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D. F. Agterberg

Publications and source records attributed to D. F. Agterberg.

At least 19 recordsLinked to original sources

Fresnel diffraction imaging of surface nanostructure using coherent resonant X-ray scattering

We investigated surface nanostructures on an antiferromagnet MnBi$_2$Te$_4$ using a novel imaging technique, direct (real)-space and real time coherent X-ray imaging (direct-CXI). This technique has provided new insights into antiferromagnetic textures, including the formation of anti-phase antiferromagnetic (AFM) domains and thermal dynamics of AFM domains and domain walls. While this method produces real-space images of AFM textures without requiring a complex imaging retrieval process, its underlying imaging mechanism has not been fully understood, limiting a deep understanding of AFM textures and the information they contain. By investigating the well-defined structural characteristics of the nanostructures fabricated on MnBi$_2$Te$_4$, we elucidate the imaging principle of this novel technique. We find that the observed images can be well explained by Fresnel diffraction integral. Using a simple model from classical optics, our calculations successfully reproduce the experimentally observed images of the nanostructures. This demonstrates that direct-CXI not only provides straightforward real-space imaging but also contains phase information through its Fresnel diffraction integral.

cond-mat.mtrl-sci

Low temperature magnetic structure and lattice response in SmCuAs$_2$

We investigated the structural and magnetic properties of single-crystalline SmCuAs$_2$ using high-resolution synchrotron X-ray diffraction and X-ray resonant magnetic scattering (XRMS) at the Sm $L_2$ and $L_3$ edges. Temperature-dependent diffraction measurements confirm that SmCuAs$_2$ maintains its tetragonal symmetry from room temperature down to 8 K, with lattice parameters showing anomalous behavior below the resistivity minimum ($T \approx$ 30 K). Notably, the \textbf{c}-axis lattice parameter exhibits a plateau and subsequent increase near the Néel temperature, indicating magnetoelastic coupling. XRMS measurements reveal a commensurate antiferromagnetic structure with a propagation vector \textbf{\textit{q}} = (0, 0, 0.5). Our measurement shows that the Sm moments are aligned within the \textbf{\textit{ab}} plane and arranged in a $++--$ stacking along the \textbf{\textit{c}}-axis. Comparison with related \textit{RE}CuAs$_2$ compounds (\textit{RE} = Pr, Nd, and Gd) suggests that in-plane moment orientation and associated magnetic frustration play a key role in the emergence of the resistivity minimum. Differences in spin-orbit and magnetoelastic coupling across the series highlight their importance in governing low-temperature transport behavior.

cond-mat.str-el

Nodeless Superconducting State in the Presence of Zero-Field Staggered Magnetization in CeRh$_{2}$As$_{2}$

The tetragonal heavy-fermion superconductor CeRh$_{2}$As$_{2}$ with a critical temperature $T_c$ $\approx$ 0.34 K exhibits an intriguing magnetic field-induced transition between likely distinct superconducting states. In zero field, an even-parity state emerges within another ordered phase of unknown origin with $T_0$ $\approx$ 0.54 K. Here, we investigated the spin-singlet state of CeRh$_{2}$As$_{2}$ at temperatures down to $\approx$ 0.02$T_c$ by means of local magnetization measurements performed using micro-Hall probe magnetometry. We determined the temperature dependencies of the lower critical field for both in-plane and out-of-plane field directions, and demonstrated their consistency with predominantly fully gapped superconductivity. In the magnetization measured along the $a$ axis, we found a clear increase below $T_0$, while no similar anomaly was observed along the $c$ axis. Our results place important constraints on the spin-singlet order parameter in CeRh$_{2}$As$_{2}$ and highlight an important role of static magnetic moments in the nature of $T_0$ phase.

