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D. Habs

Publications and source records attributed to D. Habs.

At least 19 recordsLinked to original sources

Scaling of laser-driven ion energies in the relativistic transparent regime

Laser-driven ions have compelling properties and their potential use for medical applications has attracted a huge global interest. One of the major challenges of these applications is generating beams of the required energies. To date, there has been no systematic study of the effect of laser intensity on the generation of laser-driven ions from ultrathin foils during relativistic transparency. Here we present a scaling for ion energies with respect to the on-target laser intensity and in considering target thickness we find an optimum thickness closely related to the experimentally observed relativistic transparency. A steep linear scaling with the normalized laser amplitude a0 has been measured and verified with PIC simulations. In contrast to TNSA, this scaling is much steeper and has been measured for ions with Z > 1. Following our results, ion energies exceeding 100MeV/amu are already accessible with currently available laser systems enabling realization of numerous advanced applications

physics.plasm-ph

Sub-millimeter nuclear medical imaging with high sensitivity in positron emission tomography using beta-gamma coincidences

We present a nuclear medical imaging technique, employing triple-gamma trajectory intersections from beta^+ - gamma coincidences, able to reach sub-millimeter spatial resolution in 3 dimensions with a reduced requirement of reconstructed intersections per voxel compared to a conventional PET reconstruction analysis. This '$γ$-PET' technique draws on specific beta^+ - decaying isotopes, simultaneously emitting an additional photon. Exploiting the triple coincidence between the positron annihilation and the third photon, it is possible to separate the reconstructed 'true' events from background. In order to characterize this technique, Monte-Carlo simulations and image reconstructions have been performed. The achievable spatial resolution has been found to reach ca. 0.4 mm (FWHM) in each direction for the visualization of a 22Na point source. Only 40 intersections are sufficient for a reliable sub-millimeter image reconstruction of a point source embedded in a scattering volume of water inside a voxel volume of about 1 mm^3 ('high-resolution mode'). Moreover, starting with an injected activity of 400 MBq for ^76Br, the same number of only about 40 reconstructed intersections are needed in case of a larger voxel volume of 2 x 2 x 3~mm^3 ('high-sensitivity mode'). Requiring such a low number of reconstructed events significantly reduces the required acquisition time for image reconstruction (in the above case to about 140 s) and thus may open up the perspective for a quasi real-time imaging.

physics.med-ph

Ultrasmall divergence of laser-driven ion beams from nanometer thick foils

We report on experimental studies of divergence of proton beams from nanometer thick diamond-like carbon (DLC) foils irradiated by an intense laser with high contrast. Proton beams with extremely small divergence (half angle) of 2 degree are observed in addition with a remarkably well-collimated feature over the whole energy range, showing one order of magnitude reduction of the divergence angle in comparison to the results from micrometer thick targets. We demonstrate that this reduction arises from a steep longitudinal electron density gradient and an exponentially decaying transverse profile at the rear side of the ultrathin foils. Agreements are found both in an analytical model and in particle-in-cell simulations. Those novel features make nm foils an attractive alternative for high flux experiments relevant for fundamental research in nuclear and warm dense matter physics.

physics.plasm-ph

Exploring the multi-humped fission barrier of 238U via sub-barrier photofission

The photofission cross-section of 238U was measured at sub-barrier energies as a function of the gamma-ray energy using, for the first time, a monochromatic, high-brilliance, Compton-backscattered gamma-ray beam. The experiment was performed at the High Intensity gamma-ray Source (HIgS) facility at beam energies between E=4.7 MeV and 6.0 MeV and with ~3% energy resolution. Indications of transmission resonances have been observed at gamma-ray beam energies of E=5.1 MeV and 5.6 MeV with moderate amplitudes. The triple-humped fission barrier parameters of 238U have been determined by fitting EMPIRE-3.1 nuclear reaction code calculations to the experimental photofission cross section.

nucl-ex

A Quantal, Partially Ordered Electron Structure as a Basis for a γFree Electron Laser (γ-FEL)

