arXiv subjects

D. C. Schmadel

Publications and source records attributed to D. C. Schmadel.

16 recordsLinked to original sources

arXiv2010

Terahertz Kerr and Reflectivity Measurements on the Topological Insulator Bi2Se3

We report the first terahertz Kerr measurements on bulk crystals of the topological insulator Bi2Se3. At T=10K and fields up to 8T, the real and imaginary Kerr angle and reflectance measurements utilizing both linearly and circularly polarized incident radiation were measured at a frequency of 5.24meV. A single fluid free carrier bulk response can not describe the line-shape. Surface states with a small mass and surprisingly large associated spectral weight quantitatively fit all data. However, carrier concentration inhomogeneity has not been ruled out. A method employing a gate is shown to be promising for separating surface from bulk effects.

cond-mat.str-el↗

arXiv2010

Far infrared cyclotron resonance and Faraday effect in Bi2Se3

The complex Faraday angle and transmission for the topological insulator Bi2Se3 were measured in the far infrared in magnetic fields up to 8 T and analyzed in terms of a simple Drude-Lorentz magneto-plasma dielectric model. Bulk carriers dominate the optical response. The bulk carriers are electrons as we determined from the sign of the Faraday angle. We obtain the bulk band edge cyclotron mass m_cb = 0.16 +- 0.01 m_e and free electron concentration in the 10^17 range. Electron-phonon interaction effects were found to be weak.

cond-mat.str-el↗

arXiv2010

Terahertz Hall Measurements On Optimally Doped Single Crystal Bi-2212

The infrared Hall angle in optimally doped single crystal $\rm Bi_2 Sr_2 Ca Cu_2 O_{8+x}$ was measured from 3.05 to 21.75 meV as a continuous function of temperature from 25 to 300\,K. In the normal state, the temperature dependence of the real part of the cotangent of the infrared Hall angle obeys the same power law as dc measurements. The measured Hall frequency $\rm ω_H$ is significantly larger than the expected value based upon ARPES data analyzed in terms of the relaxation time approximation. This discrepancy as well as the temperature dependence of $\rm Re(\cot{θ_H})$ and $ω_H$ is well described by a Fermi liquid theory in which current vertex corrections produced by electron-magnon scattering are included.

cond-mat.supr-con↗

arXiv2010

Simultaneous measurement of circular dichroism and Faraday rotation at terahertz frequencies using heterodyne detection

A far-infrared system measures the full complex Faraday angle, rotation as well as ellipticity, with an unprecedented accuracy of 10\,$μ$rad/T. The system operates on several far-infrared laser lines in the spectral range from 0.3 to 6 THz and produces results as a continuous function of temperature from 10 to 310K and applied fields between $\pm$ 8\,T. Materials successfully measured include GaAs 2-DEG heterostructures, various high temperature superconductors including Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$, Pr$_{2 - x}$Ce$_{x}$CuO$_4$, and La$_{2-x}$Sr$_x$CuO$_4$, and single crystals of the topological insulator Bi$_2$Se$_3$.

cond-mat.str-el↗

arXiv2009

Origin of the anomalous Hall Effect in overdoped n-type cuprates: current vertex corrections due to antiferromagnetic fluctuations

The anomalous magneto-transport properties in electron doped (n-type) cuprates were investigated using Hall measurements at THz frequencies. The complex Hall angle was measured in overdoped Pr$_{\rm 2-x}$Ce$_{\rm x}$CuO$_{\rm 4}$ samples (x=0.17 and 0.18) as a continuous function of temperature above $T_c$ at excitation energies 5.24 and 10.5 meV. The results, extrapolated to low temperatures, show that inelastic scattering introduces electron-like contributions to the Hall response. First principle calculations of the Hall angle that include current vertex corrections (CVC) induced by electron interactions mediated by magnetic fluctuations in the Hall conductivity reproduce the temperature, frequency, and doping dependence of the experimental data. These results show that CVC effects are the source of the anomalous Hall transport properties in overdoped n$\text{-}$type cuprates.

cond-mat.supr-con↗

arXiv2009

Terahertz magneto-transport measurements in underdoped PCCO and comparison with ARPES

