arXiv subjects

D. Cano-Ott

Publications and source records attributed to D. Cano-Ott.

At least 19 recordsLinked to original sources

arXiv2026

Improved $^{94}$Mo neutron resonance parameters from neutron capture and transmission measurements at n_TOF and GELINA

We report high-resolution measurements of the $^{94}\mathrm{Mo}(\mathrm{n},\gamma)^{95}\mathrm{Mo}$ cross section in the neutron energy range from a few eV up to about 250 keV, performed at the n_TOF facility (CERN), and of the $^{94}\mathrm{Mo}(\mathrm{n},\mathrm{tot})$ cross section up to 32 keV, measured at GELINA (JRC Geel). A combined R-matrix analysis of capture and transmission data yields significantly improved neutron-resonance parameters for $^{94}$Mo. A total of 186 resonances were observed in this analysis of which 127 reported here for the first time. The resulting Maxwellian-averaged cross section at stellar temperatures relevant to the slow neutron-capture process (s-process) is approximately 25% lower than previous evaluations and literature values. To assess the astrophysical impact of the revised cross section, we performed s-process nucleosynthesis calculations for low-mass asymptotic giant branch stars. Despite the substantial reduction in the $^{94}\mathrm{Mo}(\mathrm{n},\gamma)^{95}\mathrm{Mo}$ rate, the final yields vary by only 3-4%. This demonstrates that the isotopic budget of $^{94}$Mo in AGB stars is primarily governed by the branching flow at $^{94}\mathrm{Nb}$ rather than by the neutron-capture destruction on $^{94}$Mo itself. The new cross section thus helps disentangle nuclear cross-section uncertainties from branching-flow effects in the s-process production of $^{94}$Mo.

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arXiv2026

Environmental $\gamma$-Ray Flux in Hall C at LNGS and Its Correlation with Radon Activity

We report a comprehensive measurement of the environmental $\gamma$-ray flux in Hall C of the Gran Sasso National Laboratory. A spatial mapping of the radiation was carried out using a high-purity germanium detector mounted on a movable cart and deployed at eight locations within the hall. The detector response function and full-energy-peak efficiencies were determined through Geant4 simulations validated with calibrated $\gamma$-ray sources, with particular attention devoted to the efficiency modeling and associated systematic uncertainties. In the energy range of 57-2800 keV, the average $\gamma$-ray flux is measured to be $(\mathrm{0.46} \pm \mathrm{0.06}_{stat} \pm \mathrm{0.03}_{syst})$ $\mathrm{cm}^{-2}$ $\mathrm{s}^{-1}$. The radon level was monitored for about a month using a radon detector mounted on the same cart, and a clear correlation is observed between the environmental $\gamma$-ray rate and the ambient radon concentration, consistent with the short-lived daughters of $^{222}\mathrm{Rn}$. This result represents the first high-precision and efficiency-corrected mapping of the $\gamma$-ray flux in Hall C, substantially improving its radiological characterization and providing key input for future rare-event experiments operating in this hall.

physics.ins-det↗

arXiv2026

Energy-differential measurement of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions at the n_TOF facility at CERN

Energy-differential cross section of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions was measured at the neutron time of flight facility n_TOF at CERN. The measurement was performed in the first experimental area (EAR1; flight path of 182.5 m). Two position-sensitive $\Delta E$-$E$ silicon telescopes were used. Two naturally occurring carbon isotopes, $^{12}$C and $^{13}$C, contribute to the reactions on natural carbon, with the (n,p) reaction threshold at 13.7 MeV and the (n,d) threshold at 14.9 MeV (determined by the $^{12}$C isotope for both reactions). This paper provides the details of the analysis leading to the final results published previously as a Letter. The cross section results are reported up to 25 MeV. During the data analysis the population of the excited states in the daughter nuclei $^{11}$B, $^{12}$B, $^{13}$B had to be considered, requiring the adoption of the branching ratios and angular distributions of the emitted particles from an external source of information. TALYS-2.0 calculations were used as the main source and an in-depth analysis of the model-related uncertainties was performed. The n_TOF results are largely inconsistent with the major evaluation libraries. On the other hand, an unexpected agreement is found with TALYS-2.0 calculations. Specifically, the obtained cross section for the (n,p) reaction is significantly higher than in the available evaluations, fully supporting the earlier finding from an integral measurement at n_TOF.

