arXiv subjects

D. Kielpinski

Publications and source records attributed to D. Kielpinski.

At least 19 recordsLinked to original sources

arXiv2016

Scalable ion-photon quantum interface based on integrated diffractive mirrors

Quantum networking links quantum processors through remote entanglement for distributed quantum information processing (QIP) and secure long-range communication. Trapped ions are a leading QIP platform, having demonstrated universal small-scale processors and roadmaps for large-scale implementation. Overall rates of ion-photon entanglement generation, essential for remote trapped ion entanglement, are limited by coupling efficiency into single mode fibres5 and scaling to many ions. Here we show a microfabricated trap with integrated diffractive mirrors that couples 4.1(6)% of the fluorescence from a $^{174}$Yb$^+$ ion into a single mode fibre, nearly triple the demonstrated bulk optics efficiency. The integrated optic collects 5.8(8)% of the π transition fluorescence, images the ion with sub-wavelength resolution, and couples 71(5)% of the collected light into the fibre. Our technology is suitable for entangling multiple ions in parallel and overcomes mode quality limitations of existing integrated optical interconnects. In addition, the efficiencies are sufficient for fault tolerant QIP.

quant-ph↗

arXiv2016

Effects of flake size on mode-locking behavior for flake-graphene saturable absorber mirrors

After advent of graphene as a saturable absorber many experiments have been conducted to produce short pulse duration pulses. Here, we have measured the properties of flake-graphene saturable absorber mirrors of various flake sizes dependent on fabrication technique. These mirrors enabled us to obtain a large mode-locking bandwidth of 16nm in an erbium-doped fiber laser. Mirrors with large flake size and multi-layered thickness induce strong pulse shaping and reflect mode-locked train of pulses with very large bandwidths.

physics.optics↗

arXiv2016

The interaction of excited atoms and few-cycle laser pulses

This work describes the first observations of the ionisation of neon in a metastable atomic state utilising a strong-field, few-cycle light pulse. We compare the observations to theoretical predictions based on the Ammosov-Delone-Krainov (ADK) theory and a solution to the time-dependent Schrodinger equation (TDSE). The TDSE provides better agreement with the experimental data than the ADK theory. We optically pump the target atomic species and demonstrate that the ionisation rate depends on the spin state of the target atoms and provide physically transparent interpretation of such a spin dependence in the frameworks of the spin-polarised Hartree-Fock and random-phase approximations.

physics.atom-ph↗

arXiv2016

Precise and accurate measurements of strong-field photoionisation and a transferrable laser intensity calibration standard

Ionization of atoms and molecules in strong laser fields is a fundamental process in many fields of research, especially in the emerging field of attosecond science. So far, demonstrably accurate data have only been acquired for atomic hydrogen (H), a species that is accessible to few investigators. Here we present measurements of the ionization yield for argon, krypton, and xenon with percentlevel accuracy, calibrated using H, in a laser regime widely used in attosecond science. We derive a transferrable calibration standard for laser peak intensity, accurate to 1.3%, that is based on a simple reference curve. In addition, our measurements provide a much-needed benchmark for testing models of ionisation in noble-gas atoms, such as the widely employed single-active electron approximation.

physics.atom-ph↗

arXiv2016

Measuring laser carrier-envelope phase effects in the noble gases with an atomic hydrogen calibration standard

We present accurate measurements of carrier-envelope phase effects on ionisation of the noble gases with few-cycle laser pulses. The experimental apparatus is calibrated by using atomic hydrogen data to remove any systematic offsets and thereby obtain accurate CEP data on other generally used noble gases such as Ar, Kr and Xe. Experimental results for H are well supported by exact TDSE theoretical simulations however significant differences are observed in case of noble gases.

physics.atom-ph↗

arXiv2015

Isotope effect in tunnelling ionization of neutral hydrogen molecules

It has been recently predicted theoretically that due to nuclear motion light and heavy hydrogen molecules exposed to strong electric field should exhibit substantially different tunneling ionization rates (O.I. Tolstikhin, H.J. Worner and T. Morishita, Phys. Rev. A 87, 041401(R) (2013) [1]). We studied that isotope effect experimentally by measuring relative ionization yields for each species in a mixed H2/D2 gas jet interacting with intense femtosecond laser pulses. In a reaction microscope apparatus we detected ionic fragments from all contributing channels (single ionization, dissociation, and sequential double ionization) and determined the ratio of total single ionization yields for H2 and D2. The measured ratio agrees quantitatively with the prediction of the generalized weak-field asymptotic theory in an apparent failure of the frozen-nuclei approximation.

