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Cristian D. Batista

Publications and source records attributed to Cristian D. Batista.

At least 19 recordsLinked to original sources

Skyrmions of Frustrated Quantum Dimer Systems

Magnetic skyrmions are topologically protected solitons observed in various classes of real magnets. In two-dimensional systems, where the target space of local magnetization values is the two-sphere $S^2$, skyrmion textures are classified by the homotopy classes of two-loops $S^2$ in $S^2$: $Π_2(S^2) \cong Z$. Here, we demonstrate that more general topological skyrmion textures emerge in the classical limit of quantum dimer systems, where the phase space of the relevant classical theory is $\mathbb{CP}^{N-1}$ (with $N=4$ for the case of interest), because the relevant second homotopy group, $Π_2(\mathbb{CP}^{N-1}) \cong Z$ for $N\geq 2$, remains unchanged. Building on the framework established by Zhang et al. (2023), we consider a classical limit based on SU(4) coherent states, which preserve intra-dimer entanglement. We show that the zero-temperature phase diagram of frustrated spin-dimer systems on a bilayer triangular lattice with weak inter-dimer coupling includes two magnetic-field-induced $\mathbb{CP}^{3}$ skyrmion crystal phases.

cond-mat.str-el↗

Approaching the Inverse Neutron Scattering Problem with Neural Networks

Determining the microscopic Hamiltonian of a quantum magnet from inelastic neutron scattering measurements remains a central challenge in condensed matter physics. While the dynamical spin structure factor contains, in principle, sufficient information about the underlying interactions, extracting Hamiltonian parameters from experimental spectra constitutes a highly nontrivial inverse problem due to the large parameter space and the presence of experimental noise. Here we demonstrate that neural networks can efficiently solve this inverse problem for a broad class of quantum magnets. As a benchmark, we consider an eight-parameter family of honeycomb lattice Heisenberg spin models in the fully polarized phase, where the dynamical spin structure factor can be computed exactly within linear spin-wave theory. Using a large synthetic dataset of neutron scattering spectra, we train neural networks to infer the underlying Hamiltonian parameters directly from the dynamical response. We compare the performance of three different architectures---fully connected neural networks (FCNNs), one-dimensional convolutional neural networks (CNN1Ds), and two-dimensional convolutional neural networks (CNN2Ds)---and find that all achieve high predictive accuracy. Remarkably, the trained models remain robust in the presence of substantial experimental uncertainty, reliably recovering the Hamiltonian parameters even when the input spectra are contaminated by random noise with amplitudes reaching $10\%$ of the signal intensity. Our results establish machine learning as a powerful framework for quantitative Hamiltonian reconstruction from neutron scattering data and provide a practical route toward automated characterization of quantum magnetic materials.

cond-mat.str-el↗

Magnetization Plateaux as a Roadmap to Quantum Spin Liquids

We investigate the spin-1/2 $J_1-J_2$ triangular-lattice Heisenberg antiferromagnet in a magnetic field by combining large-scale density matrix renormalization group (DMRG) simulations with self-consistent spin-wave theory. The resulting field-coupling phase diagram reveals that quantum fluctuations stabilize coplanar order across the entire parameter range, giving rise to a characteristic sequence of magnetization plateaux. Near the quantum-spin-liquid window $0.06 \lesssim J_2/J_1 \lesssim 0.16$, which extends to magnetic field $B \sim J_1$, we identify overlapping $m = 1/3$ and $m = 1/2$ plateaux - a distinctive hallmark of the system's proximity to the low-field spin-liquid regime. The excellent quantitative agreement between DMRG and self-consistent one-loop spin-wave calculations demonstrates that semiclassical approaches can reliably capture and parameterize the plateau phases of triangular quantum antiferromagnets.