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arXiv2026

First $^{94}$Nb($n,\gamma$) Measurement: Constraining the Nucleosynthetic Origin of $^{94}$Mo in Presolar Grains

Isotopic measurements of presolar silicon carbide grains from dying stars have revealed a puzzling overabundance of $^{94}$Mo that stellar nucleosynthesis models have failed to reproduce for two decades. This discrepancy challenged our understanding of the slow neutron-capture process ($s$-process) that forges approximately half of the elements heavier than iron. The key uncertainty lies at $^{94}$Nb, a radiactive branching point where competition between neutron capture and beta decay governs the $^{94}$Mo production, yet the neutron-capture cross section had never been measured. Here we report the first experimental determination of the $^{94}$Nb(n,$\gamma$)$^{95}$Nb cross section important for Mo isotopic abundances. The measurement was enabled by a coordinated effort involving high-purity target preparation at Institute of Solid State and Materials Research (IFW) Dresden, radioactive sample production at the Institut Laue-Langevin (ILL) Grenoble, radiochemical characterization at Paul Scherrer Institute (PSI) Villigen, and the Time-of-Flight CERN n$\_$TOF facility using for the first time segmented total-energy detectors. Incorporation of the resulting Maxwellian-averaged cross section into fully coupled nucleosynthesis models of low-mass asymptotic giant branch (AGB) stars brings them into agreement with the presolar grain data. These results remove a major nuclear-physics input uncertainty at the $^{94}$Nb branching point and provide a firmer foundation for understanding the origin of $^{94}$Mo in the solar system.

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arXiv2025

Status of the HENSA collaboration at the Canfranc Underground Laboratory: results from two years of measurement of the neutron flux in hall B

Thiswork deals with the characterization of the neutron flux in hall B of the CanfrancUnderground Laboratory (LSC) employing the High Efficiency Neutron Spectrometry Array (HENSA). The ultimate goal of this measurement is to set a limit on the corresponding effects of the neutron flux in the background of the ANAIS-112 experiment. The preliminary neutron counting rates of two years of measurement are reported. Various data analysis techniques, including pulse shape discrimination, are discussed. The first results on the spectral reconstruction of the neutron flux are also presented.

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arXiv2025

Measurement of the $^\text{nat}$C(n,p) and $^\text{nat}$C(n,d) reactions from n_TOF at CERN

The energy dependence of the cross section of the (n,p) and (n,d) reactions on $^\text{nat}$C has been studied for the first time at the n_TOF facility at CERN, from the particle detection threshold up to 25 MeV. The measurement was performed with two telescopes made of position-sensitive silicon $\Delta E$-$E$ detectors, covering the angular range from 20{\deg} to 140{\deg}. A detector efficiency has been determined by means of Monte Carlo simulations of the experimental setup. Various assumptions on the angular distributions and branching ratios of the excited levels of the residual $^{11}$B, $^{12}$B, $^{13}$B nuclei were considered. In particular, theoretical calculations based on the TALYS-2.0 code were used and the systematic uncertainties in the analysis results were determined from the variations in these distributions. The n_TOF data on the (n,p) and (n,d) reaction on carbon are characterized by a higher accuracy and wider energy range than currently available in literature. A comparison with current evaluations from different libraries reveals a rather significant disagreement with the n_TOF results, while a remarkable agreement is observed with the prediction of TALYS-2.0 for this light element.

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arXiv2025

Neutron capture measurements for s-process nucleosynthesis; A review about CERN n_TOF developments and contributions

This article presents a review about the main CERN n\_TOF contributions to the field of neutron-capture experiments of interest for $s$-process nucleosynthesis studies over the last 25 years, with special focus on the measurement of radioactive isotopes. A few recent capture experiments on stable isotopes of astrophysical interest are also discussed. Results on $s$-process branching nuclei are appropriate to illustrate how advances in detection systems and upgrades in the facility have enabled increasingly challenging experiments and, as a consequence, have led to a better understanding and modeling of the $s$-process mechanism of nucleosynthesis. New endeavors combining radioactive-ion beams from ISOLDE for the production of radioisotopically pure samples for activation experiments at the new NEAR facility at n\_TOF are briefly discussed. On the basis of these new exciting results, also current limitations of state-of-the-art TOF and activation techniques will be depicted, thereby showing the pressing need for further upgrades and enhancements on both facilities and detection systems. A brief account of the potential technique based on inverse kinematics for direct neutron-capture measurements is also presented.