We present magneto-transport measurements performed on underdoped PCCO at THz frequencies as a function of temperature and doping. A rapidly decreasing Hall mass is observed as the doping is reduced consistent with the formation of small electron Fermi pockets. However, both dc and infrared (IR) magneto-transport data strongly deviate from the predictions of transport theory in the relaxation time approximation (RTA) based on angular resolved photoemission data. The Hall mass is observed to increase continuously with increasing temperature with no signature at the Neel temperature. In the paramagnetic state, the temperature dependence of the Hall mass is consistent with current vertex corrections to the Hall conductivity due to magnetic fluctuations as observed in overdoped PCCO. Possible causal mechanisms for the discrepancy between transport theory within the RTA and the magneto-transport data are discussed.

cond-mat.supr-con↗

arXiv2007

Silicon beamsplitter for Fourier transform spectroscopy at far infrared frequencies

We report the performance of a silicon wafer beamsplitter for use for low $Δν>0.3 cm^{-1}$ resolution Fourier transform spectroscopy at far infrared frequencies. We characterize the Si beamsplitter by comparing throughput spectra measured with it to those measured with the standard Mylar beamsplitters commonly used in that range. We find that the throughput of the silicon beamsplitter is substantially greater than that of the Mylar beamsplitters over most of the IR spectrum, and that they are comparable in some limited ranges. The 2 mm silicon beamsplitter has an etalon spacing of about 0.7 cm^{-1}, which interferes with its use for $0.1 cm^{-1}<Δν< 0.3cm^{-1}$. The average efficiency of the Si beamsplitter is 0.37 compared with a maximum efficiency of 0.35 for Mylar. The Si is particularly more efficient in the 100 to 400 cm^{-1} range because of absorption in Mylar.

physics.ins-det↗

arXiv2006

Infrared Hall Effect in the electron-doped high Tc cuprate Pr(2-x)Ce(x)CuO(4)

The electron-doped cuprate Pr(2-x)Ce(x)CuO(4) is investigated using infrared magneto-optical measurements. The optical Hall conductivity sigma_{xy} shows a strong doping, frequency and temperature dependence consistent with the presence of a temperature and doping-dependent coherent backscattering amplitude which doubles the electronic unit cell. The data suggest that the coherent backscattering vanishes at a quantum critical point inside the superconducting dome and is associated with the commensurate antiferromagnetic order observed by other workers. Using a spectral weight analysis we have further investigated the Fermi-liquid like behavior of the overdoped sample. The observed Hall-conductance spectral weight is about 10 times less than that predicted by band theory, raising the fundamental question concerning the effect of Mott and antiferromagnetic correlations on the Hall conductance of strongly correlated materials.

cond-mat.supr-con↗

arXiv2006

The infrared Hall conductivity in optimally-doped BSCCO

he frequency dependence in the mid IR from 900 to 1100 cm$^{-1}$ and far IR at 84 cm$^{-1}$ and temperature dependence from 35 to 330 K of the normal state Hall transport is reported in single crystal, optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. The results show a nearly Drude behavior in the Hall conductivity $σ_{xy}$, which stands in contrast to the more complex extended Drude behavior for the longitudinal conductivity $σ_{xx}$. The mid IR Hall scattering rate increases linearly with temperature and has a small, positive, projected intercept of 200 cm$^{-1}$ at T=0. In contrast, the longitudinal scattering rate is much larger and exhibits very little temperature dependence. The spectral weight of $σ_{xy}$ is suppressed to 0.09 times the band value, whereas the spectral weight of $σ_{xx}$ is 0.33 times the band value. These disparate behaviors are consistent with calculations based on the fluctuation-exchange interaction when current vertex corrections are included.

cond-mat.supr-con↗

arXiv2006

The mid-infrared Hall effect in optimally-doped Bi_2 Sr_2 CaCu_2 O_{8+δ}

Heterodyne polarometry is used to measure the frequency dependence in the mid IR from 900 to 1100 cm$^-1$ and temperature dependence from 35 to 330 K of the normal state Hall transport in single crystal, optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. The results show a simple Drude behavior in the Hall conductivity $σ_{xy}$ which stands in contrast to the more complex, extended Drude behavior for the longitudinal conductivity $σ_{xx}$. The mid IR Hall scattering rate $γ_{xy}$ increases linearly with temperature and has a small, positive, projected intercept at T=0. The longitudinal scatter rate, in contrast, is much larger and exhibits very little temperature dependnece. The Hall frequency indicates a carrier mass which is 6.7 times the band mass and which decreases slighly with increasing frequency. These disparate behaviors are consistent with calculations based on the fluctuation-exchange interaction using current vertex corrections.

