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D. J. Durian

Publications and source records attributed to D. J. Durian.

At least 37 records · Page 2Linked to original sources

Bubble statistics and coarsening dynamics for quasi-two dimensional foams with increasing liquid content

We report on the statistics of bubble size, topology, and shape and on their role in the coarsening dynamics for foams consisting of bubbles compressed between two parallel plates. The design of the sample cell permits control of the liquid content, through a constant pressure condition set by the height of the foam above a liquid reservoir. We find that in the scaling state, all bubble distributions are independent not only of time but also of liquid content. For coarsening, the average rate decreases with liquid content due to the blocking of gas diffusion by Plateau borders inflated with liquid. By observing the growth rate of individual bubbles, we find that von Neumann's law becomes progressively violated with increasing wetness and with decreasing bubble size. We successfully model this behavior by explicitly incorporating the border blocking effect into the von Neumann argument. Two dimensionless bubble shape parameters naturally arise, one of which is primarily responsible for the violation of von Neumann's law for foams that are not perfectly dry.

cond-mat.soft↗

Geometry dependence of the clogging transition in tilted hoppers

We report the effect of system geometry on the clogging of granular material flowing out of flat-bottomed hoppers with variable aperture size D. For such systems, there exists a critical aperture size Dc at which there is a divergence in the time for a flow to clog. To better understand the origins of Dc, we perturb the system by tilting the hopper an angle Q and mapping out a clogging phase diagram as a function of Q and D. The clogging transition demarcates the boundary between the freely-flowing (large D, small Q) and clogging (small D, large Q) regimes. We investigate how the system geometry affects Dc by mapping out this phase diagram for hoppers with either a circular hole or a rectangular narrow slit. Additionally, we vary the grain shape, investigating smooth spheres (glass beads), compact angular grains (beach sand), disk-like grains (lentils), and rod-like grains (rice). We find that the value of Dc grows with increasing Q, diverging at pi-Qr where Qr is the angle of repose. For circular apertures, the shape of the clogging transition is the same for all grain types. However, this is not the case for the narrow slit apertures, where the rate of growth of the critical hole size with tilt angle depends on the material.

cond-mat.soft↗

Effects of Particle Shape on Growth Dynamics at Edges of Evaporating Colloidal Drops

We study the influence of particle shape on growth processes at the edges of evaporating drops. Aqueous suspensions of colloidal particles evaporate on glass slides, and convective flows during evaporation carry particles from drop center to drop edge, where they accumulate. The resulting particle deposits grow inhomogeneously from the edge in two-dimensions, and the deposition front, or growth line, varies spatio-temporally. Measurements of the fluctuations of the deposition front during evaporation enable us to identify distinct growth processes that depend strongly on particle shape. Sphere deposition exhibits a classic Poisson like growth process; deposition of slightly anisotropic particles, however, belongs to the Kardar-Parisi-Zhang (KPZ) universality class, and deposition of highly anisotropic ellipsoids appears to belong to a third universality class, characterized by KPZ fluctuations in the presence of quenched disorder.

cond-mat.soft↗

Coarsening of Two Dimensional Foam on a Dome

In this paper we report on bubble growth rates and on the statistics of bubble topology for the coarsening of a dry foam contained in the narrow gap between two hemispheres. By contrast with coarsening in flat space, where six-sided bubbles neither grow nor shrink, we observe that six sided bubbles grow with time at a rate that depends on their size. This result agrees with the modification to von Neumann's law predicted by J.E. Avron and D. Levine. For bubbles with a different number of sides, except possibly seven, there is too much noise in the growth rate data to demonstrate a difference with coarsening in flat space. In terms of the statistics of bubble topology, we find fewer 3, 4, and 5 sided bubbles, and more 6 and greater sided bubbles, in comparison with the stationary distribution for coarsening in flat space. We also find good general agreement with the Aboav-Weaire law for the average number of sides of the neighbors of an n-sided bubble.