cond-mat.str-el↗

Tunable Skyrmions in a Topological Wigner Crystal

In low density systems with strong interactions electrons are expected to crystallize into a Wigner solid. Recently, advances in two-dimensional systems where electrons carry Berry curvature have added a topological dimension to Wigner crystallization. Using a model for pseudospin interactions in a topological Wigner crystal, here we show that the competition between ferromagnetic Heisenberg exchange $J$ and the chiral interaction $γ$ on the triangular lattice stabilizes a zero-field skyrmion crystal whose density is continuously tunable through the ratio $γ/J$. The chiral interaction originates from finite Berry curvature in an underlying time-reversal broken Wigner crystal. In the continuum limit, the chiral interaction acts as a chemical potential for skyrmions, while higher-order gradient terms beyond the nonlinear sigma model select the skyrmion density. At large chiral coupling, we uncover a 24-site tetra-skyrmion crystal carrying four units of topological charge per magnetic unit cell, which becomes degenerate with four-sublattice tetrahedral order as $J \to 0$. We characterize the magnon structure for these phases and discuss the transition between the tunable skyrmion crystal to these states at large $γ/J$. Our results establish the phase diagram of ferromagnetic topological Wigner crystals.

cond-mat.str-el↗

Exact Nagaoka-to-spiral transition in the doped infinite-U triangular lattice

We study the single-hole infinite-$U$ Hubbard model on the triangular lattice with nearest- and next-nearest-neighbor hoppings $t_1$ and $t_2$. A frustrating $t_2$ destabilizes Nagaoka ferromagnetism through a Lifshitz transition to a long-wavelength coplanar spiral at $t_{2,c}/t_1=-0.182$. We determine the critical point analytically by reducing the many-body problem to an effective two-body hole--magnon scattering problem in which the hard-core hole--magnon constraint is treated exactly. Numerical calculations confirm the spiral ground state and reveal a coherent spin polaron with quasiparticle weight $Z\simeq0.92$ at the Lifshitz-shifted momentum $\mathbf{K}=-\mathbf{Q}^*$. These results establish the first quantum instability of the triangular-lattice Nagaoka ferromagnet and provide the magnetic baseline for magnon-mediated pairing at finite doping.

cond-mat.str-el↗

Tunable Emergent Gauge Fields from Skyrmions in a Quasicrystalline Lattice

We study magnetic skyrmions in a two-dimensional quasicrystalline lattice using a classical Heisenberg model with Dzyaloshinskii-Moriya interactions and an external magnetic field. The competition between the skyrmion-skyrmion repulsion and an emergent quasiperiodic pinning landscape gives rise to a sequence of distinct skyrmion lattice configurations as a function of field. The resulting hierarchy of quasiperiodic pinning potentials, characterized by closely spaced quasi-degenerate minima, enables a quasi-continuous suppression of the skyrmion density as the saturation field is approached, in sharp contrast to the strongly first-order collapse of skyrmion crystals on periodic lattices. This provides a direct mechanism for controlling the topological charge and, consequently, the emergent gauge field for itinerant electrons. As a consequence, the Hall conductivity can be strongly modified with small changes in the magnetic field and driven smoothly to zero near saturation. This field-controlled tunability, rooted in the underlying multistability, identifies quasicrystalline magnets as a platform for tunable topological textures, with potential applications in magnetic memory and magnetoelectronic response.

cond-mat.str-el↗

An integrated theoretical and numerical approach to understand modern experiments on quantum magnetism

In recent decades, the study of quantum magnets, which feature unconventional behaviour such as exotic quantum phase transitions and quantum spin liquids, and unconventional magnetic states of matter, has made remarkable progress. However, each of the three foundational pillars -- numerical simulations, analytical methods and, to a lesser extent, materials synthesis and experiments -- often tends to view itself as the primary driver of the field. Even though the need for collaboration among theory, numerics and experiment to understand the complex phases of quantum magnets is well established, in our view there remains a persistent perception from experts in one area that the other two serve merely as supporting tools, primarily useful for validating the dominant ideas of one speciality, and less relevant to shaping the underlying scientific narrative. We refer to this mindset as the "pride and prejudice" in modeling and understanding modern quantum magnetism. In this Perspective, we advocate for a different, more integrated approach to overcome the challenges faced by quantum magnetism researchers. We argue that this alternative mindset has already started to advance the understanding of several important quantum magnetic models and their materials realizations.