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arXiv2025

$\beta$-delayed neutron spectroscopy of $^{85, 86}$As with MONSTER at IGISOL

The $\beta$-delayed neutron emission in the $^{85, 86}$As $\beta$-decays has been measured at the Ion Guide Isotope Separator On Line facility of the Accelerator Laboratory of the University of Jyv\"askyl\"a. The complete $\beta$-decays have been studied with a complex setup that consists of a plastic scintillator for $\beta$-particles, MONSTER -- the MOdular Neutron time-of-flight SpectromeTER -- for neutrons, and a high-purity germanium and four LaBr$_3$ crystals for $\gamma$-rays. The $\beta$-delayed neutron energy distributions have been determined by unfolding the time-of-flight spectra with an innovative methodology based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations. The results obtained for $^{85}$As are in excellent agreement with the existing evaluated data, validating the proposed methodology. In the case of $^{86}$As, a stronger neutron intensity at higher energies than previously predicted is discovered.

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arXiv2024

Radiative neutron capture cross section of $^{242}$Pu measured at n_TOF-EAR1 in the unresolved resonance region up to 600 keV

Accurate neutron capture cross sections are essential for the design and operation of fast reactors using MOX fuels. For $^{242}$Pu, the Nuclear Energy Agency (NEA) recommends 8--12% accuracy in the fast energy region (2--500 keV), compared to the current uncertainty of 35%. Moreover, integral experiments and previous measurements suggest the evaluated $^{242}$Pu(n,$\gamma$) cross section is overestimated, particularly in the JEFF-3.3 library, which shows a 14% overestimation between 1 keV and 1 MeV. Recent measurements from LANSCE reported a 20--30% reduction in the 1--40 keV range relative to evaluations. To solve these discrepancies, the $^{242}$Pu(n,$\gamma$) cross section was measured from 1 to 600 keV at CERN n_TOF-EAR1 facility using a 95(4) mg $^{242}$Pu target, enriched to 99.959%. Gamma rays from neutron capture were detected with an array of C$_6$D$_6$ scintillators and a novel application of the Pulse Height Weighting Technique was employed. The resulting cross section presents a systematic uncertainty between 8 and 12%, reducing the current uncertainties of 35\% and achieving the accuracy requested by the NEA. Analysis using FITACS produced average resonance parameters, consistent with the analysis of the resolved resonance region. Our data align well with Wisshak and Kaeppeler, and are 10--14\% lower than JEFF-3.3 in the 1--250 keV range, helping to achieve consistency with integral benchmarks. At higher energies, our results are in reasonable agreement with ENDF/B-VIII.1 and JEFF-3.3. In contrast, DANCE results appear to underestimate the cross section by a factor of 2--3 above a few keV.

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arXiv2024

Towards a new generation of solid total-energy detectors for neutron-capture time-of-flight experiments with intense neutron beams

Challenging neutron-capture cross-section measurements of small cross sections and samples with a very limited number of atoms require high-flux time-of-flight facilities. In turn, such facilities need innovative detection setups that are fast, have low sensitivity to neutrons, can quickly recover from the so-called $\gamma$-flash, and offer the highest possible detection sensitivity. In this paper, we present several steps toward such advanced systems. Specifically, we describe the performance of a high-sensitivity experimental setup at CERN n\_TOF EAR2. It consists of nine sTED detector modules in a compact cylindrical configuration, two conventional used large-volume C$_{6}$D$_{6}$ detectors, and one LaCl$_{3}$(Ce) detector. The performance of these detection systems is compared using $^{93}$Nb($n$,$\gamma$) data. We also developed a detailed \textsc{Geant4} Monte Carlo model of the experimental EAR2 setup, which allows for a better understanding of the detector features, including their efficiency determination. This Monte Carlo model has been used for further optimization, thus leading to a new conceptual design of a $\gamma$ detector array, STAR, based on a deuterated-stilbene crystal array. Finally, the suitability of deuterated-stilbene crystals for the future STAR array is investigaged experimentally utilizing a small stilbene-d12 prototype. The results suggest a similar or superior performance of STAR with respect to other setups based on liquid-scintillators, and allow for additional features such as neutron-gamma discrimination and a higher level of customization capability.

