arXiv subjects

D. H. Lu

Publications and source records attributed to D. H. Lu.

At least 55 records · Page 3Linked to original sources

arXiv2010

Strong energy-momentum dispersion of phonon-dressed carriers in the lightly doped band insulator SrTiO$_3$

Much progress has been made recently in the study of the effects of electron-phonon (el-ph) coupling in doped insulators using angle resolved photoemission (ARPES), yielding evidence for the dominant role of el-ph interactions in underdoped cuprates. As these studies have been limited to doped Mott insulators, the important question arises how this compares with doped band insulators where similar el-ph couplings should be at work. The archetypical case is the perovskite SrTiO$_3$ (STO), well known for its giant dielectric constant of 10000 at low temperature, exceeding that of La$_2$CuO$_4$ by a factor of 500. Based on this fact, it has been suggested that doped STO should be the archetypical bipolaron superconductor. Here we report an ARPES study from high-quality surfaces of lightly doped SrTiO$_3$. Comparing to lightly doped Mott insulators, we find the signatures of only moderate electron-phonon coupling: a dispersion anomaly associated with the low frequency optical phonon with a $λ'\sim0.3$ and an overall bandwidth renormalization suggesting an overall $λ'\sim0.7$ coming from the higher frequency phonons. Further, we find no clear signatures of the large pseudogap or small polaron phenomena. These findings demonstrate that a large dielectric constant itself is not a good indicator of el-ph coupling and highlight the unusually strong effects of the el-ph coupling in doped Mott insulators.

cond-mat.str-el↗

arXiv2010

Characteristic electronic structure and its doping evolution in lightly-doped to underdoped YBa2Cu3Oy

We have performed an angle resolved photoemission spectroscopy (ARPES) study of lightly-doped to underdoped YBa2Cu3Oy (YBCO) untwinned single crystals and a core-level x-ray photoemission spectroscopy (XPS) study of YBCO single and polycrystals. In the zone diagonal (nodal) direction, dispersive quasi-particle (QP) features crossing the Fermi level were observed down to the hole concentration of ~ 4%, which explains the metallic transport of the lightly-doped YBCO. The chemical potential shift estimated from XPS was more rapid than in the Bi2212 cuprates. Upon hole doping, very rapid spectral weight transfer from high binding energies to the QP feature, even faster than La2-xSrxCuO4, was observed.

cond-mat.supr-con↗

arXiv2009

Effect of strong correlations on the high energy anomaly in hole- and electron-doped high-Tc superconductors

Recently, angle-resolved photoemission spectroscopy (ARPES) has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy 'waterfall' or high energy anomaly (HEA). This paper demonstrates, using a combination of new ARPES measurements and quantum Monte Carlo simulations, that the HEA is not simply the by-product of matrix element effects, but rather represents a cross-over from a quasiparticle band at low binding energies near the Fermi level to valence bands at higher binding energy, assumed to be of strong oxygen character, in both hole- and electron-doped cuprates. While photoemission matrix elements clearly play a role in changing the aesthetic appearance of the band dispersion, i.e. the 'waterfall'-like behavior, they provide an inadequate description for the physics that underlies the strong band renormalization giving rise to the HEA. Model calculations of the single-band Hubbard Hamiltonian showcase the role played by correlations in the formation of the HEA and uncover significant differences in the HEA energy scale for hole- and electron-doped cuprates. In addition, this approach properly captures the transfer of spectral weight accompanying both hole and electron doping in a correlated material and provides a unifying description of the HEA across both sides of the cuprate phase diagram.

cond-mat.str-el↗

arXiv2009

Unconventional electronic reconstruction in undoped (Ba,Sr)Fe$_2$As$_2$ across the spin density wave transition

Through a systematic high resolution angle-resolved photoemission study of the iron pnictide compounds (Ba,Sr)Fe$_2$As$_2$, we show that the electronic structures of these compounds are significantly reconstructed across the spin density wave ordering, which cannot be described by a simple folding scenario of conventional density wave ordering. Moreover, we find that LDA calculations with an incorporated suppressed magnetic moment of 0.5$μ_{\tiny{\textrm{B}}}$ can match well the details in the reconstructed electronic structure, suggesting that the nature of magnetism in the pnictides is more itinerant than local, while the origin of suppressed magnetic moment remains an important issue for future investigations.

