arXiv subjects

Cyriaque Genet

Publications and source records attributed to Cyriaque Genet.

At least 19 recordsLinked to original sources

arXiv2026

Enantioselective optical trapping and characterization of all dielectric disorder-enabled chiral particles

We trap submicroscopic silica spheres coated with randomly distributed titanium dioxide nanoparticles in optical tweezers with Laguerre-Gaussian modes and observe orbital dynamics that differ from those of achiral silica spheres. We show that the disordered nanoparticle coating generates an effective chiral geometry, giving rise to enhanced enantioselective chiral optical forces and a measurable modification of the orbital period. A theoretical model based on the Mie-Debye formalism, including optical aberrations, not only quantitatively explains the experimental results but also allows to characterize the Pasteur parameter quantifying the chiroptical response of individual composite particles. These findings constitute direct experimental evidence of chiral optical forces exerted by structured light beams on individual chiral particles and identify disorder-enabled, all-dielectric particles as a versatile material platform to tailor chiral optical forces at the nanoscale.

physics.optics↗

arXiv2026

Consistent thermodynamics reconstructed from transitions between nonequilibrium steady-states

Constructing a thermodynamic framework for nonequilibrium systems remains a major challenge, as quantities such as temperature and free energy often become ambiguous when inferred solely from steady-state properties. Here we take a transformation-based approach and experimentally examine transitions between nonequilibrium steady states (NESS). Using an optically trapped microparticle driven by a tunable correlated stochastic force, we generate active-like steady states with controllable noise statistics. By abruptly changing the trap stiffness, we measure the stochastic work, heat, and entropy produced during NESS-to-NESS transformations. We identify a state-dependent effective temperature that restores the second law for these transitions, enabling the definition of a generalized work that incorporates the consequence of the nonequilibrium fluctuations. With this quantity, we derive and experimentally verify a Crooks-like fluctuation relation linking work distributions to a nonequilibrium free-energy difference defined through the effective temperature. Finally, we establish a fluctuation-response relation for the positional variance following stiffness changes. We demonstrate that this relation is key to distinguishing systems that can be described by a unique effective temperature (i.e., those under equilibrium or white-noise conditions) from those under colored-noise, where an equilibrium-like response cannot be restored. These results delineate the applicability and limits of effective-temperature thermodynamics in driven systems.

cond-mat.stat-mech↗

arXiv2025

Circular Dichroism without absorption in isolated chiral dielectric Mie particles

We demonstrate that an effect phenomenologically analogous to circular dichroism can arise even for dielectric and isotropic chiral spherical particles. By analyzing the polarimetry of light scattered from a chiral, lossless microsphere illuminated with linearly polarized light, we show that the scattered light becomes nearly circularly polarized, exhibiting large, nonresonant values of the Stokes parameter $S_3$ for a broad range of visible frequencies. This phenomenon occurs only in the Mie regime, with the microsphere radius comparable to the wavelength, and provided that the scattered light is collected by a high-NA objective lens, including non-paraxial Fourier components. Altogether, our findings offer a theoretical framework and motivation for an experimental demonstration of a novel chiroptical effect with isolated dielectric particles, with potential applications in enantioselection and characterization of single microparticles, each and every one with its own chiral response.

physics.optics↗

arXiv2023

Spin-momentum locking breakdown on plasmonic metasurfaces

We present a scattering formalism to analyze the spin-momentum locking in structured holey plasmonic metasurfaces. It is valid for any unit cell for arbitrary position and orientation of the holes. The spin-momentum locking emergence is found to originate from the unit cell configuration. Additionally, we find that there are several breakdown terms spoiling the perfect spin-momentum locking polarization. We prove that this breakdown also appears in systems with global symmetries of translation and rotation of the whole lattice, like the Kagome lattice. Finally, we present the excitation of surface plasmon polaritons as the paramount example of the spin-momentum locking breakdown.