cond-mat.supr-con

Observation of vortex stripes in UTe$_2$

Quantum vortices are fundamentally important for properties of superconductors. In conventional type-II superconductor they determine the magnetic response of the system and tend to form regular lattices. UTe$_2$ is a recently discovered heavy fermion superconductor exhibiting many anomalous macroscopic behaviors. However, the question whether it has a multicomponent order parameter remains open. Here, we study magnetic properties of UTe$_2$ by employing scanning superconducting quantum interference device microscopy. We find vortex behavior which is very different from that in ordinary superconductors. We imaged vortices generated by cooling in magnetic field applied along different crystalline directions. While a small out-of-plane magnetic field produces typical isolated vortices, higher field generates vortex stripe patterns which evolve with vortex density. The stripes form at different locations and along different directions in the surface plane when the vortices are crystalized along the crystalline b or c axes. The behavior is reproduced by our simulation based on an anisotropic two-component order parameter. This study shows that UTe$_2$ has a nontrivial disparity of multiple length scales, placing constraints on multicomponent superconductivity. The tendency of vortex stripe formation and their control by external field may be useful in fluxonics applications.

cond-mat.supr-con

Electron-phonon coupling and spin fluctuations in the Ising superconductor NbSe$_{2}$

Ising superconductivity, observed experimentally in NbSe$_{2}$ and similar materials, has generated tremendous interest. Recently, attention was called to the possible role that spin fluctuations (SF) play in this phenomenon, in addition to the dominant electron-phonon coupling (EPC); the possibility of a predominantly-triplet state was discussed and led to a conjecture of viable singlet-triplet Leggett oscillations. However, these hypotheses have not been put to a quantitative test. In this paper, we report first principle calculations of the EPC and also estimate coupling with SF, including full momentum dependence. We find that: (1) EPC is strongly anisotropic, largely coming from the K-K' scattering, and therefore excludes triplet symmetry even as an excited state; (2) superconductivity is substantially weakened by SF, but anisotropy remains as above; and, (3) we do find the possibility of a Leggett mode, not in a singlet-triplet but in an $s_{++}$ - $s_\pm$ channel.

cond-mat.supr-con

Field-angle dependence reveals odd-parity superconductivity in CeRh$_2$As$_2$

CeRh$_2$As$_2$ is an unconventional superconductor with multiple superconducting phases and $T_\mathrm{c} = 0.26$ K. When $H\parallel c$, it shows a field-induced transition at $μ_0H^* = 4$ T from a low-field superconducting state SC1 to a high-field state SC2 with a large critical field of $μ_0H_\mathrm{c2} = 14$ T. In contrast, for $H\perp c$, only the SC1 with $μ_0H_\mathrm{c2} = 2$ T is observed. A simple model based on the crystal symmetry was able to reproduce the phase-diagrams and their anisotropy, identifying SC1 and SC2 with even and odd parity superconducting states, respectively. However, additional orders were observed in the normal state which might have an influence on the change of the superconducting state at $H^*$. Here, we present a comprehensive study of the angle dependence of the upper critical fields using magnetic ac-susceptibility, specific heat and torque on single crystals of CeRh$_2$As$_2$. The experiments show that the state SC2 is strongly suppressed when rotating the magnetic field away from the $c$ axis and it disappears for an angle of 35$^{\circ}$. This behavior agrees perfectly with our extended model of a pseudospin triplet state with $\vec{d}$ vector in the plane and hence allows to nail down that SC2 is indeed the suggested odd-parity state.

cond-mat.supr-con

Non-symmorphic symmetry and field-driven odd-parity pairing in CeRh$_2$As$_2$

Recently, evidence has emerged for a field-induced even- to odd-parity superconducting phase transition in CeRh$_2$As$_2$ [S. Khim et al., Science 373 1012 (2021)]. Here we argue that the P4/nmm non-symmorphic crystal structure of CeRh$_2$As$_2$ plays a key role in enabling this transition by ensuring large spin-orbit interactions near the Brillouin zone boundaries, which naturally leads to the required near-degeneracy of the even- and odd-parity channels. We further comment on the relevance of our theory to FeSe, which crystallizes in the same structure.

cond-mat.supr-con

Field-induced transition from even to odd parity superconductivity in CeRh$_2$As$_2$

