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D. Lascar

Publications and source records attributed to D. Lascar.

12 recordsLinked to original sources

Compact Actively-Shielded Magnetic Field Coil within Mu-Metal Shields for ACME Electric Dipole Moment Measurements

A system of actively-shielded coils and mu-metal shields is devised, constructed and shown to provide the stable and spatially uniform magnetic field needed for the ACME III electron electric dipole moment (eEDM) measurement. Two layers of current-carrying coils, enclosed within three layers of ferromagnetic shields, produce a field that varies by less than 1 nT (10 $\uG$) within the 1 m $\times$ 4.2 cm $\times$ 4.2 cm interior volume in which a beam of ThO molecules are probed as they precess. The demountable shields are constructed from rectangular mu-metal plates. The largest, with a mass of 19 kg and an area of 2.18 m $\times$ 0.75 m, is easily carried by two people and just fits within a large available annealing oven. The assembly design facilitates low-stress mounting and handling to suppress changes in the magnetic properties of the mu metal, and also provides modular access to apparatus within the coils for maintenance and upgrades. The nearly static external ambient field is reduced within the shielded precession volume by up to a factor of $10^5$. During the magnetic field reversals that ACME uses to suppress systematic uncertainties, the ``actively-shielded'' coil largely cancels out its external fringing field to minimize the magnetization of the mu metal. Even though the shields are only 10 cm outside the coils, shield degaussing after every magnetic field reversal is not required. The non-reversing residual field stays below 1 nT for up to 17 hours when the field is reversed every 30 seconds, for example. The measured performance, compared to the previous generation ACME II apparatus, suggests that the magnetic-field-related systematic uncertainties for ACME III will be smaller by an estimated factor of 40 despite a five times longer precession volume and the use of three magnetic shielding layers rather than five.

physics.atom-ph

Precision mass measurements of $^{74-76}$Sr using TITAN's Multiple-Reflection Time-of-Flight Mass Spectrometer

We report precision mass measurements of $^{74-76}$Sr performed with the TITAN Multiple-Reflection Time-of-Flight Mass Spectrometer. This marks a first time mass measurement of $^{74}$Sr and gives increased mass precision to both $^{75}$Sr and $^{76}$Sr which were previously measured using storage ring and Penning trap methods, respectively. This completes the A = 74, T = 1 isospin triplet and gives increased precision to the A = 75, T = 1/2 isospin doublet which are both the heaviest experimentally evaluated triplets and doublets to date. The new data allow us to evaluate coefficients of the isobaric multiplet mass equation for the first time at A = 74, and with increased precision at A = 75. With increased precision of 75Sr, we confirm the recent measurement reported by CSRe which was used to remove a staggering anomaly in the doublets. New ab initio valence-space in-medium similarity renormalization group calculations of the T = 1 triplet are presented at A = 74. We also investigate the impact of the new mass data on the reaction flow of the rapid proton capture process in type I x-ray bursts using a single-zone model.

nucl-ex

Mass Measurements of Neutron-Rich Gallium Isotopes Refine Production of Nuclei of the First r-Process Abundance Peak in Neutron Star Merger Calculations

We report mass measurements of neutron-rich Ga isotopes $^{80-85}$Ga with TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The measurements determine the masses of $^{80-83}$Ga in good agreement with previous measurements. The masses of $^{84}$Ga and $^{85}$Ga were measured for the first time. Uncertainties between $25-48$ keV were reached. The new mass values reduce the nuclear uncertainties associated with the production of A $\approx$ 84 isotopes by the \emph{r}-process for astrophysical conditions that might be consistent with a binary neutron star (BNS) merger producing a blue kilonova. Our nucleosynthesis simulations confirm that BNS merger may contribute to the first abundance peak under moderate neutron-rich conditions with electron fractions $Y_e=0.35-0.38$.

nucl-ex

Dawning of the N=32 shell closure seen through precision mass measurements of neutron-rich titanium isotopes

