arXiv subjects

D. C. Ralph

Publications and source records attributed to D. C. Ralph.

At least 55 records · Page 3Linked to original sources

arXiv2012

Spin torque switching with the giant spin Hall effect of tantalum

We report a giant spin Hall effect (SHE) in β-Ta that generates spin currents intense enough to induce efficient spin-transfer-torque switching of ferromagnets, thereby providing a new approach for controlling magnetic devices that can be superior to existing technologies. We quantify this SHE by three independent methods and demonstrate spin-torque (ST) switching of both out-of-plane and in-plane magnetized layers. We implement a three-terminal device that utilizes current passing through a low impedance Ta-ferromagnet bilayer to effect switching of a nanomagnet, with a higher-impedance magnetic tunnel junction for read-out. The efficiency and reliability of this device, together with its simplicity of fabrication, suggest that this three-terminal SHE-ST design can eliminate the main obstacles currently impeding the development of magnetic memory and non-volatile spin logic technologies.

cond-mat.mtrl-sci↗

arXiv2012

Review and Analysis of Measurements of the Spin Hall Effect in Platinum

Several different experimental techniques have been used in efforts to measure the spin Hall conductivity and the spin Hall angle in Pt samples at room temperature, with results that disagree by more than a factor of 20, with spin Hall conductivities from 2.4 x 10^4 to 5.1 x 10^5 [hbar/(2e)] (Ohm-m)^-1 and spin Hall angles from 0.0037 to 0.08. We review this work, and analyze possible reasons for the discrepancies. We explain that the smallest values for the spin Hall angle that have been reported, based on measurements of lateral permalloy/copper/platinum devices, are incorrect because the original analyses did not properly take into account that copper layers in these devices will shunt charge current flowing through adjacent platinum wires, thereby greatly reducing the size of the spin-Hall-related signals. We suggest that differences between the results for the spin Hall angle found by other experimental techniques are primarily a consequence of different assumptions about the value of the spin diffusion length in Pt. We present a new measurement of the spin diffusion length in Pt within sputtered Pt/permalloy bilayer thin films at room temperature, finding 1.4 \pm 0.3 nm, a much smaller value than has generally been assumed previously. With this value for the spin diffusion length, the previously-discordant results can be brought into much better agreement, with the result that the spin Hall conductivities are (1.4 - 3.4) x 10^5 [hbar/(2e)] (Ohm-m)^-1 and the spin Hall angles are greater than 0.05. These values are sufficiently large that the spin Hall effect in Pt can be used to generate spin currents and spin transfer torques strong enough for efficient manipulation of magnetic moments in adjacent ferromagnetic layers.

cond-mat.mes-hall↗

arXiv2011

Magnetic switching by spin torque from the spin Hall effect

The spin Hall effect (SHE) generates spin currents within nonmagnetic materials. Previously, studies of the SHE have been motivated primarily to understand its fundamental origin and magnitude. Here we demonstrate, using measurement and modeling, that in a Pt/Co bilayer with perpendicular magnetic anisotropy the SHE can produce a spin transfer torque that is strong enough to efficiently rotate and reversibly switch the Co magnetization, thereby providing a new strategy both to understand the SHE and to manipulate magnets. We suggest that the SHE torque can have a similarly strong influence on current-driven magnetic domain wall motion in Pt/ferromagnet multilayers. We estimate that in optimized devices the SHE torque can switch magnetic moments using currents comparable to those in magnetic tunnel junctions operated by conventional spin-torque switching, meaning that the SHE can enable magnetic memory and logic devices with similar performance but simpler architecture than the current state of the art.

cond-mat.mtrl-sci↗

arXiv2010

Spin Torque Ferromagnetic Resonance Induced by the Spin Hall Effect

We demonstrate that the spin Hall effect in a thin film with strong spin-orbit scattering can excite magnetic precession in an adjacent ferromagnetic film. The flow of alternating current through a Pt/NiFe bilayer generates an oscillating transverse spin current in the Pt, and the resultant transfer of spin angular momentum to the NiFe induces ferromagnetic resonance (FMR) dynamics. The Oersted field from the current also generates an FMR signal but with a different symmetry. The ratio of these two signals allows a quantitative determination of the spin current and the spin Hall angle.

cond-mat.mes-hall↗

arXiv2010

Mechanical Control of Spin States in Spin-1 Molecules and the Underscreened Kondo Effect

The ability to make electrical contact to single molecules creates opportunities to examine fundamental processes governing electron flow on the smallest possible length scales. We report experiments in which we controllably stretch individual cobalt complexes having spin S = 1, while simultaneously measuring current flow through the molecule. The molecule's spin states and magnetic anisotropy were manipulated in the absence of a magnetic field by modification of the molecular symmetry. This control enabled quantitative studies of the underscreened Kondo effect, in which conduction electrons only partially compensate the molecular spin. Our findings demonstrate a mechanism of spin control in single-molecule devices and establish that they can serve as model systems for making precision tests of correlated-electron theories.