When a rather cold electron bunch is transported during laser bubble acceleration in a strongly focusing plasma channel with typical forces of 100 GeV/m, it will form partially ordered long electron cylinders due to the relativistically longitudinal reduced repulsion between electrons, resulting in a long-range pair correlation function, when reaching energies in the laboratory above 0.5 GeV. During Compton back-scattering with a second laser, injected opposite to the electron bunch, the electron bunch will be further modulated with micro bunches and due to its ordered structure will reflect coherently, Mössbauer-like, resulting in a γfree electron laser (γ-FEL). Increasing the relativistic γfactor, the quantal regime becomes more dominant. We discuss the scaling laws with γ.

physics.acc-ph

Transmission resonance spectroscopy in the third minimum of 232Pa

The fission probability of 232Pa was measured as a function of the excitation energy in order to search for hyperdeformed (HD) transmission resonances using the (d,pf) transfer reaction on a radioactive 231Pa target. The experiment was performed at the Tandem accelerator of the Maier-Leibnitz Laboratory (MLL) at Garching using the 231Pa(d,pf) reaction at a bombarding energy of E=12 MeV and with an energy resolution of dE=5.5 keV. Two groups of transmission resonances have been observed at excitation energies of E=5.7 and 5.9 MeV. The fine structure of the resonance group at E=5.7 MeV could be interpreted as overlapping rotational bands with a rotational parameter characteristic to a HD nuclear shape. The fission barrier parameters of 232Pa have been determined by fitting TALYS 1.2 nuclear reaction code calculations to the overall structure of the fission probability. From the average level spacing of the J=4 states, the excitation energy of the ground state of the 3rd minimum has been deduced to be E(III)=5.05 MeV.

nucl-ex

The Refractive Index of Silicon at Gamma Ray Energies

The index of refraction n(E_γ)=1+δ(E_γ)+iβ(E_γ) is split into a real part δand an absorptive part β. The absorptive part has the three well-known contributions to the cross section σ_{abs}: the photo effect, the Compton effect and the pair creation, but there is also the inelastic Delbrück scattering. Second-order elastic scattering cross sections σ_{sca} with Rayleigh scattering (virtual photo effect), virtual Compton effect and Delbrück scattering (virtual pair creation) can be calculated by integrals of the Kramers-Kronig dispersion relations from the cross section σ_{abs}. The real elastic scattering amplitudes are proportional to the refractive indices δ_{photo}, δ_{Compton} and δ_{pair}. While for X-rays the negative δ_{photo} dominates, we show for the first time experimentally and theoretically that the positive δ_{pair} dominates for γrays, opening a new era of γoptics applications, i.e. of nuclear photonics.

physics.atom-ph

Medical Application Studies at ELI-NP

We study the production of radioisotopes for nuclear medicine in (gamma,gamma') photoexcitation reactions or (gamma,xn + yp) photonuclear reactions for the examples of ^195mPt, ^117mSn and ^44Ti with high flux [(10^13 - 10^15) gamma/s], small beam diameter and small energy band width (Delta E/E ~ 10^-3 -10^-4) gamma beams. In order to realize an optimum gamma-focal spot, a refractive gamma-lens consisting of a stack of many concave micro-lenses will be used. It allows for the production of a high specific activity and the use of enriched isotopes. For photonuclear reactions with a narrow gamma beam, the energy deposition in the target can be reduced by using a stack of thin target wires, hence avoiding direct stopping of the Compton electrons and e^+e^- pairs. The well-defined initial excitation energy of the compound nucleus leads to a small number of reaction channels and enables new combinations of target isotope and final radioisotope. The narrow-bandwidth gamma excitation may make use of collective resonances in gamma-width, leading to increased cross sections. (gamma,gamma') isomer production via specially selected gamma cascades allows to produce high specific activity in multiple excitations, where no back-pumping of the isomer to the ground state occurs. The produced isotopes will open the way for completely new clinical applications of radioisotopes. For example ^195mPt could be used to verify the patient's response to chemotherapy with platinum compounds before a complete treatment is performed. In targeted radionuclide therapy the short-range Auger and conversion electrons of ^195mPt and ^117mSn enable a very local treatment. The generator ^44Ti allows for a PET with an additional gamma-quantum (gamma-PET), resulting in a reduced dose or better spatial resolution.

nucl-ex

Submillimeter nuclear medical imaging with a Compton Camera using triple coincidences of collinear β+ annihilation photons and γ-rays

