arXiv subjects

D. A. Pushin

Publications and source records attributed to D. A. Pushin.

At least 19 recordsLinked to original sources

arXiv2026

Probing Single-Particle Spatial Extent With Helical Neutron Wavefronts

Distinguishing transverse coherence length from single-particle wavepacket extent is fundamentally challenging, as both manifest through spatial broadening of observed intensity profiles in conventional experiments. Here we introduce a method based on helical neutron wavefronts that enables this separation. Helical neutron states produce annular intensity profiles whose peak radius depends on the transverse wavepacket extent, while coherence length only contributes to profile broadening. In our experimental geometry we measure a beam divergence of ~1.1 mrad, corresponding to a transverse coherence length of ~180 nm. In contrast, the same measurement places a lower bound of >= 2 um on the spatial extent of the individual neutron wavepackets, more than an order of magnitude larger than the coherence length. These results provide direct experimental evidence that transverse coherence length and single-particle wavepacket extent are distinct physical quantities, resolving a longstanding source of confusion in the neutron literature.

quant-ph↗

arXiv2026

Experimental Limit on Neutron Orbital Angular Momentum Detection Using Polarized 3He

A recent proposal suggested that neutron orbital angular momentum (OAM) states could be detected via spin-polarized absorption in polarized 3He, with predicted cross-section variations linked to the neutron's OAM. We experimentally tested this hypothesis using spin-polarized neutron beams with OAM =-2 to 2, generated by fork-dislocation phase-gratings, and transmitted through a polarized 3He cell. Within statistical precision, no OAM-dependent change in the absorption cross section was observed. This null result places stringent constraints on polarized 3He-based OAM detection schemes. The absence of an effect in the given regime is traced to the proposal's disregard of the spatial character of neutron OAM: unlike spin, OAM arises from the transverse phase structure of the wavefunction and couples only through spatial gradients and overlap. The transverse extent of neutron OAM modes expands rapidly, producing a doughnut-shaped intensity profile with negligible overlap with on-axis 3He nuclei, while off-axis capture samples only a locally uniform phase and reduces the interaction to the known spin dependence. These results clarify the limits of absorptive nuclear methods for probing neutron OAM and emphasize the necessity of spatially resolved interactions in any viable detection scheme.

physics.app-ph↗

arXiv2025

Design and Monte Carlo Simulation of a Phase Grating Moiré Neutron Interferometer to Measure the Gravitational Constant

The gravitational constant (G) is the least precisely known fundamental constant of nature, with persistent and significant discrepancies between measurement methods. New techniques for measuring G with systematic effects different from commonly applied pendulum methods are required. Neutrons are convenient probes of gravitational forces as they are both massive and electrically neutral, properties that allowed a single-crystal neutron interferometer (NI) to achieve the first experimental demonstration of gravitationally induced quantum interference. Despite this, the limitation of single-crystal NIs to monoenergetic beams significantly reduces neutron flux, making precision gravitational measurements unfeasible. A new NI design called the phase-grating moiré interferometer (PGMI) has been shown to increase neutron flux by orders of magnitude while allowing grating separation that maintains similar interferometer area to previous NI devices. Here, we propose and describe an experiment to measure G using the PGMI to a precision comparable to measurements from the CODATA 2022 evaluation. A Monte Carlo model for incorporating nonlinear potentials into a PGMI is introduced. This model is used to evaluate sources of systematic uncertainty and quantify the uncertainty in G arising from these effects. The effect of lunar gravitation on a torsion pendulum experiment from CODATA 2022 is calculated, and the need for possible correction factors is demonstrated. This work demonstrates that a neutron PGMI can be used to measure G to $150$ parts-per-million in the near term with the potential to achieve greater precision in future experimental designs.