cond-mat.mes-hall↗

arXiv2009

Ultrafast switching of a nanomagnet by a combined out-of-plane and in-plane polarized spin-current pulse

We report on spin valve devices that incorporate both an out-of-plane polarizer (OPP) to quickly excite spin torque (ST) switching and an in-plane polarizer/analyzer (IPP). For pulses < 200 ps we observe reliable precessional switching due largely to ST from the OPP. Compared to a conventional spin valve, for a given current in the short pulse regime the addition of the OPP can decrease the pulse width necessary for switching by a factor of 10 or more. The influence of the IPP is most obvious at longer, smaller pulses, but also has beneficial ST consequences for short pulse switching.

cond-mat.other↗

arXiv2009

Single-shot time-domain studies of spin-torque-driven switching in magnetic tunnel junctions

We report single-shot measurements of resistance versus time for thermally assisted spin-torque-driven switching in magnetic tunnel junctions. We achieve sufficient sensitivity to resolve the resistance signals leading up to switching, including the variations between individual switching events. Analyses of pre-switching thermal fluctuations allow detailed measurements of coherence times and variations in magnetization precession amplitude. We find that with a small in-plane hard-axis magnetic field the magnetization dynamics are more spatially coherent than for the case of zero field.

cond-mat.mes-hall↗

arXiv2009

Sensitivity of spin-torque diodes for frequency-tunable resonant microwave detection

We calculate the efficiency with which magnetic tunnel junctions can be used as resonant detectors of incident microwave radiation via the spin-torque diode effect. The expression we derive is in good agreement with the sensitivities we measure for MgO-based magnetic tunnel junctions with an extended (unpatterned) magnetic pinned layer. However, the measured sensitivities are reduced below our estimate for a second set of devices in which the pinned layer is a patterned synthetic antiferromagnet (SAF). We suggest that this reduction may be due to an undesirable coupling between the magnetic free layer and one of the magnetic layers within the etched SAF. Our calculations suggest that optimized tunnel junctions should achieve sensitivities for resonant detection exceeding 10,000 mV/mW.

cond-mat.mes-hall↗

arXiv2009

Bias and angular dependence of spin-transfer torque in magnetic tunnel junctions

We use spin-transfer-driven ferromagnetic resonance (ST-FMR) to measure the spin-transfer torque vector T in MgO-based magnetic tunnel junctions as a function of the offset angle between the magnetic moments of the electrodes and as a function of bias, V. We explain the conflicting conclusions of two previous experiments by accounting for additional terms that contribute to the ST-FMR signal at large |V|. Including the additional terms gives us improved precision in the determination of T(V), allowing us to distinguish among competing predictions. We determine that the in-plane component of has a weak but non-zero dependence on bias, varying by 30-35% over the bias range where the measurements are accurate, and that the perpendicular component can be large enough to be technologically significant. We also make comparisons to other experimental techniques that have been used to try to measure T(V).

cond-mat.other↗

arXiv2009

Spin Transfer Torques

This tutorial article introduces the physics of spin transfer torques in magnetic devices. We provide an elementary discussion of the mechanism of spin transfer torque, and review the theoretical and experimental progress in this field. Our intention is to be accessible to beginning graduate students. This is the introductory paper for a cluster of "Current Perspectives" articles on spin transfer torques published in volume 320 of the Journal of Magnetism and Magnetic Materials. This article is meant to set the stage for the others which follow it in this cluster; they focus in more depth on particularly interesting aspects of spin-torque physics and highlight unanswered questions that might be productive topics for future research.

cond-mat.other↗

arXiv2008

Measurement of discrete energy-level spectra in individual chemically-synthesized gold nanoparticles

We form single-electron transistors from individual chemically-synthesized gold nanoparticles, 5-15 nm in diameter, with monolayers of organic molecules serving as tunnel barriers. These devices allow us to measure the discrete electronic energy levels of individual gold nanoparticles that are, by virtue of chemical synthesis, well-defined in their composition, size and shape. We show that the nanoparticles are non-magnetic and have spectra in good accord with random-matrix-theory predictions taking into account strong spin-orbit coupling.

cond-mat.mes-hall↗

arXiv2008

Spin-Torque-Induced Rotational Dynamics of a Magnetic Vortex Dipole

We study, both experimentally and by numerical modeling, the magnetic dynamics that can be excited in a magnetic thin-film nanopillar device using the spin torque from a spatially localized current injected via a 10s-of-nm-diameter aperture. The current-driven magnetic dynamics can produce large amplitude microwave emission at zero magnetic field, with a frequency well below that of the uniform ferromagnetic resonance mode. Micromagnetic simulations indicate that the physical origin of this efficient microwave nano-oscillator is the nucleation and subsequent steady-state rotational dynamics of a magnetic vortex dipole driven by the localized spin torque. These results show this novel implementation of a spintronic nano-oscillator is a promising candidate for microwave technology applications.

cond-mat.mes-hall↗

arXiv2008

Resonant Spin-Transfer-Driven Switching of Magnetic Devices Assisted by Microwave Current Pulses