Modern PET systems reach a spatial resolution of 3-10 mm. A disadvantage of this technique is the diffusion of the positron before its decay with a typical range of ca. 1 mm (depending on its energy). This motion and Compton scattering of the 511 keV photons within the patient limit the performance of PET. We present a nuclear medical imaging technique, able to reach submillimeter spatial resolution in 3 dimensions with a reduced activity application compared to conventional PET. This 'gamma-PET' technique draws on specific positron sources simultaneously emitting an additional photon with the β+ decay. Exploiting the triple coincidence between the positron annihilation and the third photon, it is possible to separate the reconstructed 'true' events from background. In order to test the feasibility of this technique, Monte-Carlo simulations and image reconstruction has been performed. The spatial resolution amounts to 0.2 mm (FWHM) in each direction, surpassing the performance of conventional PET by about an order of magnitude. The simulated detector geometry exhibits a coincidence detection efficiency of 1.92e-7 per decay. Starting with only 0.7 MBq of source activity (ca. 200-500 times less compared to conventional PET) an exposure time of 450 s is sufficient for source reconstruction.

physics.ins-det

Seeded quantum FEL at 478 keV

We present for the first time the concept of a seeded γ quantum Free-Electron-Laser (QFEL) at 478 keV, which has very different properties compared to a classical. The basic concept is to produce a highly brilliant γ beam via SASE. To produce highly intense and coherent γ beam, we intend to use a seeded FEL scheme. Important for the production of such a γ beam are novel refractive γ -lenses for focusing and an efficient monochromator, allowing to generate a very intense and coherent seed beam. The energy of the γ beam is 478 keV, corresponding to a wavelength in the sub-Ångstrøm regime (1/38 Å). To realize a coherent γ beam at 478 keV, it is necessary to use a quantum FEL design. At such high radiation energies a classical description of the γ-FEL becomes wrong.

physics.acc-ph

Nuclear Photonics

With new gamma-beam facilities like MEGa-ray at LLNL (USA) or ELI-NP at Bucharest with 10^13 g/s and a bandwidth of Delta E_g/E_g ~10^-3, a new era of g-beams with energies <=20 MeV comes into operation, compared to the present world-leading HIGS facility (Duke Univ., USA) with 10^8 g/s and Delta E_g/E_g~0.03. Even a seeded quantum FEL for g-beams may become possible, with much higher brilliance and spectral flux. At the same time new exciting possibilities open up for focused g-beams. We describe a new experiment at the g-beam of the ILL reactor (Grenoble), where we observed for the first time that the index of refraction for g-beams is determined by virtual pair creation. Using a combination of refractive and reflective optics, efficient monochromators for g-beams are being developed. Thus we have to optimize the system of the g-beam facility, the g-beam optics and g-detectors. We can trade g-intensity for band width, going down to Delta E_g/E_g ~ 10^-6 and address individual nuclear levels. 'Nuclear photonics' stresses the importance of nuclear applications. We can address with g-beams individual nuclear isotopes and not just elements like with X-ray beams. Compared to X rays, g-beams can penetrate much deeper into big samples like radioactive waste barrels, motors or batteries. We can perform tomography and microscopy studies by focusing down to micron resolution using Nucl. Reson. Fluorescence for detection with eV resolution and high spatial resolution. We discuss the dominating M1 and E1 excitations like scissors mode, two-phonon quadrupole octupole excitations, pygmy dipole excitations or giant dipole excitations under the new facet of applications. We find many new applications in biomedicine, green energy, radioactive waste management or homeland security. Also more brilliant secondary beams of neutrons and positrons can be produced.

physics.acc-ph

Nuclear photonics at ultra-high counting rates and higher multipole excitations

Next-generation gamma beams beams from laser Compton-backscattering facilities like ELI-NP (Bucharest)] or MEGa-Ray (Livermore) will drastically exceed the photon flux presently available at existing facilities, reaching or even exceeding 10^13 gamma/sec. The beam structure as presently foreseen for MEGa-Ray and ELI-NP builds upon a structure of macro-pulses (~120 Hz) for the electron beam, accelerated with X-band technology at 11.5 GHz, resulting in a micro structure of 87 ps distance between the electron pulses acting as mirrors for a counterpropagating intense laser. In total each 8.3 ms a gamma pulse series with a duration of about 100 ns will impinge on the target, resulting in an instantaneous photon flux of about 10^18 gamma/s, thus introducing major challenges in view of pile-up. Novel gamma optics will be applied to monochromatize the gamma beam to ultimately Delta E/E~10^-6. Thus level-selective spectroscopy of higher multipole excitations will become accessible with good contrast for the first time. Fast responding gamma detectors, e.g. based on advanced scintillator technology (e.g. LaBr3(Ce)) allow for measurements with count rates as high as 10^6-10^7 gamma/s without significant drop of performance. Data handling adapted to the beam conditions could be performed by fast digitizing electronics, able to sample data traces during the micro-pulse duration, while the subsequent macro-pulse gap of ca. 8 ms leaves ample time for data readout. A ball of LaBr3 detectors with digital readout appears to best suited for this novel type of nuclear photonics at ultra-high counting rates.

