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D. Gershoni

Publications and source records attributed to D. Gershoni.

36 records · Page 2Linked to original sources

Spontaneously Localized Photonic Modes Due to Disorder in the Dielectric Constant

We present the first experimental evidence for the existence of strongly localized photonic modes due to random two dimensional fluctuations in the dielectric constant. In one direction, the modes are trapped by ordered Bragg reflecting mirrors of a planar, one wavelength long, microcavity. In the cavity plane, they are localized by disorder, which is due to randomness in the position, composition and sizes of quantum dots located in the anti-node of the cavity. We extend the theory of disorder induced strong localization of electron states to optical modes and obtain quantitative agreement with the main experimental observations.

cond-mat.mes-hall↗

Radiative cascades in charged quantum dots

We measured, for the first time, two photon radiative cascades due to sequential recombination of quantum dot confined electron hole pairs in the presence of an additional spectator charge carrier. We identified direct, all optical cascades involving spin blockaded intermediate states, and indirect cascades, in which non radiative relaxation precedes the second recombination. Our measurements provide also spin dephasing rates of confined carriers.

cond-mat.mes-hall↗

Polarization memory in single Quantum Dots

We measured the polarization memory of excitonic and biexcitonic optical transitions from single quantum dots at either positive, negative or neutral charge states. Positive, negative and no circular or linear polarization memory was observed for various spectral lines, under the same quasi-resonant excitation below the wetting layer band-gap. We developed a model which explains both qualitatively and quantitatively the experimentally measured polarization spectrum for all these optical transitions. We consider quite generally the loss of spin orientation of the photogenerated electron-hole pair during their relaxation towards the many-carrier ground states. Our analysis unambiguously demonstrates that while electrons maintain their initial spin polarization to a large degree, holes completely dephase.

cond-mat.mes-hall↗

Distilling entanglement from cascades with partial "Which Path" ambiguity

We develop a framework to calculate the density matrix of a pair of photons emitted in a decay cascade with partial "which path" ambiguity. We describe an appropriate entanglement distillation scheme which works also for certain random cascades. The qualitative features of the distilled entanglement are presented in a two dimensional "phase diagram". The theory is applied to the quantum tomography of the decay cascade of a biexciton in a semiconductor quantum dot. Agreement with experiment is obtained.

quant-ph↗

Entanglement on demand through time reordering

Entangled photons can be generated "on demand" in a novel scheme involving unitary time reordering of the photons emitted in a radiative decay cascade. The scheme yields polarization entangled photon pairs, even though prior to reordering the emitted photons carry significant "which path information" and their polarizations are unentangled. This shows that quantum chronology can be manipulated in a way that is lossless and deterministic (unitary). The theory can, in principle, be tested and applied to the biexciton cascade in semiconductor quantum dots.

quant-ph↗

Polarization sensitive spectroscopy of charged Quantum Dots

We present an experimental and theoretical study of the polarized photoluminescence spectrum of single semiconductor quantum dots in various charge states. We compare our high resolution polarization sensitive spectral measurements with a new many-carrier theoretical model, which was developed for this purpose. The model considers both the isotropic and anisotropic exchange interactions between all participating electron-hole pairs. With this addition, we calculate both the energies and polarizations of all optical transitions between collective, quantum dot confined charge carrier states. We succeed in identifying most of the measured spectral lines. In particular, the lines resulting from singly-, doubly- and triply- negatively charged excitons and biexcitons. We demonstrate that lines emanating from evenly charged states are linearly polarized. Their polarization direction does not necessarily coincide with the traditional crystallographic direction. It depends on the shells of the single carriers, which participate in the recombination process.

cond-mat.mes-hall↗

Entangled Photon Pairs from Semiconductor Quantum Dots

Tomographic analysis demonstrates that the polarization state of pairs of photons emitted from a biexciton decay cascade becomes entangled when spectral filtering is applied. The measured density matrix of the photon pair satisfies the Peres criterion for entanglement by more than 3 standard deviations of the experimental uncertainty and violates Bell's inequality. We show that the spectral filtering erases the ``which path'' information contained in the photons color and that the remanent information in the quantum dot degrees of freedom is negligible.

quant-ph↗

Emission characteristics of quantum dots in planar microcavities

The emission properties of single quantum dots in planar microcavities are studied experimentally and theoretically. Fivefold Enhanced spontaneous emission outside the microcavity is found for dots in resonance with the cavity mode, relative to detuned dots, while their radiative lifetime is only marginally decreased. Using high power excitation we obtain the in-plane cavity dispersion. Near field images of the emission show spatial distributions of several microns for resonant dots, which decrease in size with the detuning from resonance. These experimental findings are explained using a simple and intuitive model.

cond-mat.mes-hall↗

Polarized fine structure in the excitation spectrum of a negatively charged quantum dot

We report polarized photoluminescence excitation spectroscopy of the negative trion in single charge tunable InAs/GaAs quantum dots. The spectrum exhibits a p-shell resonance with polarized fine structure arising from the direct excitation of the electron spin triplet states. The energy splitting arises from the axially symmetric electron-hole exchange interaction. The magnitude and sign of the polarization are understood from the spin character of the triplet states and a small amount of quantum dot asymmetry, which mixes the wavefunctions through asymmetric e-e and e-h exchange interactions.

cond-mat.other↗

Optical pumping of electronic and nuclear spin in single charge-tunable quantum dots

We present a comprehensive examination of optical pumping of spins in individual GaAs quantum dots as we change the charge from positive to neutral to negative using a Schottky diode. We observe that photoluminescence polarization memory has the same sign as the net charge of the dot. Optical pumping of ground state electron spins enhances this effect, as demonstrated through the first measurements of the Hanle effect on an individual quantum dot. With the Overhauser effect in a high longitudinal magnetic field, we demonstrate efficient optical pumping of the quantum dot's nuclear spins for all three charge states.