physics.ins-det↗

arXiv2024

Quantum Advancements in Neutron Scattering Reshape Spintronic Devices

Topological magnetism has sparked an unprecedented age in quantum technologies. Marked by twisted spin structures with exotic dynamical modes, topological magnets have motivated a new generation of spintronic devices which transcend the limits of conventional semiconductor-based electronics. While existing material probes have biased studies and device conceptualizations for thin samples in two dimensions, advancements in three-dimensional probing techniques using beams of neutrons, are transforming our understanding of topological and emergent physics to reimagine spintronic devices. Here, we review recent neutron scattering breakthroughs which harness quantum degrees of freedom to enable three-dimensional topological investigations of quantum materials. We discuss applications of structured and tomographic neutron scattering techniques to topological magnets, with particular emphasis on magnetic skyrmion systems and their inspired three-dimensional logic device infrastructures through novel multi-bit encoding and control schemes. SANS-based dynamic visualizations and coherent manipulations of three-dimensional topological qubits are proposed using electric field controls of depth-dependant helicities and spin-orbit tuning of the neutron beam. Together, these investigations uncover a new world of three-dimensional topological physics which enhances spintronic devices through a novel set of structures, dynamics, and controls, unique to three-dimensional systems.

cond-mat.mtrl-sci↗

arXiv2024

Achieving a Near-Ideal Silicon Crystal Neutron Interferometer using Sub-Micron Fabrication Techniques

Perfect-crystal neutron interferometry which is analogous to Mach-Zehnder interferometry, uses Bragg diffraction to form interfering neutron paths. The measured phase shifts can be used to probe many types of interactions whether it be nuclear, electromagnetic, gravitational, or topological in nature. For a perfect-crystal interferometer to preserve coherence, the crystal must possess a high degree of dimensional tolerance as well as being relatively defect-free with minimal internal stresses. In the past, perfect-crystal neutron interferometers have been produced by a two step process. First, a resin diamond wheel would be used to remove excess material and shape the interferometer. Afterword, the crystal would be etched in order to remove surface defects and elevate strains. This process has had limitations in terms of repeatability and in maximizing the final contrast, or fringe visibility, of the interferometer. We have tested various fabrication and post-fabrication techniques on a single perfect-crystal neutron interferometer and measured the interferometer's performance at each step. Here we report a robust, repeatable non-etching fabrication process with high final contrast. For the interferometer used in this work, we achieved contrasts of greater than 90% several separate times and ultimately finished with an interferometer that has 92% contrast and a uniform phase distribution.

physics.ins-det↗

arXiv2023

Phase and contrast moiré signatures in two-dimensional cone beam interferometry

Neutron interferometry has played a distinctive role in fundamental science and characterization of materials. Moiré neutron interferometers are candidate next-generation instruments: they offer microscopy-like magnification of the signal, enabling direct camera recording of interference patterns across the full neutron wavelength spectrum. Here we demonstrate the extension of phase-grating moiré interferometry to two-dimensional geometries. Our fork-dislocation phase gratings reveal phase singularities in the moiré pattern, and we explore orthogonal moiré patterns with two-dimensional phase-gratings. Our measurements of phase topologies and gravitationally induced phase shifts are in good agreement with theory. These techniques can be implemented in existing neutron instruments to advance interferometric analyses of emerging materials and precision measurements of fundamental constants.

physics.app-ph↗

arXiv2023

Cone beam neutron interferometry: from modeling to applications

Phase-grating moire interferometers (PGMIs) have emerged as promising candidates for the next generation of neutron interferometry, enabling the use of a polychromatic beam and manifesting interference patterns that can be directly imaged by existing neutron cameras. However, the modeling of the various PGMI configurations is limited to cumbersome numerical calculations and backward propagation models which often do not enable one to explore the setup parameters. Here we generalize the Fresnel scaling theorem to introduce a k-space model for PGMI setups illuminated by a cone beam, thus enabling an intuitive forward propagation model for a wide range of parameters. The interference manifested by a PGMI is shown to be a special case of the Talbot effect, and the optimal fringe visibility is shown to occur at the moire location of the Talbot distances. We derive analytical expressions for the contrast and the propagating intensity profiles in various conditions, and analyze the behaviour of the dark-field imaging signal when considering sample characterization. The model's predictions are compared to experimental measurements and good agreement is found between them. Lastly, we propose and experimentally verify a method to recover contrast at typically inaccessible PGMI autocorrelation lengths. The presented work provides a toolbox for analyzing and understanding existing PGMI setups and their future applications, for example extensions to two-dimensional PGMIs and characterization of samples with non-trivial structures.