cond-mat.supr-con↗

arXiv2009

Dependence of Band Renormalization Effect on the Number of Copper-oxide Layers in Tl-based Copper-oxide Superconductor using Angle-resolved Photoemission Spectroscopy

Here we report the first angle-resolved photoemission measurement on nearly optimally-doped multi-layer Tl-based superconducting cuprates (Tl-2212 and Tl-1223) and a comparison study to single layer (Tl-2201) compound. A "kink" in the band dispersion is found in all three compounds but exhibits different momentum dependence for the single layer and multi-layer compounds, reminiscent to that of Bi-based cuprates. This layer number dependent renormalization effect strongly implies that the spin resonance mode is unlikely responsible for the dramatic renormalization effect near the antinodal region.

cond-mat.supr-con↗

arXiv2009

Enhanced superconducting gaps in the tri-layer high-$T_c$ cuprate Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$

We have investigated the optimally doped tri-layer cuprate Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ (Bi2223) by angle-resolved photoemission spectroscopy, and observed energy bands and Fermi surfaces originated from the outer and inner CuO$_2$ planes (OP and IP) separately. The OP band is overdoped (hole density $\sim$ 0.26/Cu) with a large d-wave gap of $Δ_0$ $\sim$ 43 meV while the IP is underdoped ($\sim$ 0.06/Cu) with an even large gap of $Δ_0$ $\sim$ 60 meV. We propose that the enhancement of the $Δ_0$ of IP is due to the minimal influence of out-of-plane disorder and that the OP gap is then enhanced through interlayer coupling, most likely a proximity effect from the IP.

cond-mat.supr-con↗

arXiv2009

Effects of out-of-plane disorder on the nodal quasiparticle and superconducting gap in single-layer Bi$_2$Sr$_{1.6}Ln_{0.4}$CuO$_{6+δ}$ ($Ln$ = La, Nd, Gd)

How out-of-plane disorder affects the electronic structure has been investigated for the single-layer cuprates Bi$_2$Sr$_{1.6}$$Ln$$_{0.4}$CuO$_{6+δ}$ ($Ln$ = La, Nd, Gd) by angle-resolved photoemission spectroscopy. We have observed that, with increasing disorder, while the Fermi surface shape and band dispersions are not affected, the quasi-particle width increases, the anti-nodal gap is enhanced and the superconducting gap in the nodal region is depressed. The results indicate that the superconductivity is significantly depressed by out-of-plane disorder through the enhancement of the anti-nodal gap and the depression of the superconducting gap in the nodal region.

cond-mat.supr-con↗

arXiv2009

Large Gap Topological Insulator Bi2Te3 with a Single Dirac Cone on the Surface

We investigate the surface state of Bi$_2$Te$_3$ using angle resolved photoemission spectroscopy (ARPES) and transport measurements. By scanning over the entire Brillouin zone (BZ), we demonstrate that the surface state consists of a single non-degenerate Dirac cone centered at the $Γ$ point. Furthermore, with appropriate hole (Sn) doping to counteract intrinsic n-type doping from vacancy and anti-site defects, the Fermi level can be tuned to intersect only the surface states, indicating a full energy gap for the bulk states, consistent with a carrier sign change near this doping in transport properties. Our experimental results establish for the first time that Bi$_2$Te$_3$ is a three dimensional topological insulator with a single Dirac cone on the surface, as predicted by a recent theory.

cond-mat.mtrl-sci↗

arXiv2009

Light scalar mesons in QCD sum rules with inclusion of instantons

The light scalar meson nonet above 1 GeV ({\it i.e.\}the $a_{0}$, $K^{\ast}_{0}$ and $f_{0}$) are studied within the framework of QCD sum rules. In conventional QCD sum rules, the calculated masses of this nonet are degenerate, and the mass of $K^{\ast}_{0}$ is always larger than the $a_{0}$ in contradiction with the observed spectrum. After improving the correlation function by including instanton effects, the masses are well separated from each other. In particular, our results shows glueball content plays an important role in the underlying structure of $f_{0}(1500)$. The decay constants are also discussed.

