arXiv subjects

D. Lu

Publications and source records attributed to D. Lu.

At least 19 recordsLinked to original sources

arXiv2026

Collinear Laser Spectroscopy on a Fast Atomic Beam of Boron Generated by Photodetachment of Accelerated B- Ions

Atomic beams for collinear laser spectroscopy are typically produced via charge exchange reactions in an in-beam vapor cell. This process is accompanied by the formation of a considerable amount of longer-lived excited state population, which is not accessible for spectroscopy and also induces fluorescence background to photon detectors. We present an alternative method to produce an atomic beam, consisting exclusively of ground-state atoms. Negative ions are neutralized in-flight by photodetachment and are subsequently used for fluorescence spectroscopy. As a test candidate, a negative boron ion beam was produced in a cesium sputtering source and superimposed with a co-propagating high-power pulsed infrared laser. The neutral atoms were subsequently excited along the $2s^2 2p\,{}^{2\!}P_{1/2,3/2} \rightarrow 2s^2 3s\,{}^{2\!}S_{1/2}$ transitions by a continuous-wave laser at about 250 nm. The statistics and efficiency were limited by the combination of a continuous ion beam with a low-repetition-rate laser, but a clear route for the improvement combining existing techniques is presented, which can then be applied to other elements as well as negative molecular ions.

physics.atom-ph↗

arXiv2024

X-ray magnetic circular dichroism and resonant inelastic X-ray scattering explained: role of many-body correlation and valence fluctuations

X-ray magnetic circular dichroism (XMCD) and resonant inelastic X-ray scattering with magnetic circular dichroism (RIXS-MCD) provide unparalleled insights into the electronic and magnetic dynamics of complex materials. However, interpreting their spectra in mixed-valence systems remains challenging due to intricate many-body interactions and enhanced charge fluctuations. In this study, by utilizing the Anderson impurity model with a full consideration of charge transfer (CT), many-body core-valence exchange correlation (CVEC) effects, and Jahn-Teller (JT) distortions, we systematically investigate the XMCD and RIXS-MCD spectra for a prototypical mixed-valence ferromagnet, La$_{0.7}$Sr$_{0.3}$MnO$_3$ film. We demonstrate that simple calculation with limited CT effects fails to capture characteristic substructures observed experimentally. In contrast, an adequate treatment of CT and CVEC effects yields a more consistent description of both XMCD and RIXS-MCD spectra, providing practical guidance for the interpretation of dichroic x-ray spectroscopies in mixed-valence transition-metal oxides. Furthermore, we discuss the role of the JT effect in Mn$^{3+}$ ions in the determination of their spectra.

cond-mat.str-el↗

arXiv2024

Suppression of Edge Localized Modes in ITER Baseline Scenario in EAST using Edge Localized Magnetic Perturbations

We report the suppression of Type-I Edge Localized Modes (ELMs) in the EAST tokamak under ITER baseline conditions using $n = 4$ Resonant Magnetic Perturbations (RMPs), while maintaining energy confinement. Achieving RMP-ELM suppression requires a normalized plasma beta ($\beta_N$) exceeding 1.8 in a target plasma with $q_{95}\approx 3.1$ and tungsten divertors. Quasi-linear modeling shows high plasma beta enhances RMP-driven neoclassical toroidal viscosity torque, reducing field penetration thresholds. These findings demonstrate the feasibility and efficiency of high $n$ RMPs for ELM suppression in ITER.

physics.plasm-ph↗

arXiv2023

Flat Bands at the Fermi Level in Unconventional Superconductor YFe2Ge2

We report heavy electron behavior in unconventional superconductor YFe$_2$Ge$_2$ ($T_C \,{=}\, 1.2$ K). We directly observe very heavy bands ($m_\mathrm{eff}\sim 25 m_e$) within $\sim$10 meV of the Fermi level $E_{F}$ using angle-resolved photoelectron spectroscopy (ARPES). The flat bands reside at the X points of the Brillouin zone and are composed principally of $d_{xz}$ and $d_{yz}$ orbitals. We utilize many-body perturbative theory, GW, to calculate the electronic structure of this material, obtaining excellent agreement with the ARPES data with relatively minor band renormalizations and band shifting required. We obtain further agreement at the Dynamical Mean Field Theory (DMFT) level, highlighting the emergence of the many-body physics at low energies (near $E_F$) and temperatures.

