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D. J. Norris

Publications and source records attributed to D. J. Norris.

3 recordsLinked to original sources

Optical Fourier Surfaces for Free-Space Computer-Generated Holography

Computer-generated holography can shape electromagnetic fields by encoding wavefront information in nanostructured surfaces. However, despite significant progress, hologram designs for visible and near-infrared wavelengths remain largely limited by fabrication constraints. Most implementations rely on lithographic methods that produce discretized surfaces that do not match the wave nature of light. Further advances would benefit from accurate continuous (grayscale) control of interfacial profiles, which would allow straightforward design principles from Fourier optics to be applied. In this work, we introduce optical Fourier surfaces as a versatile, intuitive platform for free-space computer-generated holograms. Exploiting these arbitrarily wavy surfaces, we demonstrate three different design strategies for computer-generated holography. First, we use an analytical linear design approach based on sinusoidal lenses and gratings as fundamental holographic building blocks. Second, we enhance diffraction efficiencies through an iterative Fourier-transform algorithm. Finally, we extend our framework with machine-learning-based inverse design, creating wavelength-multiplexed holograms that reconstruct distinct diffraction responses in a predefined image plane. Our results combine advanced thermal scanning-probe lithography with flexible design strategies to create useful structures for photonic applications, particularly in settings where rapid prototyping is crucial.

physics.optics

Comment on "Self-Purification in Semiconductor Nanocrystals"

In a recent Letter [PRL 96, 226802 (2006)], Dalpian and Chelikowsky claimed that formation energies of Mn impurities in CdSe nanocrystals increase as the size of the nanocrystal decreases, and argued that this size dependence leads to "self-purification" of small nanocrystals. They presented density-functional-theory (DFT) calculations showing a strong size dependence for Mn impurity formation energies, and proposed a general explanation. In this Comment we show that several different DFT codes, pseudopotentials, and exchange-correlation functionals give a markedly different result: We find no such size dependence. More generally, we argue that formation energies are not relevant to substitutional doping in most colloidally grown nanocrystals.

cond-mat.mtrl-sci

Elimination of cracks in self-assembled photonic band gap crystals

Thin colloidal crystals (or synthetic opals) composed of Stober silica spheres typically develop cracks when they are utilized to obtain photonic band gap crystals (or inverted opals). We find that by sintering the silica spheres prior to assembly of the opal these cracks can be avoided. We report the effects of temperature and duration of the heat treatment on 850 nm silica spheres using electron microscopy, thermogravimetry, and light scattering. We also find a large dependence of the refractive index of the silica on the temperature of the heat treatment. This may allow tuning of the refractive index of silica spheres.

cond-mat.mtrl-sci