arXiv subjects

D. Fioretto

Publications and source records attributed to D. Fioretto.

13 recordsLinked to original sources

arXiv2026

Accessing which-path information in the absorption and emission of light by a quantum dot in a Ramsey sequence

We quantify which-path information in the absorption and emission of light by a quantum dot along a Ramsey-like sequence. The quantum dot is excited by two successive classical $\pi/2$-pulses with tunable relative phase, yielding the spontaneous release of coherent superpositions of zero- and one-photon Fock states into two successive time bins. Along the sequence, the first time bin extracts information on the quantum dot energy state, behaving as a which-path detector for the Ramsey interferometer. The which-path information increases over time, and is accessed through the reduction of contrast of the Ramsey fringes. After the second pulse, the information still present in the first time bin controls the emission of coherent light into the second time bin, which is measurable through the reduction of the contrast of self-homodyne interference fringes in a Mach-Zehnder interferometer. Both measurements are in remarkable agreement with theoretical predictions. Our results quantitatively illustrate how which-path information and more generally quantum correlations impact light-matter energy exchanges in the quantum realm.

quant-ph↗

arXiv2024

Quantum interferences and gates with emitter-based coherent photon sources

Quantum emitters such as quantum dots, defects in diamond or in silicon have emerged as efficient single photon sources that are progressively exploited in quantum technologies. In 2019, it was shown that the emitted single photon states often include coherence with the vacuum component. Here we investigate how such photon-number coherence alters quantum interference experiments that are routinely implemented both for characterising or exploiting the generated photons. We show that it strongly modifies intensity correlation measurements in a Hong-Ou-Mandel experiment and leads to errors in indistinguishability estimations. It also results in additional entanglement when performing partial measurements. We illustrate the impact on quantum protocols by evidencing modifications in heralding efficiency and fidelity of two-qubit gates.

quant-ph↗

arXiv2022

High-rate entanglement between a semiconductor spin and indistinguishable photons

Photonic graph states, quantum light states where multiple photons are mutually entangled, are key resources for optical quantum technologies. They are notably at the core of error-corrected measurement-based optical quantum computing and all-optical quantum networks. In the discrete variable framework, these applications require high efficiency generation of cluster-states whose nodes are indistinguishable photons. Such photonic cluster states can be generated with heralded single photon sources and probabilistic quantum gates, yet with challenging efficiency and scalability. Spin-photon entanglement has been proposed to deterministically generate linear cluster states. First demonstrations have been obtained with semiconductor spins achieving high photon indistinguishablity, and most recently with atomic systems at high collection efficiency and record length. Here we report on the efficient generation of three partite cluster states made of one semiconductor spin and two indistinguishable photons. We harness a semiconductor quantum dot inserted in an optical cavity for efficient photon collection and electrically controlled for high indistinguishability. We demonstrate two and three particle entanglement with fidelities of 80 % and 63 % respectively, with photon indistinguishability of 88%. The spin-photon and spin-photon-photon entanglement rates exceed by three and two orders of magnitude respectively the previous state of the art. Our system and experimental scheme, a monolithic solid-state device controlled with a resource efficient simple experimental configuration, are very promising for future scalable applications.

quant-ph↗

arXiv2022

Probing the dynamics and coherence of a semiconductor hole spin via acoustic phonon-assisted excitation

Spins in semiconductor quantum dots are promising local quantum memories to generate polarization-encoded photonic cluster states, as proposed in the pioneering Rudolph-Lindner scheme [1]. However, harnessing the polarization degree of freedom of the optical transitions is hindered by resonant excitation schemes that are widely used to obtain high photon indistinguishability. Here we show that acoustic phonon-assisted excitation, a scheme that preserves high indistinguishability, also allows to fully exploit the polarization selective optical transitions to initialise and measure single spin states. We access the coherence of hole spin systems in a low transverse magnetic field and directly monitor the spin Larmor precession both during the radiative emission process of an excited state or in the quantum dot ground state. We report a spin state detection fidelity of $94.7 \pm 0.2 \%$ granted by the optical selection rules and a $20\pm5$~ns hole spin coherence time, demonstrating the potential of this scheme and system to generate linear cluster states with a dozen of photons

cond-mat.mes-hall↗

arXiv2019

Indistinguishable photons from a trapped-ion quantum network node

Trapped atomic ions embedded in optical cavities are a promising platform to enable long-distance quantum networks and their most far-reaching applications. Here we achieve and analyze photon indistinguishability in a telecom-converted ion-cavity system. First, two-photon interference of cavity photons at their ion-resonant wavelength is observed and found to reach the limits set by spontaneous emission. Second, this limit is shown to be preserved after a two-step frequency conversion replicating a distributed scenario, in which the cavity photons are converted to the telecom C band and then back to the original wavelength. The achieved interference visibility and photon efficiency would allow for the distribution and practical verification of entanglement between ion-qubit registers separated by several tens of kilometers.

quant-ph↗

arXiv2019

Inelastic x-ray scattering reveals the ergodic to nonergodic transition of salol, a liquid with local order

We have studied the high-frequency dynamics of salol by inelastic x-ray scattering over a wide temperature range between 50 and 450 K, across the glass transition. We find that salol efficiently realizes the mechanism of dynamical arrest described by the mode-coupling theory, as manifested by a cusp singularity in the behaviour of the non-ergodicity parameter and a $Q$ dependence of the critical non-ergodicity parameter that is in phase with the static structure factor. These results confront positively the mode-coupling theory with liquids with local order.