A precision mass investigation of the neutron-rich titanium isotopes $^{51-55}$Ti was performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The range of the measurements covers the $N=32$ shell closure and the overall uncertainties of the $^{52-55}$Ti mass values were significantly reduced. Our results confirm the existence of a weak shell effect at $N=32$, establishing the abrupt onset of this shell closure. Our data were compared with state-of-the-art \textit{ab-initio} shell model calculations which, despite very successfully describing where the $N=32$ shell gap is strong, overpredict its strength and extent in titanium and heavier isotones. These measurements also represent the first scientific results of TITAN using the newly commissioned Multiple-Reflection Time-of-Flight Mass Spectrometer (MR-TOF-MS), substantiated by independent measurements from TITAN's Penning trap mass spectrometer.

nucl-ex

High-precision $Q_{EC}$-value measurement of the superallowed $β^+$ emitter $^{22}$Mg and an evaluation of the $A=22$ isobaric triplet

A direct $Q_{EC}$-value measurement of the superallowed $β^+$ emitter $^{22}$Mg was performed using TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The direct ground-state to ground-state atomic mass difference between $^{22}$Mg and $^{22}$Na was determined to be $Q_{EC}=4781.40(22)$~keV, representing the most precise single measurement of this quantity to date. In a continued push towards calculating superallowed isospin-symmetry-breaking (ISB) corrections from first principles, ab-initio shell-model calculations of the $A=22$ IMME are also presented for the first time using the valence-space in-medium similarity renormalization group formalism. With particular starting two- and three-nucleon forces, this approach demonstrates a level of agreement with the experimental data that suggests reliable ab-initio calculations of superallowed ISB corrections are now possible.

nucl-ex

Precision mass measurements of $^{125-127}$Cd isotopes and isomers approaching the $N=82$ closed shell

We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}$Cd and $^{126}$Cd) in a recent TITAN experiment at TRIUMF. Finally, we compare our measurements to new \emph{ab initio} shell-model calculations and comment on the state of the field in the $N=82$ region.

nucl-ex

A Novel Transparent Charged Particle Detector for the CPET Upgrade at TITAN

The detection of an electron bunch exiting a strong magnetic field can prove challenging due to the small mass of the electron. If placed too far from a solenoid's entrance, a detector outside the magnetic field will be too small to reliably intersect with the exiting electron beam because the light electrons will follow the diverging magnetic field outside the solenoid. The TITAN group at TRIUMF in Vancouver, Canada, has made use of advances in the practice and precision of photochemical machining (PCM) to create a new kind of charge collecting detector called the "mesh detector." The TITAN mesh detector was used to solve the problem of trapped electron detection in the new Cooler PEnning Trap (CPET) currently under development at TITAN. This thin array of wires etched out of a copper plate is a novel, low profile, charge agnostic detector that can be made effectively transparent or opaque at the user's discretion.

physics.ins-det

Improvements to TITAN's Mass Measurement and Decay Spectroscopy Capabilities

The study of nuclei farther from the valley of $β$-stability goes hand-in-hand with shorter-lived nuclei produced in smaller abundances than their more stable counterparts. The measurement, to high precision, of nuclear masses therefore requires innovations in technique in order to keep up. TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN) facility deploys three ion traps, with a fourth in the commissioning phase, to perform and support Penning trap mass spectrometry and in-trap decay spectroscopy on some of the shortest-lived nuclei ever studied. We report on recent advances and updates to the TITAN facility since the 2012 EMIS Conference. TITAN's charge breeding capabilities have been improved and in-trap decay spectroscopy can be performed in TITAN's electron beam ion trap (EBIT). Higher charge states can improve the precision of mass measurements, reduce the beam-time requirements for a given measurement, improve beam purity and opens the door to access, via in-trap decay and recapture, isotopes not available from the ISOL method. This was recently demonstrated during TITAN's mass measurement of $^{30}$Al. The EBIT's decay spectroscopy setup was commissioned with a successful branching ratio and half-life measurement of $^{124}$Cs. Charge breeding in the EBIT increases the energy spread of the ion bunch sent to the Penning trap for mass measurement so a new Cooler Penning Trap (CPET), which aims to cool highly charge ions with an electron plasma, is undergoing online commissioning. Already, CPET has demonstrated the trapping and self-cooling of a room-temperature electron plasma which was stored for several minutes. A new detector has been installed inside the CPET magnetic field which will allow for in-magnet charged particle detection.