cond-mat.str-el↗

arXiv2023

Study of Enhanced MISC-Based Sparse Arrays with High uDOFs and Low Mutual Coupling

In this letter, inspired by the maximum inter-element spacing (IES) constraint (MISC) criterion, an enhanced MISC-based (EMISC) sparse array (SA) with high uniform degrees-of-freedom (uDOFs) and low mutual-coupling (MC) is proposed, analyzed and discussed in detail. For the EMISC SA, an IES set is first determined by the maximum IES and number of elements. Then, the EMISC SA is composed of seven uniform linear sub-arrays (ULSAs) derived from an IES set. An analysis of the uDOFs and weight function shows that, the proposed EMISC SA outperforms the IMISC SA in terms of uDOF and MC. Simulation results show a significant advantage of the EMISC SA over other existing SAs.

cs.LG↗

arXiv2023

Probabilistic neural networks for improved analyses with phenomenological models

Physics models typically contain adjustable parameters to reproduce measured data. While some parameters correspond directly to measured features in the data, others are unobservable. These unobservables can, in some cases, cause ambiguities in the extraction of observables from measured data, or lead to questions on the physical interpretation of fits that require these extra parameters. We propose a method based on deep learning to extract values of observables directly from the data without the need for unobservables. The key to our approach is to label the training data for the deep learning model with only the observables. After training, the deep learning model can determine the values of observables from measured data with no ambiguities arising from unobservables. We demonstrate this method on the phenomenological R-matrix that is widely utilized in nuclear physics to extract resonance parameters from cross section data. Our deep learning model based on Transformers successfully predicts nuclear properties from measurements with no need for the channel radius and background pole parameters required in traditional R-matrix analyses. Details and limitations of this method, which may be useful for studies of a wide range of phenomena, are discussed.

nucl-th↗

arXiv2021

Anisotropic quasiparticle coherence in nematic BaFe$_2$As$_2$ studied with strain-dependent ARPES

The hallmark of nematic order in iron-based superconductors is a resistivity anisotropy but it is unclear to which extent quasiparticle dispersions, lifetimes and coherence contribute. While the lifted degeneracy of the Fe $d_{xz}$ and $d_{yz}$ dispersions has been studied extensively, only little is known about the two other factors. Here, we combine in situ strain tuning with ARPES and study the nematic response of the spectral weight in BaFe$_2$As$_2$. The symmetry analysis of the ARPES spectra demonstrates that the $d_{xz}$ band gains quasiparticle spectral weight compared to the $d_{yz}$ band for negative antisymmetric strain $\Delta \epsilon_{yy}$ suggesting the same response inside the nematic phase. Our results are compatible with a different coherence of the $d_{xz}$ and $d_{yz}$ orbital within a Hund's metal picture. We also discuss the influence of orbital mixing.

cond-mat.str-el↗

arXiv2019

Momentum Dependence of the Nematic Order Parameter in Iron-Based Superconductors

The momentum dependence of the nematic order parameter is an important ingredient in the microscopic description of iron-based high-temperature superconductors. While recent reports on FeSe indicate that the nematic order parameter changes sign between electron and hole bands, detailed knowledge is still missing for other compounds. Combining angle-resolved photoemission spectroscopy (ARPES) with uniaxial strain tuning, we measure the nematic band splitting in both FeSe and BaFe$_2$As$_2$ without interference from either twinning or magnetic order. We find that the nematic order parameter exhibits the same momentum dependence in both compounds with a sign change between the Brillouin center and the corner. This suggests that the same microscopic mechanism drives the nematic order in spite of the very different phase diagrams.

cond-mat.str-el↗

arXiv2019

Electronic structure of the quadrupolar ordered heavy-fermion compound YbRu2Ge2 measured by angle-resolved photoemission

