arXiv subjects

D. Kahl

Publications and source records attributed to D. Kahl.

At least 19 recordsLinked to original sources

arXiv2025

ELIGANT-TN -- ELI Gamma Above Neutron Threshold: The Thermal Neutron setup

Here we present the thermal neutron counter from the ELI Gamma Above Neutron Threshold setup at the Extreme Light Infrastructure - Nuclear Physics. We describe the mechanical design of the setup, the properties of the ${}^{3}$He gas counters, and the hardware data-acquisition electronics and software digital signal processing. The performance of the complete detector array is demonstrated via Geant4 and MCNP simulations, and measurements with typical neutron sources. The analysis procedure for experimental measurements are outlined with a in-beam test experiment with an $\alpha$ beam to measure the ${}^{13}\mathrm{C}(\alpha,\mathrm{n}_{0}){}^{16}\mathrm{O}$ cross-section branching ratios.

physics.ins-det↗

arXiv2025

Impact of newly measured $\beta$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

nucl-ex↗

arXiv2024

High-precision mass measurements of the ground and isomeric states in $^{124,125}$Ag

The masses of the ground and isomeric states in $^{124,125}$Ag have been measured using the phase-imaging ion-cyclotron-resonance technique at the JYFLTRAP double Penning trap mass spectrometer. The ground states of $^{124}$Ag and $^{125}$Ag were found to be 30(250) keV and 250(430) keV less bound but 36 and 110 times more precise than in the Atomic Mass Evaluation 2020, respectively. The excitation energy of $^{124}$Ag$^{m}$, ${E_x = 188.2(25)}$ keV, was determined for the first time. The new precise mass values have been utilised to study the evolution of nuclear structure via two-neutron separation energies. The impact on the astrophysical rapid neutron capture process has been investigated via neutron-capture reaction rate calculations. The precision measurements indicate a more linear trend in two-neutron separation energies and reduce the mass-related uncertainties for the neutron-capture rate of $^{124}$Ag$(n,\gamma)^{125}$Ag by a factor of around 100. The new mass values also improve the mass of $^{123}$Pd, previously measured using $^{124}$Ag as a reference.

nucl-ex↗

arXiv2024

Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

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arXiv2024

First investigation on the isomeric ratio in multinucleon transfer reactions: Entrance channel effects on the spin distribution

The multinucleon transfer (MNT) reaction approach was successfully employed for the first time to measure the isomeric ratios (IRs) of $^{211}$Po (25/2$^+$) isomer and its (9/2$^+$) ground state at the IGISOL facility using a 945 MeV $^{136}$Xe beam impinged on $^{209}$Bi and $^{\rm nat}$Pb targets. The dominant production of isomers compared to the corresponding ground states was consistently revealed in the $\alpha$-decay spectra. Deduced IR of $^{211}$Po populated through the $^{136}$Xe+$^{\rm nat}$Pb reaction was found to enhance $\approx$1.8-times than observed for $^{136}$Xe+$^{209}$Bi. State-of-the-art Langevin-type model calculations have been utilized to estimate the spin distribution of an MNT residue. The computations qualitatively corroborate with the considerable increase in IRs of $^{211}$Po produced from $^{136}$Xe+$^{\rm nat}$Pb compared to $^{136}$Xe+$^{209}$Bi. Theoretical investigations indicate a weak influence of target spin on IRs. The enhancement of the $^{211}$Po isomer in the $^{136}$Xe+$^{\rm nat}$Pb over $^{136}$Xe+$^{209}$Bi can be attributed to the different proton ($p$)-transfer production routes. Estimations demonstrate an increment in the angular momentum transfer, favorable for isomer production, with increasing projectile energy. Comparative analysis indicates the two entrance channel parameters, projectile mass and $p$-transfer channels, strongly influencing the population of the high-spin isomer of $^{211}$Po (25/2$^+$). This is the first experimental and theoretical investigation on the IRs of nuclei produced via different channels of MNT reactions, with the latter quantitatively underestimating the former by a factor of two.

nucl-ex↗

arXiv2023

High-precision measurements of low-lying isomeric states in $^{120-124}$In with JYFLTRAP double Penning trap

