arXiv subjects

D. A. Shapiro

Publications and source records attributed to D. A. Shapiro.

12 recordsLinked to original sources

arXiv2024

Analyzing Near-Field Intensity Distribution in Subwavelength Gratings through Cylindrical Wave Decomposition

The investigation into the scattering of plane waves by a periodic array of parallel cylinders utilizes the method of cylindrical wave decomposition, thereby reducing the problem complexity to a series of linear algebraic equations. This methodology proves particularly efficacious when the diameter of cylinders is significantly less than the wavelength of incident wave, resulting in a rapid diminution of the solution coefficients as a function of azimuth numbers. Such a reductionist approach facilitates the computation of scattered radiation intensity in near field. Subsequent cross-validation with numerical results corroborates the theoretical findings, showcasing a qualitative concordance between the two. This study underscores the efficacy of cylindrical wave decomposition in simplifying and accurately modeling wave scattering phenomena in structured media.

physics.optics↗

arXiv2011

Scattering of evanescent wave by two cylinders near a flat boundary

Two-dimensional problem of evanescent wave scattering by dielectric or metallic cylinders near the interface between two dielectric media is solved numerically by boundary integral equations method. A special Green function was proposed to avoid the infinite integration. A pattern with a circular and a prolate elliptic cylinders, respectively, is suggested to simulate the sample and the probe in near-field optical microscopy. The energy flux in the midplane of the probe-cylinder is calculated as a function of its position.

physics.optics↗

arXiv2008

X-Ray Powder Diffraction from Sub-Micron Crystals of Photosystem-1 Membrane Protein

We demonstrate that powder diffraction data can be collected from sub-micron crystals of a mbrane protein with nearly two orders of magnitude more atoms than the molecules commonly used for powder diffraction. The crystals of photosystem-1 protein were size-selected using a 500 nm pore- size filter and delivered to a soft x-ray beam with a photon energy of 1.5 keV using a dynamically focused micro-jet developed for the serial crystallography experiment at beamline 9.0.1. The 10-micron jet places many such randomly oriented crystals in the x-ray beam simultaneously resulting in a powder diffraction pattern which extends to 28 angstrom resolution with just 200 seconds of x-ray exposure. The use of the jet for particle delivery allows for a thin sample, appropriate for the soft x-rays used, and continuously refreshes the crystals so that radiation damage is not possible. The small size of the crystals requires the use of lower energy photons for increased scattering strength and increased spacing between powder rings. The powder patterns obtained in this way, from abundant nano-crystals, could be used to provide low resolution molecular envelopes if phased using techniques such as compressive sensing which do not require atomic resolution data. The results also serve to test our aerojet injector system, with future application to femtosecond diffraction in Free Electron X-ray Laser schemes, and for Serial Crystallography using a single-file beam of aligned hydrated molecules.

physics.bio-ph↗

arXiv2008

Three-dimensional coherent X-ray diffraction imaging of a ceramic nanofoam: determination of structural deformation mechanisms

Ultra-low density polymers, metals, and ceramic nanofoams are valued for their high strength-to-weight ratio, high surface area and insulating properties ascribed to their structural geometry. We obtain the labrynthine internal structure of a tantalum oxide nanofoam by X-ray diffractive imaging. Finite element analysis from the structure reveals mechanical properties consistent with bulk samples and with a diffusion limited cluster aggregation model, while excess mass on the nodes discounts the dangling fragments hypothesis of percolation theory.

cond-mat.mtrl-sci↗

arXiv2008

Ultrafast, ultrabright, X-ray holography using a uniformly-redundant array

Advances in the development of free-electron lasers offer the realistic prospect of high-resolution imaging to study the nanoworld on the time-scale of atomic motions. We identify X-ray Fourier Transform holography, (FTH) as a promising but, so far, inefficient scheme to do this. We show that a uniformly redundant array (URA) placed next to the sample, multiplies the efficiency of X-ray FTH by more than one thousand (approaching that of a perfect lens) and provides holographic images with both amplitude- and phase-contrast information. The experiments reported here demonstrate this concept by imaging a nano-fabricated object at a synchrotron source, and a bacterial cell at a soft X-ray free-electron-laser, where illumination by a single 15 fs pulse was successfully used in producing the holographic image. We expect with upcoming hard X-ray lasers to achieve considerably higher spatial resolution and to obtain ultrafast movies of excited states of matter.

physics.optics↗

arXiv2007

Accuracy of one-dimensional collision integral in the rigid spheres approximation

