arXiv subjects

D. G. Cory

Publications and source records attributed to D. G. Cory.

At least 19 recordsLinked to original sources

arXiv2026

Probing Single-Particle Spatial Extent With Helical Neutron Wavefronts

Distinguishing transverse coherence length from single-particle wavepacket extent is fundamentally challenging, as both manifest through spatial broadening of observed intensity profiles in conventional experiments. Here we introduce a method based on helical neutron wavefronts that enables this separation. Helical neutron states produce annular intensity profiles whose peak radius depends on the transverse wavepacket extent, while coherence length only contributes to profile broadening. In our experimental geometry we measure a beam divergence of ~1.1 mrad, corresponding to a transverse coherence length of ~180 nm. In contrast, the same measurement places a lower bound of >= 2 um on the spatial extent of the individual neutron wavepackets, more than an order of magnitude larger than the coherence length. These results provide direct experimental evidence that transverse coherence length and single-particle wavepacket extent are distinct physical quantities, resolving a longstanding source of confusion in the neutron literature.

quant-ph↗

arXiv2026

Experimental Limit on Neutron Orbital Angular Momentum Detection Using Polarized 3He

A recent proposal suggested that neutron orbital angular momentum (OAM) states could be detected via spin-polarized absorption in polarized 3He, with predicted cross-section variations linked to the neutron's OAM. We experimentally tested this hypothesis using spin-polarized neutron beams with OAM =-2 to 2, generated by fork-dislocation phase-gratings, and transmitted through a polarized 3He cell. Within statistical precision, no OAM-dependent change in the absorption cross section was observed. This null result places stringent constraints on polarized 3He-based OAM detection schemes. The absence of an effect in the given regime is traced to the proposal's disregard of the spatial character of neutron OAM: unlike spin, OAM arises from the transverse phase structure of the wavefunction and couples only through spatial gradients and overlap. The transverse extent of neutron OAM modes expands rapidly, producing a doughnut-shaped intensity profile with negligible overlap with on-axis 3He nuclei, while off-axis capture samples only a locally uniform phase and reduces the interaction to the known spin dependence. These results clarify the limits of absorptive nuclear methods for probing neutron OAM and emphasize the necessity of spatially resolved interactions in any viable detection scheme.

physics.app-ph↗

arXiv2025

Design and Monte Carlo Simulation of a Phase Grating Moiré Neutron Interferometer to Measure the Gravitational Constant

The gravitational constant (G) is the least precisely known fundamental constant of nature, with persistent and significant discrepancies between measurement methods. New techniques for measuring G with systematic effects different from commonly applied pendulum methods are required. Neutrons are convenient probes of gravitational forces as they are both massive and electrically neutral, properties that allowed a single-crystal neutron interferometer (NI) to achieve the first experimental demonstration of gravitationally induced quantum interference. Despite this, the limitation of single-crystal NIs to monoenergetic beams significantly reduces neutron flux, making precision gravitational measurements unfeasible. A new NI design called the phase-grating moiré interferometer (PGMI) has been shown to increase neutron flux by orders of magnitude while allowing grating separation that maintains similar interferometer area to previous NI devices. Here, we propose and describe an experiment to measure G using the PGMI to a precision comparable to measurements from the CODATA 2022 evaluation. A Monte Carlo model for incorporating nonlinear potentials into a PGMI is introduced. This model is used to evaluate sources of systematic uncertainty and quantify the uncertainty in G arising from these effects. The effect of lunar gravitation on a torsion pendulum experiment from CODATA 2022 is calculated, and the need for possible correction factors is demonstrated. This work demonstrates that a neutron PGMI can be used to measure G to $150$ parts-per-million in the near term with the potential to achieve greater precision in future experimental designs.

physics.ins-det↗

arXiv2024

Quantum Advancements in Neutron Scattering Reshape Spintronic Devices

Topological magnetism has sparked an unprecedented age in quantum technologies. Marked by twisted spin structures with exotic dynamical modes, topological magnets have motivated a new generation of spintronic devices which transcend the limits of conventional semiconductor-based electronics. While existing material probes have biased studies and device conceptualizations for thin samples in two dimensions, advancements in three-dimensional probing techniques using beams of neutrons, are transforming our understanding of topological and emergent physics to reimagine spintronic devices. Here, we review recent neutron scattering breakthroughs which harness quantum degrees of freedom to enable three-dimensional topological investigations of quantum materials. We discuss applications of structured and tomographic neutron scattering techniques to topological magnets, with particular emphasis on magnetic skyrmion systems and their inspired three-dimensional logic device infrastructures through novel multi-bit encoding and control schemes. SANS-based dynamic visualizations and coherent manipulations of three-dimensional topological qubits are proposed using electric field controls of depth-dependant helicities and spin-orbit tuning of the neutron beam. Together, these investigations uncover a new world of three-dimensional topological physics which enhances spintronic devices through a novel set of structures, dynamics, and controls, unique to three-dimensional systems.