cond-mat.soft↗

arXiv2017

High-performance versatile setup for simultaneous Brillouin-Raman micro-spectroscopy

Brillouin and Raman scattering spectroscopy are established techniques for the nondestructive contactless and label-free readout of mechanical, chemical and structural properties of condensed matter. Brillouin-Raman investigations currently require separate measurements and a site-matching approach to obtain complementary information from a sample. Here we demonstrate a new concept of fully scanning multimodal micro-spectroscopy for simultaneous detection of Brillouin and Raman light scattering in an exceptionally wide spectral range, from fractions of GHz to hundreds of THz. It yields an unprecedented 150 dB contrast, which is especially important for the analysis of opaque or turbid media such as biomedical samples, and a spatial resolution on sub-cellular scale. We report the first applications of this new multimodal method to a range of systems, from a single cell to the fast reaction kinetics of a curing process, and the mechano-chemical mapping of highly scattering biological samples.

physics.ins-det↗

arXiv2014

Slow dynamics of salol: a pressure and temperature dependent light scattering study

We study the slow dynamics of salol by varying both temperature and pressure using photon correlation spectroscopy and pressure-volume-temperature measurements, and compare the behavior of the structural relaxation time with equations derived within the Adam-Gibbs entropy theory and the Cohen-Grest free volume theory. We find that pressure dependent data are crucial to assess the validity of these model equations. Our analysis supports the entropy-based equation, and estimates the configurational entropy of salol at ambient pressure ? 70% of the excess entropy. Finally, we investigate the evolution of the shape of the structural relaxation process, and find that a time-temperature-pressure superposition principle holds over the range investigated.

cond-mat.soft↗

arXiv2008

Effect of Polymerization on the Boson Peak, from the Liquid to Glassy Phase

Raman scattering measurements are used to follow the modification of the vibrational density of states in a reactive epoxy{amine mixture during isothermal polymerization. Combining with Brillouin light and inelastic x-ray scattering measurements, we analyze the variations of the boson peak and of the Debye level while the system passes from the uid to a glassy phase upon increasing the number of covalent bonds among the constituent molecules. We find that the shift and the intensity decrease of the boson peak are fully explained by the modification of the elastic medium throughout the reaction. Surprisingly, bond-induced modifications of the structure do not affect the relative excess of states over the Debye level.

cond-mat.soft↗

arXiv2005

Hard sphere-like dynamics in a non hard sphere liquid

The collective dynamics of liquid Gallium close to the melting point has been studied using Inelastic X-ray Scattering to probe lengthscales smaller than the size of the first coordination shell. %(momentum transfers, $Q$, $>$15 nm$^{-1}$). Although the structural properties of this partially covalent liquid strongly deviate from a simple hard-sphere model, the dynamics, as reflected in the quasi-elastic scattering, are beautifully described within the framework of the extended heat mode approximation of Enskog's kinetic theory, analytically derived for a hard spheres system. The present work demonstrates the applicability of Enskog's theory to non hard- sphere and non simple liquids.

cond-mat.dis-nn↗

arXiv2004

Microscopic dynamics and relaxation processes in liquid Hydrogen Fluoride

Inelastic x-ray scattering and Brillouin light scattering measurements of the dynamic structure factor of liquid hydrogen fluoride have been performed in the temperature range$ T=214\div 283 K$. The data, analysed using a viscoelastic model with a two timescale memory function, show a positive dispersion of the sound velocity $c(Q)$ between the low frequency value $c_0(Q)$ and the high frequency value $c_{\infty \alpha}(Q)$. This finding confirms the existence of a structural ($\alpha$) relaxation directly related to the dynamical organization of the hydrogen bonds network of the system. The activation energy $E_a$ of the process has been extracted by the analysis of the temperature behavior of the relaxation time $\tau_\alpha(T)$ that follows an Arrhenius law. The obtained value for $E_a$, when compared with that observed in another hydrogen bond liquid as water, suggests that the main parameter governing the $\alpha$-relaxation process is the number of the hydrogen bonds per molecule.

cond-mat.dis-nn↗

arXiv2000

Intra-molecular origin of the fast relaxations observed in the Brillouin light scattering spectra of molecular glass-formers

The Brillouin light scattering spectra of the o-terphenyl single crystal are compared with those of the liquid and the glass phases. This shows: i) the direct evidence of a fast relaxation at 5 GHz in both the single crystal and the glass; ii) a similar temperature dependence for the attenuation of the longitudinal sound waves in the single crystal and the glass; and iii) the absence of coupling between the fast relaxation and the transverse acoustic waves. These results allow us to assign such a relaxation to the coupling between the longitudinal acoustic waves and intra-molecular vibrations, and therefore to exclude any relationship between it and the glass transition.

cond-mat.dis-nn↗

arXiv1999

Non-dynamic origin of the acoustic attenuation at high frequency in glasses

The sound attenuation in the THz region is studied down to T=16 K in glassy glycerol by inelastic x-ray scattering. At striking variance with the decrease found below 100 K in the GHz data, the attenuation in the THz range does not show any T dependence. This result i) indicates the presence of two different attenuation mechanisms, active respectively in the high and low frequency limits; ii) demonstrates the non-dynamic origin of the attenuation of THz sound waves, and confirms a similar conclusion obtained in SiO2 glass by molecular dynamics; and iii) supports the low frequency attenuation mechanism proposed by Fabian and Allen (Phys.Rev.Lett. 82, 1478 (1999)).

cond-mat.dis-nn↗