cond-mat.mtrl-sci↗

Ultrasmall In(Ga)As Quantum Dots Grown on Strained GaxIn1-xP Layers

InAs self-assembled quantum dots were grown on strained layers of GaxIn1-xP (0 < x < 0.3) on InP substrates. We show that the quantum dots have narrow vertical dimensions, ranging between 2 to 10 monolayers only. The dot layer photoluminescence spectrum is composed of distinct spectral peaks, resulting from the discrete distribution of the dot heights. The dot height distribution depends on the total amount of InAs deposited and on the Ga content of the strained GaxIn1-xP layer underneath. Our experimental results are corroborated by an 8 band k(dot)P model calculations. In particular, we identify and quantify the diffusion of Ga from the GaxIn1-xP layer into the quantum dots.

cond-mat↗

Semiconductor quantum dot - a quantum light source of multicolor photons with tunable statistics

We investigate the intensity correlation properties of single photons emitted from an optically excited single semiconductor quantum dot. The second order temporal coherence function of the photons emitted at various wavelengths is measured as a function of the excitation power. We show experimentally and theoretically, for the first time, that a quantum dot is not only a source of correlated non-classical monochromatic photons but is also a source of correlated non-classical \emph{multicolor} photons with tunable correlation properties. We found that the emitted photon statistics can be varied by the excitation rate from a sub-Poissonian one, where the photons are temporally antibunched, to super-Poissonian, where they are temporally bunched.

cond-mat.str-el↗

Optical spectroscopy of single quantum dots at tunable positive, neutral and negative charge states

We report on the observation of photoluminescence from positive, neutral and negative charge states of single semiconductor quantum dots. For this purpose we designed a structure enabling optical injection of a controlled unequal number of negative electrons and positive holes into an isolated InGaAs quantum dot embedded in a GaAs matrix. Thereby, we optically produced the charge states -3, -2, -1, 0, +1 and +2. The injected carriers form confined collective 'artificial atoms and molecules' states in the quantum dot. We resolve spectrally and temporally the photoluminescence from an optically excited quantum dot and use it to identify collective states, which contain charge of one type, coupled to few charges of the other type. These states can be viewed as the artificial analog of charged atoms such as H$^{-}$, H$^{-2}$, H$^{-3}$, and charged molecules such as H$_{2}^{+}$ and H$_{3}^{+2}$. Unlike higher dimensionality systems, where negative or positive charging always results in reduction of the emission energy due to electron-hole pair recombination, in our dots, negative charging reduces the emission energy, relative to the charge-neutral case, while positive charging increases it. Pseudopotential model calculations reveal that the enhanced spatial localization of the hole-wavefunction, relative to that of the electron in these dots, is the reason for this effect.

cond-mat↗

Spectroscopy of a single semiconductor quantum dot at negative and positive discrete charge states

We study optically single self-assembled quantum dots embedded within the wide quantum well of a mixed type quantum structure. We compare the steady state and pulsed photoluminescence spectra of these dots to those of previously studied "regular" dots. We unambiguously identify experimentally emission from various discrete charge state of the dots. We provide means for optically tune the charge state of the dot, both negatively and positively. Our observations are used to accurately determine the asymmetry between the quantum dots' confined electron and hole envelope wavefunctions.

cond-mat.mtrl-sci↗

Radiative Lifetimes of Single Excitons in Semiconductor Quantum Dots- Manifestation of the Spatial Coherence Effect

Using time correlated single photon counting combined with temperature dependent diffraction limited confocal photoluminescence spectroscopy we accurately determine, for the first time, the intrinsic radiative lifetime of single excitons confined within semiconductor quantum dots. Their lifetime is one (two) orders of magnitude longer than the intrinsic radiative lifetime of single excitons confined in semiconductor quantum wires (wells) of comparable confining dimensions. We quantitatively explain this long radiative time in terms of the reduced spatial coherence between the confined exciton dipole moment and the radiation electromagnetic field.

cond-mat.mtrl-sci↗

Carrier-Carrier Correlations in an Optically Excited Single Semiconductor Quantum Dot

We applied low temperature diffraction limited confocal optical microscopy to spatially resolve, and spectroscopically study photoluminescence from single self-assembled semiconductor quantum dots. Using selective wavelength imaging we unambiguously demonstrated that a single photoexcited quantum dot emits light in a few very narrow spectral lines. The measured spectrum and its dependence on the power of either cw or pulsed excitation are explained by taking carrier correlations into account. We solve numerically a many body Hamiltonian for a model quantum dot, and we show that the multi line emission spectrum is due to optical transitions between confined exciton multiplexes. We furthermore show that the electron-electron and hole-hole exchange interaction is responsible for the typical appearance of pairs in the photoluminescence spectra and for the appearance of red shifted new lines as the excitation power increases. The fact that only a few spectral lines appear in the emission spectrum strongly indicates fast thermalization. This means that a multiexciton relaxes to its ground state much faster than its radiative lifetime.

cond-mat.str-el↗

Multi-Exciton Spectroscopy of a Single Self Assembled Quantum Dot

We apply low temperature confocal optical microscopy to spatially resolve, and spectroscopically study a single self assembled quantum dot. By comparing the emission spectra obtained at various excitation levels to a theoretical many body model, we show that: Single exciton radiative recombination is very weak. Sharp spectral lines are due to optical transitions between confined multiexcitonic states among which excitons thermalize within their lifetime. Once these few states are fully occupied, broad bands appear due to transitions between states which contain continuum electrons.

cond-mat.str-el↗