The torque generated by the transfer of spin angular momentum from a spin-polarized current to a nanoscale ferromagnet can switch the orientation of the nanomagnet much more efficiently than a current-generated magnetic field, and is therefore in development for use in next-generation magnetic random access memory (MRAM). Up to now, only DC currents and square-wave current pulses have been investigated in spin-torque switching experiments. Here we present measurements showing that spin transfer from a microwave-frequency pulse can produce a resonant excitation of a nanomagnet and lead to improved switching characteristics in combination with a square current pulse. With the assistance of a microwave-frequency pulse, the switching time is reduced and achieves a narrower distribution than when driven by a square current pulse alone, and this can permit significant reductions in the integrated power required for switching. Resonantly excited switching may also enable alternative, more compact MRAM circuit architectures.

cond-mat.other↗

arXiv2008

Strong linewidth variation for spin-torque nano-oscillators as a function of in-plane magnetic field angle

We measure the microwave signals produced by spin-torque-driven magnetization dynamics in patterned magnetic multilayer devices at room temperature, as a function of the angle of a magnetic field applied in the sample plane. We find strong variations in the frequency linewidth of the signals, with a decrease by more than a factor of 20 as the field is rotated from the magnetic easy axis to the in-plane hard axis. Based on micromagnetic simulations, we identify these variations as due to a transition from spatially incoherent to coherent precession.

cond-mat.other↗

arXiv2008

Magnetoresistance and spin-transfer torque in magnetic tunnel junctions

We comment on both recent progress and lingering puzzles related to research on magnetic tunnel junctions (MTJs). MTJs are already being used in applications such as magnetic-field sensors in the read heads of disk drives, and they may also be the first device geometry in which spin-torque effects are applied to manipulate magnetic dynamics, in order to make nonvolatile magnetic random access memory. However, there remain many unanswered questions about such basic properties as the magnetoresistance of MTJs, how their properties change as a function of tunnel-barrier thickness and applied bias, and what are the magnitude and direction of the spin-transfer-torque vector induced by a tunnel current.

cond-mat.other↗

arXiv2008

Coupling of Spin and Orbital Motion of Electrons in Carbon Nanotubes

Electrons in atoms possess both spin and orbital degrees of freedom. In non-relativistic quantum mechanics, these are independent, resulting in large degeneracies in atomic spectra. However, relativistic effects couple the spin and orbital motion leading to the well-known fine structure in their spectra. The electronic states in defect-free carbon nanotubes (NTs) are widely believed to be four-fold degenerate, due to independent spin and orbital symmetries, and to also possess electron-hole symmetry. Here we report measurements demonstrating that in clean NTs the spin and orbital motion of electrons are coupled, thereby breaking all of these symmetries. This spin-orbit coupling is directly observed as a splitting of the four-fold degeneracy of a single electron in ultra-clean quantum dots. The coupling favours parallel alignment of the orbital and spin magnetic moments for electrons and anti-parallel alignment for holes. Our measurements are consistent with recent theories that predict the existence of spin-orbit coupling in curved graphene and describe it as a spin-dependent topological phase in NTs. Our findings have important implications for spin-based applications in carbon-based systems, entailing new design principles for the realization of qubits in NTs and providing a mechanism for all-electrical control of spins in NTs.

cond-mat.mes-hall↗

arXiv2007

Enhancement in spin-torque efficiency by nonuniform spin current generated within a tapered nanopillar spin valve

We examine the effect a spatially non-uniform spin current with a component polarized partially out of the plane has on a low saturation magnetization nanomagnet free layer. Micromagnetic simulations indicate that the spin torque efficiency acting upon the reversing nanomagnet can be enhanced through this process, resulting in faster switching with smaller currents. In doing so, we determine that micromagnetic structure within the nanomagnets can be beneficial for reversal processes. We verify this enhancement experimentally in devices with a tapered nanopillar geometry that generates a spin current polarized partly out of plane. Finally, to take even better advantage of these effects, we examine micromagnetically the benefits of a tapered three-magnetic-layer structure that further reduces reversal times while maintaining the thermal stability of the free layer.

cond-mat.other↗

arXiv2007

Time-Domain Studies of Very-Large-Angle Magnetization Dynamics Excited by Spin Transfer Torques

We describe time-domain measurements which provide new information about the large-angle nonlinear dynamics of nanomagnets excited by spin-transfer torque from a spin-polarized current. Sampling-oscilloscope measurements, which average over thousands of experimental time traces, show that the mean reversal time for spin-transfer-driven magnetic switching has a step-like dependence on magnetic field, because an integer number of precession cycles is required for reversal. Storage-oscilloscope measurements of individual experimental traces reveal non-periodic large-amplitude resistance variations at values of magnetic field and current in a crossover region between the regimes of spin-transfer-driven switching and steady-state precession. We also observe directly the existence of time-dependent switching, on the nanosecond scale, between different precessional modes and between a precessional mode and a static state, at particular values of magnetic field and current bias.

cond-mat.mtrl-sci↗