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Cuong Dang

Publications and source records attributed to Cuong Dang.

27 records · Page 2Linked to original sources

Non-invasive optical focusing inside strongly scattering media with linear fluorescence

Non-invasive optical focusing inside scattering media is still a big challenge because inhomogeneous media scatter both incoming photons for focusing and outgoing photons for observation. Various approaches, utilizing non-linear fluorescence or ultrasound, have been reported to address this difficulty. However, implementation of these methods is complicated and highly expensive, as ultrafast laser systems or photo-acoustic equipment must be employed. Here, we demonstrate a wavefront shaping technique to achieve non-invasive focusing (NiF) inside scattering media using only a linear fluorescent signal. Contrast and mean of incoherent speckles, produced by the linear fluorescence, are utilized as feedback signals to optimize the input wavefront. While increasing speckle contrast makes the focus tighter, and increasing the speckle mean enhances the intensity, fine-tuning the contribution of these two factors in our two-step optimization is essential. An optimal wavefront is found to achieve simultaneously both a micrometer focal spot size (down to 20 um diameter) and high intensity (more than a 100-fold enhancement) inside the scattering media. Our method promises a new route in life science towards focusing, imaging or manipulating deep into biological tissues with linear fluorescent agents.

physics.optics↗

Manipulating Coherent Light Matter Interaction: Continuous Transition between Strong Coupling and Weak Coupling in MoS2 Monolayer Coupled with Plasmonic Nanocavities

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a continuous transition from weak coupling to strong coupling between excitons in MoS2 monolayer and highly localized plasmons in ultra-compact nanoantenna. The nanoantenna is assembled by a silver nanocube positioned over a gold film and separated by a dielectric spacer layer. We observed a 1570-fold enhancement in the photoluminescence at weak coupling regime in hybrid nanocavities with thick spacer layers. The interaction between excitons and plasmons is then directly prompted to strong coupling regime by shrinking down the thickness of spacer layer. Room temperature formation of polaritons with Rabi splitting up to 190 meV was observed, which is the largest plasmon-exciton Rabi splitting reported in two dimensional materials. Numerical calculations quantified the relation between coupling strength, local density of states and spacer thickness, and revealed the transition between weak coupling and strong coupling in nanocavities. The findings in this work offer a guideline for feasible designs of plasmon-exciton interaction systems with gap plasmonic cavities.

cond-mat.mes-hall↗

Noninvasive super-resolution imaging through scattering media

Super-resolution imaging with advanced optical systems has been revolutionizing technical analysis in various fields from biological to physical sciences. However, many objects are hidden by strongly scattering media such as rough wall corners or biological tissues that scramble light paths, create speckle patterns and hinder object's visualization, let alone super-resolution imaging. Here, we realize a method to do non-invasive super-resolution imaging through scattering media based on stochastic optical scattering localization imaging (SOSLI) technique. Simply by capturing multiple speckle patterns of photo-switchable emitters in our demonstration, the stochastic approach utilizes the speckle correlation properties of scattering media to retrieve an image with more than five-fold resolution enhancement compared to the diffraction limit, while posing no fundamental limit in achieving higher spatial resolution. More importantly, we demonstrate our SOSLI to do non-invasive super-resolution imaging through not only optical diffusers, i.e. static scattering media, but also biological tissues, i.e. dynamic scattering media with decorrelation of up to 80%. Our approach paves the way to non-invasively visualize various samples behind scattering media at unprecedented levels of detail.

physics.optics↗

Sustained biexciton emission in colloidal quantum wells assisted by dopant-host interaction

Biexcitons have been considered as one of the fundamental building blocks for quantum technology because of its overwhelming advantages in generating entangled photon pairs. Although many-body complexes have been demonstrated recently in mono-layer transition metal dichalcogenides (TMDs), the low emission efficiency and scale up capability hinder their applications. Colloidal nanomaterials, with high quantum efficiency and ease of synthesis/processing, are regarded to be an appealing complement to TMDs for biexciton sources. However, a progress towards biexciton emission in colloidal nanomaterials has been challenging largely by small binding energy and ultrafast non-radiative multiexciton recombination. Here, we demonstrate room-temperature biexciton emission in Cu-doped CdSe colloidal quantum wells (CQWs) under continuous-wave excitation with intensity as low as ~10 W/cm2. The characteristics of radiative biexciton states are investigated by their super linear emission with respect to excitation power, thermal stability and transient photophysics. The interaction between the quantum confined host carriers and the dopant ions increases biexciton binding energy by two folds compared to the undoped CQWs. Such strong binding energy together with suppressed Auger recombination and efficient, spectrally narrow photoluminescence in a quasi-2D semiconductor enables sustained biexciton emission at room temperature, providing a potential solution for efficient, scalable and stand-alone quantum devices.

