arXiv subjects

D. Mele

Publications and source records attributed to D. Mele.

9 recordsLinked to original sources

arXiv2023

Electroluminescence and Energy Transfer Mediated by Hyperbolic Polaritons

Under high electrical current, some materials can emit electromagnetic radiation beyond incandescence. This phenomenon, referred to as electroluminescence, leads to the efficient emission of visible photons and is the basis of domestic lighting devices (e.g., light-emitting diodes). In principle, electroluminescence can lead to mid-infrared (mid-IR) emission of confined light-matter excitations called phonon-polaritons, resulting from the coupling of photons with crystal lattice vibrations (optical phonons). In particular, phonon-polaritons arising in the van der Waals crystal hexagonal boron nitride (hBN) exhibit hyperbolic dispersion, which enhances light-matter coupling. For this reason, electroluminescence of hyperbolic phonon-polaritons (HPhPs) has been proposed as an explanation for the peculiar radiative energy transfer within hBN-encapsulated graphene transistors. However, since HPhPs are confined, they are inaccessible in the far-field, so that any hint of electroluminescence is only based on indirect electronic signatures and needs to be confirmed by direct observation. Here, we demonstrate far-field mid-IR ({\lambda} = 6.5 {\mu}m) electroluminescence of HPhPs excited by strongly biased high-mobility graphene within a van der Waals heterostructure, and we quantify the associated radiative energy transfer through the material. The presence of HPhPs is revealed via far-field mid-IR spectroscopy due to their elastic scattering at discontinuities in the heterostructure. The associated radiative flux is quantified by mid-IR pyrometry of the substrate receiving the energy. This radiative energy transfer is shown to be reduced in hBN with nanoscale inhomogeneities, demonstrating the central role of the electromagnetic environment in this process.

cond-mat.mes-hall↗

arXiv2023

Electroluminescence of the graphene 2D semi-metal

Electroluminescence, a non-thermal radiative process, is ubiquitous in semi-conductors and insulators but fundamentally precluded in metals. We show here that this restriction can be circumvented in high-quality graphene. By investigating the radiative emission of semi-metallic graphene field-effect transistors over a broad spectral range, spanning the near- and mid-infrared, we demonstrate direct far-field electroluminescence from hBN-encapsulated graphene in the mid-infrared under large bias in ambient conditions. Through a series of test experiments ruling out its incandescence origin, we determine that the electroluminescent signal results from the electrical pumping produced by interband tunneling. We show that the mid-infrared electroluminescence is spectrally shaped by a natural quarter-wave resonance of the heterostructure. This work invites a reassessment of the use of metals and semi-metals as non-equilibrium light emitters, and the exploration of their intriguing specificities in terms of carrier injection and relaxation, as well as emission tunability and switching speed.

cond-mat.mes-hall↗

arXiv2023

High-field 1/f noise in hBN-encapsulated graphene transistors

Low-frequency 1/f noise in electronics is a conductance fluctuation, that has been expressed in terms of a mobility "$\alpha$-noise" by Hooge and Kleinpenning. Understanding this noise in graphene is a key towards high-performance electronics. Early investigations in diffusive graphene have pointed out a deviation from the standard Hooge formula, with a modified expression where the free-carrier density is substituted by a constant density $n_\Delta\sim10^{12}\;\mathrm{cm^{-2}}$. We investigate hBN-encapsulated graphene transistors where high mobility gives rise to the non-linear velocity-saturation regime. In this regime, the $\alpha$-noise is accounted for by substituting conductance by differential conductance $G$, ressulting in a bell-shape dependence of flicker noise with bias voltage $V$. The same analysis holds at larger bias in the Zener regime, with two main differences: the first one is a strong enhancement of the Hooge parameter reflecting the hundred-times larger coupling of interband excitations to the hyperbolic phonon-polariton (HPhP) modes of the mid-infrared Reststrahlen (RS) bands of hBN. The second is an exponential suppression of this coupling at large fields, which we attribute to decoherence effects. We also show that the HPhP bands control the amplitude of flicker noise according to the graphene-hBN thermal coupling estimated with microwave noise thermometry. The phenomenology of $\alpha$-noise in graphene supports a quantum-coherent bremsstrahlung interpretation of flicker noise.

cond-mat.mes-hall↗

arXiv2022

Mesoscopic Klein-Schwinger effect in graphene

Strong electric field annihilation by particle-antiparticle pair creation, also known as the Schwinger effect, is a non-perturbative prediction of quantum electrodynamics. Its experimental demonstration remains elusive, as threshold electric fields are extremely strong and beyond current reach. Here, we propose a mesoscopic variant of the Schwinger effect in graphene, which hosts Dirac fermions with an approximate electron-hole symmetry. Using transport measurements, we report on universal 1d-Schwinger conductance at the pinchoff of ballistic graphene transistors. Strong pinchoff electric fields are concentrated within approximately 1 $\mu$m of the transistor's drain, and induce Schwinger electron-hole pair creation at saturation. This effect precedes a collective instability toward an ohmic Zener regime, which is rejected at twice the pinchoff voltage in long devices. These observations advance our understanding of current saturation limits in ballistic graphene and provide a direction for further quantum electrodynamic experiments in the laboratory.

cond-mat.mes-hall↗

arXiv2022

Dielectric permittivity, conductivity and breakdown field of hexagonal boron nitride