physics.optics↗

arXiv2023

Taming a Maxwell's demon for experimental stochastic resetting

A diffusive process that is reset to its origin at random times, so-called stochastic resetting (SR), is an ubiquitous expedient in many natural systems . Yet, beyond its ability to improve the efficiency of target searching, SR is a true non-equilibrium thermodynamic process that brings forward new and challenging questions . Here, we show how the recent developments of experimental information thermodynamics renew the way to address SR and can lead, beyond a new understanding, to better control on the non-equilibrium nature of SR. This thermodynamically controlled SR is experimentally implemented within a time-dependent optical trapping potential. We show in particular that SR converts heat into work from a single bath continuously and without feedback. This implements a Maxwell's demon that constantly erases information. In our experiments, the erasure takes the form of a protocol that allows to evaluate the true energetic cost of SR. We show that using an appropriate measure of the available information, this cost can be reduced to a reversible minimum while being bounded by the Landauer limit. We finally reveal that the individual trajectories generated by the demon all break ergodicity and thus demonstrate the non-ergodic nature of the demon's modus operandi. Our results offer new approaches to processes, such as SR, where the informational framework provides key experimental tools for their non-equilibrium thermodynamic control.

cond-mat.stat-mech↗

arXiv2023

Circular dichroism induction in WS2 by a chiral plasmonic metasurface

We investigate the interaction between a monolayer of WS2 and a chiral plasmonic metasurface. WS2 possesses valley excitons that selectively couple with one-handed circularly polarised light. At the same time, the chiral plasmonic metasurface exhibits spin-momentum locking, leading to a robust polarisation response in the far field. Using a scattering formalism based on the coupled mode method, we analyse various optical properties of the WS2 monolayer. Specifically, we demonstrate the generation of circular dichroism in the transition metal dichalcogenide (TMD) by harnessing the excitation of surface plasmon polaritons (SPPs) in the metasurface. Moreover, we observe the emergence of other guided modes, opening up exciting possibilities for further exploration in TMD-based devices.

physics.optics↗

arXiv2023

Optimal time-entropy bounds and speed limits for Brownian thermal shortcuts

By controlling in real-time the variance of the radiation pressure exerted on an optically trapped microsphere, we engineer temperature protocols that shortcut thermal relaxation when transferring the microsphere from one thermal equilibrium state to an other. We identify the entropic footprint of such accelerated transfers and derive optimal temperature protocols that either minimize the production of entropy for a given transfer duration or accelerate as much as possible the transfer for a given entropic cost. Optimizing the trade-off yields time-entropy bounds that put speed limits on thermalization schemes. We further show how optimization expands the possibilities for accelerating Brownian thermalization down to its fundamental limits. Our approach paves the way for the design of optimized, finite-time thermodynamic cycles at the mesoscale. It also offers a platform for investigating fundamental connections between information geometry and finite-time processes.

cond-mat.stat-mech↗

arXiv2022

Microscopic analysis of spin-momentum locking on a geometric phase metasurface

We revisit spin-orbit coupling in a plasmonic Berry metasurface comprised of rotated nanoapertures, which is known to imprint a robust far-field polarization response. We present a scattering formalism that shows how that spin-momentum locking emerges from the geometry of the unit cell without requiring global rotation symmetries. We find and confirm with Mueller polarimetry measurements that spin-momentum locking is an approximate symmetry. The symmetry breakdown is ascribed to the elliptical projection of circularly polarized light into the planar surface. This breakdown is maximal when surface waves are excited, and a new set of spin-momentum locking rules is presented for this case.

physics.optics↗

arXiv2021

Harvesting information to control non-equilibrium states of active matter

We propose to use a correlated noise bath to drive an optically trapped Brownian particle that mimics active biological matter. Thanks to the flexibility and precision of our setup, we are able to control the different parameters that drive the stochastic motion of the particle with unprecedented accuracy, thus reaching strongly correlated regimes that are not easily accessible with real active matter. In particular, by using the correlation time (i.e., the "color") of the noise as a control parameter, we can trigger transitions between two non-equilibrium steady states with no expended work, but only a calorific cost. Remarkably, the measured heat production is directly proportional to the spectral entropy of the correlated noise, in a fashion that is reminiscent of Landauer's principle. Our procedure can be viewed as a method for harvesting information from the active fluctuations.