physics.ins-det

Mass measurements of neutron-rich Rb and Sr isotopes

We report on the mass measurements of several neutron-rich $\mathrm{Rb}$ and $\mathrm{Sr}$ isotopes in the $A \approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}\mathrm{Rb}$ and $^{98-100}\mathrm{Sr}$ have been determined with a precision of $6 - 12\ \mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}\mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measurement and a deviation of $3σ$ when compared to the Atomic Mass Evaluation. We also confirm the mass of $^{100}\mathrm{Rb}$ from a previous measurement. Furthermore, our data indicates the existance of a low-lying isomer with $80\ \mathrm{keV}$ excitation energy in $^{98}\mathrm{Rb}$. We show that our updated mass values lead to minor changes in the r-process by calculating fractional abundances in the $A\approx 100$ region of the nuclear chart.

nucl-ex

First Results from the CARIBU Facility: Mass Measurements on the r-Process Path

The Canadian Penning Trap mass spectrometer has made mass measurements of 33 neutron-rich nuclides provided by the new Californium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. The studied region includes the 132Sn double shell closure and ranges in Z from In to Cs, with Sn isotopes measured out to A = 135, and the typical measurement precision is at the 100 ppb level or better. The region encompasses a possible major waiting point of the astrophysical r process, and the impact of the masses on the r process is shown through a series of simulations. These first-ever simulations with direct mass information on this waiting point show significant increases in waiting time at Sn and Sb in comparison with commonly used mass models, demonstrating the inadequacy of existing models for accurate r-process calculations.

nucl-ex

Mass measurements near the $r$-process path using the Canadian Penning Trap mass spectrometer

The masses of 40 neutron-rich nuclides from Z = 51 to 64 were measured at an average precision of $δm/m= 10^{-7}$ using the Canadian Penning Trap mass spectrometer at Argonne National Laboratory. The measurements, of fission fragments from a $^{252}$Cf spontaneous fission source in a helium gas catcher, approach the predicted path of the astrophysical $r$ process. Where overlap exists, this data set is largely consistent with previous measurements from Penning traps, storage rings, and reaction energetics, but large systematic deviations are apparent in $β$-endpoint measurements. Differences in mass excess from the 2003 Atomic Mass Evaluation of up to 400 keV are seen, as well as systematic disagreement with various mass models.

nucl-ex

Double-beta decay Q values of 130Te, 128Te, and 120Te

The double-beta decay Q values of 130Te, 128Te, and 120Te have been determined from parent-daughter mass differences measured with the Canadian Penning Trap mass spectrometer. The 132Xe-129Xe mass difference, which is precisely known, was also determined to confirm the accuracy of these results. The 130Te Q value was found to be 2527.01(32) keV which is 3.3 keV lower than the 2003 Atomic Mass Evaluation recommended value, but in agreement with the most precise previous measurement. The uncertainty has been reduced by a factor of 6 and is now significantly smaller than the resolution achieved or foreseen in experimental searches for neutrinoless double-beta decay. The 128Te and 120Te Q values were found to be 865.87(131) keV and 1714.81(125) keV, respectively. For 120Te, this reduction in uncertainty of nearly a factor of 8 opens up the possibility of using this isotope for sensitive searches for neutrinoless double-electron capture and electron capture with positron emission.

nucl-ex