hep-ph↗

arXiv2009

Electronic Structure of the BaFe$_2$As$_2$ Family of Iron Pnictides

We use high resolution angle-resolved photoemission spectroscopy to study the band structure and Fermi surface topology of the BaFe$_2$As$_2$ iron pnictides. We observe two electron bands and two hole bands near the X-point, $(π,π)$ of the Brillouin zone, in the paramagnetic state for different doping levels, including electron-doped Ba(Co$_{0.06}$Fe$_{0.94}$)$_2$As$_2$, undoped BaFe$_2$As$_2$, and hole-doped Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$. Among these four bands, only the electron bands cross the Fermi level, forming two electron pockets around X, while the hole bands approach but never reach the Fermi level. We show that the band structure of the BaFe$_2$As$_2$ family matches reasonably well with the prediction of LDA calculations after a momentum-dependent shift and renormalization. Our finding resolves a number of inconsistencies regarding the electronic structure of pnictides.

cond-mat.supr-con↗

arXiv2009

ARPES studies of the electronic structure of LaOFe(P,As)

We report a comparison study of LaOFeP and LaOFeAs, two parent compounds of recently discovered iron-pnictide superconductors, using angle-resolved photoemission spectroscopy. Both systems exhibit some common features that are very different from well-studied cuprates. In addition, important differences have also been observed between these two ferrooxypnictides. For LaOFeP, quantitative agreement can be found between our photoemission data and the LDA band structure calculations, suggesting that a weak coupling approach based on an itinerant ground state may be more appropriate for understanding this new superconducting compound. In contrast, the agreement between LDA calculations and experiments in LaOFeAs is relatively poor, as highlighted by the unexpected Fermi surface topology around (pi,pi). Further investigations are required for a comprehensive understanding of the electronic structure of LaOFeAs and related compounds.

cond-mat.supr-con↗

arXiv2008

Fermi Surface Evolution Across Multiple Charge Density Wave Transitions in ErTe3

The Fermi surface (FS) of ErTe3 is investigated using angle-resolved photoemission spectroscopy (ARPES). Low temperature measurements reveal two incommensurate charge density wave (CDW) gaps created by perpendicular FS nesting vectors. A large Delta_1 = 175 meV gap arising from a CDW with c* - q_CDW1 ~ 0.70(0) c* is in good agreement with the expected value. A second, smaller Delta_2 = 50 meV gap is due to a second CDW with a* - q_CDW2 ~ 0.68(5) a*. The temperature dependence of the FS, the two gaps and possible interaction between the CDWs are examined.

cond-mat.str-el↗

arXiv2008

Doping dependent charge transfer gap and realistic electronic model of n-type cuprate superconductors

Based on the analysis of the measurement data of angle-resolved photoemission spectroscopy (ARPES) and optics, we show that the charge transfer gap is significantly smaller than the optical one and is reduced by doping in electron doped cuprate superconductors. This leads to a strong charge fluctuation between the Zhang-Rice singlet and the upper Hubbard bands. The basic model for describing this system is a hybridized two-band $t$-$J$ model. In the symmetric limit where the corresponding intra- and inter-band hopping integrals are equal to each other, this two-band model is equivalent to the Hubbard model with an antiferromagnetic exchange interaction (i.e. the $t$-$U$-$J$ model). The mean-field result of the $t$-$U$-$J$ model gives a good account for the doping evolution of the Fermi surface and the staggered magnetization.

cond-mat.supr-con↗

arXiv2008

Electronic structure of the iron-based superconductor LaOFeP

The recent discovery of superconductivity in the so-called iron-oxypnictide family of compounds has generated intense interest. The layered crystal structure with transition metal ions in planar square lattice form and the discovery of spin-density-wave order near 130 K seem to hint at a strong similarity with the copper oxide superconductors. A burning current issue is the nature of the ground state of the parent compounds. Two distinct classes of theories have been put forward depending on the underlying band structures: local moment antiferromagnetic ground state for strong coupling approach and itinerant ground state for weak coupling approach. The local moment magnetism approach stresses on-site correlations and proximity to a Mott insulating state and thus the resemblance to cuprates; while the latter approach emphasizes the itinerant electron physics and the interplay between the competing ferromagnetic and antiferromagnetic fluctuations. Such a controversy is partly due to the lack of conclusive experimental information on the electronic structures. Here we report the first angle-resolved photoemission spectroscopy (ARPES) investigation of LaOFeP (Tc = 5.9 K), the first reported iron-based superconductor. Our results favor the itinerant ground state, albeit with band renormalization. In addition, our data reveal important differences between these and copper based superconductors.