We studied the electronic structure of the heavy fermion compound Yb(Ru$_{1-x}$Rh$_{x}$)$_2$Ge$_2$ with $x=0$ and nominally $x=0.125$ using ARPES and LDA calculations. We find a valence band structure of Yb corresponding to a non-integer valence close to $3+$. The three observed crystal electric field levels with a splitting of 32 and 75 meV confirm the suggested configuration with a quasi-quartet ground state. The experimentally determined band structure of the conduction electrons with predominantly Ru $4d$ character is well reproduced by our calculations. YbRu$_2$Ge$_2$ undergoes a non-magnetic phase transition into a ferroquadrupolar ordered state below 10.2\,K and then to an antiferromagnetically ordered state below 6.5\,K. A small hole Fermi surface shows nesting features in our calculated band structure and its size determined by ARPES is close to the magnetic ordering wave vector found in neutron scattering. The transitions are suppressed when YbRu$_2$Ge$_2$ is doped with 12.5% Rh. The electron doping leads to a shift of the band structure and successive Lifshitz transitions.

cond-mat.str-el↗

arXiv2019

Detailed band structure of twinned and detwinned BaFe$_2$As$_2$ studied with angle-resolved photoemission spectroscopy

We study the band structure of twinned and detwinned BaFe$_2$As$_2$ using angle-resolved photoemission spectroscopy (ARPES). The combination of measurements in the ordered and normal state along four high-symmetry momentum directions $\Gamma$/Z--X/Y enables us to identify the complex reconstructed band structure in the ordered state in great detail. We clearly observe the nematic splitting of the $d_{xz}$ and $d_{yz}$ orbitals as well as folding due to magnetic order with a wave vector of $(\pi,\pi,\pi)$. We are able to assign all observed bands. In particular we suggest an assignment of the electron bands different from previous reports. The high quality spectra allow us to achieve a comprehensive understanding of the band structure of BaFe$_2$As$_2$.

cond-mat.str-el↗

arXiv2018

Pseudogap in electron-doped cuprates: Strong correlation leading to band splitting

The pseudogap phenomena have been a long-standing mystery of the cuprate high-temperature superconductors. The pseudogap in the electron-doped cuprates has been attributed to band folding due to antiferromagnetic (AFM) long-range order or short-range correlation. We performed an angle-resolved photoemission spectroscopy (ARPES) study of the electron-doped cuprates Pr$_{1.3-x}$La$_{0.7}$Ce$_x$CuO$_4$ showing spin-glass, disordered AFM behaviors, and superconductivity at low temperatures and, by measurements with fine momentum cuts, found that the gap opens on the unfolded Fermi surface rather than the AFM Brillouin zone boundary. The gap did not show a node, following the full symmetry of the Brillouin zone, and its magnitude decreased from the zone-diagonal to ($\pi$,0) directions, opposite to the hole-doped case. These observations were reproduced by cluster dynamical-mean-field-theory (CDMFT) calculation, which took into account electron correlation precisely within a (CuO$_2$)$_4$ cluster. The present experimental and theoretical results are consistent with the mechanism that electron or hole doping into a Mott insulator creates an in-gap band that are separated from the upper or lower Hubbard band by the pseudogap.

cond-mat.supr-con↗

arXiv2017

3D nature of ZrTe$_5$ band structure measured by high-momentum-resolution photoemission spectroscopy

We have performed a systematic high-momentum-resolution photoemission study on ZrTe$_5$ using $6$ eV photon energy. We have measured the band structure near the $\Gamma$ point, and quantified the gap between the conduction and valence band as $18 \leq \Delta \leq 29$ meV. We have also observed photon-energy-dependent behavior attributed to final-state effects and the 3D nature of the material's band structure. Our interpretation indicates the gap is intrinsic and reconciles discrepancies on the existence of a topological surface state reported by different studies. The existence of a gap suggests that ZrTe$_5$ is not a 3D strong topological insulator nor a 3D Dirac semimetal. Therefore, our experiment is consistent with ZrTe$_5$ being a 3D weak topological insulator.

cond-mat.mtrl-sci↗

arXiv2017

Searching for Large-gap Quantum Spin Hall Insulators: Boron-Nitride/(Pb, Sn)/{\alpha}-Al2O3 Sandwich Structures

Topological insulators hold great potential for efficient information processing and storage. Using density functional theory calculations, we predict that a honeycomb lead monolayer can be stabilized on the Al2O3 (0001) substrate and becomes topologically non-trivial with a sizeable band gap (~0.27 eV). Furthermore, we propose to use hexagonal boron-nitride (h-BN) monolayer as a protection for the topological states of Pb/Al2O3 and Sn/Al2O3. Our findings suggest new possibilities for designing and protecting two-dimensional TIs for practical applications.