cond-mat.str-el↗

Design Principles for Quasi-Isotropic Exchange in Rare-Earth Quantum Magnets

Rare-earth quantum materials provide a promising platform for emergent phenomena ranging from quantum spin liquids with long-range entanglement to topological magnetic textures. However, the strong spin-orbit coupling that stabilizes their low-energy pseudospin degrees of freedom also tends to generate strongly anisotropic exchange interactions, complicating the realization of quasi-isotropic Heisenberg magnetism. Here we investigate the microscopic origin of superexchange in $\mathrm{Ce}^{3+}$- and $\mathrm{Yb}^{3+}$-based insulators with edge-sharing octahedral geometry. Using degenerate perturbation theory for a multiorbital Hubbard model, we show that isotropic exchange originates predominantly from virtual hopping within the ground-state Kramers doublet, whereas anisotropic interactions arise primarily from processes involving excited multiplets. This leads to a simple orbital design principle: quasi-isotropic exchange is promoted when the ground-state doublet has a strong maximal-angular-momentum character with respect to the quantization axis perpendicular to the superexchange plane spanned by rare-earth and ligand ions. We demonstrate this mechanism for both ideal and distorted geometries and show that it is broadly consistent with experimentally studied Yb-based insulators. Our results establish a practical framework for engineering quasi-isotropic interactions in rare-earth quantum materials.

cond-mat.str-el↗

Dynamics of Quantum Chiral Solitons

We introduce a nonperturbative framework for quantizing chiral solitons in interacting quantum spin chains. This approach provides a direct lattice extension of the well-established $S$-duality between the sine-Gordon and Thirring models, thereby bridging the gap between continuum dualities and their lattice counterparts. By constructing the quantum chiral-soliton operators explicitly, we show how their unconventional dynamics appear in the excitation spectrum and correlation functions across the full Brillouin zone. A key result is that the dominant soliton tunneling amplitude alternates in sign, $\operatorname{sgn}(t_{1+}) = (-1)^{2S+1}$, sharply distinguishing half-odd-integer from integer spin chains. We further identify characteristic signatures of these chiral excitations in the dynamical spin structure factor, demonstrating their visibility in inelastic neutron scattering. Our results open a route to experimentally probing nonperturbative features of dual quantum field theories in condensed-matter settings.

cond-mat.str-el↗

Designing electronic magnetoelectric matter with organic quantum spin trimers

Magnetoelectric (ME) phenomena are commonly driven by spin-lattice coupling. Here we demonstrate a different route based on frustrated quantum spin trimers that intrinsically intertwine magnetic moments and electric dipoles. Using molecular design principles, we realize a weakly coupled lattice of equilateral $S=1/2$ spin trimers in the organic radical crystal TNN$\cdot$CH$_3$CN. In this material, correlated electronic fluctuations within each trimer generate electric dipoles, while geometrically frustrated intertrimer interactions organize them into collective ME states. Magnetization, thermodynamic, and dielectric measurements reveal multiple magnetic-field-induced phases, including the $1/3$-magnetization plateau marked by pronounced dielectric anomalies. Effective low-energy theories and numerical simulations show that these phenomena are driven by electronically generated trimer dipoles whose collective order is stabilized by frustration relief of the intertrimer interactions, establishing a direct connection between geometric frustration and emergent magnetoelectricity. Our results identify quantum spin trimers as multifunctional building blocks, providing a bottom-up route for designing correlated ME materials from electronically active quantum spin clusters.

cond-mat.str-el↗

Semiclassical representation of the Hubbard model

By revisiting the path-integral formulation of the Hubbard model, we propose a theoretical approach based on a semiclassical approximation employing an unconventional coherent-state representation. Within this framework, a subset of the dynamical variables is treated as static, yielding a nonperturbative scheme that is applicable at finite temperature, incorporates intersite correlations, and can be naturally extended to multiorbital systems. We assess the validity of the approximation by comparing its results with exact solutions for one- and two-site systems, focusing in particular on the particle number, double occupancy, hopping amplitude, and spin correlations, and find that the present approach qualitatively reproduces the exact behavior. Quantitatively, deviations arise, which is associated with the continuum (non-discretized) character of the underlying density of states. Furthermore, we derive the exact transformation associated with the coherent-state construction, thereby providing additional insight into the representation of the Hubbard model.