We report the discovery of two-phase unconventional superconductivity in CeRh$_2$As$_2$. Using thermodynamic probes, we establish that the superconducting critical field of its high-field phase is as high as 14 T, remarkable in a material whose transition temperature is 0.26 K. Furthermore, a $c$-axis field drives a transition between two different superconducting phases. In spite of the fact that CeRh$_2$As$_2$ is globally centrosymmetric, we show that local inversion-symmetry breaking at the Ce sites enables Rashba spin-orbit coupling to play a key role in the underlying physics. More detailed analysis identifies the transition from the low- to high-field states to be associated with one between states of even and odd parity.

cond-mat.supr-con

Generalized Spin Fluctuation Feedback In Correlated Fermion Superconductors

Experiments reveal that the superconductors $\text{UPt}_3$, $\text{U}_{1-x}\text{Th}_x\text{Be}_{13}$ and $\text{PrOs}_4\text{Sb}_{12}$ undergo two superconducting transitions in the absence of an applied magnetic field. The prevalence of these multiple transitions suggests a common underlying mechanism. A natural candidate theory which accounts for these two transitions is the existence of a small symmetry breaking field, however such a field has not been observed in $\text{PrOs}_4\text{Sb}_{12}$ or $\text{U}_{1-x}\text{Th}_x\text{Be}_{13}$ and has been called into question for $\text{UPt}_3$. Motivated by arguments originally developed for superfluid $^3\text{He}$ we propose that a generalized spin fluctuation feedback effect is responsible for these two transitions. We first develop a phenomenological theory for $^3\text{He}$ that couples spin fluctuations to superfluidity, which correctly predicts that a high temperature broken time-reversal superfluid $^3\text{He}$ phase can emerge as a consequence. The transition at lower temperatures into a time-reversal invariant superfluid phase must then be first order by symmetry arguments. We then apply this phenomenological approach to the three superconductors $\text{UPt}_3$, $\text{U}_{1-x}\text{Th}_x\text{Be}_{13}$ and $\text{PrOs}_4\text{Sb}_{12}$ revealing that this naturally leads to a high-temperature time-reversal invariant nematic superconducting phase, which can be followed by a second order phase transition into a broken time-reversal symmetry phase, as observed.

cond-mat.supr-con

Loop currents and anomalous Hall effect from time-reversal symmetry-breaking superconductivity on the honeycomb lattice

We study a tight-binding model on the honeycomb lattice of chiral $d$-wave superconductivity that breaks time-reversal symmetry. Due to its nontrivial sublattice structure, we show that it is possible to construct a gauge-invariant time-reversal-odd bilinear of the pairing potential. The existence of this bilinear reflects the sublattice polarization of the pairing state. We show that it generates persistent loop current correlations around each lattice site and opens a topological mass gap at the Dirac points, resembling Haldane's model of the anomalous quantum Hall effect. In addition to the usual chiral $d$-wave edge states, there also exist electron-like edge resonances due to the topological mass gap. We show that the presence of loop-current correlations directly leads to a nonzero intrinsic ac Hall conductivity, which produces the polar Kerr effect without an external magnetic field. Similar results also hold for the nearest-neighbor chiral $p$-wave pairing. We briefly discuss the relevance of our results to superconductivity in twisted bilayer graphene.

cond-mat.supr-con

Hund's coupling stabilized superconductivity in the presence of spin-orbit interactions

The intraorbital repulsive Hubbard interaction cannot lead to attractive superconducting pairing states, except through the Kohn-Luttinger mechanism. This situation may change when we include additional local interactions such as the interorbital repulsion $U^\prime$ and Hund's interactions $J$. Adding these local interactions, we study the nature of the superconducting pairs in systems with tetragonal crystal symmetry including the $d_{xz}$ and $d_{yz}$ orbitals, and in octahedral systems including all three of $d_{xz}$, $d_{yz}$, and $d_{xy}$ orbitals. In the tetragonal case, spin-orbit interactions can stabilize attractive pairing channels containing spin triplet, orbital singlet character. Depending on the form of spin-orbit coupling, pairing channels belonging to degenerate, non-trivial irreducible representations may be stabilized. In the octahedral case, the pairing interactions of superconducting channels are found to depend critically on the number of bands crossing the Fermi energy.