physics.atom-ph↗

arXiv2015

Experimental observation of the elusive double-peak structure in R-dependent strong-field ionization rate of H2+

When a diatomic molecule is ionized by an intense laser field, the ionization rate depends very strongly on the inter-nuclear separation. That dependence exhibits a pronounced maximum at the inter-nuclear separation known as the critical distance. This phenomenon was first demonstrated theoretically in H2+ and became known as charge-resonance enhanced ionization (CREI, in reference to a proposed physical mechanism) or simply enhanced ionisation (EI). All theoretical models of this phenomenon predict a double-peak structure in the R-dependent ionization rate of H2+. However, such double-peak structure has never been observed experimentally. It was even suggested that it is impossible to observe due to fast motion of the nuclear wavepackets. Here we report a few-cycle pump-probe experiment which clearly resolves that elusive double-peak structure. In the experiment, an expanding H2+ ion produced by an intense pump pulse is probed by a much weaker probe pulse. The predicted double-peak structure is clearly seen in delay-dependent kinetic energy spectra of protons when pump and probe pulses are polarized parallel to each other. No structure is seen when the probe is polarized perpendicular to the pump.

physics.chem-ph↗

arXiv2015

Detection-Enhanced Steady State Entanglement with Ions

Driven dissipative steady state entanglement schemes take advantage of coupling to the environment to robustly prepare highly entangled states. We present a scheme for two trapped ions to generate a maximally entangled steady state with fidelity above 0.99, appropriate for use in quantum protocols. Furthermore, we extend the scheme by introducing detection of our dissipation process, significantly enhancing the fidelity. Our scheme is robust to anomalous heating and requires no sympathetic cooling.

quant-ph↗

arXiv2015

Transverse electron momentum distribution in tunneling and over the barrier ionization by laser pulses with varying ellipticity

We study transverse electron momentum distribution (TEMD) in strong field atomic ionization driven by laser pulses with varying ellipticity. We show, both experimentally and theoretically, that the TEMD in the tunneling and over the barrier ionization regimes evolves in a qualitatively different way when the ellipticity parameter describing polarization state of the driving laser pulse increases.

physics.atom-ph↗

arXiv2014

Benchmarking strong-field ionisation with atomic hydrogen

As the simplest atomic system, the hydrogen atom plays a key benchmarking role in laser and quantum physics. Atomic hydrogen is a widely used atomic test system for theoretical calculations of strong-field ionization, since approximate theories can be directly compared to numerical solutions of the time-dependent Schrödinger equation. However, relatively little experimental data is available for comparison to these calculations, since atomic hydrogen sources are difficult to construct and use. We review the existing experimental results on strong-field ionization of atomic hydrogen in multi-cycle and few-cycle laser pulses. Quantitative agreement has been achieved between experiment and theoretical predictions at the 10% uncertainty level, and has been used to develop an intensity calibration method with 1% uncertainty. Such quantitative agreement can be used to certify experimental techniques as being free from systematic errors, guaranteeing the accuracy of data obtained on species other than H. We review the experimental and theoretical techniques that enable these results.

physics.atom-ph↗

arXiv2014

Three-photon excitation of quantum dots with a telecom band ultrafast fiber laser

We demonstrate three-photon excitation in quantum dots with a mode-locked fiber laser operating in the telecommunications band. We compare spectra and intensity dependence of fluorescence from one- and three-photon excitation of commercially available 640 nm quantum dots, using a 372 nm diode laser for one-photon excitation and 116 fs pulses from a mode-locked fiber laser with a center wavelength of 1575 nm for three-photon excitation.

physics.optics↗

arXiv2013

Fast gates for ion traps by splitting laser pulses

We present a fast phase gate scheme that is experimentally achievable and has an operation time more than two orders of magnitude faster than current experimental schemes for low numbers of pulses. The gate time improves with the number of pulses following an inverse power law. Unlike implemented schemes which excite precise motional sidebands, thus limiting the gate timescale, our scheme excites multiple motional states using discrete ultra-fast pulses. We use beam-splitters to divide pulses into smaller components to overcome limitations due to the finite laser pulse repetition rate. This provides gate times faster than proposed theoretical schemes when we optimise a practical setup.