cond-mat.str-el↗

Superconductivity and fractionalized magnetic excitations in CeCoIn5

Recent experiments on CeCoIn5 -- a prototypical d-wave superconductor -- indicate that its normal state lies near an unconventional quantum critical point (QCP). One intriguing hypothesis is that quantum-critical fluctuations promote fractionalization of localized 4f moments into fermionic spinons. This fractionalized Fermi liquid (FL*) scenario provides a comprehensive framework for the unconventional QCP and superconductivity, and can reconcile a "missing" Fermi-surface volume relative to the Luttinger count in the normal state of CeCoIn5. To test this possibility, we performed inelastic neutron scattering (INS) measurements on CeCoIn5 across the superconducting transition and corresponding theoretical analysis. Our high-precision spectra reveal detailed momentum and temperature dependence of the spin resonance and a structured spin excitation continuum persisting even in the normal state, placing stringent constraints on the physical picture of pairing in a d-wave superconductor. We show that a Kondo-lattice framework incorporating proximity to FL* physics and d-wave pairing reproduces key features of the data. The model suggests that both the quasi-localized nature of the f-moments above Tc and the resonance below Tc arise from common underlying gauge dynamics, implying a unifying organizing principle linking spin fractionalization and unconventional superconductivity in strongly correlated metals.

cond-mat.str-el↗

Spin dynamics of the spin-1 triangular lattice Heisenberg antiferromagnet K$_2$Ni(SeO$_3$)$_2$

Strong quantum fluctuations and unconventional spin dynamics are well established in the spin-1/2 triangular lattice Heisenberg antiferromagnet. However, their survival in the spin-1 case remains an open question. We investigate the spin dynamics of K$_2$Ni(SeO$_3$)$_2$, a nearly ideal spin-1 triangular lattice Heisenberg antiferromagnet, using inelastic neutron scattering. Below the ordering temperature $T_{\rm N}$, we observe coherent one-magnon excitations coexisting with a broad high-energy continuum. Two complementary approaches, a spectrally consistent $1/S$-corrected spin wave theory and a beyond-mean-field Schwinger boson theory, reproduce different facets of the continuum. Neither alone is complete, demonstrating substantial quantum fluctuations survive for $S\!=\!1$ and are reflected primarily in the spectral distribution of the continuum. Above $T_{\rm N}$, the continuum bandwidth is conserved while spectral weight is redistributed as magnons lose spatial coherence. Our results establish K$_2$Ni(SeO$_3$)$_2$ as a model triangular antiferromagnet, identifying bandwidth conservation and the distribution of spectral weight within the continuum as organizing principles to understand the spin dynamics of ordered quantum magnets beyond spin-1/2. Our results highlight the need for controlled calculations of the interacting multi-magnon sector of 2D antiferromagnets.

cond-mat.mtrl-sci↗

Experimental confirmation of the magnetic ordering transition induced by an electronic structure change in the metallic triangular antiferromagnet Co$_{1/3}$TaS$_2$

We report ARPES studies combined with DFT+DMFT calculations to confirm that the magnetic ordering vector transition from \textbf{Q}=(1/2,0,0) to \textbf{Q}=(1/3,0,0) in the metallic triangular antiferromagnets Co$_{1/3\pmε}$TaS$_2$ ($ε\approx$0.007) is induced by the electronic structure change in the system. The ARPES-measured Fermi surface (FS) maps of Co$_{0.325}$TaS$_2$ show two hexagonal and one circular hole-like FSs around $Γ$, which matches well with the triple-\textbf{Q} state by taking into account the contribution of nesting vectors occurring between Co 3$d$ and Ta 5$d$ orbitals. In the case of Co$_{0.340}$TaS$_2$, a new electron pocket around K appears and the FS geometry changes as a result of the correlation effect of Co$_4$S$_{18}$ tripods forming in the system. The magnetic susceptibility calculations based on the charge-self-consistent DFT+DMFT band structures and the random phase approximation indicate that the most stable magnetic ordering vector (1/2,0,0) split into (1/6,0,0) and (1/2,0,0), which is consistent with the magnetic phase transition around $x$=1/3 in Co$_{x}$TaS$_2$.