In view of the extensive use of hexagonal boron nitride (hBN) in 2D material electronics, it becomes important to refine its dielectric characterization in terms of low-field permittivity and high-field strength and conductivity up to the breakdown voltage. The present study aims at filling this gap using DC and RF transport in two Au-hBN-Au capacitor series of variable thickness in the 10--100 nm range, made of large high-pressure, high-temperature (HPHT) crystals and a polymer derivative ceramics (PDC) crystals. We deduce an out-of-plane low field dielectric constant $\epsilon_\parallel=3.4\pm0.2$ consistent with the theoretical prediction of Ohba et al., that narrows down the generally accepted window $\epsilon_\parallel=3$--$4$. The DC-current leakage at high-field is found to obey the Frenkel-Pool law for thermally-activated trap-assisted electron transport with a dynamic dielectric constant $\epsilon_\parallel\simeq3.1$ and a trap energy $\Phi_B\simeq1.3\;\mathrm{eV}$, that is comparable with standard technologically relevant dielectrics.

cond-mat.mtrl-sci↗

arXiv2019

A corner reflector of graphene Dirac fermions as a phonon-scattering sensor

Dirac fermion optics exploits the refraction of chiral fermions across optics-inspired Klein-tunneling barriers defined by high-transparency p-n junctions. We consider the corner reflector (CR) geometry introduced in optics or radars. We fabricate Dirac fermion CRs using bottom-gate-defined barriers in hBN-encapsulated graphene. By suppressing transmission upon multiple internal reflections, CRs are sensitive to minute phonon scattering rates. We report on doping-independent CR transmission in quantitative agreement with a simple scattering model including thermal phonon scattering. As a new signature of CRs, we observe Fabry-Pérot oscillations at low temperature, consistent with single-path reflections. Finally, we demonstrate high-frequency operation which promotes CRs as fast phonon detectors. Our work establishes the relevance of Dirac fermion optics in graphene and opens a route for its implementation in topological Dirac matter.

cond-mat.mes-hall↗

arXiv2018

Ultra-long wavelength Dirac plasmons in graphene capacitors

Graphene is a valuable 2D platform for plasmonics as illustrated in recent THz and mid-infrared optics experiments. These high-energy plasmons however, couple to the dielectric surface modes giving rise to hybrid plasmon-polariton excitations. Ultra-long-wavelengthes address the low energy end of the plasmon spectrum, in the GHz-THz electronic domain, where intrinsic graphene Dirac plasmons are essentially decoupled from their environment. However experiments are elusive due to the damping by ohmic losses at low frequencies. We demonstrate here a plasma resonance capacitor (PRC) using hexagonal boron-nitride (hBN) encapsulated graphene at cryogenic temperatures in the near ballistic regime. We report on a $100\;\mathrm{μm}$ quarter-wave plasmon mode, at $40\;\mathrm{GHz}$, with a quality factor $Q\simeq2$. The accuracy of the resonant technique yields a precise determination of the electronic compressibility and kinetic inductance, allowing to assess residual deviations from intrinsic Dirac plasmonics. Our capacitor GHz experiment constitutes a first step toward the demonstration of plasma resonance transistors for microwave detection in the sub-THz domain for wireless communications and sensing. It also paves the way to the realization of doping modulated superlattices where plasmon propagation is controlled by Klein tunneling.

cond-mat.mes-hall↗

arXiv2007

Improved tests on the relationship between the kinetic energy of galaxies and the mass of their central black holes

We support, with new fitting instruments and the analysis of more recent experimental data, the proposal of a relationship between the mass of a Supermassive Black Hole (SMBH) and the kinetic energy of random motions in the host elliptical galaxy. The first results obtained in a previous paper with 13 elliptical galaxies are now confirmed by the new data and an enlarged sample. We find $M_{BH} \propto (M_{G} σ^{2}/c^2)^β$ with $0.8 \leq β\leq 1$ depending on the different fitting methods and samples used. The meaningful case $β= 1$ is carefully analyzed. Furthermore, we test the robustness of our relationship including in the sample also lenticular and spiral galaxies and we show that the result does not change. Finally we find a stronger correlation between the mass of the galaxy and the corresponding velocity dispersion that allows to connect our relationship to the $M_{BH} \propto σ^α$ law. With respect to this law, our relationship has the advantage to have a smaller scatter.

astro-ph↗

arXiv2005

Is there a relationship between the mass of a SMBH and the kinetic energy of its host elliptical galaxy?

We use a restricted sample of elliptical galaxies, whose kinematical parameters inside the semimajor axis were calculated correcting the effect of the integration of the light along the line of sight, in order to analyze a possible relationship between the mass of a Supermassive Black Hole (SMBH) and the kinetic energy of random motions in the host galaxy. We find $M_{BH} \propto (M_{G} σ^{2})^α$ with $0.87 \leq α\leq 1$ depending on the different fitting methods and samples used. This result could be interpreted as a new fundamental relationship or as a new way to explain the old $M_{BH} - σ$ law. In fact, the relations of the velocity dispersion both with the mass of the SMBH ($M_{BH} \propto σ^{4.12}$) and with the mass of the host galaxy ($M_{G} \propto σ^{2.16}$) induce us to infer an almost direct proportionality: $M_{BH} \propto M_{G} σ^{2}$. A similar relationship is found for the total kinetic energy involving the rotation velocity too.

astro-ph↗