arXiv subjects

D. A. Chareev

Publications and source records attributed to D. A. Chareev.

At least 37 records · Page 2Linked to original sources

arXiv2017

Direct Evidence of Two Superconducting Gaps in FeSe$_{0.5}$Te$_{0.5}$: SnS-Andreev Spectroscopy and Lower Critical Field

We present direct measurements of the superconducting order parameter in nearly optimal FeSe$_{0.5}$Te$_{0.5}$ single crystals with critical temperature $T_C \approx 14$ K. Using intrinsic multiple Andreev reflection effect (IMARE) spectroscopy and measurements of lower critical field, we directly determined two superconducting gaps, $Δ_L \approx 3.3 - 3.4$ meV and $Δ_S \approx 1$ meV, and their temperature dependences. We show that a two-band model fits well the experimental data. The estimated electron-boson coupling constants indicate a strong intraband and a moderate interband interaction.

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arXiv2016

Gossamer bulk high-temperature superconductivity in FeSe

The cuprates and iron-based high-temperature superconductors share many common features: layered strongly anisotropic crystal structure, strong electronic correlations, interplay between different types of electronic ordering, the intrinsic spatial inhomogeneity due to doping. The understanding of complex interplay between these factors is crucial for a directed search of new high-temperature superconductors. Here we show the appearance of inhomogeneous gossamer superconductivity in bulk FeSe compound at ambient pressure and at temperature 5 times higher than its zero-resistance $T_c$. This discovery helps to understand numerous remarkable superconducting properties of FeSe. We also find and prove a general property: if inhomogeneous superconductivity in a anisotropic conductor first appears in the form of isolated superconducting islands, it reduces electric resistivity anisotropically with maximal effect along the least conducting axis. This gives a simple and very general tool to detect inhomogeneous superconductivity in anisotropic compounds, which is critically important to study the onset of high-temperature superconductivity.

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arXiv2016

Highly mobile carriers in orthorhombic phases of iron-based superconductors FeSe${}_{1-x}$S${}_{x}$

The field and temperature dependencies of the longitudinal and Hall resistivity have been measured for FeSe${}_{1-x}$S${}_{x}$ (x=0.04, 0.09 and 0.19) single crystals. The sample FeSe${}_{0.81}$S${}_{0.19}$ does not show a transition to an orthorhombic phase and exhibits at low temperatures the transport properties quite different from those of orthorhombic samples. The behavior of FeSe${}_{0.81}$S${}_{0.19}$ is well described by the simple two band model with comparable values of hole and electron mobility. In particular, at low temperatures the transverse resistance shows a linear field dependence, the magnetoresistance follow a quadratic field dependence and obeys to Kohler's rule. In contrast, Kohler's rule is strongly violated for samples having an orthorhombic low temperature structure. However, the transport properties of the orthorhombic samples can be satisfactory described by the three band model with the pair of almost equivalent to the tetragonal sample hole and electron bands, supplemented with the highly mobile electron band which has two order smaller carrier number. Therefore, the peculiarity of the low temperature transport properties of the orthorhombic Fe(SeS) samples, as probably of many other orthorhombic iron superconductors, is due to the presence of a small number of highly mobile carriers which originate from the local regions of the Fermi surface, presumably, nearby the Van Hove singularity points.

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arXiv2016

Magnetic ground state of FeSe

Elucidating the nature of the magnetism of a high-temperature superconductor is crucial for establishing its pairing mechanism. The parent compounds of the cuprate and iron-pnictide superconductors exhibit Néel and stripe magnetic order, respectively. However, FeSe, the structurally simplest iron-based superconductor, shows nematic order (Ts = 90 K), but not magnetic order in the parent phase, and its magnetic ground state is intensely debated. Here, we report inelastic neutron-scattering experiments that reveal both stripe and Néel spin fluctuations over a wide energy range at 110 K. On entering the nematic phase, a substantial amount of spectral weight is transferred from the Néel to the stripe spin fluctuations. Moreover, the total fluctuating magnetic moment of FeSe is ~ 60% larger than that in the iron pnictide BaFe2As2. Our results suggest that FeSe is a novel S = 1 nematic quantum-disordered paramagnet interpolating between the Néel and stripe magnetic instabilities.