cond-mat.supr-con

Residual spin susceptibility in the spin-triplet, orbital-singlet model

Nuclear magnetic resonance (NMR) and Knight shift measurements are critical tools in the identification of spin-triplet superconductors. We discuss the effects of spin orbit coupling on the Knight shift and susceptibilities for a variety of spin triplet multi-orbital gap functions with orbital-singlet character and compare their responses to "traditional" single band spin-triplet ($p_x+ip_y$) superconductors. We observe a non-negligible residual spin-susceptibility at low temperature.

cond-mat.supr-con

Bogoliubov Fermi surfaces: General theory, magnetic order, and topology

We present a comprehensive theory for Bogoliubov Fermi surfaces in inversion-symmetric superconductors which break time-reversal symmetry. A requirement for such a gap structure is that the electrons posses internal degrees of freedom apart from the spin (e.g., orbital or sublattice indices), which permits a nontrivial internal structure of the Cooper pairs. We develop a general theory for such a pairing state, which we show to be nonunitary. A time-reversal-odd component of the nonunitary gap product is found to be essential for the appearance of Bogoliubov Fermi surfaces. These Fermi surfaces are topologically protected by a $\mathbb{Z}_2$ invariant. We examine their appearance in a generic low-energy effective model and then study two specific microscopic models supporting Bogoliubov Fermi surfaces: a cubic material with a $j=3/2$ total-angular-momentum degree of freedom and a hexagonal material with distinct orbital and spin degrees of freedom. The appearance of Bogoliubov Fermi surfaces is accompanied by a magnetization of the low-energy states, which we connect to the time-reversal-odd component of the gap product. We additionally calculate the surface spectra associated with these pairing states and demonstrate that the Bogoliubov Fermi surfaces are characterized by additional topological indices. Finally, we discuss the extension of phenomenological theories of superconductors to include Bogoliubov Fermi surfaces, and identify the time-reversal-odd part of the gap product as a composite order parameter which is intertwined with superconductivity.

cond-mat.supr-con

Resilient nodeless $d$-wave superconductivity in monolayer FeSe

Monolayer FeSe exhibits the highest transition temperature among the iron based superconductors and appears to be fully gapped, seemingly consistent with $s$-wave superconductivity. Here, we develop a theory for the superconductivity based on coupling to fluctuations of checkerboard magnetic order (which has the same translation symmetry as the lattice). The electronic states are described by a symmetry based ${\bf k}\cdot {\bf p}$-like theory and naturally account for the states observed by angle resolved photoemission spectroscopy. We show that a prediction of this theory is that the resultant superconducting state is a fully gapped, nodeless, $d$-wave state. This state, which would usually have nodes, stays nodeless because, as seen experimentally, the relevant spin-orbit coupling term has an energy scale smaller than the superconducting gap.

cond-mat.supr-con

Inflated nodes and surface states in superconducting half-Heusler compounds

Two topics of high current interest in the field of unconventional superconductivity are non-centrosymmetric superconductors and multiband superconductivity. Half-Heusler superconductors such as YPtBi exemplify both. In this paper, we study bulk and surface states in nodal superconducting phases of the half-Heusler compounds, belonging to the $A_1$ ($s+p$-like) and $T_2$ ($k_zk_x+ik_zk_y$-like) irreducible representations of the point group. These two phases preserve and break time-reversal symmetry, respectively. For the $A_1$ case, we find that flat surface bands persist in the multiband system. In addition, the system has dispersive surface bands with zero-energy crossings forming Fermi arcs, which are protected by mirror symmetries. For the $T_2$ case, there is an interesting coexistence of point and line nodes, known from the single-band case, with Bogoliubov Fermi surfaces (two-dimensional nodes). There are no flat-band surface states, as expected, but dispersive surface bands with Fermi arcs exist. If these arcs do not lie in high-symmetry planes, they are split by the antisymmetric spin-orbit coupling so that their number is doubled compared to the inversion-symmetric case.