cond-mat.mtrl-sci↗

arXiv2024

Achieving a Near-Ideal Silicon Crystal Neutron Interferometer using Sub-Micron Fabrication Techniques

Perfect-crystal neutron interferometry which is analogous to Mach-Zehnder interferometry, uses Bragg diffraction to form interfering neutron paths. The measured phase shifts can be used to probe many types of interactions whether it be nuclear, electromagnetic, gravitational, or topological in nature. For a perfect-crystal interferometer to preserve coherence, the crystal must possess a high degree of dimensional tolerance as well as being relatively defect-free with minimal internal stresses. In the past, perfect-crystal neutron interferometers have been produced by a two step process. First, a resin diamond wheel would be used to remove excess material and shape the interferometer. Afterword, the crystal would be etched in order to remove surface defects and elevate strains. This process has had limitations in terms of repeatability and in maximizing the final contrast, or fringe visibility, of the interferometer. We have tested various fabrication and post-fabrication techniques on a single perfect-crystal neutron interferometer and measured the interferometer's performance at each step. Here we report a robust, repeatable non-etching fabrication process with high final contrast. For the interferometer used in this work, we achieved contrasts of greater than 90% several separate times and ultimately finished with an interferometer that has 92% contrast and a uniform phase distribution.

physics.ins-det↗

arXiv2023

Phase and contrast moiré signatures in two-dimensional cone beam interferometry

Neutron interferometry has played a distinctive role in fundamental science and characterization of materials. Moiré neutron interferometers are candidate next-generation instruments: they offer microscopy-like magnification of the signal, enabling direct camera recording of interference patterns across the full neutron wavelength spectrum. Here we demonstrate the extension of phase-grating moiré interferometry to two-dimensional geometries. Our fork-dislocation phase gratings reveal phase singularities in the moiré pattern, and we explore orthogonal moiré patterns with two-dimensional phase-gratings. Our measurements of phase topologies and gravitationally induced phase shifts are in good agreement with theory. These techniques can be implemented in existing neutron instruments to advance interferometric analyses of emerging materials and precision measurements of fundamental constants.

physics.app-ph↗

arXiv2023

Cone beam neutron interferometry: from modeling to applications

Phase-grating moire interferometers (PGMIs) have emerged as promising candidates for the next generation of neutron interferometry, enabling the use of a polychromatic beam and manifesting interference patterns that can be directly imaged by existing neutron cameras. However, the modeling of the various PGMI configurations is limited to cumbersome numerical calculations and backward propagation models which often do not enable one to explore the setup parameters. Here we generalize the Fresnel scaling theorem to introduce a k-space model for PGMI setups illuminated by a cone beam, thus enabling an intuitive forward propagation model for a wide range of parameters. The interference manifested by a PGMI is shown to be a special case of the Talbot effect, and the optimal fringe visibility is shown to occur at the moire location of the Talbot distances. We derive analytical expressions for the contrast and the propagating intensity profiles in various conditions, and analyze the behaviour of the dark-field imaging signal when considering sample characterization. The model's predictions are compared to experimental measurements and good agreement is found between them. Lastly, we propose and experimentally verify a method to recover contrast at typically inaccessible PGMI autocorrelation lengths. The presented work provides a toolbox for analyzing and understanding existing PGMI setups and their future applications, for example extensions to two-dimensional PGMIs and characterization of samples with non-trivial structures.

physics.app-ph↗

arXiv2023

Psychophysical discrimination of radially varying polarization entoptic phenomena

The incorporation of structured light techniques into vision science has enabled more selective probes of polarization related entoptic phenomena. Diverse sets of stimuli have become accessible in which the spatially dependant optical properties can be rapidly controlled and manipulated. For example, past studies with human perception of polarization have dealt with stimuli that appear to vary azimuthally. This is mainly due to the constraint that the typically available degree of freedom to manipulate the phase shift of light rotates the perceived pattern around a person's point of fixation. Here we create a structured light stimulus that is perceived to vary purely along the radial direction and test discrimination sensitivity to inwards and outwards radial motion. This is accomplished by preparing a radial state coupled to an orbital angular momentum state that matches the orientation of the dichroic elements in the macula. The presented methods offering a new dimension of exploration serve as a direct compliment to previous studies and may provide new insights into characterizing macular pigment density profiles and assessing the health of the macula.

