SearcharxivSearch

arXiv subjects

D. Dai

Publications and source records attributed to D. Dai.

2 recordsLinked to original sources

Sign-resolved nanoscale readout and control of hidden antiferromagnetic spin order

Antiferromagnetic memories promise ultrafast, stray-field-free information storage. Yet perfect magnetic compensation conceals the information carrier itself: the sign of the N\'eel vector distinguishing two time-reversed states. Moreover, in future dense memories, the local polarity of N\'eel domains would need to be read out on the nanoscale. We make this hidden polarity visible in a fully-compensated, high-N\'eel-temperature, PT-symmetric antiferromagnet by driving interband electric-dipole transitions by mid-infrared near-fields confined at a scanning probe. The excitation generates a N\'eel-order-dependent quantum-metric photocurrent, a Hall-like signal reversing with N\'eel order, which we term the optical nonlinear anomalous Hall effect. This optically induced electrical readout maps opposite N\'eel polarities with sub-100-nm resolution at room temperature and, combined with spin-orbit-torque writing, reveals N\'eel-texture polarization and reversible domain-wall motion, establishing electrical-write/optoelectronic-read antiferromagnetic functionality.

cond-mat.mtrl-sci

On the Origin of the Metallic and Anisotropic Magnetic Properties of Na_xCoO_2 (x~~0.75)

Non-stoichiometric NaxCoO2 (0.5 < x < 1) consists of CoO2 layers made up of edge-sharing CoO6 octahedra, and exhibits strongly anisotropic magnetic susceptibilities as well as metallic properties. A modified Curie-Weiss law was proposed for systems containing anisotropic magnetic ions to analyze the magnetic susceptibilities of NaxCoO2 (x ~~ 0.75), and implications of this analysis were explored. Our study shows that the lowspin Co4+ (S = 1/2) ions of NaxCoO2 generated by the Na vacancies cause the anisotropic magnetic properties of NaxCoO2, and suggests that the six nearest-neighbor Co3+ ions of each Co4+ ion adopt the intermediate-spin electron configuration thereby behaving magnetically like low-spin Co4+ ions. The Weiss temperature of NaxCoO2 is more negative along the direction of the lower g-factor (i.e., Theta_parallel < Theta_perp < 0, and g_parallel < g_perp). The occurrence of intermediate-spin Co3+ ions surrounding each Co4+ ion account for the apparently puzzling magnetic properties of NaxCoO2 (x ~~ 0.75), i.e., the large negative Weiss temperature, the three-dimensional antiferromagnetic ordering below ~22 K, and the metallic properties. The picture of the magnetic structure derived from neutron scattering studies below ~22 K are in apparent conflict with that deduced from magnetic susceptibility measurements between ~50 - 300 K. These conflicting pictures are resolved by noting that the spin exchange between Co3+ ions is more strongly antiferromagnetic than that between Co4+ and Co3+ ions.

cond-mat.str-el