cond-mat.supr-con

Anisotropy of magnetic interactions and symmetry of the order parameter in unconventional superconductor Sr$_{2}$RuO$_{4}$

Sr$_2$RuO$_4$ is the best candidate for spin-triplet superconductivity, an unusual and elusive superconducting state of fundamental importance. In the last three decades Sr$_2$RuO$_4$ has been very carefully studied and despite its apparent simplicity when compared with strongly correlated high-$T_{c}$ cuprates, for which the pairing symmetry is understood, there is no scenario that can explain all the major experimental observations, a conundrum that has generated tremendous interest. Here we present a density-functional based analysis of magnetic interactions in Sr$_{2}$RuO$_{4}$ and discuss the role of magnetic anisotropy in its unconventional superconductivity. Our goal is twofold. First, we access the possibility of the superconducting order parameter rotation in an external magnetic field of 200 Oe, and conclude that the spin-orbit interaction in this material is several orders of magnitude too strong to be consistent with this hypothesis. Thus, the observed invariance of the Knight shift across $T_{c}$ has no plausible explanation, and casts doubt on using the Knight shift as an ultimate litmus paper for the pairing symmetry. Second, we propose a quantitative double-exchange-like model for combining itinerant fermions with an anisotropic Heisenberg magnetic Hamiltonian. This model is complementary to the Hubbard-model-based calculations published so far, and forms an alternative framework for exploring superconducting symmetry in Sr$_{2}$RuO$_{4}.$ As an example, we use this model to analyze the degeneracy between various $p-$triplet states in the simplest mean-field approximation, and show that it splits into a single and two doublets with the ground state defined by the competition between the "Ising" and "compass" anisotropic terms.

cond-mat.supr-con

Bogoliubov Fermi surfaces in superconductors with broken time-reversal symmetry

It is commonly believed that in the absence of disorder or an external magnetic field, there are three possible types of superconducting excitation gaps: the gap is nodeless, it has point nodes, or it has line nodes. Here, we show that for an even-parity nodal superconducting state which spontaneously breaks time-reversal symmetry, the low-energy excitation spectrum generally does not belong to any of these categories, instead it has extended Bogoliubov Fermi surfaces. These Fermi surfaces can be visualized as two-dimensional surfaces generated by "inflating" point or line nodes into spheroids or tori, respectively. These inflated nodes are topologically protected from being gapped by a $\mathbb{Z}_2$ invariant, which we give in terms of a Pfaffian. We also show that superconducting states possessing these Fermi surfaces can be energetically stable. A crucial ingredient in our theory is that more than one band is involved in the pairing, since all candidate materials for even-parity superconductivity with broken time-reversal symmetry are multiband systems, we expect these $\mathbb{Z}_2$-protected Fermi surfaces to be ubiquitous.

cond-mat.supr-con

Effects of interface oxygen vacancies on electronic bands of FeSe/SrTiO3(001)

Modifications of the electronic bands of thin FeSe films due to oxygen vacancies in the supporting SrTiO 3 (001) substrate - and the interplay with spin-orbit coupling, magnetism, and epitaxy - are investigated by first-principles supercell calculations. Unfolded (k-projected) bands show that the oxygen vacancies both provide electron doping to the interface FeSe layer and also have notable effects on the details of the bands around the Fermi level, including renormalizing the width of the Fe-3d band near the Fermi level by a factor of about 0.6, and causing a splitting of ~40 meV at the M point for the checkerboard antiferromagnetic configuration. For an FeSe bilayer, the modifications to the bands are mainly limited to the interface FeSe layer. While spin-orbit-coupling induced band splittings of ~30 meV at M for the ideal FeSe/SrTiO3 (001) interfaces are comparable to the splitting due to oxygen vacancies, the effects are not simply additive. Calculations and comparison to our scanning tunneling microscopy images of MBE-grown FeSe films on SrTiO3 (001) suggest that a common defect may be Se bound to an oxygen vacancy at the interface

cond-mat.mtrl-sci