quant-ph↗

arXiv2013

Unavoidable decoherence in the quantum control of an unknown state

A common objective for quantum control is to force a quantum system, initially in an unknown state, into a particular target subspace. We show that if the subspace is required to be a decoherence-free subspace of dimension greater than 1, then such control must be decoherent. That is, it will take almost any pure state to a mixed state. We make no assumptions about the control mechanism, but our result implies that for this purpose coherent control offers no advantage, in principle, over the obvious measurement-based feedback protocol.

quant-ph↗

arXiv2012

Controllable optical phase shift over one radian from a single isolated atom

Fundamental optics such as lenses and prisms work by applying phase shifts to incoming light via the refractive index. In these macroscopic devices, many particles each contribute a miniscule phase shift, working together to impose a total phase shift of many radians. In principle, even a single isolated particle can apply a radian-level phase shift, but observing this phenomenon has proven challenging. We have used a single trapped atomic ion to induce and measure a large optical phase shift of $1.3 \pm 0.1$ radians in light scattered by the atom. Spatial interferometry between the scattered light and unscattered illumination light enables us to isolate the phase shift in the scattered component. The phase shift achieves the maximum value allowed by atomic theory over the accessible range of laser frequencies, validating the microscopic model that underpins the macroscopic phenomenon of the refractive index. Single-atom phase shifts of this magnitude open up new quantum information protocols, including long-range quantum phase-shift-keying cryptography [1,2] and quantum nondemolition measurement [3,4].

quant-ph↗

arXiv2012

Absorption imaging of a single atom

Absorption imaging has played a key role in the advancement of science from van Leeuwenhoek's discovery of red blood cells to modern observations of dust clouds in stellar nebulas and Bose-Einstein condensates. Here we show the first absorption imaging of a single atom isolated in vacuum. The optical properties of atoms are thoroughly understood, so a single atom is an ideal system for testing the limits of absorption imaging. A single atomic ion was confined in an RF Paul trap and the absorption imaged at near wavelength resolution with a phase Fresnel lens. The observed image contrast of 3.1(3)% is the maximum theoretically allowed for the imaging resolution of our setup. The absorption of photons by single atoms is of immediate interest for quantum information processing (QIP). Our results also point out new opportunities in imaging of light-sensitive samples both in the optical and x-ray regimes.

quant-ph↗

arXiv2011

Low-loss flake-graphene saturable absorber mirror for laser mode-locking at sub-200-fs pulse duration

Saturable absorbers are a key component for mode-locking femtosecond lasers. Polymer films containing graphene flakes have recently been used in transmission as laser mode-lockers, but suffer from high nonsaturable loss, limiting their application in low-gain lasers. Here we present a saturable absorber mirror based on a film of pure graphene flakes. The device is used to mode lock an erbium-doped fiber laser, generating pulses with state-of-the-art, sub-200-fs duration. The laser characteristic indicate that the film exhibits low nonsaturable loss (13% per pass) and large absorption modulation depth (45% of low-power absorption).

physics.optics↗

arXiv2011

Quantum interface between an electrical circuit and a single atom

We show how to bridge the divide between atomic systems and electronic devices by engineering a coupling between the motion of a single ion and the quantized electric field of a resonant circuit. Our method can be used to couple the internal state of an ion to the quantized circuit with the same speed as the internal-state coupling between two ions. All the well-known quantum information protocols linking ion internal and motional states can be converted to protocols between circuit photons and ion internal states. Our results enable quantum interfaces between solid state qubits, atomic qubits, and light, and lay the groundwork for a direct quantum connection between electrical and atomic metrology standards.

quant-ph↗

arXiv2011

Phase-coherent repetition rate multiplication of a mode-locked laser from 40 MHz to 1 GHz by injection locking

We have used injection locking to multiply the repetition rate of a passively mode-locked femtosecond fiber laser from 40 MHz to 1 GHz while preserving optical phase coherence between the master laser and the slave output. The system is implemented almost completely in fiber and incorporates gain and passive saturable absorption. The slave repetition rate is set to a rational harmonic of the master repetition rate, inducing pulse formation at the least common multiple of the master and slave repetition rates.

physics.optics↗