arXiv subjects
Publications and source records attributed to D. Brinkmann.
A two-band model of a disordered semiconductor is used to analyze dynamical interaction induced weakening of localization in a system that is accessible to experimental verification. The results show a dependence on the sign of the two-particle interaction and on the optical excitation energy of the Coulomb-correlated electron-hole pair.
We present a 17O nuclear magnetic resonance study in the stoichiometric superconductor YBa_2Cu_4O_8. A double irradiation method enables us to show that, below around 180 K, the spin-lattice relaxation rate of plane oxygen is not only driven by magnetic, but also significantly by quadrupolar fluctuations, i.e. low-frequency charge fluctuations. In the superconducting state, on lowering the temperature, the quadrupolar relaxation diminishes faster than the magnetic one. These findings show that, with the opening of the pseudo spin gap, a charge degree of freedom of mainly oxygen character is present in the electronic low-energy excitation spectrum.
We present a NMR pulse double-irradiation method which allows one to separate magnetic from quadrupolar contributions in the spin-lattice relaxation. The pulse sequence fully saturates one transition while another is observed. In the presence of a Delta m = 2 quadrupolar contribution, the intensity of the observed line is altered compared to a standard spin-echo experiment. We calculated analytically this intensity change for spins I=1, 3/2, 5/2, thus providing a quantitative analysis of the experimental results. Since the pulse sequence we used takes care of the absorbed radio-frequency power, no problems due to heating arise. The method is especially suited when only one NMR sensitive isotope is available. Different cross-checks were performed to prove the reliability of the obtained results. The applicability of this method is demonstrated by a study of the plane oxygen 17O (I = 5/2) in the high-temperature superconductor YBa_2Cu_4O_8: the 17O spin-lattice relaxation rate consists of magnetic as well as quadrupolar contributions.
We report measurements of the Gaussian contribution, T_{2G}, to the plane ^{63}Cu nuclear spin--spin relaxation time in the YBa_2Cu_3O_7 and YBa_2Cu_4O_8 blocks of normal and superconducting Y_2Ba_4Cu_7O_{15}. The data confirm our previous results that adjacent CuO_2 planes have different doping levels and that these planes are strongly coupled. -- The static spin susceptibility at the anti-ferromagnetic wave vector exhibits a Curie--Weiss like temperature dependence in the normal state. -- The Y_2Ba_4Cu_7O_{15} data are incompatible with a phase diagram based on a single CuO_2 plane theory and suggest that the appearance of a spin gap implies interplane coupling. Additional data for YBa_2Cu_4O_8 and YBa_2Cu_3O_{6.982} are in accord with the single plane theory. -- The temperature dependence of T_{2G,ind} below T_c excludes isotropic s-wave superconductivity in all three compounds.