cond-mat.mes-hall↗

Temperature-dependent Optoelectronic Properties of Quasi-2D Colloidal Cadmium Selenide Nanoplatelets

Colloidal Cadmium Selenide (CdSe) nanoplatelets (NPLs) are a recently developed class of efficient luminescent nanomaterial suitable for optoelectronic device applications. A change in temperature greatly affects their electronic bandstructure and luminescence properties. It is important to understand how-and-why the characteristics of NPLs are influenced, particularly at elevated temperature, where both reversible and irreversible quenching processes come into picture. Here we present a study on the effect of elevated temperature on the characteristics of colloidal CdSe NPLs. We used an effective-mass envelope function theory based 8-band k$\cdot$p model and density-matrix theory considering exciton-phonon interaction. We observed the photoluminescence (PL) spectra at various temperatures for their photon emission energy, PL linewidth and intensity by considering the exciton-phonon interaction with both acoustic and optical phonons using Bose-Einstein statistical factors. With rise in temperature we observed a fall in the transition energy (emission redshift), matrix element, Fermi factor and quasi Fermi separation, with reduction in intraband state gaps and increased interband coupling. Also, there was a fall in the PL intensity, along with spectral broadening due to an intraband scattering effect. The predicted transition energy values and simulated PL spectra at varying temperatures exhibit appreciable consistency with experimental results. Our findings have important implications for application of NPLs in optoelectronic devices, such as NPL lasers and LEDs, operating much above room temperature.

cond-mat.mes-hall↗

Single shot large field of view imaging with scattering media by spatial demultiplexing

Optically focusing and imaging through strongly scattering media are challenging tasks but have widespread applications from scientific research to biomedical applications and daily life. Benefiting from the memory effect (ME) for speckle intensity correlations, only one single-shot speckle pattern can be used for the high quality recovery of the objects and avoiding some complicated procedures to reduce scattering effects. In spite of all the spatial information from a large object being embedded in a single speckle image, ME gives a strict limitation to the field of view (FOV) for imaging through scattering media. Objects beyond the ME region cannot be recovered and only produce unwanted speckle patterns, causing reduction in the speckle contrast and recovery quality. Here, we extract the spatial information by utilizing these unavoidable speckle patterns, and enlarge the FOV of the optical imaging system. Regional point spreading functions (PSFs), which are fixed and only need to be recorded once for all time use, are employed to recover corresponding spatial regions of an object by deconvolution algorithm. Then an automatic weighted averaging in an iterative process is performed to obtain the object with significantly enlarged FOV. Our results present an important step toward an advanced imaging technique with strongly scattering media.

physics.optics↗

Single-shot multispectral imaging with a monochromatic camera

Multispectral imaging plays an important role in many applications from astronomical imaging, earth observation to biomedical imaging. However, the current technologies are complex with multiple alignment-sensitive components, predetermined spatial and spectral parameters by manufactures. Here, we demonstrate a single-shot multispectral imaging technique that gives flexibility to end-users with a very simple optical setup, thank to spatial correlation and spectral decorrelation of speckle patterns. These seemingly random speckle patterns are point spreading functions (PSFs) generated by light from point sources propagating through a strongly scattering medium. The spatial correlation of PSFs allows image recovery with deconvolution techniques, while the spectral decorrelation allows them to play the role of tune-able spectral filters in the deconvolution process. Our demonstrations utilizing optical physics of strongly scattering media and computational imaging present the most cost-effective approach for multispectral imaging with great advantages.

physics.optics↗

Enhancing security of optical cryptosystem with position-multiplexing and ultra-broadband illumination

A position-multiplexing based cryptosystem is proposed to enhance the information security with an ultra-broadband illumination. The simplified optical encryption system only contains one diffuser acting as the random phase mask (RPM). Light coming from a plaintext passes through this RPM and generates the corresponding ciphertext on a camera. The proposed system effectively reduces problems of misalignment and coherent noise that are found in the coherent illumination. Here, the use of ultra-broadband illumination has the advantage of making a strong scattering and complex ciphertext by reducing the speckle contrast. Reduction of the ciphertext size further increases the strength of the ciphering. The unique spatial keys are utilized for the individual decryption as the plaintext locates at different spatial positions, and a complete decrypted image could be concatenated with high fidelity. Benefiting from the ultra-broadband illumination and position-multiplexing, the information of interest is scrambled together in a small ciphertext. Only the authorized user can decrypt this information with the correct keys. Therefore, a high performance security for a cryptosystem could be achieved.

physics.optics↗