physics.med-ph↗

arXiv2023

Roadmap on structured waves

Structured waves are ubiquitous for all areas of wave physics, both classical and quantum, where the wavefields are inhomogeneous and cannot be approximated by a single plane wave. Even the interference of two plane waves, or a single inhomogeneous (evanescent) wave, provides a number of nontrivial phenomena and additional functionalities as compared to a single plane wave. Complex wavefields with inhomogeneities in the amplitude, phase, and polarization, including topological structures and singularities, underpin modern nanooptics and photonics, yet they are equally important, e.g., for quantum matter waves, acoustics, water waves, etc. Structured waves are crucial in optical and electron microscopy, wave propagation and scattering, imaging, communications, quantum optics, topological and non-Hermitian wave systems, quantum condensed-matter systems, optomechanics, plasmonics and metamaterials, optical and acoustic manipulation, and so forth. This Roadmap is written collectively by prominent researchers and aims to survey the role of structured waves in various areas of wave physics. Providing background, current research, and anticipating future developments, it will be of interest to a wide cross-disciplinary audience.

physics.optics↗

arXiv2022

Quantum Information Approach to the Implementation of a Neutron Cavity

Using the quantum information model of dynamical diffraction we consider a neutron cavity composed of two perfect crystal silicon blades capable of containing the neutron wavefunction. We show that the internal confinement of the neutrons through Bragg diffraction can be modelled by a quantum random walk. Good agreement is found between the simulation and the experimental implementation. Analysis of the standing neutron waves is presented in regards to the crystal geometry and parameters; and the conditions required for well-defined bounces are derived. The presented results enable new approaches to studying the setups utilizing neutron confinement, such as the experiments to measure neutron magnetic and electric dipole moments.

quant-ph↗

arXiv2022

Skyrmion Alignment and Pinning Effects in a Disordered Multi-Phase Skyrmion Material Co8Zn8Mn4

Underlying disorder in skyrmion materials may both inhibit and facilitate skyrmion reorientations and changes in topology. The identification of these disorder-induced topologically active regimes is critical to realizing robust skyrmion spintronic implementations, yet few studies exist for disordered bulk samples. Here, we employ small-angle neutron scattering (SANS) and micromagnetic simulations to examine the influence of skyrmion order on skyrmion lattice formation, transition, and reorientation dynamics across the phase space of a disordered polycrystalline Co$_{8}$Zn$_{8}$Mn$_{4}$ bulk sample. Our measurements reveal a new disordered-to-ordered skyrmion square lattice transition pathway characterized by the novel promotion of four-fold order in SANS and accompanied by a change in topology of the system, reinforced through micromagnetic simulations. Pinning responses are observed to dominate skyrmion dynamics in the metastable triangular lattice phase, enhancing skyrmion stabilization through a remarkable and previously undetected skyrmion memory effect which reproduces previous ordering processes and persists in zero field. These results uncover the cooperative interplay of anisotropy and disorder in skyrmion formation and restructuring dynamics, establishing new tunable pathways for skyrmion manipulation.

cond-mat.mtrl-sci↗

arXiv2022

Three-Dimensional Neutron Far-Field Tomography of a Bulk Skyrmion Lattice

Skyrmions are topologically-protected spin textures thought to nucleate and annihilate on points of vanishing magnetization, called Bloch points. However, owing to a lack of bulk techniques, experimental visualizations of skyrmion lattices and their stabilization through defects in three-dimensions remain elusive. Here, we present a tomographic algorithm applied to a Co$_8$Zn$_8$Mn$_4$ skyrmion lattice host, processing multi-projection small angle neutron scattering measurements to generate mean scattering feature reconstructions (MSFR) of the bulk spin textures. Digital phantoms validated the algorithm; reconstructions of the sample show a disordered skyrmion lattice with a topological saturation of 63~\%, exhibiting three-dimensional topological transitions through two different emergent (anti)monopole defect pathways with densities of 147~$μ$m$^{-3}$ and 21~$μ\mathrm{m}^{-3}$ for branching and segmentation events, respectively. Our techniques produce experimentally-informed visualizations of bulk skyrmion lattice structures and defects, enabling future bulk studies over a wide variety of sample shapes and chemistries, magnetic phases, and external parameters.

cond-mat.mtrl-sci↗

arXiv2022

Experimental Realization of Neutron Helical Waves

Methods of preparation and analysis of structured waves of light, electrons, and atoms have been advancing rapidly. Despite the proven power of neutrons for material characterization and studies of fundamental physics, neutron science has not been able to fully integrate such techniques due to small transverse coherence lengths, the relatively poor resolution of spatial detectors, and low fluence rates. Here, we demonstrate methods that are practical with the existing technologies, and show the experimental achievement of neutron helical wavefronts that carry well-defined orbital angular momentum (OAM) values. We discuss possible applications and extensions to spin-orbit correlations and material characterization techniques.