cond-mat.soft↗

arXiv2021

Planar chirality and optical spin-orbit coupling for chiral Fabry-Perot cavities

We design, in a most simple way, Fabry-Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin-orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry.

physics.optics↗

arXiv2021

Galilean relativity for Brownian dynamics and energetics

We study experimentally the impact of inertial reference frame changes on overdamped Brownian motion. The reference frame changes are implemented by inducing, with a laser, laminar convection flows in a column of fluid where Brownian microspheres are dispersed. The convection flow plays the role of the relative velocity between the laboratory and the fluid comoving frames, and enables us to analyse the consequences of Galilean transformations on Brownian diffusion. We verify in particular how the Brownian dynamics remains "weakly" Galilean invariant, in agreement with recent discussions. We also carefully look at the consequences of Galilean relativity on the Brownian energetics. This leads us to derive a Galilean invariant expression of the stochastic thermodynamic first law, consistent with existing theoretical results. We finally discuss a potential ambiguity of the Galilean relativistic features of diffusive systems that has obvious practical implications in the context of force measurements in external flows.

cond-mat.stat-mech↗

arXiv2021

Large Enhancement of Ferro-Magnetism under Collective Strong Coupling of YBCO Nanoparticles

Light-matter strong coupling in the vacuum limit has been shown to enhance material properties over the past decade. Oxide nanoparticles are known to exhibit weak ferromagnetism due to vacancies in the lattice. Here we report the 700-fold enhancement of the ferromagnetism of YBa$_2$Cu$_3$O$_{7-x}$ nanoparticles under cooperative strong coupling at room temperature. The magnetic moment reaches 0.90 $\mu_{\rm B}$/mol, and with such a high value, it competes with YBa$_2$Cu$_3$O$_{7-x}$ superconductivity at low temperature. This strong ferromagnetism at room temperature suggest that strong coupling is a new tool for the development of next generations of magnetic and spintronic nanodevices.

cond-mat.mtrl-sci↗

arXiv2020

Chiral thermodynamics in tailored chiral optical environments

We present an optomechanical model that describes the stochastic motion of an overdamped chiral nanoparticle diffusing in the optical bistable potential formed in the standing-wave of two counter-propagating Gaussian beams. We show how chiral optical environments can be induced in the standing-wave with no modification of the initial bistability by controlling the polarizations of each beam. Under this control, optical chiral densities and/or an optical chiral fluxes are generated, associated respectively with reactive vs. dissipative chiral optical forces exerted on the diffusing chiral nanoparticle. This optomechanical chiral coupling bias the thermodynamics of the thermal activation of the barrier crossing, in ways that depend on the nanoparticle enantiomer and on the optical field enantiomorph. We show that reactive chiral forces, being conservative, contribute to a global, enantiospecific, change of the Helmholtz free energy bistable landscape. In contrast, when the chiral nanoparticle is immersed in a dissipative chiral environment, the symmetry of the bistable potential is broken by non-conservative chiral optical forces. In this case, the chiral electromagnetic fields continuously transfer, through dissipation, mechanical energy to the chiral nanoparticle. For this chiral nonequilibrium steady-state, the thermodynamic changes of the barrier crossing take the form of heat transferred to the thermal bath and yield chiral deracemization schemes that can be explicitly calculated within the framework of our model. Three-dimensional stochastic simulations confirm and further illustrate the thermodynamic impact of chirality. Our results reveal how chiral degrees of freedom both of the nanoparticle and of the optical fields can be transformed into true thermodynamics control parameters, thereby demonstrating the significance of optomechanical chiral coupling in stochastic thermodynamics.

quant-ph↗

arXiv2020

Probing quantum effects with classical stochastic analogs

We propose a method to construct a classical analog of an open quantum system, namely a single quantum particle confined in a potential well and immersed in a thermal bath. The classical analog is made out of a collection of identical wells where classical particles of mass $m$ are trapped. The distribution $n(x,t)$ of the classical positions is used to reconstruct the quantum Bohm potential $V_{\rm Bohm} = -\frac{\hbar^2}{2 m} \frac{\Delta \sqrt{n}}{\sqrt{n}}$, which in turn acts on the shape of the potential wells. As a result, the classical particles experience an effective "quantum" force. This protocol is tested with numerical simulations using single- and double-well potentials, evidencing typical quantum effects such as long-lasting correlations and quantum tunneling. For harmonic confinement, the analogy is implemented experimentally using micron-sized dielectric beads optically trapped by a laser beam.

