atmospheres of substellar objects such as gas giant planets. Calculations show that modest electron temperatures of $\approx 1$ eV ($\approx 10^{4}$ K) are enough to accelerate ions to sufficient energies that exceed the activation energies required for the formation of formaldehyde, ammonia, hydrogen cyanide and the amino acid glycine.

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arXiv2013

Ionization in Atmospheres of Brown Dwarfs and Extrasolar Planets V: Alfvén Ionization

Observations of continuous radio and sporadic X-ray emission from low-mass objects suggest they harbour localized plasmas in their atmospheric environments. For low-mass objects, the degree of thermal ionization is insufficient to qualify the ionized component as a plasma, posing the question: what ionization processes can efficiently produce the required plasma that is the source of the radiation? We propose Alfvén ionization as a mechanism for producing localized pockets of ionized gas in the atmosphere, having sufficient degrees of ionization ($\geq10^{-7}$) that they constitute plasmas. We outline the criteria required for Alfvén ionization and demonstrate it's applicability in the atmospheres of low-mass objects such as giant gas planets, brown dwarfs and M-dwarfs for both solar and sub-solar metallicities. We find that Alfvén ionization is most efficient at mid to low atmospheric pressures where a seed plasma is easier to magnetize and the pressure gradients needed to drive the required neutral flows are the smallest. For the model atmospheres considered, our results show that degrees of ionization of $10^{-6}-1$ can be obtained as a result of Alfvén ionization. Observable consequences include continuum Bremsstrahlung emission, superimposed with spectral lines from the plasma ion species (e.g. He, Mg, H$_{2}$ or CO lines). Forbidden lines are also expected from the metastable population. The presence of an atmospheric plasma opens the door to a multitude of plasma and chemical processes not yet considered in current atmospheric models. The occurrence of Alfvén ionization may also be applicable to other astrophysical environments such as protoplanetary disks.

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