Neutron-rich $^{120-124}$In isotopes have been studied utilizing the double Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. Using the phase-imaging ion-cyclotron-resonance technique, the isomeric states were resolved from ground states and their excitation energies measured with high precision in $^{121,123,124}$In. In $^{120,122}$In, the $1^+$ states were separated and their masses were measured while the energy difference between the unresolved $5^+$ and $8^-$ states, whose presence was confirmed by post-trap decay spectroscopy was determined to be $\leq15$ keV. In addition, the half-life of $^{122}$Cd, $T_{1/2} = 5.98(10)$ s, was extracted. Experimental results were compared with energy density functionals, density functional theory and shell-model calculations.

nucl-ex↗

arXiv2023

High-precision Penning-trap mass measurements of Cd and In isotopes at JYFLTRAP remove the fluctuations in the two-neutron separation energies

We report on the first direct mass measurements of the $^{118,119}$Cd and $^{117-119}$In isotopes performed at the Ion Guide Isotope Separator On-Line facility using the JYFLTRAP double Penning trap mass spectrometer. The masses of $^{117}$In and $^{118}$Cd isotopes are in agreement with the literature, while $^{118,119}$In and $^{119}$Cd differ from literature by 49, 13 and 85 keV (6.1, 1.9 and 2.1 standard deviations), respectively. The excitation energy of the $^{118}$In first isomeric state, $E_x = 40.3(25)$ keV, was determined for the first time. The updated mass values removed the fluctuations observed in the two-neutron separation energies and lead to a smoother linear decrease of both isotopic chains. The $\log(ft)$ value for the $^{118}$Cd decay is also found to increase from 3.93(6) to 4.089(8). The reported results indicate an absence of significant structural changes around $N=70$.

nucl-ex↗

arXiv2021

Advancement of Photospheric Radius Expansion and Clocked Type-I X-Ray Burst Models with the New $^{22}$Mg$(α,p)^{25}$Al Reaction Rate Determined at Gamow Energy

We report the first (in)elastic scattering measurement of $^{25}\mathrm{Al}+p$ with the capability to select and measure in a broad energy range the proton resonances in $^{26}$Si contributing to the $^{22}$Mg$(α,p)$ reaction at type I x-ray burst energies. We measured spin-parities of four resonances above the $α$ threshold of $^{26}$Si that are found to strongly impact the $^{22}$Mg$(α,p)$ rate. The new rate advances a state-of-the-art model to remarkably reproduce light curves of the GS 1826$-$24 clocked burster with mean deviation $<9$ % and permits us to discover a strong correlation between the He abundance in the accreting envelope of photospheric radius expansion burster and the dominance of $^{22}$Mg$(α,p)$ branch.

nucl-ex↗

arXiv2021

Isomeric states in neutron-rich nuclei around $N = 40$

Neutron-rich nuclei in the vicinity of the $N=40$ island of inversion are characterized by shell evolution and exhibit deformed ground states. In several nuclei isomeric states have been observed and attributed to excitations to the intruder neutron $1g_{9/2}$ orbital. In the present study we searched for isomeric states in nuclei around $N=40$, $Z=22$ produced by projectile fragmentation at RIBF. Delayed $γ$ rays were detected by the EURICA germanium detector array. High statistics data allowed for an updated decay scheme of $^{60}$V. The lifetime of an isomeric state in $^{64}$V was measured for the first time in the present experiment. A previously unobserved isomeric state was discovered in $^{58}$Sc. The measured lifetime suggests a parity changing transition, originating from an odd number of neutrons in the $1g_{9/2}$ orbital. The nature of the isomeric state in $^{58}$Sc is thus different from isomers in the less exotic V and Sc nuclei.

nucl-ex↗

arXiv2021

Uncertainties in the $^{18}$F(p,$α$)$^{15}$O reaction rate in classical novae

Context. Direct observation of gamma-ray emission from the decay of $^{18}$F ejected in classical nova outbursts remains a major focus of the nuclear astrophysics community. However, modeling the abundance of ejected $^{18}$F, and thus the predicted detectability distance of a gamma-ray signal near 511 keV emitted from these transient thermonuclear episodes, is hampered by significant uncertainties in our knowledge of the key $^{18}$F(p,$α$) reaction rate. Aims. We analyze uncertainties in the most recent nuclear physics experimental results employed to calculate the $^{18}$F(p,$α$) reaction rate. Our goal is to determine which uncertainties have the most profound influence on the predicted abundance of $^{18}$F ejected from novae, in order to guide future experimental works. Methods. We calculated a wide range of $^{18}$F(p,$α$) reaction rates using R-Matrix formalism, allowing us to take into account all interference effects. Using a selection of 16 evenly-spaced rates over the full range, we performed 16 new hydrodynamic nova simulations. Results. We performed one of the most thorough theoretical studies of the impact of the $^{18}$F(p,$α$) reaction in classical novae to date. The $^{18}$F(p,$α$) rate remains highly uncertain at nova temperatures, resulting in a factor ~10 uncertainty in the predicted abundance of $^{18}$F ejected from nova explosions. We also found that the abundance of $^{18}$F may be strongly correlated with that of $^{19}$F. Conclusions. Despite numerous nuclear physics uncertainties affecting the $^{18}$F(p,$α$) reaction rate, which are dominated by unknown interference signs between 1/2$^+$ and 3/2$^+$ resonances, future experimental work should focus on firmly and precisely determining the directly measurable quantum properties of the subthreshold states in the compound nucleus $^{19}$Ne near 6.13 and 6.29 MeV.