physics.ins-det

High-Intensity and High-Brightness Source of Moderated Positrons Using a Brilliant gamma Beam

Presently large efforts are conducted towards the development of highly brilliant gamma beams via Compton back scattering of photons from a high-brilliance electron beam, either on the basis of a normal-conducting electron linac or a (superconducting) Energy Recovery Linac (ERL). Particularly ERL's provide an extremely brilliant electron beam, thus enabling to generate highest-quality gamma beams. A 2.5 MeV gamma beam with an envisaged intensity of 10^15 s^-1, as ultimately envisaged for an ERL-based gamma-beam facility, narrow band width (10^-3), and extremely low emittance (10^-4 mm^2 mrad^2) offers the possibility to produce a high-intensity bright polarized positron beam. Pair production in a face-on irradiated W converter foil (200 micron thick, 10 mm long) would lead to the emission of 2 x 10^13 (fast) positrons per second, which is four orders of magnitude higher compared to strong radioactive ^22Na sources conventionally used in the laboratory.Using a stack of converter foils and subsequent positron moderation, a high-intensity low-energy beam of moderated positrons can be produced. Two different source setups are presented: a high-brightness positron beam with a diameter as low as 0.2 mm, and a high-intensity beam of 3 x 10^11 moderated positrons per second. Hence, profiting from an improved moderation efficiency, the envisaged positron intensity would exceed that of present high-intensity positron sources by a factor of 100.

nucl-ex

Neutron Halo Isomers in Stable Nuclei and their Possible Application for the Production of Low Energy, Pulsed, Polarized Neutron Beams of High Intensity and High Brilliance

We propose to search for neutron halo isomers populated via $γ$-capture in stable nuclei with mass numbers of about A=140-180 or A=40-60, where the $4s_{1/2}$ or $3s_{1/2}$ neutron shell model state reaches zero binding energy. These halo nuclei can be produced for the first time with new $γ$-beams of high intensity and small band width ($\le$ 0.1%) achievable via Compton back-scattering off brilliant electron beams thus offering a promising perspective to selectively populate these isomers with small separation energies of 1 eV to a few keV. Similar to single-neutron halo states for very light, extremely neutron-rich, radioactive nuclei \cite{hansen95,tanihata96,aumann00}, the low neutron separation energy and short-range nuclear force allows the neutron to tunnel far out into free space much beyond the nuclear core radius. This results in prolonged half lives of the isomers for the $γ$-decay back to the ground state in the 100 ps-$μ$s range. Similar to the treatment of photodisintegration of the deuteron, the neutron release from the neutron halo isomer via a second, low-energy, intense photon beam has a known much larger cross section with a typical energy threshold behavior. In the second step, the neutrons can be released as a low-energy, pulsed, polarized neutron beam of high intensity and high brilliance, possibly being much superior to presently existing beams from reactors or spallation neutron sources.

nucl-ex

Introducing the Fission-Fusion Reaction Process: Using a Laser-Accelerated Th Beam to produce Neutron-Rich Nuclei towards the N=126 Waiting Point of the r Process