cond-mat.soft↗

Temperature-pressure scaling for air-fluidized grains on approaches to Point J

We present experiments on a monolayer of air-fluidized beads in which a jamming transition is approached by increasing pressure, increasing packing fraction, and decreasing kinetic energy. This is accomplished, along with a noninvasive measurement of pressure, by tilting the system and examining behavior vs depth. We construct an equation of state and analyze relaxation time vs effective temperature. By making time and effective temperature dimensionless using factors of pressure, bead size, and bead mass, we obtain a good collapse of the data but to a functional form that differs from that of thermal hard-sphere systems. The relaxation time appears to diverge only as the effective temperature to pressure ratio goes to zero.

cond-mat.soft↗

Dynamical heterogeneity in soft particle suspensions under shear

We present experimental measurements of dynamical heterogeneities in a dense system of microgel spheres, sheared at different rates and at different packing fractions in a microfluidic channel, and visualized with high speed digital video microscopy. A four-point dynamic susceptibility is deduced from video correlations, and is found to exhibit a peak that grows in height and shifts to longer times as the jamming transition is approached from two different directions. In particular, the time for particle-size root-mean square relative displacements is found to scale as $τ^* \sim (\dot γΔϕ^4)^{-1}$ where $\dotγ$ is the strain rate and $Δϕ=|ϕ-ϕ_c|$ is the distance from the random close packing volume fraction. The typical number of particles in a dynamical heterogeneity is deduced from the susceptibility peak height and found to scale as $n^* \sim (\dot γΔϕ^4)^{-0.3}$. Exponent uncertainties are less than ten percent. We emphasize that the same power-law behavior is found at packing fractions above and below $ϕ_c$. Thus, our results considerably extend a previous observation of $n^* \sim \dotγ^{-0.3}$ for granular heap flow at fixed packing below $ϕ_c$. Furthermore, the implied result $n^*\sim (τ^*)^{0.3}$ compares well with expectation from mode-coupling theory and with prior observations for driven granular systems.

cond-mat.soft↗

Abrasion of flat rotating shapes

We report on the erosion of flat linoleum "pebbles" under steady rotation in a slurry of abrasive grit. To quantify shape as a function of time, we develop a general method in which the pebble is photographed from multiple angles with respect to the grid of pixels in a digital camera. This reduces digitization noise, and allows the local curvature of the contour to be computed with a controllable degree of uncertainty. Several shape descriptors are then employed to follow the evolution of different initial shapes toward a circle, where abrasion halts. The results are in good quantitative agreement with a simple model, where we propose that points along the contour move radially inward in proportion to the product of the radius and the derivative of radius with respect to angle.

cond-mat.soft↗

Air fluidized balls in a background of smaller beads

We report on quasi-two-dimensional granular systems in which either one or two large balls is fluidized by an upflow of air in the presence of a background of several hundred smaller beads. A single large ball is observed to propel ballistically in nearly circular orbits, in direct contrast to the Brownian behavior of a large ball fluidized in the absence of this background. Further, the large ball motion satisfies a Langevin equation with an additional speed-dependent force acting in the direction of motion. This results in a non-zero average speed of the large ball that is an order of magnitude faster than the root mean square speed of the background balls. Two large balls fluidized in the absence of the small-bead background experience a repulsive force depending only on the separation of the two balls. With the background beads present, by contrast, the ball-ball interaction becomes velocity-dependent and attractive. The attraction is long-ranged and inconsistent with a depletion model; instead, it is mediated by local fluctuations in the density of the background beads which depends on the large balls' motion.