cond-mat.str-el↗

arXiv2003

Magneto-optical evidence for a gapped Fermi surface in underdoped YBa2Cu3O6+x

The infrared (900-1100 cm-1) Faraday rotation and circular dichroism are measured in the normal state of underdoped High Tc superconductors and used to study the magneto-transport. YBa2Cu3O6+x thin films are investigated in the temperature range 10-300 K in magnetic fields up to 8 Tesla and as a function of oxygen concentration. A dramatic increase of the Hall frequency is observed for underdoped samples which is not consistent with the approach to a Mott transition but is consistent with a partial gapping of the Fermi surface as predicted in charge density wave models.

cond-mat.supr-con↗

arXiv2002

The mid-infrared AC Hall effect in optimally-doped BSCCO

A novel heterodyne polarimetry system determines the frequency dependence from 900 to 1100 cm^-1 and temperature dependence from 35 to 330 K of the Hall transport in single crystal, optimally doped BSCCO. The results show a significant disconnect from the behavior of the Hall angle in the existing data for YBCO in the far-infrared, which indicate a negative value for the real part of the Hall angle above 250 cm^-1, whereas that of the current work at 1000 cm^-1 is positive. The current work when analyzed using an extended Drude formalism results in a Hall mass comparable to the ARPES Fermi mass and a scattering rate comparable to the low frequency conductivity and Hall effect scattering rates, which, however, are only 1/4 of the ARPES values.

cond-mat.supr-con↗

arXiv2002

Measurement of the complex Faraday angle in thin-film metals and high temperature superconductors

A sensitive polarization modulation technique uses photoelastic modulation and hetrodyne detection to simultaneously measure the Faraday rotation and induced ellipticity in light transmitted by semiconducting and metallic samples. The frequencies measured are in the mid-infrared and correspond to the spectral lines of a CO2 laser. The measured temperature range is continuous and extends from 35 to 330K. Measured samples include GaAs and Si substrates, gold and copper films, and YBCO and BSCCO high temperature superconductors.

cond-mat.supr-con↗

arXiv2002

Spectral measurement of the Hall angle response in normal state cuprate superconductors

We measure the temperature and frequency dependence of the complex Hall angle for normal state YBa$_2$Cu$_3$O$_7$ films from dc to far-infrared frequencies (20-250 cm$^{-1}$) using a new modulated polarization technique. We determine that the functional dependence of the Hall angle on scattering does not fit the expected Lorentzian response. We find spectral evidence supporting models of the Hall effect where the scattering $Γ_H$ is linear in T, suggesting that a single relaxation rate, linear in temperature, governs transport in the cuprates.

cond-mat.supr-con↗

arXiv1999

Infrared Hall effect in high Tc superconductors: Evidence for non-Fermi liquid Hall scattering

Infrared (20-120 cm-1 and 900-1100 cm-1) Faraday rotation and circular dichroism are measured in high Tc superconductors using sensitive polarization modulation techniques. Optimally doped YBCO thin films are studied at temperatures down to 15 K and magnetic fields up to 8 T. At 1000 cm-1 the Hall conductivity varies strongly with temperature in contrast to the longitudinal conductivity which is nearly independent of temperature. The Hall scattering rate has a T^2 temperature dependence but, unlike a Fermi liquid, depends only weakly on frequency. The experiment puts severe constraints on theories of transport in the normal state of high Tc superconductors.

cond-mat.supr-con↗

arXiv1999

Mid-infrared Hall effect in thin-film metals: Probing the Fermi surface anisotropy in Au and Cu

A sensitive mid-infrared (MIR, 900-1100 cm-1, 112-136 meV) photo-elastic polarization modulation technique is used to measure simultaneously Faraday rotation and circular dichroism in thin metal films. These two quantities determine the complex AC Hall conductivity. This novel technique is applied to study Au and Cu thin films at temperatures down to 20 K and magnetic fields up to 8 T. The Hall frequency is consistent with band theory predictions. We report the first measurement of the MIR Hall scattering rate, which is significantly lower than that derived from Drude analysis of zero magnetic field MIR transmission measurements. This difference is qualitatively explained in terms of the anisotropy of the Fermi surface in Au and Cu.

cond-mat.mtrl-sci↗