nucl-th↗

arXiv2020

Study of the $^{25}$Mg(d,p)$^{26}$Mg reaction to constrain the $^{25}$Al(p,$γ$)$^{26}$Si resonant reaction rates in nova burning conditions

The rate of the $^{25}$Al($p$,$γ$)$^{26}$Si reaction is one of the few key remaining nuclear uncertainties required for predicting the production of the cosmic $γ$-ray emitter $^{26}$Al in explosive burning in novae. This reaction rate is dominated by three key resonances ($J^π=0^{+}$, $1^{+}$ and $3^{+}$) in $^{26}$Si. Only the $3^{+}$ resonance strength has been directly constrained by experiment. A high resolution measurement of the $^{25}$Mg($d$,$p$) reaction was used to determine spectroscopic factors for analog states in the mirror nucleus, $^{26}$Mg. A first spectroscopic factor value is reported for the $0^{+}$ state at 6.256 MeV, and a strict upper limit is set on the value for the $1^{+}$ state at 5.691 MeV, that is incompatible with an earlier ($^{4}$He,$^{3}$He) study. These results are used to estimate proton partial widths, and resonance strengths of analog states in $^{26}$Si contributing to the $^{25}$Al($p$,$γ$)$^{26}$Si reaction rate in nova burning conditions.

nucl-ex↗

arXiv2019

Single-particle shell strengths near the doubly magic nucleus $^{56}$Ni and the $^{56}$Ni(p,$γ$)$^{57}$Cu reaction rate in explosive astrophysical burning

Angle-integrated cross-section measurements of the $^{56}$Ni(d,n) and (d,p) stripping reactions have been performed to determine the single-particle strengths of low-lying excited states in the mirror nuclei pair $^{57}$Cu-$^{57}$Ni situated adjacent to the doubly magic nucleus $^{56}$Ni. The reactions were studied in inverse kinematics utilizing a beam of radioactive $^{56}$Ni ions in conjunction with the GRETINA $γ$-array. Spectroscopic factors are compared with new shell-model calculations using a full $pf$ model space with the GPFX1A Hamiltonian for the isospin-conserving strong interaction plus Coulomb and charge-dependent Hamiltonians. These results were used to set new constraints on the $^{56}$Ni(p,$γ$)$^{57}$Cu reaction rate for explosive burning conditions in x-ray bursts, where $^{56}$Ni represents a key waiting point in the astrophysical rp-process.

nucl-ex↗

arXiv2019

First spectroscopy of 61Ti and the transition to the Island of Inversion at N = 40

Isomeric states in 59,61Ti have been populated in the projectile fragmentation of a 345 AMeV 238U beam at the Radioactive Isotope Beam Factory. The decay lifetimes and delayed gamma-ray transitions were measured with the EURICA array. Besides the known isomeric state in 59Ti, two isomeric states in 61Ti are observed for the first time. Based on the measured lifetimes, transition multipolarities as well as tentative spins and parities are assigned. Large-scale shell model calculations based on the modified LNPS interaction show that both 59Ti and 61Ti belong to the Island of Inversion at N=40 with ground state configurations dominated by particle-hole excitations to the g_9/2 and d_5/2 orbits.

nucl-ex↗

arXiv2018

Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

physics.ins-det↗

arXiv2018

First measurement of $^{30}$S+$α$ resonant elastic scattering for the $^{30}$S($α$,p) reaction rate