physics.app-ph↗

arXiv2023

Final Measurement of the U235 Antineutrino Energy Spectrum with the PROSPECT-I Detector at HFIR

This Letter reports one of the most precise measurements to date of the antineutrino spectrum from a purely U235-fueled reactor, made with the final dataset from the PROSPECT-I detector at the High Flux Isotope Reactor. By extracting information from previously unused detector segments, this analysis effectively doubles the statistics of the previous PROSPECT measurement. The reconstructed energy spectrum is unfolded into antineutrino energy and compared with both the Huber-Mueller model and a spectrum from a commercial reactor burning multiple fuel isotopes. A local excess over the model is observed in the 5MeV to 7MeV energy region. Comparison of the PROSPECT results with those from commercial reactors provides new constraints on the origin of this excess, disfavoring at 2.2 and 3.2 standard deviations the hypotheses that antineutrinos from U235 are solely responsible and non-contributors to the excess observed at commercial reactors respectively.

nucl-ex↗

arXiv2023

Psychophysical discrimination of radially varying polarization entoptic phenomena

The incorporation of structured light techniques into vision science has enabled more selective probes of polarization related entoptic phenomena. Diverse sets of stimuli have become accessible in which the spatially dependant optical properties can be rapidly controlled and manipulated. For example, past studies with human perception of polarization have dealt with stimuli that appear to vary azimuthally. This is mainly due to the constraint that the typically available degree of freedom to manipulate the phase shift of light rotates the perceived pattern around a person's point of fixation. Here we create a structured light stimulus that is perceived to vary purely along the radial direction and test discrimination sensitivity to inwards and outwards radial motion. This is accomplished by preparing a radial state coupled to an orbital angular momentum state that matches the orientation of the dichroic elements in the macula. The presented methods offering a new dimension of exploration serve as a direct compliment to previous studies and may provide new insights into characterizing macular pigment density profiles and assessing the health of the macula.

physics.med-ph↗

arXiv2023

Calibration strategy of the PROSPECT-II detector with external and intrinsic sources

This paper presents an energy calibration scheme for an upgraded reactor antineutrino detector for the Precision Reactor Oscillation and Spectrum Experiment (PROSPECT). The PROSPECT collaboration is preparing an upgraded detector, PROSPECT-II (P-II), to advance capabilities for the investigation of fundamental neutrino physics, fission processes and associated reactor neutrino flux, and nuclear security applications. P-II will expand the statistical power of the original PROSPECT (P-I) dataset by at least an order of magnitude. The new design builds upon previous P-I design and focuses on improving the detector robustness and long-term stability to enable multi-year operation at one or more sites. The new design optimizes the fiducial volume by elimination of dead space previously occupied by internal calibration channels, which in turn necessitates the external deployment. In this paper, we describe a calibration strategy for P-II. The expected performance of externally deployed calibration sources is evaluated using P-I data and a well-benchmarked simulation package by varying detector segmentation configurations in the analysis. The proposed external calibration scheme delivers a compatible energy scale model and achieves comparable performance with the inclusion of an additional AmBe neutron source, in comparison to the previous internal arrangement. Most importantly, the estimated uncertainty contribution from the external energy scale calibration model meets the precision requirements of the P-II experiment.

physics.ins-det↗

arXiv2023

Neutron interferometric measurement of the scattering length difference between the triplet and singlet states of n-$^3$He

We report a determination of the n-$^3$He scattering length difference $Δb^{\prime} = b_{1}^{\prime}-b_{0}^{\prime} = $ ($-5.411$ $\pm$ $0.031$ (statistical) $\pm$ $0.039$ (systematic)) fm between the triplet and singlet states using a neutron interferometer. This revises our previous result $Δb^{\prime} = $ (-5.610 $\pm$ $0.027$ (statistical) $\pm$ $0.032$ (systematic) fm obtained using the same technique in 2008. This revision is due to a re-analysis of the 2008 experiment that includes a more robust treatment of the phase shift caused by magnetic field gradients near the $^3$He cell. Furthermore, we more than doubled our original data set from 2008 by acquiring six months of additional data in 2013. Both the new data set and a re-analysis of the older data are in good agreement. Scattering lengths of low Z isotopes are valued for use in few-body nuclear effective field theories, provide important tests of modern nuclear potential models and in the case of $^3$He aid in the interpretation of neutron scattering from quantum liquids. The difference $Δb^{\prime}$ was determined by measuring the relative phase shift between two incident neutron polarizations caused by the spin-dependent interaction with a polarized $^3$He target. The target $^3$He gas was sealed inside a small, flat windowed glass cell that was placed in one beam path of the interferometer. The relaxation of $^3$He polarization was monitored continuously with neutron transmission measurements. The neutron polarization and spin flipper efficiency were determined separately using $^3$He analyzers and two different polarimetry analysis methods. A summary of the measured scattering lengths for n-$^3$He with a comparison to nucleon interaction models is given.