physics.ins-det↗

arXiv2024

Measurement and analysis of the $^{246}$Cm and $^{248}$Cm neutron capture cross-sections at the EAR2 of the n TOF facility

The $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) cross-sections have been measured at the Experimental Area 2 (EAR2) of the n_TOF facility at CERN with three C$_6$D$_6$ detectors. This measurement is part of a collective effort to improve the capture cross-section data for Minor Actinides (MAs), which are required to estimate the production and transmutation rates of these isotopes in light water reactors and innovative reactor systems. In particular, the neutron capture in $^{246}$Cm and $^{248}$Cm open the path for the formation of other Cm isotopes and heavier elements such as Bk and Cf and the knowledge of (n,$\gamma$) cross-sections of these Cm isotopes plays an important role in the transport, transmutation and storage of the spent nuclear fuel. The reactions $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) have been the two first capture measurements analyzed at n_TOF EAR2. Until this experiment and two recent measurements performed at J-PARC, there was only one set of data of the capture cross-sections of $^{246}$Cm and $^{248}$Cm, that was obtained in 1969 in an underground nuclear explosion experiment. In the measurement at n_TOF a total of 13 resonances of $^{246}$Cm between 4 and 400 eV and 5 of $^{248}$Cm between 7 and 100 eV have been identified and fitted. The radiative kernels obtained for $^{246}$Cm are compatible with JENDL-5, but some of them are not with JENDL-4, which has been adopted by JEFF-3.3 and ENDF/B-VIII.0. The radiative kernels obtained for the first three $^{248}$Cm resonances are compatible with JENDL-5, however, the other two are not compatible with any other evaluation and are 20% and 60% larger than JENDL-5.

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arXiv2024

Review of Neutron Yield from (${\alpha}$, n) Reactions: Data, Methods, and Prospects

Understanding the radiogenic neutron production rate through the (${\alpha}$, n) reaction is crucial in many areas of physics, including dark matter searches, neutrino studies, and nuclear astrophysics. In addition to its relevance for fundamental research, the (${\alpha}$, n) reaction also plays a significant role in nuclear energy technologies, for example by contributing to neutron production in subcritical systems using UO$_{2}$, as well as in applications such as medical physics. This review examines the current state of (${\alpha}$, n) yield calculations and neutron spectra, describes the computational tools used for their estimation, and discusses the available cross-section data. We explore the uncertainties affecting (${\alpha}$, n) yield estimations and propose a strategy to enhance their accuracy. Furthermore, this paper discusses and emphasizes the need for new measurements of (${\alpha}$, n) cross-sections for a variety of relevant materials. Such measurements are essential for improving neutron flux predictions, which are crucial for reducing uncertainties in sensitivity estimates for next-generation physics experiments operating in the keV--MeV range.

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arXiv2024

A Segmented Total Energy Detector (sTED) optimized for $(n,\gamma)$ cross-section measurements at n_TOF EAR2

The neutron time-of-flight facility n_TOF at CERN is a spallation source dedicated to measurements of neutron-induced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of $4\times 10^7$ neutrons per nominal proton pulse, which is 50 times higher than the one of Experimental ARea 1 (EAR1) of $8\times10^5$ neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detectors response, by reducing the active volume per module and by using a photomultiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to $\gamma$-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at n_TOF EAR2.