cond-mat.supr-con↗

arXiv2008

Fermi surface and van Hove singularities in the itinerant metamagnet Sr3Ru2O7

The low-energy electronic structure of the itinerant metamagnet Sr3Ru2O7 is investigated by angle resolved photoemission and density functional calculations. We find well-defined quasiparticle bands with resolution limited line widths and Fermi velocities up to an order of magnitude lower than in single layer Sr2RuO4. The complete topography, the cyclotron masses and the orbital character of the Fermi surface are determined, in agreement with bulk sensitive de Haas - van Alphen measurements. An analysis of the dxy band dispersion reveals a complex density of states including van Hove singularities (vHs) near the Fermi level; a situation which is favorable for magnetic instabilities.

cond-mat.str-el↗

arXiv2008

Superconductivity-Induced Self-Energy Evolution of the Nodal Electron of Optimally-Doped Bi2212

The temperature dependent evolution of the renormalization effect in optimally-doped Bi2212 along the nodal direction has been studied via angle-resolved photoemission spectroscopy. Fine structure is observed in the real part of the self-energy (Re$Σ$), including a subkink and maximum, suggesting that electrons couple to a spectrum of bosonic modes, instead of just one mode. Upon cooling through the superconducting phase transition, the fine structures of the extracted Re$Σ$ exhibit a two-processes evolution demonstrating an interplay between kink renormalization and superconductivity. We show that this two-process evolution can be qualitatively explained by a simple Holstein model in which a spectrum of bosonic modes is considered.

cond-mat.supr-con↗

arXiv2008

Doping evolution of the electronic structure in the single-layer cuprates Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$: Comparison with other single-layer cuprates

We have performed angle-resolved photoemission and core-level x-ray photoemission studies of the single-layer cuprate Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$ (Bi2201) and revealed the doping evolution of the electronic structure from the lightly-doped to optimally-doped regions. We have observed the formation of the dispersive quasi-particle band, evolution of the Fermi ``arc'' into the Fermi surface and the shift of the chemical potential with hole doping as in other cuprates. The doping evolution in Bi2201 is similar to that in Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_2$ (Na-CCOC), where a rapid chemical potential shift toward the lower Hubbard band of the parent insulator has been observed, but is quite different from that in La$_{2-x}$Sr$_{x}$CuO$_{4}$ (LSCO), where the chemical potential does not shift, yet the dispersive band and the Fermi arc/surface are formed around the Fermi level already in the lightly-doped region. The (underlying) Fermi surface shape and band dispersions are quantitatively analyzed using tight-binding fit, and the deduced next-nearest-neighbor hopping integral $t'$ also confirm the similarity to Na-CCOC and the difference from LSCO.

cond-mat.supr-con↗

arXiv2008

Extracting the spectral function of the cuprates by a full two-dimensional analysis: Angle-resolved photoemission spectra of Bi2Sr2CuO6

Recently, angle-resolved photoemission spectroscopy (ARPES) has revealed a dispersion anomaly at high binding energy near 0.3-0.5eV in various families of the high-temperature superconductors. For further studies of this anomaly we present a new two-dimensional fitting-scheme and apply it to high-statistics ARPES data of the strongly-overdoped Bi2Sr2CuO6 cuprate superconductor. The procedure allows us to extract theself-energy in an extended energy and momentum range. It is found that the spectral function of Bi2Sr2CuO6 can be parameterized using a small set of tight-binding parameters and a weakly-momentum-dependent self-energy up to 0.7 eV in binding energy and over the entire first Brillouin zone. Moreover the analysis gives an estimate of the momentum dependence of the matrix element, a quantity, which is often neglected in ARPES analyses.

cond-mat.supr-con↗