The accuracy of calculation of spectral line shapes in one-dimensional approximation is studied analytically in several limiting cases for arbitrary collision kernel and numerically in the rigid spheres model. It is shown that the deviation of the line profile is maximal in the center of the line in case of large perturber mass and intermediate values of collision frequency. For moderate masses of buffer molecules the error of one-dimensional approximation is found not to exceed 5%.

physics.optics↗

arXiv2006

Efficient numerical method of the fiber Bragg grating synthesis

A new numerical method is developed for solution of the Gel'fand - Levitan - Marchenko inverse scattering integral equations. The method is based on the fast inversion procedure of a Toeplitz Hermitian matrix and special bordering technique. The method is highly competitive with the known discrete layer peeling method in speed and exceeds it noticeably in accuracy at high reflectance.

physics.optics↗

arXiv2006

Group delay in Bragg grating with linear chirp

An analytic solution for Bragg grating with linear chirp in the form of confluent hypergeometric functions is analyzed in the asymptotic limit of long grating. Simple formulas for reflection coefficient and group delay are derived. The simplification makes it possible to analyze irregularities of the curves and suggest the ways of their suppression. It is shown that the increase in chirp at fixed other parameters decreases the oscillations in the group delay, but gains the oscillations in the reflection spectrum. The conclusions are in agreement with numerical calculations.

physics.optics↗

arXiv2005

An assessment of the resolution limitation due to radiation-damage in x-ray diffraction microscopy

X-ray diffraction microscopy (XDM) is a new form of x-ray imaging that is being practiced at several third-generation synchrotron-radiation x-ray facilities. Although only five years have elapsed since the technique was first introduced, it has made rapid progress in demonstrating high-resolution threedimensional imaging and promises few-nm resolution with much larger samples than can be imaged in the transmission electron microscope. Both life- and materials-science applications of XDM are intended, and it is expected that the principal limitation to resolution will be radiation damage for life science and the coherent power of available x-ray sources for material science. In this paper we address the question of the role of radiation damage. We use a statistical analysis based on the so-called "dose fractionation theorem" of Hegerl and Hoppe to calculate the dose needed to make an image of a lifescience sample by XDM with a given resolution. We conclude that the needed dose scales with the inverse fourth power of the resolution and present experimental evidence to support this finding. To determine the maximum tolerable dose we have assembled a number of data taken from the literature plus some measurements of our own which cover ranges of resolution that are not well covered by reports in the literature. The tentative conclusion of this study is that XDM should be able to image frozen-hydrated protein samples at a resolution of about 10 nm with "Rose-criterion" image quality.

physics.optics↗

arXiv1997

Strong nonlinear regime of resonant four-wave mixing in a gas

The explicit solution is obtained for Raman four-wave mixing $ω_4=ω_1-ω_2+ω_3$ of two strong fields $E_1, E_3$ and two weak fields $E_2, E_4$ in a four-level system with the large Doppler broadening. The resonance of the mixing coefficient vs intensity is found near equal Rabi frequencies of strong fields and interpreted as an intersection of quasi-energy levels. Up to 6 peaks appear in the dependence of conversion coefficient on the detuning of the probe field. An unexpected additional pair of peaks is a result of averaging over velocities and disappears at low temperature. The effects allow explaining saturation behavior in recent experiments on the mixing in sodium molecular vapor.

physics.atom-ph↗

arXiv1996

Giant Coulomb broadening and Raman lasing on ionic transitions

CW generation of anti-Stokes Raman laser on a number of blue-green argon-ion lines (4p-4s, 4p-3d) has been demonstrated with optical pumping from metastable levels 3d'^2G, 3d^4F. It is found, that the population transfer rate is increased by a factor of 3-5 (and hence, the output power of such Raman laser) owing to Coulomb diffusion in the velocity space. Measured are the excitation and relaxation rates for the metastable level. The Bennett hole on the metastable level has been recorded using the probe field technique. It has been shown that the Coulomb diffusion changes shape of the contour to exponential cusp profile while its width becomes 100 times the Lorentzian one and reaches values close to the Doppler width. Such a giant broadening is also confirmed by the shape of the absorption saturation curve.

atom-ph↗

arXiv1995

Narrowing of Bennett Hole in Collisional Plasma

The profile of a Bennett hole induced by laser field in ionic distribution in collisional plasma is calculated. Influence of Chandrasekhar's dependence of coefficients of velocity space transport on the profile is included into the calculation for the first time. It is found that the hole narrows down as the field detuning frequency increases. Physical cause of the effect is the falling dependence of Coulomb collision frequency on the ionic velocity. Estimations show that the effect is quite observable under conditions of high-current gas-discharge plasma.

plasm-ph↗