quant-ph↗

arXiv2020

Noise and ergodic properties of Brownian motion in an optical tweezer: looking at the crossover between Wiener and Ornstein-Uhlenbeck processes

We characterize throughout the spectral range of an optical trap the nature of the noise at play and the ergodic properties of the corresponding Brownian motion of an overdamped trapped single microsphere, comparing experimental, analytical and simulated data. We carefully analyze noise and ergodic properties $(i)$ using the Allan variance for characterizing the noise and $(ii)$ exploiting a test of ergodicity tailored for experiments done over finite times. We derive these two observables in the low-frequency Ornstein-Uhlenbeck trapped-diffusion regime and study analytically their evolution towards the high-frequency Wiener free-diffusion regime, in a very good agreement with simulated and experimental results. This leads to reveal noise and ergodic spectral signatures associated with the distinctive features of both regimes.

cond-mat.stat-mech↗

arXiv2020

Large optical nonlinearity enhancement under electronic strong coupling

Nonlinear optical responses provide a powerful way to understand the microscopic interactions between laser fields and matter. They are critical for plenty of applications, such as in lasers, integrated photonic circuits, biosensing and medical tools. However, most materials exhibit weak optical nonlinearities or long response times when they interact with intense optical fields. Here, we strongly couple the exciton of organic molecules to an optical mode of a Fabry-Perot cavity, and achieve an enhancement of the nonlinear complex refractive index by two orders of magnitude compared with that of the uncoupled condition. Moreover, the coupled system shows an ultrafast response of ~120 fs that we extract from optical cross-correlation measurements. The ultrafast and large enhancement of the nonlinar coefficients in this work paves the way for exploring strong coupling effects on various third-order nonlinear optical phenomena and for technological applications.

physics.optics↗

arXiv2019

Exploring Superconductivity under Strong Coupling with the Vacuum Electromagnetic Field

Light-matter interactions have generated considerable interest as a means to manipulate material properties. Light-induced superconductivity has been demonstrated using pulsed lasers. An attractive alternative possibility is to exploit strong light-matter interactions arising by coupling phonons to the vacuum electromagnetic field of a cavity mode as has been suggested and theoretically studied. Here we explore this possibility for two very different superconductors, namely YBCO (YBa$_2$Cu$_3$O$_{6+x}$) and Rb$_3$C$_{60}$, coupled to surface plasmon polaritons, using a novel cooperative effect based on the presence of a strongly coupled vibrational environment allowing efficient dressing of the otherwise weakly coupled phonon bands of these compounds. By placing the superconductor-surface plasmon system in a SQUID magnetometer, we find that the superconducting transition temperatures ($T_{c}$) for both compounds are modified in the absence of any external laser field. For YBCO, $T_{c}$ decreases from 92 K to 86 K while for Rb$_3$C$_{60}$, it increases from 30 K to 45 K at normal pressures. In the latter case, a simple theoretical framework is provided to understand these results based on an enhancement of the electron-phonon coupling. This proof-of-principle study opens a new tool box to not only modify superconducting materials but also to understand the mechanistic details of different superconductors.

cond-mat.supr-con↗

arXiv2019

Subfemtonewton force fields measured with ergodic Brownian ensembles

We demonstrate that radiation pressure force fields can be measured and reconstructed with a resolution of $0.3$ fN (at a $99.7\%$ confidence level) using an ergodic ensemble of overdamped colloidal particles. The outstanding force resolution level is provided by the large size of the statistical ensemble built by recording all displacements from all diffusing particles, regardless of trajectory and time. This is only possible because the noise driving the particles is thermal, white and stationary, so that the colloidal system is ergodic, as we carefully verify. Using an ergodic colloidal dispersion for performing ultra-sensitive measurements of external forces is not limited to non-conservative optical force fields. Our experiments therefore give way to interesting opportunities in the context of weak force measurements in fluids.

physics.optics↗