cond-mat.str-el↗

Nonperturbative Semiclassical Spin Dynamics for Ordered Quantum Magnets

In ordered quantum magnets where interactions between elementary excitations dominate over their kinetic energy, perturbative approaches often fail, making non-perturbative methods essential to capture spectral features such as bound states and the redistribution of weight within excitation continua. Although an increasing number of experiments report anomalous spin excitation continua in such systems, their microscopic interpretation remains an open challenge. Here, we investigate the spin dynamics of the triangular-lattice antiferromagnet in its 1/3-plateau phase using two complementary non-perturbative approaches: exact diagonalization in a truncated Hilbert space for a gas of elementary excitations (THED) and matrix product state (MPS) simulations. Alongside cross-validation between these methods, we benchmark our results against inelastic neutron scattering (INS) data. The THED analysis confirms the presence of two-magnon bound states and identifies the anomalous scattering continuum observed in both MPS and INS as a two-magnon resonance, arising from hybridization between the bound state and the two-magnon continuum. Furthermore, THED reveals bound states overlapping with the continuum, enriching the interpretation of continuum anomalies. More broadly, THED provides a robust framework for investigating anomalous spin excitation continua and bound-state effects in other materials with gapped spectra. Its combination of accuracy and computational efficiency makes it a powerful tool for extracting reliable microscopic models in semiclassical regimes.

cond-mat.str-el↗

Magnon-Mediated Superconductivity in the Infinite-$U$ Triangular Lattice

We demonstrate that the infinite-$U$ triangular-lattice Hubbard model supports a superconducting state built from tightly bound Cooper pairs composed of two holes and one magnon ($2h1m$). Building on the seminal prediction of repulsively bound $2h1m$ states, we show that next-nearest-neighbor hopping $t_{2}$ coherently mixes symmetry-related configurations, stabilizing an $s$-wave bound state with substantial binding energy and a light effective mass. Large-scale DMRG calculations at finite doping identify a magnetization plateau corresponding to a gas of such bound states and quasi--long--range superconducting order with power-law $2h1m$ pair correlations. Our results establish a magnon-mediated superconducting mechanism driven by kinetic frustration, with immediate detectable signatures for moiré Hubbard materials and ultracold-atom simulators.

cond-mat.supr-con↗

Skyrmion and Meron Crystals in Intermetallic Gd$_3$Ru$_4$Al$_{12}$: Microscopic Model Insights into Chiral Phases

Topological spin textures in frustrated intermetallics hold great promise for spintronics applications. However, understanding their origin and properties remains a significant challenge due to competing and often long-range interactions mediated by conduction electrons. Here, by combining neutron scattering experiments with theoretical modeling via unprecedented multi-target fits that further incorporate the ferromagnentic resonance data and magnetization curve, we construct a realistic microscopic model for the prototypical intermetallic skyrmion host \text{Gd}$_3$\text{Ru}$_4$\text{Al}$_{12}$. Beyond magnetic frustration, we identify the competition between dipolar interactions and easy-plane single-ion anisotropy as a key ingredient for stabilizing the rich chiral magnetic phases observed in this compound -- including a hexagonal skyrmion crystal and two distinct meron crystals. Remarkably, the meron crystal in lower field is revealed to be commensurate with the underlying lattice, and its unique three-meron-one-antimeron spin texture is verified by the polarized x-ray diffraction data. At elevated temperatures, the short-range spin correlations in \text{Gd}$_3$\text{Ru}$_4$\text{Al}$_{12}$ are well described by a codimension-two spiral spin-liquid. Perturbations from staggered Dzyaloshinskii-Moriya interactions give rise to chiral fluctuations that account for the temperature and field dependence of the anomalous Hall response. Our results highlight the unique power of neutron scattering, especially when combined with complementary experimental techniques, to unravel complex magnetic phase transitions and provide new insights into the rich variety of topological spin textures in frustrated systems.

cond-mat.str-el↗

A resonant valence bond spin liquid in the dilute limit of doped frustrated Mott insulators

Ideas about resonant valence bond liquids and spin-charge separation have led to key concepts in physics such as quantum spin liquids, emergent gauge symmetries, topological order, and fractionalisation. Despite extensive efforts to demonstrate the existence of a resonant valence bond phase in the Hubbard model that originally motivated the concept, a definitive realisation has yet to be achieved. Here we present a solution to this long-standing problem by uncovering a resonant valence bond phase exhibiting spin-charge separation in realistic Hamiltonians. We show analytically that this ground state emerges in the dilute-doping limit of a half-filled Mott insulator on corner-sharing tetrahedral lattices with frustrated hopping, in the absence of exchange interactions. We confirm numerically that the results extend to finite exchange interactions, finite-sized systems and finite dopant density. Although much attention has been devoted to the emergence of unconventional states from geometrically frustrated interactions, our work demonstrates that kinetic energy frustration in doped Mott insulators may be essential for stabilising robust, topologically ordered states in real materials.

cond-mat.str-el↗