physics.app-ph↗

arXiv2021

Next-generation high transmission neutron optical devices utilizing micro-machined structures

Neutrons have emerged as a unique probe at the forefront of modern material science, unrivaled in their penetrating abilities. A major challenge stems from the fact that neutron optical devices are limited to refractive indices on the order of $n\approx 1 \pm 10^{-5}$. By exploiting advances in precision manufacturing, we have designed and constructed a micro-meter period triangular grating with a high aspect ratio of $14.3$. The manufacturing quality is demonstrated with white-light interferometric data and microscope imaging. Neutron scattering experiment results are presented, showing agreement to refraction modelling. The capabilities of neutron Fresnel lenses based on this design are contrasted to existing neutron focusing techniques and the path separation of a prism-based neutron interferometer is estimated.

physics.app-ph↗

arXiv2021

Generalizing the Quantum Information Model for Dynamic Diffraction

The development of novel neutron optics devices that rely on perfect crystals and nano-scale features are ushering a new generation of neutron science experiments, from fundamental physics to material characterization of emerging quantum materials. However, the standard theory of dynamical diffraction (DD) that analyzes neutron propagation through perfect crystals does not consider complex geometries, deformations, and/or imperfections which are now becoming a relevant systematic effect in high precision interferometric experiments. In this work, we expand upon a quantum information (QI) model of DD that is based on propagating a particle through a lattice of unitary quantum gates. We show that the model output is mathematically equivalent to the spherical wave solution of the Takagi-Taupin equations when in the appropriate limit, and that the model can be extended to the Bragg as well as the Laue-Bragg geometry where it is consistent with experimental data. The presented results demonstrate the universality of the QI model and its potential for modeling scenarios that are beyond the scope of the standard theory of DD.

quant-ph↗

arXiv2020

Characterization of a Disordered Above Room Temperature Skyrmion Material Co8Zn8Mn4

Topologically non trivial spin textures host great promise for future spintronic applications. Skyrmions in particular are of burgeoning interest owing to their nanometric size, topological protection, and high mobility via ultra-low current densities. It has been previously reported through magnetic susceptibility, microscopy, and scattering techniques that Co$_{8}$Zn$_{8}$Mn$_{4}$ forms an above room temperature triangular skyrmion lattice. Here we report the synthesis procedure and characterization of a polycrystalline Co$_{8}$Zn$_{8}$Mn$_{4}$ bulk sample. We employ powder x-ray diffraction, backscatter Laue diffraction, and neutron diffraction as characterization tools of the crystallinity of the samples, while magnetic susceptibility and Small Angle Neutron Scattering (SANS) measurements are performed to study the skyrmion phase. Magnetic susceptibility measurements show a dip anomaly in the magnetization curves which persists over a range of approximately 305 K- 315 K. SANS measurements reveal a rotationally disordered polydomain skymrion lattice. Applying a recently developed symmetry-breaking magnetic field sequence, we were able to orient and order the previously jammed state to yield the prototypical hexagonal diffraction patterns, with secondary diffraction rings.

cond-mat.mtrl-sci↗

arXiv2019

Direct discrimination of structured light by humans

We predict and experimentally verify an entoptic phenomenon through which humans are able to perceive and discriminate structured light with space-varying polarization. Direct perception and discrimination is possible through the observation of distinct profiles induced by the interaction between the polarization gradients in a uniform-intensity beam and the radially symmetric dichroic elements that are centered on the foveola in the macula of the human eye. A psychophysical study was conducted where optical states with coupled polarization and orbital angular momentum (OAM) were directed onto the retina of participants. The participants were able to correctly discriminate between two states, differentiated by OAM =\pm7, with an average success probability of 77.6 % (average sensitivity d^\prime=1.7, t(9) = 5.9, p = 2\times 10^{-4}). These results enable new methods of robustly characterizing the structure of the macula, probing retina signalling pathways, and conducting experiments with non-separable optical states and human detectors.

physics.optics↗

arXiv2019

Generation and detection of spin-orbit coupled neutron beams

Spin-orbit coupling of light has come to the fore in nano-optics and plasmonics, and is a key ingredient of topological photonics and chiral quantum optics. We demonstrate a basic tool for incorporating analogous effects into neutron optics: the generation and detection of neutron beams with coupled spin and orbital angular momentum. $^3$He neutron spin-filters are used in conjunction with specifically oriented triangular coils to prepare neutron beams with lattices of spin-orbit correlations, as demonstrated by their spin-dependant intensity profiles. These correlations can be tailored to particular applications, such as neutron studies of topological materials.

quant-ph↗