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arXiv2016

Pressure effect on magnetic susceptibility of SmS in semiconducting phase: experimental study

Magnetic susceptibility $χ$ of the polycrystalline sample of samarium monosulfide was measured as a function of the hydrostatic pressure $P$ up to 2 kbar at liquid nitrogen and room temperatures using a pendulum-type magnetometer. A pronounced magnitude of the pressure effect is found to be positive in sign and strongly temperature dependent: the pressure derivatives of $χ$, d\,ln$χ$/d$P$, are $6.3\pm0.5$ and $14.2\pm1$ Mbar$^{-1}$ at 300 and 78 K, respectively. The obtained experimental results are discussed within phenomenological approaches.

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arXiv2016

Doubling of the critical temperature of FeSe observed in point contacts

Rise in superconducting critical temperature Tc more than two times (exceeding 20 K) is discov- ered in point-contacts created between iron-chalcogenide FeSe single crystal and Cu. The possible reasons of such Tc increase in point-contacts are discussed. The most probable cause for this may be the interfacial carriers doping and/or interfacial enhanced electron-phonon interaction.

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arXiv2016

Highly anisotropic and two-fold symmetric superconducting gap in nematically ordered FeSe$_{0.93}$S$_{0.07}$

FeSe exhibits a novel ground state in which superconductivity coexists with a nematic order in the absence of any long-range magnetic order. Here we report an angle-resolved photoemission study on the superconducting gap structure in the nematic state of FeSe$_{0.93}$S$_{0.07}$, without the complication caused by Fermi surface reconstruction induced by magnetic order. We found that the superconducting gap shows a pronounced 2-fold anisotropy around the elliptical hole pocket near the Z point of the Brillouin zone, with gap minima at the endpoints of its major axis, while no detectable gap was observed around the zone center and zone corner. The large anisotropy and nodal gap distribution demonstrate the substantial effects of the nematicity on the superconductivity, and thus put strong constraints on the current theories.

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arXiv2015

Analysis of nonlinear conductivity of point contacts on the base of FeSe in the normal and superconducting state

Nonlinear conductivity of point contacts (PCs) on the base of FeSe single crystals has been investigated. Measured dV/dI dependencies demonstrate the prevailing contribution to the PC conductivity caused by the degraded surface. Superconducting (SC) feature in dV/dI like a sharp zero-bias minimum develops for relatively low ohmic PCs, where the deep areas of FeSe are involved. Analysis of dV/dI has shown that the origin of the zero-bias minimum is connected with the Maxwell part of the PC resistance, what masks energy dependent spectral peculiarities. Even so, we have found the specific features in dV/dI - the sharp side maxima, which may have connection to the SC gap, since their position follows the BCS temperature dependence. Exploring the dV/dI spectra of the rare occurrence with Andreev-like structure, the two gaps with Delta = 2.5 and 3.5 meV were identified.

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arXiv2015

Anomalous correlation effects and unique phase diagram of electron doped FeSe revealed by angle resolved photoemission spectroscopy

In FeSe-derived superconductors, the lack of a systematic and clean control on the carrier concentration prevents the comprehensive understanding on the phase diagram and the interplay between different phases. Here by K dosing and angle resolved photoemission study on thick FeSe films and FeSe$_{0.93}$S$_{0.07}$ bulk crystals, the phase diagram of FeSe as a function of electron doping is established, which is extraordinarily different from other Fe-based superconductors. The correlation strength remarkably increases with increasing doping, while an insulting phase emerges in the heavily overdoped regime. Between the nematic phase and the insulating phase, a dome of enhanced superconductivity is observed, with the maximum superconducting transition temperature of 44$\pm$2~K. The enhanced superconductivity is independent of the thickness of FeSe, indicating that it is intrinsic to FeSe. Our findings provide an ideal system with variable doping for understanding the different phases and rich physics in the FeSe family.