cond-mat.soft↗

Propagating Waves in a Monolayer of Gas-Fluidized Rods

We report on an observation of propagating compression waves in a quasi-two-dimensional monolayer of apolar granular rods fluidized by an upflow of air. The collective wave speed is an order of magnitude faster than the speed of the particles. This gives rise to anomalously large number fluctuations dN ~ $N^{0.72 \pm 0.04}$, which are greater than ordinary number fluctuations of N^{1/2}. We characterize the waves by calculating the spatiotemporal power spectrum of the density. The position of observed peaks, as a function of frequency w and wavevector k, yields a linear dispersion relationship in the long-time, long-wavelength limit and a wavespeed c = w/k. Repeating this analysis for systems at different densities and air speeds, we observe a linear increase in the wavespeed with increasing packing fraction with no dependence on the airflow. Although air-fluidized rods self-propel individually or in dilute collections, the parallel and perpendicular root-mean-square speeds of the rods indicate that they no longer self-propel when propagating waves are present. Based on this mutual exclusivity, we map out the phase behavior for the existence of waves vs self-propulsion as a function of density and fluidizing airflow.

cond-mat.soft↗

Microfluidic rheology of soft colloids above and below jamming

The rheology near jamming of a suspension of soft colloidal spheres is studied using a custom microfluidic rheometer that provides stress versus strain rate over many decades. We find non-Newtonian behavior below the jamming concentration and yield stress behavior above it. The data may be collapsed onto two branches with critical scaling exponents that agree with expectations based on Hertzian contacts and viscous drag. These results support the conclusion that jamming is similar to a critical phase transition, but with interaction-dependent exponents.

cond-mat.soft↗

Centrifugal compression of soft particle packings - theory and experiment

An exact method is developed for computing the height of an elastic medium subjected to centrifugal compression, for arbitrary constitutive relation between stress and strain. Example solutions are obtained for power-law media and for cases where the stress diverges at a critical strain -- for example as required by packings composed of deformable but incompressible particles. Experimental data are presented for the centrifugal compression of thermo-responsive N-isopropylacrylamide (NIPA) microgel beads in water. For small radial acceleration, the results are consistent with Hertzian elasticity, and are analyzed in terms of the Young elastic modulus of the bead material. For large radial acceleration, the sample compression asymptotes to a value corresponding to a space-filling particle volume fraction of unity. Therefore we conclude that the gel beads are incompressible, and deform without deswelling. In addition, we find that the Young elastic modulus of the particulate gel material scales with cross-link density raised to the power 3.3+-0.8, somewhat larger than the Flory expectation.

cond-mat.soft↗

Jamming and growth of dynamical heterogeneities versus depth for granular heap flow

We report on grain dynamics versus depth for steady-state gravity-driven flow of grains along a heap formed between two parallel sidewalls. Near the surface the flow is steady and fast, while far below there is no flow whatsoever; therefore, a jamming transition occurs where depth is an effective control parameter for setting the distance from the transition. As seen previously, the time-averaged velocity profile along the sidewall exhibits a nearly exponential decay vs depth. Using speckle-visiblility spectroscopy (SVS), we find that velocity fluctuations grow relative to the average on approach to jamming. Introducing an image-based order parameter and the variance in its temporal decay at a given depth, we also characterize the spatially heterogeneous nature of the dynamics and find that it increases on approach to jamming. In particular, the important time and length scales for dynamical heterogeneities are found to grow almost exponentially as a function of depth. These dynamical changes occur without noticeable change in structure, and are compared to behavior found by experiment and simulation elsewhere in order to test the universality of the jamming concept. In particular we find that the size of the heterogeneities scales as the inertia number raised to the -1/3 power, in agreement with two recent simulations.

cond-mat.soft↗

Granular discharge and clogging for tilted hoppers

We measure the flux of spherical glass beads through a hole as a systematic function of both tilt angle and hole diameter, for two different size beads. The discharge increases with hole diameter in accord with the Beverloo relation for both horizontal and vertical holes, but in the latter case with a larger small-hole cutoff. For large holes the flux decreases linearly in cosine of the tilt angle, vanishing smoothly somewhat below the angle of repose. For small holes it vanishes abruptly at a smaller angle. The conditions for zero flux are discussed in the context of a {\it clogging phase diagram} of flow state vs tilt angle and ratio of hole to grain size.

