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Cuihong Li

Publications and source records attributed to Cuihong Li.

4 recordsLinked to original sources

Flash annealing-engineered wafer-scale relaxor antiferroelectrics for enhanced energy storage performance

Dielectric capacitors are essential for energy storage systems due to their high-power density and fast operation speed. However, optimizing energy storage density with concurrent thermal stability remains a substantial challenge. Here, we develop a flash annealing process with ultrafast heating and cooling rates of 1000 oC/s, which facilitates the rapid crystallization of PbZrO3 film within a mere second, while locking its high-temperature microstructure to room temperature. This produces compact films with sub-grain boundaries fraction of 36%, nanodomains of several nanometers, and negligible lead volatilization. These contribute to relaxor antiferroelectric film with a high breakdown strength (4800 kV/cm) and large polarization (70 uC/cm2). Consequently, we have achieved a high energy storage density of 63.5 J/cm3 and outstanding thermal stability with performance degradation less than 3% up to 250 oC. Our approach is extendable to ferroelectrics like Pb(Zr0.52Ti0.48)O3 and on wafer scale, providing on-chip nonlinear dielectric energy storage solutions with industrial scalability.

cond-mat.mtrl-sci

Investigating and Controlling the Libration and Rotation Dynamics of Nanoparticles in an Optomechanical System

In optomechanical systems, the libration and rotation of nanoparticles offer profound insights for ultrasensitive torque measurement and macroscopic quantum superpositions. Achievements include transitioning libration to rotation up to 6 GHz and cooling libration to millikelvin temperatures. It is undoubted that the libration and rotation are respectively driven by restoring and constant optical torques. The transition mechanisms between these two states, however, demand further exploration. In this perspective, it is demonstrated in this manuscript that monitoring lateral-scattered light allows real-time observation of libration/rotation transitions and associated hysteresis as ellipticities of trapping laser fields vary. By calculating optical torques and solving the Langevin equation, transitions are linked to the balance between anisotropic-polarization-induced sinusoidal optical torques and constant ones, with absorption identified as the main contributor to constant torques. These findings enable direct weak torque sensing and precise nanoparticle control in rotational degrees, paving the way for studying quantum effects like nonadiabatic phase shifts and macroscopic quantum superpositions, thereby enriching quantum optomechanics research.

physics.optics

Morphological tracking and tuning of silica NPs for stable levitation in vacuum optomechanical systems

Optically levitated nanomechanical resonators in vacuum perform ultrahigh sensitivity for mechanical quantities by overcoming the limitations of clamped resonators. However, the generally levitated silica nanoparticles (NPs) with low absorption and high transparence still face difficulties surviving in high vacuum with unclear reason. By monitoring the physicochemical properties like scattering, mass and density of amorphous silica NPs during pumping process. we propose that the loss of NPs may arises from the motional instability induced by laser heating lead releasing at low pressure. In this work, two types of NPs are heat treated from 100 to 1200 degree Celsius to release impurities before being loaded into an optical trap. The high vacuum levitation ratio for both NPs increase obviously after heat treatment. In particular, for NPs heated to 600 degree Celsius, the ratio strikingly improves from ~30% to 100% and ~0 to 85% for two types of NPs. The loss mechanism is further confirmed by their relatively stable physicochemical parameters during pumping process. This work paves a way for wide application of levitated nano-resonators and indicates that levitated vacuum optomechanical systems could be a promising tool for dynamics and in-situ studying of small particles like aerosols and dusts.

physics.optics

Nanoscale Electric Field Sensing Using Levitated Nano-resonator with Net Charge

Nanomechanical resonator based on levitated particle exhibits unique advantages in the development of ultrasensitive electric field detector. We demonstrate a three-dimensional, high-sensitivity electric field measurement technology using the optically levitated nanoparticle with a known net charge. By changing the relative position between nanoparticle and parallel electrodes, the three-dimensional electric field distribution is scanned. The measured noise equivalent electric intensity with charge amount of 100 reaches the order of {\rm{1μV/cm/H}}{\rm{z}^{\rm{1/2}}} at 1.4 \times {10^{ - 7}}mbar. Linearity analysis near resonance frequency shows a measured linear range over 91dB limited only by the maximum output voltage of the driving equipment. This work may provide avenue for developing a high-sensitive electric field sensor based on optically levitated nano-resonator.

physics.app-ph