nucl-ex↗

arXiv2022

PROSPECT-II Physics Opportunities

The Precision Reactor Oscillation and Spectrum Experiment, PROSPECT, has made world-leading measurements of reactor antineutrinos at short baselines. In its first phase, conducted at the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory, PROSPECT produced some of the strongest limits on eV-scale sterile neutrinos, made a precision measurement of the reactor antineutrino spectrum from $^{235}$U, and demonstrated the observation of reactor antineutrinos in an aboveground detector with good energy resolution and well-controlled backgrounds. The PROSPECT collaboration is now preparing an upgraded detector, PROSPECT-II, to probe yet unexplored parameter space for sterile neutrinos and contribute to a full resolution of the Reactor Antineutrino Anomaly, a longstanding puzzle in neutrino physics. By pressing forward on the world's most precise measurement of the $^{235}$U antineutrino spectrum and measuring the absolute flux of antineutrinos from $^{235}$U, PROSPECT-II will sharpen a tool with potential value for basic neutrino science, nuclear data validation, and nuclear security applications. Following a two-year deployment at HFIR, an additional PROSPECT-II deployment at a low enriched uranium reactor could make complementary measurements of the neutrino yield from other fission isotopes. PROSPECT-II provides a unique opportunity to continue the study of reactor antineutrinos at short baselines, taking advantage of demonstrated elements of the original PROSPECT design and close access to a highly enriched uranium reactor core.

hep-ex↗

arXiv2022

Quantum Information Approach to the Implementation of a Neutron Cavity

Using the quantum information model of dynamical diffraction we consider a neutron cavity composed of two perfect crystal silicon blades capable of containing the neutron wavefunction. We show that the internal confinement of the neutrons through Bragg diffraction can be modelled by a quantum random walk. Good agreement is found between the simulation and the experimental implementation. Analysis of the standing neutron waves is presented in regards to the crystal geometry and parameters; and the conditions required for well-defined bounces are derived. The presented results enable new approaches to studying the setups utilizing neutron confinement, such as the experiments to measure neutron magnetic and electric dipole moments.

quant-ph↗

arXiv2022

Skyrmion Alignment and Pinning Effects in a Disordered Multi-Phase Skyrmion Material Co8Zn8Mn4

Underlying disorder in skyrmion materials may both inhibit and facilitate skyrmion reorientations and changes in topology. The identification of these disorder-induced topologically active regimes is critical to realizing robust skyrmion spintronic implementations, yet few studies exist for disordered bulk samples. Here, we employ small-angle neutron scattering (SANS) and micromagnetic simulations to examine the influence of skyrmion order on skyrmion lattice formation, transition, and reorientation dynamics across the phase space of a disordered polycrystalline Co$_{8}$Zn$_{8}$Mn$_{4}$ bulk sample. Our measurements reveal a new disordered-to-ordered skyrmion square lattice transition pathway characterized by the novel promotion of four-fold order in SANS and accompanied by a change in topology of the system, reinforced through micromagnetic simulations. Pinning responses are observed to dominate skyrmion dynamics in the metastable triangular lattice phase, enhancing skyrmion stabilization through a remarkable and previously undetected skyrmion memory effect which reproduces previous ordering processes and persists in zero field. These results uncover the cooperative interplay of anisotropy and disorder in skyrmion formation and restructuring dynamics, establishing new tunable pathways for skyrmion manipulation.