We propose to produce neutron-rich nuclei in the range of the astrophysical r-process around the waiting point N=126 by fissioning a dense laser-accelerated thorium ion bunch in a thorium target (covered by a CH2 layer), where the light fission fragments of the beam fuse with the light fission fragments of the target. Via the 'hole-boring' mode of laser Radiation Pressure Acceleration using a high-intensity, short pulse laser, very efficiently bunches of 232Th with solid-state density can be generated from a Th layer, placed beneath a deuterated polyethylene foil, both forming the production target. Th ions laser-accelerated to about 7 MeV/u will pass through a thin CH2 layer placed in front of a thicker second Th foil closely behind the production target and disintegrate into light and heavy fission fragments. In addition, light ions (d,C) from the CD2 production target will be accelerated as well to about 7 MeV/u, inducing the fission process of 232Th also in the second Th layer. The laser-accelerated ion bunches with solid-state density, which are about 10^14 times more dense than classically accelerated ion bunches, allow for a high probability that generated fission products can fuse again. In contrast to classical radioactive beam facilities, where intense but low-density radioactive beams are merged with stable targets, the novel fission-fusion process draws on the fusion between neutron-rich, short-lived, light fission fragments both from beam and target. The high ion beam density may lead to a strong collective modification of the stopping power in the target, leading to significant range enhancement. Using a high-intensity laser as envisaged for the ELI-Nuclear Physics project in Bucharest (ELI-NP), estimates promise a fusion yield of about 10^3 ions per laser pulse in the mass range of A=180-190, thus enabling to approach the r-process waiting point at N=126.

nucl-ex

Dynamics of Nanometer-Scale Foil Targets Irradiated with Relativistically Intense Laser Pulses

In this letter we report on an experimental study of high harmonic radiation generated in nanometer-scale foil targets irradiated under normal incidence. The experiments constitute the first unambiguous observation of odd-numbered relativistic harmonics generated by the $\vec{v}\times\vec{B}$ component of the Lorentz force verifying a long predicted property of solid target harmonics. Simultaneously the observed harmonic spectra allow in-situ extraction of the target density in an experimental scenario which is of utmost interest for applications such as ion acceleration by the radiation pressure of an ultraintense laser.

physics.plasm-ph

Production of Medical Radioisotopes with High Specific Activity in Photonuclear Reactions with $γ$ Beams of High Intensity and Large Brilliance

We study the production of radioisotopes for nuclear medicine in $(γ,x{\rm n}+y{\rm p})$ photonuclear reactions or ($γ,γ'$) photoexcitation reactions with high flux [($10^{13}-10^{15}$)$γ$/s], small diameter $\sim (100 \, μ$m$)^2$ and small band width ($ΔE/E \approx 10^{-3}-10^{-4}$) $γ$ beams produced by Compton back-scattering of laser light from relativistic brilliant electron beams. We compare them to (ion,$x$n$ + y$p) reactions with (ion=p,d,$α$) from particle accelerators like cyclotrons and (n,$γ$) or (n,f) reactions from nuclear reactors. For photonuclear reactions with a narrow $γ$ beam the energy deposition in the target can be managed by using a stack of thin target foils or wires, hence avoiding direct stopping of the Compton and pair electrons (positrons). $(γ,γ')$ isomer production via specially selected $γ$ cascades allows to produce high specific activity in multiple excitations, where no back-pumping of the isomer to the ground state occurs. We discuss in detail many specific radioisotopes for diagnostics and therapy applications. Photonuclear reactions with $γ$ beams allow to produce certain radioisotopes, e.g. $^{47}$Sc, $^{44}$Ti, $^{67}$Cu, $^{103}$Pd, $^{117m}$Sn, $^{169}$Er, $^{195m}$Pt or $^{225}$Ac, with higher specific activity and/or more economically than with classical methods. This will open the way for completely new clinical applications of radioisotopes. For example $^{195m}$Pt could be used to verify the patient's response to chemotherapy with platinum compounds before a complete treatment is performed. Also innovative isotopes like $^{47}$Sc, $^{67}$Cu and $^{225}$Ac could be produced for the first time in sufficient quantities for large-scale application in targeted radionuclide therapy.

physics.med-ph

Collective deceleration: toward a compact beam dump

With the increasing development of laser accelerators, the electron energy is already beyond GeV and even higher in near future. Conventional beam dump based on ionization or radiation loss mechanism is cumbersome and costly, also has radiological hazards. We revisit the stopping power of high-energy charged particles in matter and discuss the associated problem of beam dump from the point of view of collective deceleration. The collective stopping length in an ionized gas can be several orders of magnitude shorter than the Bethe-Bloch and multiple electromagnetic cascades' stopping length in solid. At the mean time, the tenuous density of the gas makes the radioactivation negligible. Such a compact and non-radioactivating beam dump works well for short and dense bunches, which is typically generated from laser wakefield accelerator.

physics.plasm-ph