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arXiv2015

Strong Interplay between Stripe Spin Fluctuations, Nematicity and Superconductivity in FeSe

Elucidating the microscopic origin of nematic order in iron-based superconducting materials is important because the interactions that drive nematic order may also mediate the Cooper pairing. Nematic order breaks fourfold rotational symmetry in the iron plane, which is believed to be driven by either orbital or spin degrees of freedom. However, as the nematic phase often develops at a temperature just above or coincides with a stripe magnetic phase transition, experimentally determining the dominant driving force of nematic order is difficult. Here, we use neutron scattering to study structurally the simplest iron-based superconductor FeSe, which displays a nematic (orthorhombic) phase transition at $T_s=90$ K, but does not order antiferromagnetically. Our data reveal substantial stripe spin fluctuations, which are coupled with orthorhombicity and are enhanced abruptly on cooling to below $T_s$. Moreover, a sharp spin resonance develops in the superconducting state, whose energy (~4 meV) is consistent with an electron boson coupling mode revealed by scanning tunneling spectroscopy, thereby suggesting a spin fluctuation-mediated sign-changing pairing symmetry. By normalizing the dynamic susceptibility into absolute units, we show that the magnetic spectral weight in FeSe is comparable to that of the iron arsenides. Our findings support recent theoretical proposals that both nematicity and superconductivity are driven by spin fluctuations.

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arXiv2015

Superconducting properties of sulfur-doped iron selenide

The recent discovery of high-temperature superconductivity in single-layer iron selenide has generated significant experimental interest for optimizing the superconducting properties of iron-based superconductors through the lattice modification. For simulating the similar effect by changing the chemical composition due to S doping, we investigate the superconducting properties of high-quality single crystals of FeSe$_{1-x}$S$_{x}$ ($x$=0, 0.04, 0.09, and 0.11) using magnetization, resistivity, the London penetration depth, and low temperature specific heat measurements. We show that the introduction of S to FeSe enhances the superconducting transition temperature $T_{c}$, anisotropy, upper critical field $H_{c2}$, and critical current density $J_{c}$. The upper critical field $H_{c2}(T)$ and its anisotropy are strongly temperature dependent, indicating a multiband superconductivity in this system. Through the measurements and analysis of the London penetration depth $λ_{ab}(T)$ and specific heat, we show clear evidence for strong coupling two-gap $s$-wave superconductivity. The temperature-dependence of $λ_{ab}(T)$ calculated from the lower critical field and electronic specific heat can be well described by using a two-band model with $s$-wave-like gaps. We find that a $d$-wave and single-gap BCS theory under the weak-coupling approach can not describe our experiments. The change of specific heat induced by the magnetic field can be understood only in terms of multiband superconductivity.

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arXiv2014

Temperature dependence of lower critical field Hc1(T) shows nodeless superconductivity in FeSe

We investigate the temperature dependence of the lower critical field Hc1(T) of a high-quality FeSe single crystal under static magnetic fields H parallel to the c axis. The temperature dependence of the first vortex penetration field has been experimentally obtained by two independent methods and the corresponding Hc1(T) was deduced by taking into account demagnetization factors. A pronounced change in the Hc1(T) curvature is observed, which is attributed to anisotopic s-wave or multiband superconductivity. The London penetration depth λab(T) calculated from the lower critical field does not follow an exponential behavior at low temperatures, as it would be expected for a fully gapped clean s-wave superconductor. Using either a two-band model with s-wave-like gaps of magnitudes ?delta 1 = 0.41 meV and delta ?2 = 3.33 meV or a single anisotropic s-wave order parameter, the temperature dependence of the lower critical field Hc1(T) can be well described. These observations clearly show that the superconducting energy gap in FeSe is nodeless.

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arXiv2014

Spin-dependent conductivity of iron-based superconductors in a magnetic field

We report the results of a study of magnetic field features of electron transport in heterojunctions with NS boundary inside iron-based superconductors, represented by a binary phase of $α$ - FeSe and oxyarsenide pnictide LaO(F)FeAs. We used the ability of self magnetic field of the transport current to partially destroy superconductivity, no matter how low the field may be, in the NS interface area, where, due to the proximity effect, the superconducting order parameter, $Δ$, disperses from 1 to 0 within the scale of the Ginzburg-Landau coherence length. The following features of transport were found:(i) at $T<T_{c}$, magnetoresistance in systems with different superconductors has different sign;(ii) sign and magnitude of the magnetoresistance depend on the magnitude of current and temperature, and (iii) in all operating modes where the contribution from Andreev reflection is suppressed ($(T + eV) \gtrsim Δ$),the hysteresis of the magnetoresistance is present. Based on the results of the experiment and analysis it has been concluded that there is along-range magnetic order in th eground normal state of the iron-based superconductors studied, in the presence of itinerant magnetism of conduction electrons which determines the possibility of anisotropic spin-dependent exchange interaction with the local magnetic moments of the ions.