cond-mat.mtrl-sci↗

arXiv2015

Effects of electric field polarizations on pair production

The effects of electric field polarizations on pair production from a vacuum are investigated numerically by employing the real-time Dirac-Heisenberg-Wigner formalism. For few-cycle fields, it is found that the interference pattern in momentum spectra is absent and the circular distortion of momentum distribution becomes more apparent with the increase of polarization. For multi-cycle fields, it is found that the interference effects in momentum spectra are obvious. And as the polarization increases, the momentum distribution is split into two parts in the momentum $q_y$ direction first and then two separated parts are connected into a ring. The effects of polarizations on the number density of created particles exhibits two different characteristics. For a small laser frequency, the particle number density deceases with the polarization, while for a large laser frequency, the relation between them is sensitive to the field frequency nonlinearly. Some interpretations for the obtained results in this study, which is expected to be valuable to deepen the understanding of pair production in complex fields and also helpful for the study associated to strong-field ionization.

quant-ph↗

arXiv2015

Nonperturbative signatures in pair production for general elliptic polarization fields

The momentum signatures in nonperturbative multiphoton pair production for general elliptic polarization electric fields are investigated by employing the real-time Dirac-Heisenberg-Wigner formalism. For a linearly polarized electric field we find that the positions of the nodes in momenta spectra of created pairs depend only on the electric field frequency. The polarization of external fields could not only change the node structures or even make the nodes disappear but also change the thresholds of pair production. The momentum signatures associated to the node positions in which the even-number-photon pair creation process is forbid could be used to distinguish the orbital angular momentum of created pairs on the momenta spectra. These distinguishable momentum signatures could be relevant for providing the output information of created particles and also the input information of ultrashort laser pulses.

quant-ph↗

arXiv2015

Dual Fano and Lorentzian line profile poperties of autoionizing states

Ott et al. (Science (340, 716 (2013)) successfully transferred Fano profile into Lorentzian lineshape using an intense infrared laser, after excitation of autoionizing states in helium by attosecond XUV pulse. This is a very important step forward of quantum phase control. However, here we show experimentally that an autoionizing state can have both Fano and Lorentzian behavior naturally, depending on the process involved. This study utilized the inverse process of photon absorption ionization, i.e. electron ion recombination with photon emission, making sure the resonant autoionizing state is not perturbed by the laser fields. Our result implies that excitation of the state through different paths can lead to different Fano profiles for the same resonant state. This allows more options for the combination of laser fields and lead to more opportunities for quantum phase control. Our result also indicates the breakdown of the classical two step picture for dielectronic recombination.

physics.atom-ph↗

arXiv2014

Mass shift effects in nonperturbative multiphoton pair production for arbitrary polarized electric fields

The mass shift effects in multiphoton pair production of a nonperturbative nature for arbitrary polarized electric fields are investigated numerically by employing the real-time Dirac-Heisenberg-Wigner formalism, and theoretically by proposing an effective energy concept. It is found that the theoretical results are agreement with the numerical ones very well. It is the first time to consider the roles of the momenta of created particles and the polarizations of external fields played in the mass shift effects. These results can deepen the understanding of pair production in the nonperturbative threshold regime. Moreover, the distinct mass shift effects are observable in the forthcoming experiments and can be used as a probe to distinguish the electron-positron pair production from other background events.

hep-ph↗

arXiv2013

Spectroscopic evidence for polaronic behaviour of the strong spin-orbit insulator Sr$_3$Ir$_2$O$_7$

We investigate the bilayer Ruddlesden-Popper iridate Sr$_3$Ir$_2$O$_7$ by temperature-dependent angle-resolved photoemission. We find a narrow-gap correlated insulator, with spectral features indicative of a polaronic ground state, strikingly similar to that observed previously for the parent compounds of the cuprate superconductors. We additionally observe similar behaviour for the single-layer cousin Sr$_2$IrO$_4$, indicating that strong electron-boson coupling dominates the low-energy excitations of this exotic family of materials, and providing a microscopic link between the insulating ground states of the seemingly-disparate 3d cuprates and 5d iridates.

cond-mat.str-el↗