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arXiv2024

Analysis of neutron time-of-flight spectra with a Bayesian unfolding methodology

We have developed an innovative methodology for obtaining the neutron energy distribution from a time-of-flight (TOF) measurement based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations. This methodology has been validated through the analysis of a realistic virtual $\beta$-decay experiment, including the most relevant systematic effects in a real experiment. The proposed methodology allowed for obtaining accurate results over the energy range above the neutron detection threshold.

physics.data-an↗

arXiv2023

Pushing the high count rate limits of scintillation detectors for challenging neutron-capture experiments

One of the critical aspects for the accurate determination of neutron capture cross sections when combining time-of-flight and total energy detector techniques is the characterization and control of systematic uncertainties associated to the measuring devices. In this work we explore the most conspicuous effects associated to harsh count rate conditions: dead-time and pile-up effects. Both effects, when not properly treated, can lead to large systematic uncertainties and bias in the determination of neutron cross sections. In the majority of neutron capture measurements carried out at the CERN n\_TOF facility, the detectors of choice are the C$_{6}$D$_{6}$ liquid-based either in form of large-volume cells or recently commissioned sTED detector array, consisting of much smaller-volume modules. To account for the aforementioned effects, we introduce a Monte Carlo model for these detectors mimicking harsh count rate conditions similar to those happening at the CERN n\_TOF 20~m fligth path vertical measuring station. The model parameters are extracted by comparison with the experimental data taken at the same facility during 2022 experimental campaign. We propose a novel methodology to consider both, dead-time and pile-up effects simultaneously for these fast detectors and check the applicability to experimental data from $^{197}$Au($n$,$γ$), including the saturated 4.9~eV resonance which is an important component of normalization for neutron cross section measurements.

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arXiv2023

New detection systems for an enhanced sensitivity in key stellar (n,$\gamma$) measurements

Neutron capture cross-section measurements are fundamental in the study of astrophysical phenomena, such as the slow neutron capture (s-) process of nucleosynthesis operating in red-giant and massive stars. However, neutron capture measurements via the time-of-flight (TOF) technique on key $s$-process nuclei are often challenging. Difficulties arise from the limited mass ($\sim$mg) available and the high sample-related background in the case of the unstable $s$-process branching points. Measurements on neutron magic nuclei, that act as $s$-process bottlenecks, are affected by low (n,$\gamma$) cross sections and a dominant neutron scattering background. Overcoming these experimental challenges requires the combination of facilities with high instantaneous flux, such as n\_TOF-EAR2, with detection systems with an enhanced detection sensitivity and high counting rate capabilities. This contribution reviews some of the latest detector developments in detection systems for (n,$\gamma$) measurements at n\_TOF, such as i-TED, an innovative detection system which exploits the Compton imaging technique to reduce the dominant neutron scattering background and s-TED, a highly segmented total energy detector intended for high flux facilities. The discussion will be illustrated with results of the first measurement of key the $s$-process branching-point reaction $^{79}$Se(n,$\gamma$).

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arXiv2023

First measurement of the $^{94}$Nb($n$,$γ$) cross section at the CERN n\_TOF facility

One of the crucial ingredients for the improvement of stellar models is the accurate knowledge of neutron capture cross-sections for the different isotopes involved in the $s$-,$r$- and $i$- processes. These measurements can shed light on existing discrepancies between observed and predicted isotopic abundances and help to constrain the physical conditions where these reactions take place along different stages of stellar evolution.In the particular case of the radioactive $^{94}$Nb, the $^{94}$Nb($n$,$γ$) cross-section could play a role in the determination of the $s$-process production of $^{94}$Mo in AGB stars, which presently cannot be reproduced by state-of-the-art stellar models. There are no previous $^{94}$Nb($n$,$γ$) experimental data for the resolved and unresolved resonance regions mainly due to the difficulties in producing high-quality samples and also due to limitations in conventional detection systems commonly used in time-of-flight experiments.Motivated by this situation, a first measurement of the $^{94}$Nb($n$,$γ$) reaction was carried out at CERN n\_TOF, thereby exploiting the high luminosity of the EAR2 area in combination with a new detection system of small-volume C6D6-detectors and a high quality $^{94}$Nb-sample. The latter was based on hyper-pure $^{93}$Nb material activated at the high-flux reactor of ILL-Grenoble. An innovative ring-configuration detection system in close geometry around the capture sample allowed us to significantly enhance the signal-to-background ratio. This set-up was supplemented with two conventional C$_{6}$D$_{6}$ detectors and a high-resolution LaCl$_{3}$(Ce)-detector, which will be employed for addressing reliably systematic effects and uncertainties.At the current status of the data analysis, 18 resonance in $^{94}$Nb+$n$ have been observed for the first time in the neutron energy range from thermal up to 10 keV.

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arXiv2022

Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV

Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,${\alpha}$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.

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