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arXiv2013

Interplay of superconductivity and magnetism in FeSe$_{1-x}$Te$_x$ compounds. Pressure effects

The influence of uniform pressures $P$ up to 5 kbar on the superconducting transition temperature $T_c$ was studied for the FeSe$_{1-x}$Te$_x$ ($x=0$, 0.85, 0.88 and 0.9) system. For the first time, we observed a change in sign of the pressure effect on $T_c$ when going from FeSe to tellurium rich alloys. This has allowed to specify the pressure derivative d$T_c$/d$P$ for the system as a function of composition. The observed dependence was compared with results of the {\em ab initio} calculations of electronic structure and magnetism of FeSe, FeTe and FeSe$_{0.5}$Te$_{0.5}$, and also with our recent experimental data on pressure effects on magnetic susceptibilities of FeSe and FeTe compounds in the normal state. This comparison demonstrates a competing interplay between superconductivity and magnetism in tellurium rich FeSe$_{1-x}$Te$_x$ compounds

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arXiv2013

Piezomagnetism of FeSe single crystals

The acoustic-electric transformation in high-quality FeSe single crystals is studied. In zero magnetic field we observe an abnormally strong electromagnetic radiation induced by a transverse elastic wave. Usually a radiation of such intensity and polarization is observed only in metals subjected to a high magnetic field (the radiation is caused by the Hall current). We argue that in FeSe in zero magnetic field it is caused by the piezomagnetic effect which is most probably of dynamical origin. We find that the piezomagnetism survives under the transition from the normal to superconducting state. In the superconducting state the electromagnetic signal decreases with decreasing temperature that is connected with the change in the London penetration depth.

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arXiv2013

Unusual band renormalization in the simplest iron based superconductor

The electronic structure of the iron chalcogenide superconductor FeSe_{1-x} was investigated by high- resolution angle-resolved photoemission spectroscopy (ARPES). The results were compared to DFT calculations showing some significant differences between the experimental electronic structure of FeSe_{1-x}, DFT calculations and existing data on FeSe_{x}Te_{1-x}. The bands undergo a pronounced orbital dependent renormalization, different from what was observed for FeSe_{x}Te_{1-x} and any other pnictides.

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arXiv2013

Acoustic characteristics of FeSe single crystals Acoustic characteristics of FeSe single crystals

The results of the comprehensive ultrasonic research of high quality single crystals of FeSe are presented. Absolute values of sound velocities and their temperature dependences were measured; elastic constants and Debye temperature were calculated. The elastic C11-C12 and C11 constants undergo significant softening under the structural tetra-ortho transformation. The significant influence of the superconducting transition on the velocity and attenuation of sound was revealed and the value of the superconducting energy gap was estimated.

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arXiv2012

Magnetic properties of FeSe superconductor

A detailed magnetization study for the novel FeSe superconductor is carried out to investigate the behavior of the intrinsic magnetic susceptibility $χ$ in the normal state with temperature and under hydrostatic pressure. The temperature dependencies of $χ$ and its anisotropy $Δχ=χ_{|}-χ_{\bot}$ are measured for FeSe single crystals in the temperature range 4.2-300 K, and a substantial growth of susceptibility with temperature is revealed. The observed anisotropy $Δχ$ is very large and comparable with the averaged susceptibility at low temperatures. For a polycrystalline sample of FeSe, a significant pressure effect on $χ$ is determined to be essentially dependent on temperature. Ab initio calculations of the pressure dependent electronic structure and magnetic susceptibility indicate that FeSe is close to magnetic instability with dominating enhanced spin paramagnetism. The calculated paramagnetic susceptibility exhibits a strong dependence on the unit cell volume and especially on the height $Z$ of chalcogen species from the Fe plane. The change of $Z$ under pressure determines a large positive pressure effect on $χ$ which is observed at low temperatures. It is shown that the literature experimental data on the strong and nonmonotonic pressure dependence of the superconducting transition temperature in FeSe correlate qualitatively with calculated behavior of the density of electronic states at the Fermi level.

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