cond-mat.soft↗

Dynamics of Gas-Fluidized Granular Rods

We study a quasi-two-dimensional monolayer of granular rods fluidized by a spatially and temporally homogeneous upflow of air. By tracking the position and orientation of the particles, we characterize the dynamics of the system with sufficient resolution to observe ballistic motion at the shortest time scales. Particle anisotropy gives rise to dynamical anisotropy and superdiffusive dynamics parallel to the rod's long axis, causing the parallel and perpendicular mean squared displacements to become diffusive on different timescales. The distributions of free times and free paths between collisions deviate from exponential behavior, underscoring the non-thermal character of the particle motion. The dynamics show evidence of rotational-translational coupling similar to that of an anisotropic Brownian particle. We model rotational-translation coupling in the single-particle dynamics with a modified Langevin model using non-thermal noise sources. This suggests a phenomenological approach to thinking about collections of self-propelling particles in terms of enhanced memory effects.

cond-mat.soft↗

Effective temperatures and activated dynamics for a two-dimensional air-driven granular system on two approaches to jamming

We present experiments on several distinct effective temperatures in a granular system at a sequence of increasing packing densities and at a sequence of decreasing driving rates. This includes single-grain measurements based on the mechanical energies of both the grains and an embedded oscillator, as well as a collective measurement based on the Einstein relation between diffusivity and mobility, which all probe different time scales. Remarkably, all effective temperatures agree. Furthermore, mobility data along the two trajectories collapse when plotted vs effective temperature and exhibit an Arrhenius form with the same energy barrier as the microscopic relaxation time.

cond-mat.soft↗

Statistics of bubble rearrangement dynamics in a coarsening foam

We use speckle-visibility spectroscopy to measure the time-dependence of bubble rearrangement events that are driven by coarsening in an aqueous foam. This technique gives the time-trace for the average scattering site speed within a prescribed volume of the sample. Results are analyzed in terms of distributions of event times, event speeds, and event displacements. The distribution of rest times between successive events is also measured; comparison with diffusing-wave spectroscopy results shows that the spatial structure of a typical event consists of a core of only a few bubbles which undergo topology change plus a surrounding halo of bubbles which shift by an amount that decays to one wavelength at four to five bubbles away. No correlations are found between the durations, speeds, and rest times between successive events.

cond-mat.soft↗

Projectile interactions in granular impact cratering

We present evidence for the interactions between a ball and the container boundaries, as well as between two balls, that are mediated by the granular medium during impact cratering. The presence of the bottom boundary affects the final penetration depth only for low drop heights with shallow filling, in which case, surprisingly, the penetration becomes deeper. By contrast the presence of the side wall causes less penetration and also an effective repulsion. Repulsion is also found for two balls dropped side-by-side.

cond-mat.soft↗

Polymeric filament thinning and breakup in microchannels

The effects of elasticity on filament thinning and breakup are investigated in microchannel cross flow. When a viscous solution is stretched by an external immiscible fluid, a low 100 ppm polymer concentration strongly affects the breakup process, compared to the Newtonian case. Qualitatively, polymeric filaments show much slower evolution, and their morphology features multiple connected drops. Measurements of filament thickness show two main temporal regimes: flow- and capillary-driven. At early times both polymeric and Newtonian fluids are flow-driven, and filament thinning is exponential. At later times, Newtonian filament thinning crosses over to a capillary-driven regime, in which the decay is algebraic. By contrast, the polymeric fluid first crosses over to a second type of flow-driven behavior, in which viscoelastic stresses inside the filament become important and the decay is again exponential. Finally, the polymeric filament becomes capillary-driven at late times with algebraic decay. We show that the exponential flow thinning behavior allows a novel measurement of the extensional viscosities of both Newtonian and polymeric fluids.

physics.flu-dyn↗