cond-mat.mtrl-sci↗

arXiv2022

Three-Dimensional Neutron Far-Field Tomography of a Bulk Skyrmion Lattice

Skyrmions are topologically-protected spin textures thought to nucleate and annihilate on points of vanishing magnetization, called Bloch points. However, owing to a lack of bulk techniques, experimental visualizations of skyrmion lattices and their stabilization through defects in three-dimensions remain elusive. Here, we present a tomographic algorithm applied to a Co$_8$Zn$_8$Mn$_4$ skyrmion lattice host, processing multi-projection small angle neutron scattering measurements to generate mean scattering feature reconstructions (MSFR) of the bulk spin textures. Digital phantoms validated the algorithm; reconstructions of the sample show a disordered skyrmion lattice with a topological saturation of 63~\%, exhibiting three-dimensional topological transitions through two different emergent (anti)monopole defect pathways with densities of 147~$μ$m$^{-3}$ and 21~$μ\mathrm{m}^{-3}$ for branching and segmentation events, respectively. Our techniques produce experimentally-informed visualizations of bulk skyrmion lattice structures and defects, enabling future bulk studies over a wide variety of sample shapes and chemistries, magnetic phases, and external parameters.

cond-mat.mtrl-sci↗

arXiv2022

Physics Opportunities with PROSPECT-II

The PROSPECT experiment has substantially addressed the original 'Reactor Antineutrino Anomaly' by performing a high-resolution spectrum measurement from an enriched compact reactor core and a reactor model-independent sterile neutrino oscillation search based on the unique spectral distortions the existence of eV$^2$-scale sterile neutrinos would impart. But as the field has evolved, the current short-baseline (SBL) landscape supports many complex phenomenological interpretations, establishing a need for complementary experimental approaches to resolve the situation. While the global suite of SBL reactor experiments, including PROSPECT, have probed much of the sterile neutrino parameter space, there remains a large region above 1 eV$^2$ that remains unaddressed. Recent results from BEST confirm the Gallium Anomaly, increasing its significance to $\sim 5σ$, with sterile neutrinos providing a possible explanation of this anomaly. Separately, the MicroBooNE exclusion of electron-like signatures causing the MiniBooNE low-energy excess does not eliminate the possibility of sterile neutrinos as an explanation. Focusing specifically on the future use of reactors as a neutrino source for beyond-the-standard-model physics and applications, higher-precision spectral measurements still have a role to play. These recent results have created a confusing landscape which requires new data to disentangle the seemingly contradictory measurements. To directly probe $\overlineν_{e}$ disappearance from high $Δm^2$ sterile neutrinos, the PROSPECT collaboration proposes to build an upgraded and improved detector, PROSPECT-II. It features an evolutionary detector design which can be constructed and deployed within one year and have impactful physics with as little as one calendar year of data.

hep-ex↗

arXiv2022

Experimental Realization of Neutron Helical Waves

Methods of preparation and analysis of structured waves of light, electrons, and atoms have been advancing rapidly. Despite the proven power of neutrons for material characterization and studies of fundamental physics, neutron science has not been able to fully integrate such techniques due to small transverse coherence lengths, the relatively poor resolution of spatial detectors, and low fluence rates. Here, we demonstrate methods that are practical with the existing technologies, and show the experimental achievement of neutron helical wavefronts that carry well-defined orbital angular momentum (OAM) values. We discuss possible applications and extensions to spin-orbit correlations and material characterization techniques.

physics.app-ph↗

arXiv2021

Next-generation high transmission neutron optical devices utilizing micro-machined structures

Neutrons have emerged as a unique probe at the forefront of modern material science, unrivaled in their penetrating abilities. A major challenge stems from the fact that neutron optical devices are limited to refractive indices on the order of $n\approx 1 \pm 10^{-5}$. By exploiting advances in precision manufacturing, we have designed and constructed a micro-meter period triangular grating with a high aspect ratio of $14.3$. The manufacturing quality is demonstrated with white-light interferometric data and microscope imaging. Neutron scattering experiment results are presented, showing agreement to refraction modelling. The capabilities of neutron Fresnel lenses based on this design are contrasted to existing neutron focusing techniques and the path separation of a prism-based neutron interferometer is estimated.

physics.app-ph↗