Background: Type I x-ray bursts are the most frequent thermonuclear explosions in the galaxy, resulting from thermonuclear runaway on the surface of an accreting neutron star. The $^{30}$S($α$,p) reaction plays a critical role in burst models, yet insufficient experimental information is available to calculate a reliable, precise rate for this reaction. Purpose: Our measurement was conducted to search for states in $^{34}$Ar and determine their quantum properties. In particular, natural-parity states with large $α$-decay partial widths should dominate the stellar reaction rate. Method: We performed the first measurement of $^{30}$S+$α$ resonant elastic scattering up to a center-of-mass energy of 5.5 MeV using a radioactive ion beam. The experiment utilized a thick gaseous active target system and silicon detector array in inverse kinematics. Results: We obtained an excitation function for $^{30}$S($α$,$α$) near $150^{\circ}$ in the center-of-mass frame. The experimental data were analyzed with an $R$-Matrix calculation, and we observed three new resonant patterns between 11.1 and 12.1 MeV, extracting their properties of resonance energy, widths, spin, and parity. Conclusions: We calculated the resonant thermonuclear reaction rate of $^{30}$S($α$,p) based on all available experimental data of $^{34}$Ar and found an upper limit about one order of magnitude larger than a rate determined using a statistical model. The astrophysical impact of these two rates has been investigated through one-zone postprocessing type I x-ray burst calculations. We find that our new upper limit for the $^{30}$S($α$,p)$^{33}$Cl rate significantly affects the predicted nuclear energy generation rate during the burst.

nucl-ex↗

arXiv2017

Non-extensive Statistics Solution to the Cosmological Lithium Problem

Big Bang nucleosynthesis (BBN) theory predicts the abundances of the light elements D, $^3$He, $^4$He and $^7$Li produced in the early universe. The primordial abundances of D and $^4$He inferred from observational data are in good agreement with predictions, however, the BBN theory overestimates the primordial $^7$Li abundance by about a factor of three. This is the so-called "cosmological lithium problem". Solutions to this problem using conventional astrophysics and nuclear physics have not been successful over the past few decades, probably indicating the presence of new physics during the era of BBN. We have investigated the impact on BBN predictions of adopting a generalized distribution to describe the velocities of nucleons in the framework of Tsallis non-extensive statistics. This generalized velocity distribution is characterized by a parameter $q$, and reduces to the usually assumed Maxwell-Boltzmann distribution for $q$ = 1. We find excellent agreement between predicted and observed primordial abundances of D, $^4$He and $^7$Li for $1.069\leq q \leq 1.082$, suggesting a possible new solution to the cosmological lithium problem.

astro-ph.CO↗

arXiv2016

Experimental investigation of a linear-chain structure in the nucleus 14C

It is a well-known fact that a cluster of nucleons can be formed in the interior of an atomic nucleus, and such clusters may occupy molecular-like orbitals, showing characteristics similar to normal molecules consisting of atoms. Chemical molecules having a linear alignment are commonly seen in nature, such as carbon dioxide. A similar linear alignment of the nuclear clusters, referred to as linear-chain cluster state (LCCS), has been studied since the 1950s, however, up to now there is no clear experimental evidence demonstrating the existence of such a state. Recently, it was proposed that an excess of neutrons may offer just such a stabilizing mechanism, revitalizing interest in the nuclear LCCS, specifically with predictions for their emergence in neutron-rich carbon isotopes. Here we present the experimental observation of α-cluster states in the radioactive 14C nucleus. Using the 10Be+α resonant scattering method with a radioactive beam, we observed a series of levels which completely agree with theoretically predicted levels having an explicit linear-chain cluster configuration. We regard this as the first strong indication of the linear-chain clustered nucleus.

nucl-ex↗

arXiv2016

First direct measurement of the $^{11}$C($α$, p)$^{14}$N stellar reaction by an extended thick-target method

The $^{11}$C($α$, p) reaction is an important $α$-induced reaction competing with $β$-limited hydrogen-burning processes in high-temperature explosive stars. We directly measured its reaction cross sections both for the ground-state transition ($α$, $p_{0}$) and the excited-state transitions ($α$, $p_{1}$) and ($α$, $p_{2}$) at relevant stellar energies 1.3 - 4.5 MeV by an extended thick-target method featuring time of flight for the first time. We revised the reaction rate by numerical integration including the ($α$, $p_{1}$) and ($α$, $p_{2}$) contributions and also low-lying resonances of ($α$, $p_{0}$) using both the present and the previous experimental data which were totally neglected in the previous compilation works. The present total reaction rate lies between the previous ($α$, $p_{0}$) rate and the total rate of the Hauser-Feshbach statistical model calculation, which is consistent with the relevant explosive hydrogen-burning scenarios such as the $νp$-process.

nucl-ex↗